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rays from a neutron-induced 
-wave resonance of 
XeOkudaira, Takuya*; Tani, Yuika*; Endo, Shunsuke; Doskow, J.*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kameda, Kento*; Kimura, Atsushi; Kitaguchi, Masaaki*; Luxnat, M.*; et al.
Physical Review C, 107(5), p.054602_1 - 054602_7, 2023/05
Times Cited Count：2 Percentile：83.53(Physics, Nuclear)no abstracts in English
Sn in concrete rubbleDo, V. K.; Furuse, Takahiro; Ota, Yuki; Iwahashi, Hiroyuki; Hirosawa, Takashi; Watanabe, Masahisa; Sato, Soichi
Journal of Radioanalytical and Nuclear Chemistry, 331(12), p.5631 - 5640, 2022/12
Times Cited Count：2 Percentile：50.96(Chemistry, Analytical)Sn is one of the long-lived fission products that might have been released into the environment after the Fukushima nuclear accident in Japan in 2011. The presence of radionuclides must be monitored for the proper treatment of wastes obtained from decommissioning accident-related nuclear facilities and the surrounding environment. In the work, we propose a reliable method for verifying the presence of Sn in construction materials by combining the HCl-free solid phase extraction on TEVA resin and a selective measurement by inductively coupled plasma tandem mass spectrometry (ICP-MS/MS). The method has been optimized and characterized step by step. More than 95% of chemical recovery was achieved for Sn from typical concrete matrixes. The interference caused by an isobar Te and possible polyatomic interferences from matrixes were effectively suppressed by the developed chemical separation and the tandem MS/MS configuration. The total decontamination factor for the Te interference was of the order of 10
. The estimated method detection limit for Sn in concrete as measured at m/z = 160 was 12.1 pg g
, which is equivalent to 6.1 mBq g.
rays in the 
Sn(
)
Sn reactionEndo, Shunsuke; Okudaira, Takuya*; Abe, Ryota*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Oku, Takayuki; Sakai, Kenji; Shima, Tatsushi*; et al.
Physical Review C, 106(6), p.064601_1 - 064601_7, 2022/12
Times Cited Count：3 Percentile：49.92(Physics, Nuclear)no abstracts in English
Yamano, Hidemasa; Takai, Toshihide; Emura, Yuki; Fukuyama, Hiroyuki*; Higashi, Hideo*; Nishi, Tsuyoshi*; Ota, Hiromichi*; Morita, Koji*; Nakamura, Kinya*; Fukai, Hirofumi*; et al.
Proceedings of 13th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation and Safety (NUTHOS-13) (Internet), 12 Pages, 2022/09
This paper describes the project overview and progress of experimental and analytical studies conducted until 2020. Specific results in this paper are the measurement of the eutectic reaction rates and the validation of physical model describing the eutectic reaction in the analysis code through the numerical analysis of the B
C-SS eutectic reaction rate experiments in which a BC pellet was placed in a SS crucible.
Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.
Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07
This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.
Fe
GeO
with andalusite structureKakimoto, Kazuo*; Takada, Saki*; Ota, Hiroto*; Hayaguchi, Yuya*; Hagihara, Masato; Torii, Shuki*; Kamiyama, Takashi*; Mitamura, Hiroyuki*; Tokunaga, Masashi*; Hatakeyama, Atsushi*; et al.
Journal of the Physical Society of Japan, 91(5), p.054704_1 - 054704_7, 2022/05
Times Cited Count：1 Percentile：26.42(Physics, Multidisciplinary) rays from the -wave resonance of SnKoga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.
Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05
Times Cited Count：4 Percentile：64.25(Physics, Nuclear)no abstracts in English
Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.
Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12
Times Cited Count：6 Percentile：49.29(Geosciences, Multidisciplinary)The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.
Yamano, Hidemasa; Takai, Toshihide; Furukawa, Tomohiro; Kikuchi, Shin; Emura, Yuki; Kamiyama, Kenji; Fukuyama, Hiroyuki*; Higashi, Hideo*; Nishi, Tsuyoshi*; Ota, Hiromichi*; et al.
Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 11 Pages, 2021/08
One of the key issues in a core disruptive accident (CDA) evaluation in sodium-cooled fast reactors is eutectic reactions between boron carbide (BC) and stainless steel (SS) as well as its relocation. Such behaviors have never been simulated in CDA numerical analyses in the past, therefore it is necessary to develop a physical model and incorporate the model into the CDA analysis code. This study focuses on BC-SS eutectic melting experiments, thermophysical property measurement of the eutectic melt, and physical model development for the eutectic melting reaction. The eutectic experiments involve the visualization experiments, eutectic reaction rate experiments and material analyses. The thermophysical properties are measured in a range from solid to liquid state. The physical model is developed for a CDA computer code based on the measured data of the eutectic reaction rate and the physical properties. This paper describes the project overview and progress of experimental and analytical studies conducted until 2019. Specific results in this paper are the validation of physical model describing BC-SS eutectic reaction in the CDA analysis code, SIMMER-III, through the numerical analysis of the BC-SS eutectic melting experiments in which a BC block was placed in a SS pool.
rays in the 
La(
)
La
reactionOkudaira, Takuya*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Niinomi, Yudai*; Sakai, Kenji; et al.
Physical Review C, 104(1), p.014601_1 - 014601_6, 2021/07
Times Cited Count：4 Percentile：55.56(Physics, Nuclear)
studied with high-pressure 
SRSugiyama, Jun; Higemoto, Wataru; Andreica, D.*; Forslund, O. K.*; Nocerino, E.*; M
nsson, M.*; Sassa, Y.*; Gupta, R.*; Khasanov, R.*; Ota, Hiroto*; et al.
Physical Review B, 103(10), p.104418_1 - 104418_10, 2021/03
Times Cited Count：8 Percentile：60.77(Materials Science, Multidisciplinary)The magnetic nature of a quasi-one-dimensional compound, BaVSe, has been investigated with positive muon spin rotation and relaxation measurements at ambient and high pressures. At ambient pressure, the spectrum recorded under zero external magnetic field exhibited a clear oscillation below the Curie temperature due to the formation of quasistatic ferromagnetic order. As pressure increased from ambient pressure, 
was found to decrease slightly up to about 1.5 GPa, at which point started to increase rapidly with the further increase of the pressure. Based on a strong ferromagnetic interaction along the 
-axis, the result revealed that there are two magnetic interactions in the ab-plane.
Arai, Yoichi; Watanabe, So; Ono, Shimpei; Nomura, Kazunori; Nakamura, Fumiya*; Arai, Tsuyoshi*; Seko, Noriaki*; Hoshina, Hiroyuki*; Hagura, Naoto*; Kubota, Toshio*
Nuclear Instruments and Methods in Physics Research B, 477, p.54 - 59, 2020/08
Times Cited Count：5 Percentile：52.81(Instruments & Instrumentation)Yamano, Hidemasa; Takai, Toshihide; Furukawa, Tomohiro; Kikuchi, Shin; Emura, Yuki; Kamiyama, Kenji; Fukuyama, Hiroyuki*; Higashi, Hideo*; Nishi, Tsuyoshi*; Ota, Hiromichi*; et al.
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 10 Pages, 2020/08
One of the key issues in a core disruptive accident (CDA) evaluation in sodium-cooled fast reactors is eutectic reactions between boron carbide (BC) and stainless steel (SS) as well as its relocation. Such behaviors have never been simulated in CDA numerical analyses in the past, therefore it is necessary to develop a physical model and incorporate the model into the CDA analysis code. This study focuses on BC-SS eutectic melting experiments, thermophysical property measurement of the eutectic melt, and physical model development for the eutectic melting reaction. The eutectic experiments involve the visualization experiments, eutectic reaction rate experiments and material analyses. The thermophysical properties are measured in a range from solid to liquid state. The physical model is developed for a severe accident computer code based on the measured data of the eutectic reaction rate and the physical properties. This paper describes the project overview and progress of experimental and analytical studies conducted until 2018. Specific results in this paper are boron concentration distributions of solidified BC-SS eutectic sample in the eutectic melting experiments, which would be used for the validation of the eutectic physical model implemented into the computer code.
rays from neutron-induced compound states of LaYamamoto, Tomoki*; Okudaira, Takuya; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ino, Takashi*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; et al.
Physical Review C, 101(6), p.064624_1 - 064624_8, 2020/06
Times Cited Count：9 Percentile：72.89(Physics, Nuclear)
F from 
O
?Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.
Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05
Times Cited Count：14 Percentile：73.46(Physics, Multidisciplinary)The structure of a neutron-rich F nucleus is investigated by a quasifree (
) knockout reaction. The sum of spectroscopic factors of 
orbital is found to be 1.0 
0.3. The result shows that the O core of F nucleus significantly differs from a free O nucleus, and the core consists of 
35% O
, and 65% excited O. The result shows that the O core of F nucleus significantly differs from a free O nucleus. The result may infer that the addition of the 
proton considerably changes the neutron structure in F from that in O, which could be a possible mechanism responsible for the oxygen dripline anomaly.
Arai, Yoichi; Watanabe, So; Ono, Shimpei; Nomura, Kazunori; Nakamura, Fumiya*; Arai, Tsuyoshi*; Seko, Noriaki*; Hoshina, Hiroyuki*; Kubota, Toshio*
QST-M-23; QST Takasaki Annual Report 2018, P. 59, 2020/03
Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11
Times Cited Count：4 Percentile：21.22(Chemistry, Analytical)We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the 
Cs results were within 2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.
O(
He,
)F reaction; Identification of the low-energy "super" -Gamow-Teller stateFujita, Hirohiko*; Fujita, Yoshitaka*; Utsuno, Yutaka; Yoshida, Kenichi*; Adachi, Tatsuya*; Algora, A.*; Csatl
s, M.*; Deaven, J. M.*; Estevez-Aguado, E.*; Guess, C. J.*; et al.
Physical Review C, 100(3), p.034618_1 - 034618_13, 2019/09
Times Cited Count：12 Percentile：76.6(Physics, Nuclear)no abstracts in English
Yamano, Hidemasa; Takai, Toshihide; Furukawa, Tomohiro; Kikuchi, Shin; Emura, Yuki; Kamiyama, Kenji; Fukuyama, Hiroyuki*; Higashi, Hideo*; Nishi, Tsuyoshi*; Ota, Hiromichi*; et al.
Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.418 - 427, 2019/09
Eutectic reactions between boron carbide (BC) and stainless steel (SS) as well as its relocation are one of the key issues in a core disruptive accident (CDA) evaluation in sodium-cooled fast reactors. Since such behaviors have never been simulated in CDA numerical analyses, it is necessary to develop a physical model and incorporate the model into the CDA analysis code. This study is focusing on BC-SS eutectic melting experiments, thermophysical property measurement of the eutectic melt, and physical model development for the eutectic melting reaction. The eutectic experiments involve the visualization experiments, eutectic reaction rate experiments and material analyses. The thermophysical properties are measured in the range from solid to liquid state. The physical model is developed for a severe accident computer code based on the measured data of the eutectic reaction rate and the physical properties. This paper describes the project overview and progress of experimental and analytical studies by 2017. Specific results in this paper is boron concentration distributions of solidified BC-SS eutectic sample in the eutectic melting experiments, which would be used for the validation of the eutectic physical model implemented into the computer code.
Arai, Yoichi; Watanabe, So; Ono, Shimpei; Nakamura, Masahiro; Shibata, Atsuhiro; Nakamura, Fumiya*; Arai, Tsuyoshi*; Seko, Noriaki*; Hoshina, Hiroyuki*; Hagura, Naoto*; et al.
International Journal of PIXE, 29(1&2), p.17 - 31, 2019/00
The spent PUREX solvent containing U and Pu is generated from the reprocessing process of spent nuclear fuel. The nuclear material removal is important for the safe storage or disposal of the spent solvent. Our previous study revealed that the adsorbent with the iminodiacetic acid (IDA) functional group is one of the most promising materials for designing the nuclear material recovery process. Accordingly, an IDA-type adsorbent was synthesized by using graft polymerization technology or a chemical reaction to improve the adsorption rate and capacity. The synthesized IDA-type adsorbent was characterized by micro particle-induced X-ray emission (PIXE) and extended X-ray absorption fine structure (EXAFS) analyses. The micro-PIXE analysis revealed that Zr was adsorbed on the whole synthesized adsorbents and quantified the microamount of adsorbed Zr. Moreover, EXAFS suggested that Zr in the aqueous solution and solvent can be trapped by the IDA group with different mechanisms.
