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Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Journal of Neutron Research, 26(2-3), p.69 - 74, 2024/09
Slow neutrons, such as cold neutrons, are important non-destructive probes not only for basic physics but also for the structural genomics advancements in the life sciences and the battery technology advancements needed for the transition to a hydrogen society. Neutron-based science is also known as high-neutron-intensity-dependent science. A new unique method focusing on nanosized particle aggregation has been proposed to increase neutron intensity in that energy region. The method is based on intensity enhancement by multiple coherent scatterings with nanosized particle aggregation. The aggregation of nanosized particles matches the wavelength of below cold neutrons, causing a similar effect to coherent scattering, so-called Bragg scattering, leading to neutron intensity enhancement by several orders of magnitude. Nanodiamonds and magnesium hydride have recently been studied numerically and experimentally. The major challenge with nanodiamonds in practical applications is the molding method. Another carbon structure, graphene is focused on to find a solution to this problem. It is hypothesized that nanosized graphene could aid coherent neutron scattering under particle size conditions similar to nanodiamonds. We report the potential of nanosized graphene as a reflector material below cold neutrons, together with experimental results.
Teshigawara, Makoto; Ikeda, Yujiro*; Yan, M.*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*
Nanomaterials (Internet), 13(1), p.76_1 - 76_9, 2023/01
Times Cited Count:4 Percentile:50.15(Chemistry, Multidisciplinary)To enhance neutron intensity below cold neutrons, it is proposed that nanosized graphene aggregation could facilitate neutron coherent scattering under particle size conditions similar to nanodiamond. It might also be possible to use it in high neutron radiation conditions due to graphene's strong sp2 bonds. Using the RIKEN accelerator-driven compact neutron source and iMATERIA at J-PARC, we performed neutron measurement experiments, total neutron cross-section, and small-angle neutron scattering on nanosized graphene aggregation. The measured data revealed, for the first time, that nanosized graphene aggregation increased the total cross-sections and small-angle scattering in the cold neutron energy region, most likely due to coherent scattering, resulting in higher neutron intensities, similar to nanodiamond.
Iwamoto, Chihiro*; Takamura, Masato*; Ueno, Kota*; Kataoka, Minami*; Kurihara, Ryo*; Xu, P. G.; Otake, Yoshie*
ISIJ International, 62(5), p.1013 - 1022, 2022/05
Times Cited Count:3 Percentile:23.47(Metallurgy & Metallurgical Engineering)Xu, P. G.; Takamura, Masato*; Iwamoto, Chihiro*; Hakoyama, Tomoyuki*; Otake, Yoshie*; Suzuki, Hiroshi
Isotope News, (774), p.7 - 10, 2021/04
no abstracts in English
Ma, B.*; Teshigawara, Makoto; Wakabayashi, Yasuo*; Yan, M.*; Hashiguchi, Takao*; Yamagata, Yutaka*; Wang, S.*; Ikeda, Yujiro*; Otake, Yoshie*
Nuclear Instruments and Methods in Physics Research A, 995, p.165079_1 - 165079_7, 2021/04
Times Cited Count:2 Percentile:25.50(Instruments & Instrumentation)We have optimized a cold neutron moderator to be operated at the RIKEN accelerator-driven compact neutron source. We selected a safe and easy to manage material, mesitylene, as the RANS cold moderator. An efficient moderator system was designed by studying and optimizing a coupled cold neutron moderator of mesitylene at 20 K with a polyethylene (PE) pre-moderator at room temperature in the slab geometry with Particle and Heavy Ion Transport code System (PHITS) simulations. The parameters of mesitylene and PE thickness, the reflector, and the shielding configuration were studied to increase cold neutron intensities. Consequently, an integrated cold neutron intensity of 1.1510
n/cm
/
A at 2 m from the neutron-producing target was finally achieved, which was 12 times higher than that of the current PE moderator. The results showed attractive application prospect of mesitylene as cold neutron moderator material.
Xu, P. G.; Ikeda, Yoshimasa*; Hakoyama, Tomoyuki*; Takamura, Masato*; Otake, Yoshie*; Suzuki, Hiroshi
Journal of Applied Crystallography, 53(2), p.444 - 454, 2020/04
Times Cited Count:10 Percentile:69.52(Chemistry, Multidisciplinary)Kumagai, Masayoshi*; Uchida, Tomohiro*; Murasawa, Kodai*; Takamura, Masato*; Ikeda, Yoshimasa*; Suzuki, Hiroshi; Otake, Yoshie*; Hama, Takayuki*; Suzuki, Shinsuke*
Materials Research Proceedings, Vol.6, p.57 - 62, 2018/10
Times Cited Count:0 Percentile:0.00(Metallurgy & Metallurgical Engineering)Murasawa, Kodai*; Takamura, Masato*; Kumagai, Masayoshi*; Ikeda, Yoshimasa*; Suzuki, Hiroshi; Otake, Yoshie*; Hama, Takayuki*; Suzuki, Shinsuke*
Materials Transactions, 59(7), p.1135 - 1141, 2018/07
Times Cited Count:10 Percentile:38.70(Materials Science, Multidisciplinary)Ikeda, Yoshimasa*; Takamura, Masato*; Hakoyama, Tomoyuki*; Otake, Yoshie*; Kumagai, Masayoshi*; Suzuki, Hiroshi
Tetsu To Hagane, 104(3), p.138 - 144, 2018/03
Times Cited Count:5 Percentile:23.65(Metallurgy & Metallurgical Engineering)Neutron engineering diffraction is a powerful technique which provides the information of the micro structure of steels in bulk-average, while X-ray diffraction or Electron backscatter diffraction can provide information only from the surface layer. However, such measurement using neutron diffraction is typically performed in a large facility such as a reactor and a synchrotron, while a compact neutron source has never been used for this purpose. Authors have recently developed a neutron diffractometer installed in Riken Accelerator driven compact Neutron Source (RANS) and succeeded in the measurement of texture evolution of a steel sheet. In this study, we made an attempt to measure the volume fraction of retained austenite by RANS. Background noise was carefully eliminated in order to detect as many diffraction peaks as possible with low flux neutrons. The volume fraction was estimated by Rietveld analysis. The accuracy of the measurement result was discussed by comparing with those obtained by a large neutron facility (J-PARC TAKUMI). The volume fraction obtained by RANS with reasonable measurement time, i.e. 30 to 300 min, showed only 1 to 2 % discrepancies with those obtained in J-PARC. These comparisons suggest that neutron diffraction by RANS is capable of quantitative analysis of the volume fraction of crystal phases, showing the possibility of practical use of an in-house compact neutron source in the industry.
Seki, Yoshichika; Shinohara, Takenao; Parker, J. D.*; Yashiro, Wataru*; Momose, Atsushi*; Kato, Kosuke*; Kato, Hidemi*; Sadeghilaridjani, M.*; Otake, Yoshie*; Kiyanagi, Yoshiaki*
Journal of the Physical Society of Japan, 86(4), p.044001_1 - 044001_5, 2017/03
Times Cited Count:14 Percentile:64.96(Physics, Multidisciplinary)For the effective phase imaging at pulsed neutron sources, we have designed and developed the multi-colored Talbot-Lau interferometer which works at several wavelengths. At the Energy Resolved Neutron Imaging System RADEN in J-PARC, we demonstrated its operation by observing the visibilities of moire fringes derived from different wavelengths (0.25, 0.50, and 0.75 nm). We also investigated the variation of moire fringes dependent on the wavelength resolution from 18% to 50% and showed the advantage of pulsed beams. At the central wavelength of 0.5 nm, we have succeeded in interferometric imaging for the samples of metal rods made of aluminum, lead, and copper. An absorption grating as an analyzer was fabricated by imprinting of metallic glass for the first time, and showed a clear moire fringe with the high visibility of 68% and a well-controlled shape in comparison with previous ones fabricated by oblique evaporation of gadolinium.
Ikeda, Yoshimasa*; Taketani, Atsushi*; Takamura, Masato*; Sunaga, Hideyuki*; Kumagai, Masayoshi*; Oba, Yojiro*; Otake, Yoshie*; Suzuki, Hiroshi
Nuclear Instruments and Methods in Physics Research A, 833, p.61 - 67, 2016/10
Times Cited Count:41 Percentile:96.16(Instruments & Instrumentation)A compact accelerator-based neutron source has been lately discussed on engineering applications such as transmission imaging and small angle scattering as well as reflectometry. However, nobody considers using it for neutron diffraction experiment because of its low neutron flux. In this study, therefore, the neutron diffraction experiments are carried out using Riken Accelerator-driven Compact Neutron Source (RANS), to clarify the capability of the compact neutron source for neutron engineering diffraction. The diffraction pattern from a ferritic steel was successfully measured by suitable arrangement of the optical system to reduce the background noise, and it was confirmed that the recognizable diffraction pattern can be measured by the large sampling volume with 10 mm in cubic for an acceptable measurement time, i.e. 10 minutes. The minimum resolution of the 110 reflection for RANS is approximately 2.5 % at 8 s of the proton pulse width, which is insufficient to perform the strain measurement by neutron diffraction. The moderation time width at the wavelength corresponding to the 110 reflection is estimated to be approximately 30
s, which is the most dominant factor to determine the resolution. Therefore, refinements of the moderator system to decrease the moderation time are important to improve the resolution of the diffraction experiment using the compact neutron source. In contrast, the texture evolution due to plastic deformation was successfully observed by measuring a change in the diffraction peak intensity by RANS. Furthermore, the volume fraction of the austenite phase was also successfully evaluated by fitting the diffraction pattern using a Rietveld code. Consequently, RANS was proved to be capable for neutron engineering diffraction aiming for the easy access measurement of the texture and the amount of retained austenite.
Sunaga, Hideyuki*; Takamura, Masato*; Ikeda, Yoshimasa*; Otake, Yoshie*; Hama, Takayuki*; Kumagai, Masayoshi*; Suzuki, Hiroshi; Suzuki, Shinsuke*
Journal of Physics; Conference Series, 734(Part B), p.032027_1 - 032027_4, 2016/09
Times Cited Count:0 Percentile:0.00(Physics, Applied)A neutron diffraction measurement was performed to reveal microstructural aspects of the ductile fracture in ferritic steel. The diffraction patterns were continuously measured at the center of the reduced area while a tensile specimen was loaded under tension until the end of the fracture process. The measurement results showed that the volume fraction of (110)-oriented grains increased when the texture evolved as a result of plastic deformation. But the mechanism of texture evolution may be changed during necking, decreasing an increase rate of the volume fraction.
Takamura, Masato*; Ikeda, Yoshimasa*; Sunaga, Hideyuki*; Taketani, Atsushi*; Otake, Yoshie*; Suzuki, Hiroshi; Kumagai, Masayoshi*; Hama, Takayuki*; Oba, Yojiro*
Journal of Physics; Conference Series, 734(Part B), p.032047_1 - 032047_4, 2016/08
Times Cited Count:5 Percentile:84.66(Physics, Applied)Neutron diffraction is well known to be a useful technique for measuring a bulk texture of metallic materials taking advantage of a large penetration depth of the neutron beam. However, this technique has not been widely utilized for the texture measurement because large facilities like a reactor or a large accelerator are required in general. In contrast, RANS (Riken Accelerator-driven Compact Neutron Source) has been developed as a neutron source which can be used easily in laboratories. In this study, texture evolution in steel sheets with plastic deformation was successfully measured using RANS. The results show the capability of the compact neutron source for the analysis of the crystal structure of metallic materials, which leads us to a better understanding of plastic deformation behavior.
Uesaka, Mitsuru*; Kobayashi, Hitoshi*; Kureta, Masatoshi; Nakatsuka, Shigehiro*; Nishimura, Kazuya*; Igashira, Masayuki*; Hori, Junichi*; Kiyanagi, Yoshiaki*; Tagi, Kazuhiro*; Seki, Toshichika*; et al.
Reviews of Accelerator Science and Technology, 8, p.181 - 207, 2015/00
We choose nuclear data and nuclear material inspection for energy application and nondestructive testing of explosive and hidden nuclear materials for security application. 90 keV electrostatic accelerators of deuterium are commercially available for nondestructive testing. For nuclear data measurement, electrostatic ion accelerators and L-band and S-band electron linear accelerators (linac) are used for the neutron source. Compact or mobile X-band electron linac neutron sources are under development. Compact proton linac neutron source is used for nondestructive testing especially water in solids. Several efforts for more neutron intensity using proton and deuteron accelerators are also introduced.
Mishima, Kenji*; Ino, Takashi*; Sakai, Kenji; Shinohara, Takenao; Hirota, Katsuya*; Ikeda, Kazuaki*; Sato, Hiromi*; Otake, Yoshie*; Omori, Hitoshi*; Muto, Suguru*; et al.
Nuclear Instruments and Methods in Physics Research A, 600, p.342 - 345, 2009/02
Times Cited Count:32 Percentile:87.48(Instruments & Instrumentation)A new beamline for a fundamental physics experiment is under construction at BL05 port in the Materials and Life Science Facility (MLF) at Japan Proton Accelerator Research Complex (J-PARC), this beamline is designed using novel techniques of neutron optics and it is termed "Neutron Optics and Physics". The beam from the moderator is deflected by multi-channel supermirrors and split into three branches for individual experiments. In this study, we have optimized the design of the beam optics and shields using the Monte Carlo simulation package PHITS. The neutron fluxes of beams are expected to be cm
str
s
MW,
cm
s
MW,
cm
s
MW, with polarization of 99.8%.
Xu, P. G.; Takamura, Masato*; Ikeda, Yoshimasa*; Kakuta, Ryunosuke*; Iwamoto, Chihiro*; Hakoyama, Tomoyuki*; Otake, Yoshie*; Suzuki, Hiroshi
no journal, ,
Takamura, Masato*; Iwamoto, Chihiro*; Xu, P. G.; Ueno, Kota*; Kurihara, Ryo*; Suzuki, Hiroshi; Otake, Yoshie*
no journal, ,
Iwamoto, Chihiro*; Takamura, Masato*; Ueno, Kota*; Kurihara, Ryo*; Xu, P. G.; Suzuki, Hiroshi; Otake, Yoshie*
no journal, ,
no abstracts in English
Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; Otake, Yoshie*
no journal, ,
Science using neutrons in the nanometer (nm) wavelength region as probes is expanding into a wide range of fields, from basic research in materials and life science to industrial applications. Dramatic increase in the intensity of the beam source is required to drive such research. To increase the intensity of neutron beams, we have focused on coherent scattering caused by nano-sized particle aggregations. We focused on graphene, which is different from nanodiamond that has been vigorously researched and developed, and started to develop its nano-sized aggregates, which have high van der Waals force of more than one order of magnitude and stronger bonding force between carbons than nanodiamond, so that they can be easily formed into a lump shape and adapted to higher radiation fields. The graphene is expected to be formable into clumps and adaptable to higher radiation fields. By promoting chemical vapor deposition (CVD), we have established a technique to form nano-sized graphene (graphene flower) with a shape similar to a sunflower flower. In this talk, we report on the neutron scattering characteristics that contribute to the coherent scattering of the newly developed graphene flowers.
Muramatsu, Kazuo*; Sutani, Koichi*; Kimishima, Koichi*; Teshigawara, Makoto; Ikeda, Yujiro*; Fukuzumi, Masafumi*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; Otake, Yoshie*
no journal, ,
The use of nano-diamonds has been vigorously investigated to increase the intensity of neutron beams, focusing on the coherent scattering caused by nano-sized particle aggregations. Sp2 intercarbon-bonded graphene has a larger van der Waals force than sp3 intercarbon-bonded nano-diamonds. It is expected to be more easily formed into a lump shape and adaptability to higher radiation fields. On the other hand, the large cohesive nature of graphene makes it difficult to construct nano-sized three-dimensional structures. To solve this problem, we focused on the Hot Isostatic Pressing (HIP) method, which uses resin powder as a raw material and produces vapor-phase grown graphene. In this talk, we will report on the preparation of graphene flower structures, in which nano-sized graphene is three-dimensionally freestanding, how to control the nano-size of graphene, and a prototype of graphene neutron reflector material.