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Journal Articles

Development of nanosized graphene material for neutron intensity enhancement below cold neutron energy

Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*

Journal of Neutron Research, 26(2-3), p.69 - 74, 2024/09

Slow neutrons, such as cold neutrons, are important non-destructive probes not only for basic physics but also for the structural genomics advancements in the life sciences and the battery technology advancements needed for the transition to a hydrogen society. Neutron-based science is also known as high-neutron-intensity-dependent science. A new unique method focusing on nanosized particle aggregation has been proposed to increase neutron intensity in that energy region. The method is based on intensity enhancement by multiple coherent scatterings with nanosized particle aggregation. The aggregation of nanosized particles matches the wavelength of below cold neutrons, causing a similar effect to coherent scattering, so-called Bragg scattering, leading to neutron intensity enhancement by several orders of magnitude. Nanodiamonds and magnesium hydride have recently been studied numerically and experimentally. The major challenge with nanodiamonds in practical applications is the molding method. Another carbon structure, graphene is focused on to find a solution to this problem. It is hypothesized that nanosized graphene could aid coherent neutron scattering under particle size conditions similar to nanodiamonds. We report the potential of nanosized graphene as a reflector material below cold neutrons, together with experimental results.

Journal Articles

New material exploration to enhance neutron intensity below cold neutrons; Nanosized graphene flower aggregation

Teshigawara, Makoto; Ikeda, Yujiro*; Yan, M.*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Saruta, Koichi; Otake, Yoshie*

Nanomaterials (Internet), 13(1), p.76_1 - 76_9, 2023/01

 Times Cited Count:4 Percentile:47.87(Chemistry, Multidisciplinary)

To enhance neutron intensity below cold neutrons, it is proposed that nanosized graphene aggregation could facilitate neutron coherent scattering under particle size conditions similar to nanodiamond. It might also be possible to use it in high neutron radiation conditions due to graphene's strong sp2 bonds. Using the RIKEN accelerator-driven compact neutron source and iMATERIA at J-PARC, we performed neutron measurement experiments, total neutron cross-section, and small-angle neutron scattering on nanosized graphene aggregation. The measured data revealed, for the first time, that nanosized graphene aggregation increased the total cross-sections and small-angle scattering in the cold neutron energy region, most likely due to coherent scattering, resulting in higher neutron intensities, similar to nanodiamond.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Optimization of a slab geometry type cold neutron moderator for RIKEN accelerator-driven compact neutron source

Ma, B.*; Teshigawara, Makoto; Wakabayashi, Yasuo*; Yan, M.*; Hashiguchi, Takao*; Yamagata, Yutaka*; Wang, S.*; Ikeda, Yujiro*; Otake, Yoshie*

Nuclear Instruments and Methods in Physics Research A, 995, p.165079_1 - 165079_7, 2021/04

 Times Cited Count:2 Percentile:24.88(Instruments & Instrumentation)

We have optimized a cold neutron moderator to be operated at the RIKEN accelerator-driven compact neutron source. We selected a safe and easy to manage material, mesitylene, as the RANS cold moderator. An efficient moderator system was designed by studying and optimizing a coupled cold neutron moderator of mesitylene at 20 K with a polyethylene (PE) pre-moderator at room temperature in the slab geometry with Particle and Heavy Ion Transport code System (PHITS) simulations. The parameters of mesitylene and PE thickness, the reflector, and the shielding configuration were studied to increase cold neutron intensities. Consequently, an integrated cold neutron intensity of 1.15$$times$$10$$^{3}$$n/cm$$^{2}$$/$$mu$$A at 2 m from the neutron-producing target was finally achieved, which was 12 times higher than that of the current PE moderator. The results showed attractive application prospect of mesitylene as cold neutron moderator material.

Journal Articles

Enhancement of critical current densities in (Ba,K)Fe$$_{2}$$As$$_{2}$$ by 320 MeV Au irradiation in single crystals and by high-pressure sintering in powder-in-tube wires

Pyon, S.*; Taen, Toshihiro*; Otake, Fumiaki*; Tsuchiya, Yuji*; Inoue, Hiroshi*; Akiyama, Hiroki*; Kajitani, Hideki; Koizumi, Norikiyo; Okayasu, Satoru; Tamegai, Tsuyoshi*

Applied Physics Express, 6(12), p.123101_1 - 123101_4, 2013/12

 Times Cited Count:22 Percentile:64.22(Physics, Applied)

We demonstrate a large enhancement of critical current density ($$J$$$$_{rm c}$$) up to 1.0 $$times$$ 10$$^{7}$$ A/cm$$^{2}$$ at 5 K under self-field in (Ba,K)Fe$$_{2}$$As$$_{2}$$ single crystals by irradiating 320 MeV Au ions. With the very promising potential of this material in mind, we have fabricated a (Ba,K)Fe$$_{2}$$As$$_{2}$$ superconducting wire through a powder-in-tube method combined with the hot isostatic pressing technique, whose effectiveness has been proven in industrial Bi2223 tapes. The Jc in the wire at 4.2 K has reached 37 kA/cm$$^{2}$$ under self-field and 3.0 kA/cm$$^{2}$$ at 90 kOe. Magneto-optical imaging of the wire confirmed the large intergranular Jc in the wire core.

Journal Articles

Full-coherent free electron laser seeded by 13th- and 15th-order harmonics of near-infrared femtosecond laser pulses

Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Togashi, Tadashi*; Fukami, Kenji*; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 46(16), p.164006_1 - 164006_6, 2013/08

 Times Cited Count:3 Percentile:18.14(Optics)

By introducing 13th- (61.7 nm) and 15th-order harmonics (53.4 nm) of femtosecond laser pulses at 800 nm into an undulator of SCSS (SPring-8 Compact SASE Source) test accelerator at RIKEN, these harmonic pulses were amplified by a factor of more than 10$$^{2}$$ with a high contrast ratio through the interaction between accelerated electron bunches and the harmonic pulses. From numerical simulations of the amplification processes of high-order harmonic pulses in the undulator, optimum conditions of the electron bunch duration interacting with the high-order harmonic pulses were investigated for generating full-coherent and intense pulses in the extreme ultraviolet wavelength region.

Journal Articles

Full-coherent HHG-seeded EUV-FEL locked by EOS timing feedback

Ogawa, Kanade*; Sato, Takahiro*; Matsubara, Shinichi*; Okayasu, Yuichi*; Togashi, Tadashi*; Watanabe, Takahiro*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; et al.

Proceedings of 10th Conference on Lasers and Electro-Optics Pacific Rim and 18th OptoElectronics and Communications Conference and Photonics in Switching 2013 (CLEO-PR & OECC/PS 2013) (USB Flash Drive), 2 Pages, 2013/06

no abstracts in English

Journal Articles

High intense full-coherent radiation of free electron laser seeded by high-order harmonics in extreme-ultraviolet region

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of Ultrafast Optics IX (CD-ROM), 2 Pages, 2013/03

We have demonstrated free-electron laser radiation seeded by high-order harmonics in the extreme-ultraviolet region. Strong enhancement of the radiation intensity by a factor of 104 was observed with timing control of an electro-optical sampling technique.

Journal Articles

Extreme ultraviolet free electron laser seeded by high-order harmonic

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of 11th International School and Symposium on Synchrotron Radiation in Natural Science (ISSRNS 2012), p.1 - 21, 2012/05

The 13th harmonic of a Ti:sapphire laser has been significantly amplified with the SCSS test accelerator. The temporal and spatial overlap of the electron beam and the high harmonic radiation were precisely tuned for achieving the seeded free electron laser operation. With numerical simulation the present HH-seeded FEL scheme could readily be applied to the wavelength region down to 10 nm.

Journal Articles

A Preliminary assessment of the adoption of innovative technologies in the Fast Reactor Cycle Technology Development (FaCT) project in Japan

Sato, Koji; Kotake, Shoji; Fujita, Yuji; Mizuno, Tomoyasu

Energy Procedia, 7, p.140 - 145, 2011/09

 Times Cited Count:4 Percentile:90.70(Nuclear Science & Technology)

JAEA has been implementing the FaCT project in cooperation with electric utilities toward the commercialization of fast reactor cycle system before 2050. In this FaCT project, many innovative technologies with technical challenges are actively used in order to provide significant improvements in economic competitiveness, enhancement of safety and reliability, sustainability, and nonproliferation. The work of deciding on the adoption of innovative technologies by the end of JFY2010 is in progress. This paper describes current preliminary assessment results.

Journal Articles

Seeding of extreme ultraviolet free electron laser with high-order harmonic

Takahashi, Eiji*; Togashi, Tadashi*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of European Conference on Lasers and Electro-Optics and the 12th European Quantum Electronics Conference (CLEO/Europe-EQEC 2011) (CD-ROM), 1 Pages, 2011/05

We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.

Journal Articles

EUV-FEL seeded by high-order harmonic

Takahashi, Eiji*; Togashi, Tadashi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; Matsubara, Shinichi*; et al.

Proceedings of International Quantum Electronics Conference and the Pacific Rim Conference on Lasers and Electro-Optics (IQEC/CLEO Pacific Rim 2011) (CD-ROM), p.199 - 200, 2011/05

We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.

Journal Articles

Extreme ultraviolet free electron laser seeded with high-order harmonic of Ti:sapphore laser

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Okino, Tomoya*; Yamanouchi, Kaoru*; et al.

Optics Express (Internet), 19(1), p.317 - 324, 2011/01

 Times Cited Count:97 Percentile:96.04(Optics)

The 13th harmonic of a Ti:sapphire (Ti:S) laser in the plateau region was injected as a seeding source to a 250-MeV free-electron-laser (FEL) amplifier. When the amplification conditions were fulfilled, strong enhancement of the radiation intensity by a factor of 650 was observed. The random and uncontrollable spikes, which appeared in the spectra of the Self-Amplified Spontaneous Emission (SASE) based FEL radiation without the seeding source, were found to be suppressed drastically to form to a narrow-band, single peak profile at 61.2 nm. The properties of the seeded FEL radiation were well reproduced by numerical simulations. We discuss the future precept of the seeded FEL scheme to the shorter wavelength region.

Journal Articles

Target station design of 1 MW spallation neutron source at the high intensity proton accelerator facilities J-PARC

Takada, Hiroshi; Maekawa, Fujio; Honmura, Shiro*; Yoshida, Katsuhiko*; Teraoku, Takuji*; Meigo, Shinichiro; Sakai, Akio*; Kasugai, Yoshimi; Kanechika, Shuji*; Otake, Hidenori*; et al.

Proceedings of ICANS-XVI, Volume 3, p.1115 - 1125, 2003/07

no abstracts in English

Oral presentation

Development of neutron reflector material brought about by nano-sized flowers; Structural control of nano-sized graphene and application for neutron reflector

Muramatsu, Kazuo*; Sutani, Koichi*; Kimishima, Koichi*; Teshigawara, Makoto; Ikeda, Yujiro*; Fukuzumi, Masafumi*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; Otake, Yoshie*

no journal, , 

The use of nano-diamonds has been vigorously investigated to increase the intensity of neutron beams, focusing on the coherent scattering caused by nano-sized particle aggregations. Sp2 intercarbon-bonded graphene has a larger van der Waals force than sp3 intercarbon-bonded nano-diamonds. It is expected to be more easily formed into a lump shape and adaptability to higher radiation fields. On the other hand, the large cohesive nature of graphene makes it difficult to construct nano-sized three-dimensional structures. To solve this problem, we focused on the Hot Isostatic Pressing (HIP) method, which uses resin powder as a raw material and produces vapor-phase grown graphene. In this talk, we will report on the preparation of graphene flower structures, in which nano-sized graphene is three-dimensionally freestanding, how to control the nano-size of graphene, and a prototype of graphene neutron reflector material.

Oral presentation

Development of neutron reflector material brought about by nano-sized flowers; Intensify neutron beam caused by coherent scattering

Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; Otake, Yoshie*

no journal, , 

Science using neutrons in the nanometer (nm) wavelength region as probes is expanding into a wide range of fields, from basic research in materials and life science to industrial applications. Dramatic increase in the intensity of the beam source is required to drive such research. To increase the intensity of neutron beams, we have focused on coherent scattering caused by nano-sized particle aggregations. We focused on graphene, which is different from nanodiamond that has been vigorously researched and developed, and started to develop its nano-sized aggregates, which have high van der Waals force of more than one order of magnitude and stronger bonding force between carbons than nanodiamond, so that they can be easily formed into a lump shape and adapted to higher radiation fields. The graphene is expected to be formable into clumps and adaptable to higher radiation fields. By promoting chemical vapor deposition (CVD), we have established a technique to form nano-sized graphene (graphene flower) with a shape similar to a sunflower flower. In this talk, we report on the neutron scattering characteristics that contribute to the coherent scattering of the newly developed graphene flowers.

Oral presentation

Human resource development for radionuclide analysis in nuclear science research institute

Kitatsuji, Yoshihiro; Fukaya, Hiroyuki; Haraga, Tomoko; Oka, Toshitaka; Otake, Yoshinori; Tambo, Masaki; Inada, Arisa; Aono, Ryuji; Kinase, Akari; Ikarugi, Riko; et al.

no journal, , 

To proceed with the decommissioning of Fukushima Daiichi Nuclear Power Station Accident (1F), it is necessary to secure human resources for radionuclide analysis, which is a prerequisite for the safe treatment and disposal of treated water and waste containing radionuclides generated as a result of the decommissioning. The Nuclear Science Research Institute of JAEA, together with the Fukushima Research and Engineering Institute, has started a project to train analytical personnel who will be responsible for decommissioning in the future. In this presentation, we will introduce the training of analytical operators, managers, and engineers for young staff members and our efforts using the summer intern program.

Oral presentation

Sustained lasing of HHG-seeded FEL by using EOS-based timing control

Watanabe, Takahiro*; Aoyama, Makoto; Iwasaki, Atsushi*; Otake, Yuji*; Oshima, Takashi*; Okayasu, Yuichi*; Ogawa, Kanade*; Owada, Shigeki*; Sato, Takahiro*; Togashi, Tadashi*; et al.

no journal, , 

no abstracts in English

Oral presentation

Temporal overlapping for an HH seeded EUV-FEL operation by using EO-based timing-drift controlling system

Matsubara, Shinichi*; Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; et al.

no journal, , 

no abstracts in English

Oral presentation

None

Yanagisawa, Kayo; Ikarugi, Riko; Morii, Shiori; Oka, Toshitaka; Kitatsuji, Yoshihiro; Fukaya, Hiroyuki; Haraga, Tomoko; Otake, Yoshinori; Tambo, Masaki; Inada, Arisa; et al.

no journal, , 

no abstracts in English

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