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JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2022

Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Nagaoka, Mika; Koike, Yuko; Kubota, Tomohiro; Hirao, Moe; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; et al.

JAEA-Review 2023-052, 118 Pages, 2024/03

JAEA-Review-2023-052.pdf:3.67MB

Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2022. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2021

Nakada, Akira; Kanai, Katsuta; Kokubun, Yuji; Nagaoka, Mika; Koike, Yuko; Yamada, Ryohei*; Kubota, Tomohiro; Hirao, Moe; Yoshii, Hideki*; Otani, Kazunori*; et al.

JAEA-Review 2022-079, 116 Pages, 2023/03

JAEA-Review-2022-079.pdf:2.77MB

Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2021. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.

JAEA Reports

Annual report on the effluent control of low level liquid waste in Nuclear Fuel Cycle Engineering Laboratories FY2020

Nakano, Masanao; Nakada, Akira; Kanai, Katsuta; Nagaoka, Mika; Koike, Yuko; Yamada, Ryohei; Kubota, Tomohiro; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; et al.

JAEA-Review 2021-040, 118 Pages, 2021/12

JAEA-Review-2021-040.pdf:2.48MB

Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2020. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.

Journal Articles

Auger electron spectroscopic analysis of corrosion products formed on A3003 aluminum alloy in model fresh water with different Zn$$^{2+}$$ concentration

Otani, Kyohei; Islam, M. S.*; Sakairi, Masatoshi*; Kaneko, Akira*

Surface and Interface Analysis, 51(12), p.1207 - 1213, 2019/12

 Times Cited Count:1 Percentile:2.04(Chemistry, Physical)

The corrosion morphology and composition of corrosion products of A3003 formed in model fresh water with different Zn$$^{2+}$$ concentrations were investigated by immersion tests combined with surface observations and analysis using an auger electron spectroscope (AES). The cross-sectional AES observations showed that the thickness of the corrosion product layer formed on A3003 decreases with increases in the Zn$$^{2+}$$ concentration of the model fresh water. A cross-sectional AES point analysis suggested that the corrosion products formed on the A3003 in the Zn$$^{2+}$$ containing model fresh water (Zn$$^{2+}$$ $$>$$ 0.1 mM) have a multi-layer structure, and that the inner of Zn-rich layer would have high corrosion protective properties.

Journal Articles

Numerical and experimental study of H$$^{-}$$ beam dynamics in J-PARC LEBT

Shibata, Takanori*; Ikegami, Kiyoshi*; Liu, Y.*; Miura, Akihiko; Naito, Fujio*; Nammo, Kesao*; Oguri, Hidetomo; Okoshi, Kiyonori; Otani, Masashi*; Shinto, Katsuhiro; et al.

Proceedings of 29th International Linear Accelerator Conference (LINAC 2018) (Internet), p.519 - 521, 2019/01

Transport process of negative hydrogen ion (H$$^{-}$$) in LEBT (Low Energy Beam Transport) is investigated by comparison of experimental and numerical results. A three dimensional Particle-In-Cell (PIC) particle transport model has been developed in order to take into account (i) axial magnetic field by two solenoids in J-PARC LEBT and (ii) radial electric field by space charge (SC) effect. Ratio of H$$^-$$ beam particles inside the RFQ (Radio Frequency Quadrupole) acceptance to the total particles at the RFQ entrance is calculated for different current conditions in LEBT solenoid 1 and 2. The results are compared with RFQ transmission rate measured in the J-PARC linac commissioning. The double peak of RFQ transmission rate to the solenoid applied current seen in the measurement is explained by the calculation results. The results indicate that presence of the LEBT orifice for differential pumping plays a role as a collimator to reduce emittance at RFQ entrance.

Journal Articles

Local structure study of the iron-based systems of BaFe$$_2$$As$$_2$$ and LiFeAs by X-ray PDF and XAFS analyses

Li, S.*; Toyoda, Masayuki*; Kobayashi, Yoshiaki*; Ito, Masayuki*; Ikeuchi, Kazuhiko*; Yoneda, Yasuhiro; Otani, Akira*; Matsumura, Daiju; Asano, Shun*; Mizuki, Junichiro*; et al.

Physica C, 555, p.45 - 53, 2018/12

 Times Cited Count:1 Percentile:5.02(Physics, Applied)

${it T}$-dependence of local distortions in BaFe$$_2$$As$$_2$$ and LiFeAs by X-ray PDF and XAFS methods. Although PDF data exhibit anomaly at the structure transition temperature, EXAFS data exhibit no anomaly. Data supporting the local orthorhombicity at 300 K in the tetragonal phase for BaFe$$_2$$As$$_2$$. Arguments on the origins of the 4-fold symmetry breaking in the ground average structure of the tetragonal phase.

Journal Articles

Crack formation in cementitious materials used for an engineering barrier system and their impact on hydraulic conductivity from the viewpoint of performance assessment of a TRU Waste disposal system

Hirano, Fumio; Otani, Yoshiteru*; Kyokawa, Hiroyuki*; Mihara, Morihiro; Shimizu, Hiroyuki*; Honda, Akira

Nihon Genshiryoku Gakkai Wabun Rombunshi, 15(2), p.97 - 114, 2016/06

A mechanical analysis code MACBECE2014 has been developed at the Japan Atomic Energy Agency to make realistic simulations of the physical integrity of the near-field for performance assessment of geological disposal of TRU waste in Japan. The MACBECE2014 code can be used to evaluate long-term changes in the mechanical behavior and any subsequent changes in the permeability of engineering barrier components, including crack formation in cementitious materials caused by expansion due to metal corrosion. Simulated results of the TRU waste disposal system with a bentonite buffer using the MACBECE2014 code demonstrated that the low permeability of the engineering barrier system could be maintained for long time periods after disposal because the physical integrity of the bentonite buffer remained intact. Simulated results of the disposal system with a concrete backfill, showed that crack formation leads to a significant increase in permeability of the system.

Journal Articles

Proton-exchange mechanism of specific Cs$$^{+}$$ adsorption $$via$$ lattice defect sites of Prussian blue filled with coordination and crystallization water molecules

Ishizaki, Manabu*; Akiba, Sae*; Otani, Asako*; Hoshi, Yuji*; Ono, Kenta*; Matsuba, Mayu*; Togashi, Takanari*; Kanaizuka, Katsuhiko*; Sakamoto, Masatomi*; Takahashi, Akira*; et al.

Dalton Transactions, 42(45), p.16049 - 16055, 2013/12

 Times Cited Count:178 Percentile:99.58(Chemistry, Inorganic & Nuclear)

We have revealed the fundamental mechanism of specific Cs$$^{+}$$ adsorption into Prussian blue (PB) in order to develop high-performance PB-based Cs$$^{+}$$ adsorbents in the wake of the Fukushima nuclear accident. We compared two types of PB nanoparticles with formulae of Fe$$^{III}$$$$_{4}$$[Fe$$^{II}$$(CN)$$_{6}$$]3$$cdot$$xH$$_{2}$$O (x = 10-15) (PB-1) and (NH$$_{4}$$)0.70Fe$$^{III}$$1.10[Fe$$^{II}$$(CN)$$_{6}$$]$$cdot$$1.7H$$_{2}$$O (PB-2) with respect to the Cs$$^{+}$$ adsorption ability. The synthesised PB-1, by a common stoichiometric aqueous reaction between 4Fe$$^{3+}$$ and 3[Fe$$^{II}$$(CN)$$_{6}$$]$$^{4-}$$, showed much more efficient Cs$$^{+}$$ adsorption ability than did the commercially available PB-2.

Journal Articles

Japanese FR deployment scenario study after the Fukushima accident

Ono, Kiyoshi; Shiotani, Hiroki; Ohtaki, Akira; Mukaida, Kyoko; Abe, Tomoyuki

Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Safe Technologies and Sustainable Scenarios (FR-13) (USB Flash Drive), 10 Pages, 2013/03

In parallel to the mid-term analyses by the AEC after the Fukushima-accident, JAEA implemented the long-term scenario analyses for the nuclear fuel cycle options including FR cycle deployment. As a result, it was revealed that FR cycle deployment brings great benefits to reduction of uranium demand, spent fuel storage, radioactive waste generation, and Pu stockpiles in addition to potential hazard of HLW in "20 GWe constant after 2030" case. Meanwhile, it was also revealed the benefits of reduction of radioactive waste generation and Pu stockpiles in "Gradual decrease from 20 GWe after 2030" case.

JAEA Reports

Document collection of the 24th Technical Special Committee on Fugen Decommissioning

Otani, Hiroshi; Matsushima, Akira; Mori, Naoto; Kutsuna, Hideki; Higashiura, Norikazu

JAEA-Review 2011-041, 55 Pages, 2012/01

JAEA-Review-2011-041.pdf:6.08MB

In planning and carrying out decommissioning technical development of Fugen, "Technical special committee on Fugen decommissioning", which consists of the members well-informed, is established, aiming to make good use of Fugen as a place for technological development which is opened inside and outside the country, as the central point in the energy research and development base making project of Fukui prefecture, and to utilize the outcome in our decommissioning to the technical development effectively. This report compiles presentation materials "Current Situation of Fugen Decommissioning", "Radioactive Corrosion Products Decontamination Experiment with using Heavy Water System Equipment", "Laser Cutting Test on Dust Behavior in Cutting Work in Air", "Preparatory Situation for Operation of Clearance System" of this committee.

Journal Articles

Angle-resolved photoemission spectroscopy study of PrFeAsO$$_{0.7}$$; Comparison with LaFePO

Nishi, Ichiro*; Ishikado, Motoyuki; Ideta, Shinichiro*; Malaeb, W.*; Yoshida, Teppei*; Fujimori, Atsushi*; Kotani, Yoshinori*; Kubota, Masato*; Ono, Kanta*; Yi, M.*; et al.

Physical Review B, 84(1), p.014504_1 - 014504_5, 2011/07

 Times Cited Count:22 Percentile:65.72(Materials Science, Multidisciplinary)

We have performed an angle-resolved photoemission spectroscopy (ARPES) study of the iron-based superconductor PrFeAsO$$_{0.7}$$ and examined the Fermi surfaces and band dispersions near the fermi level. Heavily hole-doped electronic states have been observed due to the polar nature of the cleaved surfaces. Nevertheless, we have found that the ARPES spectra basically agree with band dispersions calculated in the local density approximation (LDA) if the bandwidth is reduced by a factor of $$sim$$ 2.5 and then the chemical potential is lowered by $$sim$$ 70 meV. Comparison with previous ARPES results on LaFePO reveals that the energy positions of the $$d$$$$_{3z^{2}-r^{2}}$$- and $$d$$$$_{yz,zx}$$-derived bands are considerably different between the two materials, which we attribute to the different pnictogen height as predicted by the LDA calculation.

Journal Articles

XMCD spectroscopy on valence fluctuating and heavy fermion compounds in very high magnetic fields up to 40 T

Matsuda, Yasuhiro*; Her, J. L.*; Inami, Toshiya; Owada, Kenji; Ouyang, Z. W.*; Okada, Kyoko*; Nojiri, Hiroyuki*; Mitsuda, Akihiro*; Wada, Hirofumi*; Yoshimura, Kazuyoshi*; et al.

Journal of Physics; Conference Series, 190, p.012019_1 - 012019_6, 2009/11

 Times Cited Count:7 Percentile:85.24(Physics, Condensed Matter)

Journal Articles

Complementary spectroscopy of tin ions using ion and electron beams

Ohashi, Hayato*; Suda, Shintaro*; Tanuma, Hajime*; Fujioka, Shinsuke*; Nishimura, Hiroaki*; Nishihara, Katsunobu*; Kai, Takeshi; Sasaki, Akira; Sakaue, Hiroyuki*; Nakamura, Nobuyuki*; et al.

Journal of Physics; Conference Series, 163, p.012071_1 - 012071_4, 2009/06

 Times Cited Count:7 Percentile:89.27(Physics, Multidisciplinary)

Extreme ultra-violet (EUV) emission spectra of multiply charged tin ions were measured in the wavelength range of 10-22 nm following charge exchange collisions or the electron impact excitation of tin ions. In charge exchange collisions, we observed both the resonance lines and the emission lines corresponding to the transitions between the excited states. On the other hand, we observed mainly the resonance lines in the electron impact experiments. We can distinguish the resonance lines from other emission lines in the charge exchange spectrum by comparison with the emission lines in the electron impact spectrum.

JAEA Reports

Feasibility Study on Commercialization of Fast Breeder Reactor Cycle System Interim Report of Phase II -Technical Study Report on Synthetic Evaluation for FBR Cycle-

Shiotani, Hiroki; Ohtaki, Akira; Ono, Kiyoshi; Hirao, Kazunori; Kato, Atsushi; Yasumatsu, Naoto*; Kubota, Sadae*

JNC TN9400 2004-052, 514 Pages, 2004/09

JNC-TN9400-2004-052.pdf:8.85MB

This report presents the outline of the development and the results of characteristic evaluation on the candidate Fast Reactor (FR) cycle system concepts, scenario study on FR cycle deployment and cost-benefit analysis on the candidate FR cycle system concepts in the interim evaluation (FY2001 through FY2003) of the second phase of the Japanese "Feasibility Study on Commercialization of Fast Breeder Reactor Cycle System (FS)".

Journal Articles

Development of 10kA Bi2212 conductor for fusion application

Isono, Takaaki; Nunoya, Yoshihiko; Ando, Toshinari*; Okuno, Kiyoshi; Ono, Michitaka*; Ozaki, Akira*; Koizumi, Tsutomu*; Otani, Nozomu*; Hasegawa, Takayo*

IEEE Transactions on Applied Superconductivity, 13(2), p.1512 - 1515, 2003/06

 Times Cited Count:21 Percentile:67.71(Engineering, Electrical & Electronic)

Japan Atomic Energy Research Institute has started development work on a large current conductor using high Tc superconductor (HTS) aiming at a fusion power reactor after the International Thermonuclear Experimental Reactor (ITER). HTS has a capability to produce a magnetic field of higher than 16 T, which is required in such a fusion power reactor. A trial fabrication of a 10-kA 12-T conductor was started using round Ag-alloy sheathed Bi-2212 strands, which has best performance at 4.2K, 16T at present. The conductor has about 34-mm diameter, and is composed of 729 HTS strands. Operating temperature is designed at not only 4 K but also 20K. The conductor sample is indirectly cooled and is solder-coated on the surface to use specific heat of the lead as much as possible, which at 20 K is almost comparable with specific heat of SHe at 4.5K, 0.6MPa. From the tests of the conductor, the fabrication of large HTS conductor and 10kA operation at 12 T and about 12.5 K were successfully performed and the possibility of HTS to use fusion application was demonstrated.

Oral presentation

Development of eddy current testing technique for fast reactor fuel pins; ECT results of irradiated fuel pins

Miyaji, Noriko; Katsuyama, Kozo; Nagamine, Tsuyoshi; Nakamura, Yasuo; Otani, Akira*

no journal, , 

no abstracts in English

Oral presentation

Multidimensional evaluation of FR cycle systems in the Phase II of the feasibility study, 1; Evaluations of economics and efficient utilization of resource

Kato, Atsushi; Mukaida, Kyoko; Ohtaki, Akira; Shiotani, Hiroki; Ono, Kiyoshi; Yasumatsu, Naoto*; Kubota, Sadae*

no journal, , 

no abstracts in English

Oral presentation

Dynamic analysis of FR cycle systems, 1; Perspectives and environmental burden reduction

Shiotani, Hiroki; Heta, Masanori*; Ohtaki, Akira; Kubota, Sadae*; Kawasaki, Hirotsugu; Ono, Kiyoshi

no journal, , 

Methodologies for the dynamic analysis of nuclear energy system from current LWR cycle to FR cycle which will replace the LWR cycle system are developed in the "Feasibility Study on Commercialized Fast Raector cycle systems". The role and perspectives of the dynamic analysis are shown, and status and tentative results of the developmnent of the environmental burden reduction evaluation methodology are reported.

Oral presentation

Dissolution test on the sludge of the dissolver

Sugai, Eiji; Terunuma, Hirotaka; Otani, Takehisa; Hikita, Keiichi; Hatanaka, Akira; Samoto, Hirotaka; Okano, Masanori; Hayashi, Shinichiro

no journal, , 

A dissolution test of the sludge gathered from the dissolver of Tokai Reprocessing Plant (TRP) was performed for the purpose of eliminating of the sludge, which deposited in the dissolver and clogged pipes equipped in the dissolver. In the result, the sludge consisted primarily of ZrMo$$_{2}$$O$$_{7}$$(OH)$$_{2}$$(H$$_{2}$$O)$$_{2}$$ and was possible to eliminate at the rate of about 80% by using NaOH and HNO$$_{3}$$ reagent which was commonly-used in the PUREX process. From this experimental result, it is thought that the method of using NaOH and HNO$$_{3}$$ reagent is effective method for the elimination of the sludge which deposited in the dissolver.

Oral presentation

Replacement of butterfly valves installed in shearing off-gas treatment process of TRP, 2; Survey results of replaced valves

Sugai, Eiji; Kikuchi, Hideki; Hatanaka, Akira; Otani, Takehisa; Suzuki, Kazuyuki; Taguchi, Katsuya

no journal, , 

no abstracts in English

28 (Records 1-20 displayed on this page)