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Journal Articles

Field-tuned quantum renormalization of spin dynamics in the honeycomb lattice Heisenberg antiferromagnet YbCl$$_3$$

Sala, G.*; Stone, M. B.*; Hal$'a$sz, G. B.*; Lumsden, M. D.*; Fay, A, F,*; Pajerowski, D. M.*; Kawamura, Seiko; Kaneko, Koji; Mazzone, D. G.*; Simutis, G.*; et al.

Communications Physics (Internet), 6, p.234_1 - 234_7, 2023/08

Journal Articles

The $$f$$-electron state of the heavy fermion superconductor NpPd$$_5$$Al$$_2$$ and the isostructural family

Metoki, Naoto; Aczel, A. A.*; Aoki, Dai*; Chi, S.*; Fernandez-Baca, J. A.*; Griveau, J.-C.*; Hagihara, Masato*; Hong, T.*; Haga, Yoshinori; Ikeuchi, Kazuhiko*; et al.

JPS Conference Proceedings (Internet), 30, p.011123_1 - 011123_6, 2020/03

Rare earths (4$$f$$) and actinides (5$$f$$) provide variety of interesting states realized with competing interactions between the increasing number of $$f$$ electrons. Since crystal field splitting of many-body $$f$$ electron system is smaller than the bandwidth, (1) high resolution experiments are needed, (2) essentially no clear spectrum with well defined peaks is expected in itinerant Ce and U compounds, and (3) Np and Pu is strictly regulated. Therefore, systematic research on magnetic excitations by neutron scattering experiments of localized compounds and rare earth iso-structural reference is useful. We describe the $$f$$ electron states of heavy electron compounds NpPd$$_5$$Al$$_2$$ and actinide and rare earth based iso-structural family.

Journal Articles

$$f$$-electron states in PrPd$$_5$$Al$$_2$$

Metoki, Naoto; Yamauchi, Hiroki; Suzuki, Hiroyuki*; Kitazawa, Hideaki*; Hagihara, Masato*; Masuda, Takatsugu*; Aczel, A. A.*; Chi, S.*; Hong, T.*; Matsuda, Masaaki*; et al.

Journal of the Physical Society of Japan, 87(9), p.094704_1 - 094704_8, 2018/09

 Times Cited Count:6 Percentile:46.89(Physics, Multidisciplinary)

The $$f$$-electron states of PrPd$$_5$$Al$$_2$$ were revealed by neutron inelastic scattering. The flat $$f$$-orbitals with large $$J_z$$ become stable under the two-dimensional CEF potential of unique crystal structure, which is the origin of the Ising anisotropy. A systematic understanding is possible in RPd$$_5$$Al$$_2$$ based on this CEF potential. Especially the $$XY$$-type anisotropy in NpPd$$_5$$Al$$_2$$ can be qualitatively understood with the positive Stevens factors. It mean that the local property is important for the physical properties of RPd$$_5$$Al$$_2$$ including the heavy fermion superconductivity in NpPd$$_5$$Al$$_2$$.

Journal Articles

Magnetic structure and dispersion relation of the $$S$$=1/2 quasi-one-dimensional Ising-like antiferromagnet BaCo$$_{2}$$V$$_{2}$$O$$_{8}$$ in a transverse magnetic field

Matsuda, Masaaki*; Onishi, Hiroaki; Okutani, Akira*; Ma, J.*; Agrawal, H.*; Hong, T.*; Pajerowski, D. M.*; Copley, J. R. D.*; Okunishi, Koichi*; Mori, Michiyasu; et al.

Physical Review B, 96(2), p.024439_1 - 024439_8, 2017/07

 Times Cited Count:12 Percentile:51.78(Materials Science, Multidisciplinary)

Oral presentation

$$f$$-electron states in RPd$$_5$$Al$$_2$$ (R: Pr, Nd)

Metoki, Naoto; Yamauchi, Hiroki; Kitazawa, Hideaki*; Suzuki, Hiroyuki*; Hagihara, Masato*; Masuda, Takatsugu*; Matsuda, Masaaki*; Aczel, A. A.*; Songxue, C.*; Hong, T.*; et al.

no journal, , 

In order to elucidate the 5$$f$$-electron states in the heavy electron superconductor NpPd$$_5$$Al$$_2$$, neutron scattering experiments of the rare earth based iso-structural family have been carried out. The observed crystal field excitations of PrPd$$_5$$Al$$_2$$ and NdPd$$_5$$Al$$_2$$ were analyzed via the crystal field Hamiltonian with tetragonal symmetry, diagonalized analytically. The experimentally obtained crystal field parameters $$A_{lm}$$were very similar in CePd$$_5$$Al$$_2$$, PrPd$$_5$$Al$$_2$$, and NdPd$$_5$$Al$$_2$$, indicating a common effective charge potential in this series. We succeeded to clarify the 5$$f$$ electron states of NpPd$$_5$$Al$$_2$$ and UPd$$_5$$Al$$_2$$ in comparison with these results.

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