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Journal Articles

Main outputs from the OECD/NEA ARC-F Project

Maruyama, Yu; Sugiyama, Tomoyuki*; Shimada, Asako; Lind, T.*; Bentaib, A.*; Sogalla, M.*; Pellegrini, M.*; Albright, L.*; Clayton, D.*

Proceedings of 20th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-20) (Internet), p.4782 - 4795, 2023/08

Journal Articles

Integration of pool scrubbing research to enhance source-term calculations (IPRESCA) project

Gupta, S.*; Herranz, L. E.*; Lebel, L. S.*; Sonnenkalb, M.*; Pellegrini, M.*; Marchetto, C.*; Maruyama, Yu; Dehbi, A.*; Suckow, D.*; K$"a$rkel$"a$, T.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

Journal Articles

Review of Fukushima Daiichi Nuclear Power Station debris endstate location in OECD/NEA preparatory study on analysis of fuel debris (PreADES) project

Nakayoshi, Akira; Rempe, J. L.*; Barrachin, M.*; Bottomley, D.; Jacquemain, D.*; Journeau, C.*; Krasnov, V.; Lind, T.*; Lee, R.*; Marksberry, D.*; et al.

Nuclear Engineering and Design, 369, p.110857_1 - 110857_15, 2020/12

 Times Cited Count:7 Percentile:30.13(Nuclear Science & Technology)

Much is still not known about the end-state of core materials in each of the units at Fukushima Daiichi Nuclear Power Station (Daiichi) that were operating on March 11, 2011. The Nuclear Energy Agency of the Organization for Economic Development has launched the Preparatory Study on Analysis of Fuel Debris (PreADES) project as a first step to reduce some of these uncertainties. As part of the PreADES Task 1, relevant information was reviewed to confirm the accuracy of graphical depictions of the debris endstates at the damaged Daiichi units, which provides a basis for suggesting future debris examinations. Two activities have been completed within the PreADES Task 1. First, relevant knowledge from severe accidents at the Three Mile Island Unit 2 and the Chernobyl Nuclear Power Plant Unit 4 was reviewed, along with results from prototypic tests and hot cell examinations, to glean insights that may inform future decommissioning activities at Daiichi. Second, the current debris endstate diagrams for the damaged reactors at Daiichi were reviewed to confirm that they incorporate relevant knowledge from plant observations and from severe accident code analyses of the BSAF (Benchmark Study of the Accident at Daiichi Nuclear Power Station) 1 and 2 projects. This paper highlights Task 1 insights, which have the potential to not only inform future Decontamination and Decommissioning activities at Daiichi, but also provide important perspectives for severe accident analyses and management, particularly regarding the long term management of a damaged nuclear site following a severe accident.

Journal Articles

Main findings, remaining uncertainties and lessons learned from the OECD/NEA BSAF Project

Pellegrini, M.*; Herranz, L.*; Sonnenkalb, M.*; Lind, T.*; Maruyama, Yu; Gauntt, R.*; Bixler, N.*; Morreale, A.*; Dolganov, K.*; Sevon, T.*; et al.

Nuclear Technology, 206(9), p.1449 - 1463, 2020/09

 Times Cited Count:35 Percentile:98.28(Nuclear Science & Technology)

Journal Articles

Main findings, remaining uncertainties and lessons learned from the OECD/NEA BSAF Project

Pellegrini, M.*; Herranz, L.*; Sonnenkalb, M.*; Lind, T.*; Maruyama, Yu; Gauntt, R.*; Bixler, N.*; Morreale, A.*; Dolganov, K.*; Sevon, T.*; et al.

Proceedings of 18th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-18) (USB Flash Drive), p.1147 - 1162, 2019/08

Journal Articles

Development of a reactive transport code MC-CEMENT ver.2 and its verification using 15-year ${it in-situ}$ concrete/clay interactions at the Tournemire URL

Yamaguchi, Tetsuji; Kataoka, Masaharu; Sawaguchi, Takuma; Mukai, Masayuki; Hoshino, Seiichi; Tanaka, Tadao; Marsal, F.*; Pellegrini, D.*

Clay Minerals, 48(2), p.185 - 197, 2013/05

 Times Cited Count:3 Percentile:9.54(Chemistry, Physical)

Highly alkaline environments induced by cement based materials are likely to deteriorate the physical and/or chemical properties of the bentonite buffer materials in radioactive waste repositories. Predicting long-term alteration of concrete/clay systems requires physico-chemical models and a number of input parameters. In order to provide reliability to the long-term prediction of bentonite buffer performance under disposal conditions, it is necessary to develop and verify reactive transport codes for concrete/clay systems. In this study, a PHREEQC-based, reactive transport analysis code (MC-CEMENT ver.2) was developed and was verified by comparing results of the calculations with ${it in situ}$ observations of the mineralogical evolution at the concrete/argillite interface. The calculation reproduced the observations such as the mineralogical changes limited within one cm in thickness, formation of CaCO$$_{3}$$ and CSH, dissolution of quartz, decrease of porosity in argillite and increase in concrete. These agreements indicate possibility that the models based on lab-scale ($$sim$$ 1 y) experiments can be applied to longer time scale. The fact that the calculation did not reproduce the dissolution of clays and the formation of gypsum indicates that there is still room for improvement in our model.

Oral presentation

Verification of a reactive transport model for long-term alteration of cement-clay systems based on laboratory experiments and in situ observations

Yamaguchi, Tetsuji; Mitsumoto, Yoshibumi; Kadowaki, Mitsushi; Hoshino, Seiichi; Maeda, Toshikatsu; Tanaka, Tadao; Nakayama, Shinichi; Marsal, F.*; Pellegrini, D.*

no journal, , 

It is important to assess long-term alteration of engineered barrier composed of bentonite and cement for the safety assessment of radioactive waste disposal. A mineral model for bentonite-cement-seawater systems and a hydraulic conductivity model for bentonite buffer materials were developed and verified by comparing results of the model calculations with experimental observations. Changes in mineralogy of bentonite buffer materials and accompanying changes in the hydraulic conductivity over 10,000 y were calculated to identify key issues in the long-term alteration analysis. The calculation showed that the temperature, the slow kinetics of the dissolution of montmorillonite, the diffusive mass transfer and the initial (1000 y) mineralogical changes were identified as the key issues. The salinity of the groundwater was identifies as another key issue, which has both positive and negative effects on the hydraulic conductivity.

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