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論文

Leaching behavior of prototypical Corium samples; A Step to understand the interactions between the fuel debris and water at the Fukushima Daiichi reactors

仲吉 彬; Jegou, C.*; De Windt, L.*; Perrin, S.*; 鷲谷 忠博

Nuclear Engineering and Design, 360, p.110522_1 - 110522_18, 2020/04

 被引用回数:1 パーセンタイル:24.17(Nuclear Science & Technology)

Simulated in-vessel and ex-vessel fuel debris, fabricated in the Colima experimental facility set up in the PLINIUS platform at CEA Cadarache, were selected and leaching experiments were carried out under oxidizing conditions. In parallel, geochemical modeling was performed to better understand the experimental concentrations, pH evolutions and secondary phase's formation. Finally, the Fractional Release Rates of the (U, Zr)O$$_{2}$$ matrix for the two kinds of samples (in-vessel and ex-vessel) were found to be close to or one order of magnitude lower than that of SF under oxidizing conditions (from 10$$^{-6}$$ to 10$$^{-7}$$ per day), but the release processes are different.

論文

Characterization of the PTW 34031 ionization chamber (PMI) at RCNP with high energy neutrons ranging from 100 - 392 MeV

Theis, C.*; Carbonez, P.*; Feldbaumer, E.*; Forkel-Wirth, D.*; Jaegerhofer, L.*; Pangallo, M.*; Perrin, D.*; Urscheler, C.*; Roesler, S.*; Vincke, H.*; et al.

EPJ Web of Conferences, 153, p.08018_1 - 08018_5, 2017/09

 被引用回数:0 パーセンタイル:100

欧州原子核研究機構(CERN)の放射線モニタとして、中性子、陽子、$$gamma$$線等の様々な放射線に対して有感な空気入り電離箱PTW-34031(PMI)が使用されている。PMIの各放射線に対する応答関数の計算では、CERNが開発を支援している放射線輸送計算コードFLUKAが用いられている。本研究では、このうち高エネルギー中性子に対するPMIの応答関数の精度検証のため、大阪大学核物理研究センター(RCNP)の$$^{7}$$Li(p,n)反応を利用した準単色中性子照射場において、100-392MeVの準単色中性子に対するPMIの応答関数を測定した。その結果、200MeV以下の準単色中性子照射において、中性子エネルギースペクトルの測定値を線源としたFLUKAによる応答関数の計算値と実験値はよく一致しすることがわかった。一方、250及び392MeVの場合、中性子場に$$^{7}$$Li(p,n)反応から生成する$$pi$$$$^{0}$$の崩壊に伴う$$gamma$$線が混在するため、中性子のみを線源とした計算値は実験値を過小評価することがわかった。

口頭

In situ Raman spectroscopy on nuclear materials in hot cell

Miro, S.*; Peuget, S.*; Tupin, M.*; Fayette, L.*; 仲吉 彬; Perrin, S.*; Jegou, C.*

no journal, , 

Micro-Raman spectroscopy is a powerful technique for analyzing nuclear materials (fuels, claddings and simulated fuel debris). For this purpose, the confocal Raman spectrometer of the Atalante facility (CEA/Marcoule), coupled to an optical microscope in a hot cell, is used to study the aging of nuclear materials in service conditions (reactor, interim storage, waste disposal) or in accidental conditions, subjected to complex scenarios of irradiation, temperature and interaction with the surrounding environment. This contribution aims to illustrate, through examples, the interest of Raman spectroscopy in the characterization of nuclear materials in a wide range of chemical composition and solicitation.

口頭

Leaching behavior of prototypical Corium samples; A Step to understand the interactions between the corium debris and water at the Fukushima Daiichi reactors

仲吉 彬; Jegou, C.*; De Windt, L.*; Perrin, S.*; Peuget, S.*; 鷲谷 忠博

no journal, , 

Simulated in-vessel and ex-vessel corium debris, fabricated in the Colima experimental facility set up in the Severe Accident PLINIUS platform at CEA Cadarache, were selected and leaching experiments were carried out under oxidizing conditions. In parallel, geochemical modeling was performed to better understand the experimental concentrations, pH evolutions and secondary phase's formation. Finally, the Fractional Release Rates of the (U, Zr)O$$_{2}$$ matrix for the two kinds of samples (in-vessel and ex-vessel) were found to be close to or one order of magnitude lower than that of SF under oxidizing conditions (from 10$$^{-6}$$ to 10$$^{-7}$$ per day) but the release processes are different.

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