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坪田 陽一; Porcheron, E.*; Journeau, C.*; Delacroix, J.*; Suteau, C.*; Lallot, Y.*; Bouland, A.*; Roulet, D.*; 三次 岳志
Proceedings of International Conference on Environmental Remediation and Radioactive Waste Management (ICEM2023) (Internet), 6 Pages, 2023/10
福島第一原子力発電所(1F)における燃料デブリ取出しを安全に実施するためには、燃料デブリの切断時に発生する放射性微粒子の定量評価が必要である。我々はウラン含有のIn/Ex-Vessel組成を持つ模擬燃料デブリを作製し、それらを加熱した際に生じるエアロゾルの物理、化学的特性を評価した。それらを基に1F-Unit2の燃料デブリを加熱法の代表例であるレーザー切断した際に生じるエアロゾルの同位体組成と放射能を推定したところ、
Pu、
Am、
Cmを主とするプルトニウムが
核種として、Pu、
Cs-Ba、
Sr-Yが
核種としての着目核種であることが分かった。
Porcheron, E.*; Journeau, C.*; Delacroix, J.*; Berlemont, R.*; Bouland, A.*; Lallot, Y.*; 坪田 陽一; 池田 篤史; 三次 岳志
Proceedings of International Conference on Environmental Remediation and Radioactive Waste Management (ICEM2023) (Internet), 5 Pages, 2023/10
福島第一原子力発電所(1F)の損傷した原子炉の廃止措置における重要な課題である燃料デブリの切断作業における放射性エアロゾルの発生と飛散を評価する目的で行われたURASOLプロジェクトにおいて、模擬燃料デブリの加熱および機械的切断に伴い生成するエアロゾルの質量濃度、リアルタイム数密度、質量基準の粒径分布、形態、および化学的特性の観点からの特性評価について報告する。加熱試験においては温度上昇に伴う粒径増大が観察され、粒子数密度に関しては劣化ウランを用いた模擬燃料デブリを用いた例がHf含有模擬燃料デブリを用いた試験よりも小さい数密度であった。機械的切断においてはエアロゾルの空気動力学的質量中央径は、放射性試料と非放射性試料でほぼ同程度(約3.7
4.4
m)であった。
Journeau, C.*; Delacroix, J.*; Gu
var, C.*; Testud, V.*; Brackx, E.*; Porcheron, E.*; Bouland, A.*; Berlemont, R.*; 池田 篤史
Science Talks (Internet), 6, p.100215_1 - 100215_9, 2023/05
One of the important challenges for the decommissioning of the damaged reactors of the Fukushima Daiichi Nuclear Power Station (1F) is the fuel debris retrieval. The URASOL (URAnium and aeroSOL) project has been undertaken by the French consortium laboratories consisting of ONET, CEA, and IRSN for JAEA. It aims at acquiring basic data on the generation and characteristics of radioactive aerosols from the thermal or mechanical processing of fuel debris simulant. Prototypic fuel debris samples were fabricated based on the average of the lower head compositions computed in the OECD/BSAF benchmark. Samples were heated in an induction furnace to simulate thermal cutting and released aerosols were collected during three temperature ramps using impactors. The collected aerosols were chemically analyzed by ICP-AES and ICP-MS. Iron and tin are the major elements found in these aerosols, followed by chromium and silicon. Significant releases of tellurium, barium and cerium were observed.
孫 昊旻; Leblois, Y.*; Gelain, T.*; Porcheron, E.*
Journal of Nuclear Science and Technology, 59(11), p.1356 - 1369, 2022/11
被引用回数：0 パーセンタイル：0.01(Nuclear Science & Technology)PWRのシビアアクシデントシナリオにおいて、格納容器内エアロゾル状放射性物質の除去・保持のために、格納容器スプレイを用いることができる。そのために、高精度な除去効率の予測は安全評価上重要である。PWRの格納容器スプレイでは、84%-95%と高いスプレイカバー率が要求されるのに対して、既往研究では、そのような高いカバー率におけるエアロゾル除去実験はかなり限られている。本論文では、カバー率に着目し、スプレイによるエアロゾル除去現象の理解と除去効率評価モデル高度化のために、大型容器において実機相当のカバー率を有する体系のエアロゾル除去実験を実施し、詳細なエアロゾルと液滴特性の計測結果から除去特性を調査した。また、MELCORの除去モデルと実験結果を比較し、粒子径に対する除去効率の傾向が再現でき、大きい粒子径に対して過小評価となるものの、最小除去効率を有する小さい粒子径(
0.52m)において良好な一致が得られることを示した。
Porcheron, E.*; Leblois, Y.*; Journeau, C.*; Delacroix, J.*; Molina, D.*; Suteau, C.*; Berlemont, R.*; Bouland, A.*; Lallot, Y.*; Roulet, D.*; et al.
Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR2022) (Internet), 5 Pages, 2022/10
福島第一原子力発電所(1F)の事故炉廃止措置における重要な課題の一つが、燃料デブリの取り出しである。ONET Technologies, CEA, IRSNからなるフランスのコンソーシアムがJAEA/CLADSのために実施したURASOLプロジェクトは、燃料デブリ模擬物質の熱的・機械的加工による放射性エアロゾルの生成と特性に関する科学的基礎データの取得に取り組んでいる。VITAE施設で行われる加熱試験はレーザーによる熱的切断の代表的な条件を模擬している。機械的切断では、FUJISAN施設においてコアボーリング試験を実施した。燃料デブリ模擬物質は、非放射性試験と放射性試験のために開発されている。化学的特性評価と粒径情報の取得は、デブリ取り出しで発生する可能性のある放射性粒子の特性推定のために実施された。これらの情報は1Fにおける燃料デブリ取り出し作業において放射線防護上の対策を評価するうえで重要な情報である。
孫 昊旻; Porcheron, E.*; Magne, S.*; Leroy, M.*; Dhote, J.*; Ruffien Ciszak, A.*; Bentaib, A.*
Proceedings of OECD/NEA Specialist Workshop on Advanced Measurement Method and Instrumentation for enhancing Severe Accident Management in an NPP addressing Emergency, Stabilization and Long-term Recovery Phases (SAMMI 2020) (Internet), 10 Pages, 2020/12
During a severe accident (SA), hydrogen may be generated. To avoid a hydrogen explosion, it is important to monitor gas concentrations of e.g. H
, O, N, HO, CO and CO in the containment during a SA. A spontaneous Raman spectrometry (SRS) associated with a fiber-coupled probe had been developed. Since the probe had been designed to be implemented in the reactor containment, the SRS was qualified experimentally with the probe being surrounded by aerosols. Particles attached on the probe optical components (contamination) due to a continuous aerosol exposure as well as those in the atmosphere (aerosol) can cause photon-particle interactions such as light scattering (Mie) and fluorescence which may influence the Raman spectrum (RS). In our experiment, the contamination effect and the aerosol effect on the RS were investigated separately. It was found both effects increase the spectrum counts in whole wavelength range. Elementary criterion for the onset of each effect was suggested.
Bentaib, A.*; Janin, T.*; Porcheron, E.*; Magne, S.*; Leroy, M.*; Dhote, J.*; Ruffien Ciszak, A.*; 孫 昊旻
Proceedings of OECD/NEA Specialist Workshop on Advanced Measurement Method and Instrumentation for enhancing Severe Accident Management in an NPP addressing Emergency, Stabilization and Long-term Recovery Phases (SAMMI 2020) (Internet), 6 Pages, 2020/12
To prevent hydrogen explosion hazard during a severe accident, dedicated mitigation strategies were adopted according to plants design and improved as results of stress tests after the Fukushima accident. The strategies commonly used combine the implementation of safety components, as the passive autocatalytic recombiners (PARs), and the definition of adequate SAMGs (Severe Accident Management Guidelines). Concerning French PWRs, SAMGs procedure relies on information provided by limited monitoring systems as pressure, core exit temperature and dose rate sensors. The containment atmosphere gaseous composition is not monitored and only PARs are equipped with thermocouples to detect hydrogen through the heat release of the exothermic recombination reaction. In the framework of the MITHYGENE project, a prototypic device had been developed based on Raman probes connected by optical fibers to a transportable unit. Several qualification campaigns had been conducted to check the effect of severe accident representative conditions, including radiation, on the device response. This paper aims to present an overview of the device development and qualification and presents its potential implementation inside the containment.
孫 昊旻; Leblois, Y.*; Gelain, T.*; Porcheron, E.*
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 11 Pages, 2020/08
During a severe accident of PWR, fission products (FPs) may be released. Containment spray can be utilized to remove the aerosols of FPs. Therefore, it is important to develop an analytical model for predicting aerosol removal efficiency. The containment spray has high spray coverage ratio where the droplets are expected to impact side walls. In such condition, the gas flow induced by droplets will behave differently from that without droplet impaction where a stable gas circulation is expected. Since the aerosol removal efficiency depends on gas flow, to develop the removal model for the containment spray from this viewpoint, several experiments were carried out in TOSQAN facility. It was confirmed that the spray coverage ratios were comparable to that of the containment spray and many droplets impacted side wall. Aerosol removal was found to be more effective in higher spray water flow rates. Aerosol concentration decay calculated by CFD was in agreement with measured one.
