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Detlefs, B.*; Wilkins, S. B.*; Caciuffo, R.*; Paixo, J. A.*; Kaneko, Koji; Honda, Fuminori*; Metoki, Naoto; Bernhoeft, N.*; Rebizant, J.*; Lander, G. H.*
Physical Review B, 77(2), p.024425_1 - 024425_10, 2008/01
Times Cited Count:17 Percentile:57.23(Materials Science, Multidisciplinary)We report a resonant X-ray scattering study of the antiferromagnetic neptunium compounds NpCoGa and NpRhGa
. Large resonant signals of magnetic dipole character are observed below the N
el temperatures. The signals at the Np edges confirm the behavior determined previously from neutron diffraction. On application of a magnetic field of 9 T along the [010] direction in NpRhGa
, we observe a change in the population of different [110]-type domains. We also observe a magnetic dipole signal at the Ga
edge, similarly to the reported UGa
case, that can be interpreted within a semilocalized model as an orbital polarization of the Ga 4
states induced via strong hybridization with the Np 5
valence band. Quantitative analysis of the signal shows that the Ga dipole on the two different Ga sites follows closely the Np magnetic moment reorientation in NpRhGa
. The ratios of the signals on the two inequivalent Ga sites are not the same for the different compounds.
Raymond, S.*; Piekarz, P.*; Sanchez, J. P.*; Serrano, J.*; Kirsch, M.*; Detlefs, B.*; Rebizant, J.*; Metoki, Naoto; Kaneko, Koji; Jochym, P. T.*; et al.
Journal of Alloys and Compounds, 444-445, p.104 - 108, 2007/10
Times Cited Count:2 Percentile:20.92(Chemistry, Physical)The phonon dispersion curves of the unconventional superconductor PuCoGa were studied by inelastic X-ray scattering at room temperature. The experimental data agree well with ab initio lattice dynamics calculations. An accurate theoretical description of the phonon spectrum is obtained only when a local Coulomb repulsion
3 eV among 5f electrons is taken into account. This implies partial localization of the 5f electrons in this compound. A comparison made with the phonon spectrum of UCoGa
suggests that the latter compound is better described with a fully itinerant f electrons model.
Raymond, S.*; Piekarz, P.*; Sanchez, J. P.*; Serrano, J.*; Kirsch, M.*; Janousova, B.*; Rebizant, J.*; Metoki, Naoto; Kaneko, Koji; Jochym, P. T.*; et al.
Physical Review Letters, 96(23), p.237003_1 - 237003_4, 2006/06
Times Cited Count:26 Percentile:74.02(Physics, Multidisciplinary)The phonon dispersion curves of the superconductor PuCoGa were studied by inelastic X-ray scattering at room temperature. The experimental data agree well with
lattice dynamics calculations. An accurate description of the phonon spectrum is obtained only when a local Coulomb repulsion U
3 eV among 5
electrons is taken into account.
Metoki, Naoto; Kaneko, Koji; Colineau, E.*; Javorsk, P.*; Aoki, Dai*; Homma, Yoshiya*; Boulet, P.*; Wastin, F.*; Shiokawa, Yoshinobu; Bernhoeft, N.*; et al.
Physical Review B, 72(1), p.014460_1 - 014460_8, 2005/07
Times Cited Count:50 Percentile:83.11(Materials Science, Multidisciplinary)no abstracts in English
Metoki, Naoto; Kaneko, Koji; Ikeda, Shugo; Matsuda, Tatsuma; Haga, Yoshinori; Onuki, Yoshichika; Raymond, S.*; Piekarz, P.*; Sanchez, J. P.*; Serrano, J.*; et al.
no journal, ,
no abstracts in English