Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Martin, P. G.*; Jones, C. P.*; Cipiccia, S.*; Batey, D. J.*; Hallam, K. R.*; Satou, Yukihiko; Griffiths, I.*; Rau, C.*; Richards, D. A.*; Sueki, Keisuke*; et al.
Scientific Reports (Internet), 10(1), p.1636_1 - 1636_11, 2020/01
Times Cited Count:8 Percentile:34.78(Multidisciplinary Sciences)Martin, P. G.*; Louvel, M.*; Cipiccia, S.*; Jones, C. P.*; Batey, D. J.*; Hallam, K. R.*; Yang, I. A. X.*; Satou, Yukihiko; Rau, C.*; Mosselmans, J. F. W.*; et al.
Nature Communications (Internet), 10, p.2801_1 - 2801_7, 2019/06
Times Cited Count:26 Percentile:77.9(Multidisciplinary Sciences)Synchrotron radiation (SR) analysis techniques alongside secondary ion mass spectrometry (SIMS) measurements have been made on sub-mm particulate material derived from reactor Unit 1 of the Fukushima Daiichi Nuclear Power Plant (FDNPP). Using these methods, it has been possible to investigate the distribution, state and isotopic composition of micron-scale U particulate contained within the larger Si-based ejecta material. Through combined SR micro-focused X-ray fluorescence (SR-micro-XRF) and absorption contrast SR micro-focused X-ray tomography (SR-micro-XRT), the U particulate was found to be located around the exterior circumference of the highly-porous particle. Synchrotron radiation micro-focused X-ray absorption near edge structure (SR-micro-XANES) analysis of a number of these entrapped particles revealed them to exist within the U(IV) oxidation state, as UO, and identical in structure to reactor fuel. Confirmation that this U was of nuclear origin (U-enriched) was provided through secondary ion mass spectrometry (SIMS) analysis with an isotopic enrichment ratio characteristic of a provenance from reactor Unit 1 at the FDNPP. These results provide clear evidence of the event scenario (that a degree of core fragmentation and release occurred from reactor Unit 1), with such spent fuel ejecta existing; (i) within the stable U(IV) oxidation state; and (ii) contained within a bulk Si-based particle. While this U is unlikely to represent an environmental or health hazard, such assertions would likely change, however, should break-up of the Si-containing bulk particle occur. However, more important to the long-term decommissioning of the reactors (and clean-up) on the FDNPP, is the knowledge that core integrity of reactor Unit 1 was compromised with nuclear material existing outside of the reactors primary containment.
Kondoh, Takashi; Richards, R. K.*; Hutchinson, D. P.*; Sugie, Tatsuo; Costley, A. E.*; Miura, Yukitoshi; Lee, S.*
Proceedings of 30th EPS Conference on Controlled Fusion and Plasma Physics (CD-ROM), 4 Pages, 2003/07
In order to understand the behavior of alpha-particles which are the dominant heat source in a burning plasma, it is necessary to measure the spatial distribution of the number of the alpha-particles and their energy spectrum. A collective Thomson scattering (CTS) system based on a pulsed CO laser is being developed and is under consideration for alpha-particle measurements on ITER. Heating beam ions (E = 1 MeV) are normally co-injected and have a similar velocity with alpha-particles in ITER. The CTS measurement can not, in general, distinguish beam ions and alpha-particles which have the same velocity. A vertical scattering geometry to distinguish between beam ions and alpha-particles is proposed. Calculations have shown that the vertically viewing CTS can resolve counter-travelling alphas without being masked by beam ions. Preliminary design of a beam line and a receiver system with the vertical scattering geometry has been developed. A proof-of-principle test on the CTS system using the JT-60U plasma is being conducted.
Kondoh, Takashi; Miura, Yukitoshi; Lee, S.*; Richards, R. K.*; Hutchinson, D. P.*; Bennett, C. A.*
Review of Scientific Instruments, 74(3), p.1642 - 1645, 2003/03
Times Cited Count:20 Percentile:68.22(Instruments & Instrumentation)Measurements of energy spectrum and density profile of confined alpha-particles are required for ITER. Several methods have been proposed, however, a measurement technique hasn't been established yet. A collective Thomson scattering (CTS) system based on a pulsed CO laser is being developed to demonstrate feasibility of alpha-particle diagnostics for ITER. The pulse laser (15J, 1m, 0.6 m) and a wide band (~ 8GHz) heterodyne receiver with a quantum-well infrared photodetector (QWIP) have been developed and installed in the JT-60U tokamak. Stray light is reduced by a notch filter with hot CO gas. Heterodyne receiver is absolutely calibrated using large area blackbody radiation source. Scattered signal from JT-60U plasma has not detected because of electrical noise originated from discharge of the pulsed laser and stray signal caused by impurity of the spectrum of the pulsed laser.