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Journal Articles

Compositional and structural analysis of Fukushima-derived particulates using high-resolution X-ray imaging and synchrotron characterisation techniques

Martin, P. G.*; Jones, C. P.*; Cipiccia, S.*; Batey, D. J.*; Hallam, K. R.*; Satou, Yukihiko; Griffiths, I.*; Rau, C.*; Richards, D. A.*; Sueki, Keisuke*; et al.

Scientific Reports (Internet), 10(1), p.1636_1 - 1636_11, 2020/01

 Times Cited Count:8 Percentile:34.78(Multidisciplinary Sciences)

Journal Articles

Provenance of uranium particulate contained within Fukushima Daiichi Nuclear Power Plant Unit 1 ejecta material

Martin, P. G.*; Louvel, M.*; Cipiccia, S.*; Jones, C. P.*; Batey, D. J.*; Hallam, K. R.*; Yang, I. A. X.*; Satou, Yukihiko; Rau, C.*; Mosselmans, J. F. W.*; et al.

Nature Communications (Internet), 10, p.2801_1 - 2801_7, 2019/06

 Times Cited Count:26 Percentile:77.9(Multidisciplinary Sciences)

Synchrotron radiation (SR) analysis techniques alongside secondary ion mass spectrometry (SIMS) measurements have been made on sub-mm particulate material derived from reactor Unit 1 of the Fukushima Daiichi Nuclear Power Plant (FDNPP). Using these methods, it has been possible to investigate the distribution, state and isotopic composition of micron-scale U particulate contained within the larger Si-based ejecta material. Through combined SR micro-focused X-ray fluorescence (SR-micro-XRF) and absorption contrast SR micro-focused X-ray tomography (SR-micro-XRT), the U particulate was found to be located around the exterior circumference of the highly-porous particle. Synchrotron radiation micro-focused X-ray absorption near edge structure (SR-micro-XANES) analysis of a number of these entrapped particles revealed them to exist within the U(IV) oxidation state, as UO$$_{2}$$, and identical in structure to reactor fuel. Confirmation that this U was of nuclear origin ($$^{235}$$U-enriched) was provided through secondary ion mass spectrometry (SIMS) analysis with an isotopic enrichment ratio characteristic of a provenance from reactor Unit 1 at the FDNPP. These results provide clear evidence of the event scenario (that a degree of core fragmentation and release occurred from reactor Unit 1), with such spent fuel ejecta existing; (i) within the stable U(IV) oxidation state; and (ii) contained within a bulk Si-based particle. While this U is unlikely to represent an environmental or health hazard, such assertions would likely change, however, should break-up of the Si-containing bulk particle occur. However, more important to the long-term decommissioning of the reactors (and clean-up) on the FDNPP, is the knowledge that core integrity of reactor Unit 1 was compromised with nuclear material existing outside of the reactors primary containment.

Journal Articles

Prospects for $$alpha$$-particle diagnostics by CO$$_{2}$$ laser collective Thomson scattering in ITER

Kondoh, Takashi; Richards, R. K.*; Hutchinson, D. P.*; Sugie, Tatsuo; Costley, A. E.*; Miura, Yukitoshi; Lee, S.*

Proceedings of 30th EPS Conference on Controlled Fusion and Plasma Physics (CD-ROM), 4 Pages, 2003/07

In order to understand the behavior of alpha-particles which are the dominant heat source in a burning plasma, it is necessary to measure the spatial distribution of the number of the alpha-particles and their energy spectrum. A collective Thomson scattering (CTS) system based on a pulsed CO$$_{2}$$ laser is being developed and is under consideration for alpha-particle measurements on ITER. Heating beam ions (E = 1 MeV) are normally co-injected and have a similar velocity with alpha-particles in ITER. The CTS measurement can not, in general, distinguish beam ions and alpha-particles which have the same velocity. A vertical scattering geometry to distinguish between beam ions and alpha-particles is proposed. Calculations have shown that the vertically viewing CTS can resolve counter-travelling alphas without being masked by beam ions. Preliminary design of a beam line and a receiver system with the vertical scattering geometry has been developed. A proof-of-principle test on the CTS system using the JT-60U plasma is being conducted.

Journal Articles

Collective Thomson scattering based on CO$$_{2}$$ laser for ion energy spectrum measurements in JT-60U

Kondoh, Takashi; Miura, Yukitoshi; Lee, S.*; Richards, R. K.*; Hutchinson, D. P.*; Bennett, C. A.*

Review of Scientific Instruments, 74(3), p.1642 - 1645, 2003/03

 Times Cited Count:20 Percentile:68.22(Instruments & Instrumentation)

Measurements of energy spectrum and density profile of confined alpha-particles are required for ITER. Several methods have been proposed, however, a measurement technique hasn't been established yet. A collective Thomson scattering (CTS) system based on a pulsed CO$$_{2}$$ laser is being developed to demonstrate feasibility of alpha-particle diagnostics for ITER. The pulse laser (15J, 1$$mu$$m, 0.6 $$mu$$m) and a wide band (~ 8GHz) heterodyne receiver with a quantum-well infrared photodetector (QWIP) have been developed and installed in the JT-60U tokamak. Stray light is reduced by a notch filter with hot CO$$_{2}$$ gas. Heterodyne receiver is absolutely calibrated using large area blackbody radiation source. Scattered signal from JT-60U plasma has not detected because of electrical noise originated from discharge of the pulsed laser and stray signal caused by impurity of the spectrum of the pulsed laser.

Journal Articles

Collective Thomson scattering using a pulsed CO$$_{2}$$ laser in JT-60U

Kondoh, Takashi; Lee, S.; Hutchinson, D. P.*; Richards, R. K.*

Review of Scientific Instruments, 72(1), p.1143 - 1146, 2001/01

 Times Cited Count:13 Percentile:59.42(Instruments & Instrumentation)

no abstracts in English

Journal Articles

Fast ion diagnostics in JT-60U; $$gamma$$-ray and collective Thomson scattering measurements

Kondoh, Takashi; Nagashima, Akira; ; Richards, R. K.*; Hutchinson, D. P.*; Moriyama, Shinichi; Morioka, Atsuhiko; Tobita, Kenji; Kusama, Yoshinori; V.G.Kiptily*

Proc. of 1998 Int. Congress on Plasma Physics, p.1478 - 1481, 1998/00

no abstracts in English

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