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Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.
Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12
Times Cited Count:7 Percentile:34.52(Geosciences, Multidisciplinary)The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.
Sb
uncovered by soft X-ray magnetic circular dichroismSaito, Yuji; Fujiwara, Hidenori*; Yasui, Akira*; Kadono, Toshiharu*; Sugawara, Hitoshi*; Kikuchi, Daisuke*; Sato, Hideyuki*; Suga, Shigemasa*; Yamasaki, Atsushi*; Sekiyama, Akira*; et al.
Physical Review B, 102(16), p.165152_1 - 165152_8, 2020/10
Times Cited Count:1 Percentile:4.03(Materials Science, Multidisciplinary)Kudo, Hideyuki*; Otani, Yuichi*; Hara, Masahide*; Kato, Atsushi; Ishikawa, Nobuyuki; Otaka, Masahiko; Nagai, Keiichi; Saito, Junichi; Ara, Kuniaki; Ide, Akihiro*
Proceedings of 2019 International Congress on Advances in Nuclear Power Plants (ICAPP 2019) (Internet), 10 Pages, 2019/05
A next generation SFR in Japan has adopted an advanced dry cleaning system which consists of the argon gas blowing process to reduce the amount of metallic residual sodium remaining on spent fuel assemblies. This paper describes experimental and analytical work focusing on the amount of residual sodium remaining on a fuel pin bundle before and after the argon gas blowing process. The experiments were conducted using a sodium test loop and a short specimen consisting of a 7 pin bundle. The effects of the blowing gas velocity and the blowing time were quantitatively analyzed in the experiments. On the basis of these experimental results, evaluation models predicting the amount of the residual sodium were constructed.
Ide, Akihiro*; Kudo, Hideyuki*; Inuzuka, Taisuke*; Hara, Masahide*; Kato, Atsushi; Ishikawa, Nobuyuki; Otaka, Masahiko; Nagai, Keiichi; Saito, Junichi; Ara, Kuniaki
Proceedings of 2019 International Congress on Advances in Nuclear Power Plants (ICAPP 2019) (Internet), 10 Pages, 2019/05
A next generation SFR in Japan has adopted an advanced dry cleaning system which consists of the following process of argon gas blowing to reduce the amount of metallic sodium, moist argon gas blowing to deactivate the residual sodium, and direct storage in the SFP without using storage containers. This three-step process increases economic competitiveness and reduces waste products. In this Research and Development work, the amount of residual sodium and performance of the dry cleaning process were investigated. This paper describes experimental and analytical work for all parts of a fuel assembly except for a fuel pin bundle.
Zr determination with isotope dilution ICP-MSAsai, Shiho; Hanzawa, Yukiko; Konda, Miki; Suzuki, Daisuke; Magara, Masaaki; Kimura, Takaumi; Ishihara, Ryo*; Saito, Kyoichi*; Yamada, Shinsuke*; Hirota, Hideyuki*
Talanta, 185, p.98 - 105, 2018/08
Times Cited Count:9 Percentile:29.53(Chemistry, Analytical)Estimating the risks associated with radiation from long-lived fission products (LLFP) in radioactive waste is essential to ensure the long-term safety of potential disposal sites. In this study, the amount of
Zr, a LLFP, was determined by ICP-MS after separating Zr from a spent nuclear fuel solution using a microvolume anion-exchange cartridge (TEDA cartridge). The TEDA cartridge achieved highly selective separation of Zr regardless of its small bed volume of 0.08 cm
. The time taken to complete the Zr separation was 1.2 min with a flow rate of 1.5 mL/min, which was 10 times faster than that for a conventional anion-exchange resin column. Almost all the other elements were removed, leading to accurate measurement of
Zr. The result connects experimental value to theoretical prediction provided by ORIGEN2, which requires verification. With the measured value, we demonstrated that the theoretical value is reliable enough to estimate radiation risks.
Furumoto, Kenichiro*; Watanabe, Seiichi*; Yamamoto, Teruhisa*; Teshima, Hideyuki*; Yamashita, Shinichiro; Saito, Hiroaki; Shirasu, Noriko
Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 10 Pages, 2017/09
Since 2015, Mitsubishi Nuclear Fuel (MNF) has joined in a Japanese R&D project of ATF founded by the Ministry of Economy, Trade and Industry (METI) as a subcontractor to Japan Atomic Energy Agency (JAEA) which is the prime contractor to METI. In this program, MNF plans to evaluate an influence of Silicon Carbide (SiC) composite cladding upon fuel rod behavior in current pressurized water reactors (PWR). This paper reports the evaluation result of the applicability of fuel rod with SiC composite cladding for a conventional PWR. For the applicability evaluations of SiC composite to conventional PWR, both of analytical evaluations and out-of-pile tests for SiC composite were conducted. Analytical evaluations were performed by Mitsubishi's own fuel rod design code and the fuel rod behavior evaluation code developed by JAEA. These codes were modified to evaluate the behavior of the fuel rod with SiC composite cladding. As out-of-pile tests, thermal diffusivity measurement and autoclave corrosion test for SiC composite samples were performed. Test apparatus were developed for evaluation of performance of SiC composite under the condition simulated design basis accident (DBA).
Np content in spent nuclear fuelAsai, Shiho; Hanzawa, Yukiko; Konda, Miki; Suzuki, Daisuke; Magara, Masaaki; Kimura, Takaumi; Ishihara, Ryo*; Saito, Kyoichi*; Yamada, Shinsuke*; Hirota, Hideyuki*
Analytical Chemistry, 88(6), p.3149 - 3155, 2016/03
Times Cited Count:8 Percentile:25.93(Chemistry, Analytical)Neptunium-237 (
Np) is one of the major long-lived radionuclides found in spent nuclear fuel. To evaluate the long-term safety of a HLW repository, the
Np content in spent nuclear fuel must be determined. In this study, micro-volume anion-exchange porous polymer disk-packed cartridges were prepared for Am-Np separation, which is required prior to the measurement of
Np with ICP-MS. Disks with a volume of 0.08 cm
were cut out from porous sheets having triethylenediamine (TEDA)-containing polymer chains densely attached on the pore surface. The resulting TEDA-introduced disk cartridge was applied to a spent nuclear fuel sample. The chemical yield of Np was 90.4%, which is sufficiently high for ICP-MS measurement of
Np. Compared with the conventional separation technique using commercially available anion-exchange resin columns, the time required to adsorb, wash and elute Np using the TEDA-introduced disk cartridge was reduced by 75%.
Tanaka, Ryota*; Ishihara, Ryo*; Miyoshi, Kazuyoshi*; Umeno, Daisuke*; Saito, Kyoichi*; Asai, Shiho; Yamada, Shinsuke*; Hirota, Hideyuki*
Separation Science and Technology, 49(1), p.154 - 159, 2014/01
Times Cited Count:4 Percentile:15.65(Chemistry, Multidisciplinary)Uchiyama, Shoichiro*; Ishihara, Ryo*; Umeno, Daisuke*; Saito, Kyoichi*; Yamada, Shinsuke*; Hirota, Hideyuki*; Asai, Shiho
Journal of Chemical Engineering of Japan, 46(6), p.414 - 419, 2013/06
Times Cited Count:7 Percentile:24.12(Engineering, Chemical)Wada, Go*; Ishihara, Ryo*; Miyoshi, Kazuyoshi*; Umeno, Daisuke*; Saito, Kyoichi*; Asai, Shiho; Yamada, Shinsuke*; Hirota, Hideyuki*
Solvent Extraction and Ion Exchange, 31(2), p.210 - 220, 2013/02
Times Cited Count:2 Percentile:11.45(Chemistry, Multidisciplinary)A crosslinked chelating porous sheet was prepared by cografting ethylene glycol dimethacrylate (EGDMA) with glycidyl methacrylate onto an electron-beam-irradiated porous polyethylene sheet, followed by the introduction of an iminodiacetate group. At a molar percentage of EGDMA of 1.0 mol%, the sheet exhibited a maximum dynamic binding capacity for copper ions of 0.93 mmol/g, while the equilibrium binding capacity remained the same (1.2 mmol/g) as that of a non-crosslinked chelating porous sheet. The crosslinking of the grafted chain causes copper ions to lower their diffusion rate along the sheet thickness driven by the gradient of the amount of copper ions adsorbed.
Ishihara, Ryo*; Asai, Shiho; Otosaka, Shigeyoshi; Yamada, Shinsuke*; Hirota, Hideyuki*; Miyoshi, Kazuyoshi*; Umeno, Daisuke*; Saito, Kyoichi*
Solvent Extraction and Ion Exchange, 30(2), p.171 - 180, 2012/02
Times Cited Count:8 Percentile:30.31(Chemistry, Multidisciplinary)Wada, Go*; Ishihara, Ryo*; Miyoshi, Kazuyoshi*; Umeno, Daisuke*; Saito, Kyoichi*; Asai, Shiho; Yamada, Shinsuke*; Hirota, Hideyuki*
Nihon Ion Kokan Gakkai-Shi, 22(2), p.47 - 52, 2011/01
no abstracts in English
-octylphosphine oxide, and its adsorption/elution of bismuth ionsTanaka, Ryota*; Ishihara, Ryo*; Miyoshi, Kazuyoshi*; Umeno, Daisuke*; Saito, Kyoichi*; Asai, Shiho; Yamada, Shinsuke*; Hirota, Hideyuki*
Reactive and Functional Polymers, 70(12), p.986 - 990, 2010/12
Times Cited Count:7 Percentile:27.77(Chemistry, Applied)Kumada, Hiroaki*; Saito, Kimiaki; Nakamura, Takemi; Sakae, Takeji*; Sakurai, Hideyuki*; Matsumura, Akira*; Ono, Koji*
Proceedings of 14th International Congress on Neutron Capture Therapy (ICNCT-14) (CD-ROM), p.238 - 241, 2010/10
Asai, Shiho; Kimura, Takaumi; Miyoshi, Kazuyoshi*; Saito, Kyoichi*; Yamada, Shinsuke*; Hirota, Hideyuki*
Nihon Ion Kokan Gakkai-Shi, 21(3), p.334 - 339, 2010/07
Saito, Takakazu; Imaizumi, Kazuyuki; Oka, Kiyoshi; Aizawa, Hideyuki*; Katagiri, Genichi*
FAPIG, (179), p.3 - 9, 2009/07
The experimental fast reactor Joyo is the first sodium cooled fast reactor in Japan. In-vessel visual inspections have been conducted with an obstacle on the in-vessel storage rack in Joyo. Because of the high radiation dose in the reactor vessel, radiation-resistant fiberscope was applied to Joyo. The radiation-resistant fiberscope was inserted into the reactor vessel thorough the inspection hole and fuel handling hole on rotating plugs. In order to observe the top of the subassemblies and in-vessel storage rack, an I-shape device which had a downward and side view monitoring radiation-resistant fiberscopes was used. To observe the bottom face of the upper core structure, a remote handling visual device whose tip could bend into an L-shape was developed to insert the radiation-resistant fiberscope into the 70 mm gap between the bottom of the upper core structure and the top of the subassemblies. The observations of the top of the subassemblies and in-vessel storage rack were conducted from October 2007 to February 2008. The bottom face of the upper core structure was observed in July 2008. The number of photographs of the entire bottom face of the upper core structure reached approximately 35,000. Confirmation was made that the remote handling device equipped with the radiation-resistant fiberscope would achieve the expected performance. These observations results provided useful information on incident investigations. In addition, fundamental findings and the experience gained during this study, which included the design of equipment, operating procedures, resolution, lighting adjustments, photograph composition and the durability of the radiation-resistant fiberscope under radiation exposure, provided valuable insights into possible further improvements and verifications for in-vessel visual observation techniques in an sodium fast reactor.
Nakano, Takashi*; Arakawa, Kazuo; Sakurai, Hideyuki*; Hasegawa, Masatoshi*; Yuasa, Kazuhisa*; Saito, Etsuko*; Takagi, Hitoshi*; Nagamine, Takeaki*; Kusakabe, Takahiko*; Takada, Hisashi*; et al.
International Journal of PIXE, 16(1&2), p.69 - 76, 2006/00
A new program was started out to create a new medical scientific field, which is consisting of radiation oncology and nuclear medicine, utilizing the advanced accelerator and ion beam technology. An in-air micro-PIXE analyzer system, which is among the most important technical basis of the program, was upgraded to improve accuracy of elemental mapping for samples having thickness variation in a scope of microbeam scanning. In the program, on the other hand, in order to approach important bio-medical problems on cancer, intracellular dynamics of the trace elements according to mechanism of development of diseases were studied using this system. This paper outlines this program and shows the system upgraded, and results of preliminary studied about the problems.
Miyahara, Tsuneaki*; Ishii, Hiroyoshi*; Takayama, Yasuhiro*; Hirose, Masaaki*; Maruyama, Kenichi*; Obu, Kenji*; Shinoda, Motoki*; Muro, Takayuki*; Saito, Yuji; Matsuda, Tatsuma*; et al.
Journal of the Physical Society of Japan, 70(10), p.2977 - 2981, 2001/10
Times Cited Count:6 Percentile:41.61(Physics, Multidisciplinary)no abstracts in English
Saito, Yuji; Kimura, Hiroaki*; Suzuki, Yoshio*; Nakatani, Takeshi*; Matsushita, Tomohiro*; Muro, Takayuki*; Miyahara, Tsuneaki*; Fujisawa, M.*; Soda, Kazuo*; Ueda, Shigenori*; et al.
Review of Scientific Instruments, 71(9), p.3254 - 3259, 2000/09
Times Cited Count:188 Percentile:98.94(Instruments & Instrumentation)no abstracts in English
Asai, Shiho; Hanzawa, Yukiko; Konda, Miki; Suzuki, Daisuke; Magara, Masaaki; Kimura, Takaumi; Ishihara, Ryo*; Saito, Kyoichi*; Yamada, Shinsuke*; Hirota, Hideyuki*
no journal, ,
Zr is a long-lived fission product which can be found in spent nuclear fuel and HLW. The estimation of the
Zr content is indispensable to achieve a safety disposal of HLW because
Zr is predicted to be one of the major contributors to radiation dose. However, only a few measured
Zr values have been reported, leading to a high demand for development of an efficient analytical method. Our group has been prepared a new porous filter cartridge which has densely bound ion-exchanger onto the pore surface of the filter, enabling a high-capacity and rapid adsorption. In order to apply this filter cartridge to a pretreatment for the
Zr measurement with ICP-MS, an elution profiles of Zr and the other coexisting elements were examined. According to the resultant separation conditions, Zr in a spent nuclear fuel sample was successfully separated. The measured
Zr content is 98.2
5.1 ng, which agrees with the theoretical value.