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Journal Articles

Purification of anionic fluorescent probes through precise fraction collection with a two-point detection system using multiple-stacking preparative capillary transient isotachophoresis

Haraga, Tomoko; Tsujimura, Hiroto*; Miyauchi, Saori*; Kamimura, Takuya*; Shibukawa, Masami*; Saito, Shingo*

Electrophoresis, 41(13-14), p.1152 - 1159, 2020/07

 Times Cited Count:0 Percentile:100(Biochemical Research Methods)

A novel combination of CE-based separation techniques was used for the precise fractionation of ionic compounds from impurities. The combination of on-capillary concentration and separation using transient isotachophoresis, with multiple injections and a two-point detection system provided higher efficiency, and accuracy at a microliter-scale injection volume, than when CE was individually used for purification. In this paper, we present successful applications of the CE fractionation techniques for the purification of fluorescein, fluorescein-4-isothiocyanate, two fluorescent metal ion probes, and a fluorescein-modified DNA aptamer. The purity of the isolated fluorescent probes ranged from 95 to 99%. The purified probe solutions were practical for use as purified stock solutions. The method developed was useful for the purification of anionic fluorescent reagents to be of ultratrace analytical grade for use with CE-LIF.

Journal Articles

Experimental observation of temperature and magnetic-field evolution of the 4${it f}$ states in CeFe$$_{2}$$ revealed by soft X-ray magnetic circular dichroism

Saito, Yuji; Yasui, Akira*; Fuchimoto, Hiroto*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Imada, Shin*; Narumi, Yasuo*; Kindo, Koichi*; Takahashi, Minoru*; Ebihara, Takao*; et al.

Physical Review B, 96(3), p.035151_1 - 035151_5, 2017/07

AA2017-0611.pdf:0.36MB

 Times Cited Count:1 Percentile:100(Materials Science, Multidisciplinary)

We revisit the delocalized character of the 4$$f$$ states of CeFe$$_2$$ in the ferromagnetically ordered phase by X-ray magnetic circular dichroism (XMCD) in X-ray absorption spectroscopy (XAS) with improved data quality using single crystals. Surprisingly, the Ce $$M_{4,5}$$ XMCD spectral shape changes significantly as a function of temperature and applied magnetic field, with no concomitant changes in the spectral shape of the Ce $$M_{4,5}$$ XAS as well as the Fe $$L_{2,3}$$ XAS and XMCD. This unusual behavior is characterized by the $$J=7/2$$ states in a 4$$f^1$$ configuration mixed into the $$J=5/2$$ ground state. Such extreme sensitivity of the Ce 4$$f$$ states to the external perturbations can be related to the magnetic instability toward an antiferromagnetic phase in CeFe$$_2$$. Our experimental data presented here provide valuable insights into the underlying physics in strongly-hybridized ferromagnetic Ce compounds.

Journal Articles

2016 Professional Engineer (PE) test preparation course; Nuclear and radiation technical disciplines

Takahashi, Naoki; Suzuki, Soju; Saito, Hiroto; Ueno, Takashi; Abe, Sadayoshi; Yamanaka, Atsushi; Tanigawa, Masafumi; Nakamura, Daishi; Sasaki, Shunichi; Mine, Tadaharu

Nippon Genshiryoku Gakkai Homu Peji (Internet), 20 Pages, 2017/05

no abstracts in English

Journal Articles

Electronic structures of ferromagnetic CeAgSb$$_{2}$$; Soft X-ray absorption, magnetic circular dichroism, and angle-resolved photoemission spectroscopies

Saito, Yuji; Fujiwara, Hidenori*; Yamaguchi, Takashi*; Nakatani, Yasuhiro*; Mori, Takeo*; Fuchimoto, Hiroto*; Kiss, Takayuki*; Yasui, Akira*; Miyawaki, Jun*; Imada, Shin*; et al.

Journal of the Physical Society of Japan, 85(11), p.114713_1 - 114713_7, 2016/11

 Times Cited Count:7 Percentile:39.4(Physics, Multidisciplinary)

We report on the electronic structures of ferromagnetic CeAgSb$$_{2}$$ using soft X-ray absorption (XAS), magnetic circular dichroism (XMCD), and angle-resolved photoemission (ARPES) spectroscopies. The Ce $$M_{4,5}$$ XAS spectra show very small satellite structures, reflecting a strongly localized character of the Ce 4${it f}$ electrons. The linear dichroism effects in the Ce $$M_{4,5}$$ XAS spectra demonstrate the ground-state Ce 4${it f}$ symmetry of $$Gamma$$$$_{6}$$, the spatial distribution of which is directed along the ${it c}$-axis. Nevertheless, ARPES spectra at the Ce 3$$d$$-4$$f$$ resonance show the momentum dependence of the intensity ratio between Ce 4$$f^{1}_{5/2}$$ and 4$$f^{1}_{7/2}$$ peaks in a part of the Brillouin zone, suggesting the non negligible momentum-dependent hybridization effect between the Ce 4${it f}$ and the conduction electrons. This is associated with the moderate mass enhancement in CeAgSb$$_{2}$$.

Journal Articles

Thermoelectric generation based on spin Seebeck effects

Uchida, Kenichi*; Adachi, Hiroto; Kikkawa, Takashi*; Kirihara, Akihiro*; Ishida, Masahiko*; Yorozu, Shinichi*; Maekawa, Sadamichi; Saito, Eiji*

Proceedings of the IEEE, 104(10), p.1946 - 1973, 2016/10

 Times Cited Count:118 Percentile:0.71(Engineering, Electrical & Electronic)

Journal Articles

Origin of the spin Seebeck effect in compensated ferrimagnets

Gepr$"a$gs, S.*; Kehlberger, A.*; Coletta, F.*; Qiu, Z.*; Guo, E.-J.*; Schulz, T.*; Mix, C.*; Meyer, S.*; Kamra, A.*; Althammer, M.*; et al.

Nature Communications (Internet), 7, p.10452_1 - 10452_6, 2016/02

 Times Cited Count:80 Percentile:2.93(Multidisciplinary Sciences)

Journal Articles

2016 Professional Engineer (PE) test preparation course "Nuclear and Radiation Technical Disciplines"

Takahashi, Naoki; Yoshinaka, Kazuyuki; Harada, Akio; Yamanaka, Atsushi; Ueno, Takashi; Kurihara, Ryoichi; Suzuki, Soju; Takamatsu, Misao; Maeda, Shigetaka; Iseki, Atsushi; et al.

Nippon Genshiryoku Gakkai Homu Peji (Internet), 64 Pages, 2016/00

no abstracts in English

Journal Articles

Unconventional scaling and significant enhancement of the spin Seebeck effect in multilayers

Ramos, R.*; Kikkawa, Takashi*; Aguirre, M.*; Lucas, I.*; Anad$'o$n, A.*; Oyake, Takafumi*; Uchida, Kenichi*; Adachi, Hiroto; Shiomi, Junichiro*; Algarabel, P. A.*; et al.

Physical Review B, 92(22), p.220407_1 - 220407_5, 2015/12

 Times Cited Count:49 Percentile:8.14(Materials Science, Multidisciplinary)

Journal Articles

Magnon instability driven by heat current in magnetic bilayers

Onuma, Yuichi*; Adachi, Hiroto; Saito, Eiji; Maekawa, Sadamichi

Physical Review B, 92(22), p.224404_1 - 224404_8, 2015/12

 Times Cited Count:7 Percentile:58.13(Materials Science, Multidisciplinary)

Journal Articles

Generation of spin currents by surface plasmon resonance

Uchida, Kenichi*; Adachi, Hiroto; Kikuchi, Daisuke*; Ito, Shun*; Qiu, Z.*; Maekawa, Sadamichi; Saito, Eiji

Nature Communications (Internet), 6, p.5910_1 - 5910_8, 2015/01

 Times Cited Count:36 Percentile:13.08(Multidisciplinary Sciences)

Journal Articles

Enhanced dc spin pumping into a fluctuating ferromagnet near Tc

Onuma, Yuichi*; Adachi, Hiroto; Saito, Eiji; Maekawa, Sadamichi

Physical Review B, 89(17), p.174417_1 - 174417_10, 2014/05

 Times Cited Count:61 Percentile:6.75(Materials Science, Multidisciplinary)

Journal Articles

Separation of longitudinal spin Seebeck effect from anomalous Nernst effect; Determination of origin of transverse thermoelectric voltage in metal/insulator junctions

Kikkawa, Takashi*; Uchida, Kenichi*; Daimon, Shunsuke*; Shiomi, Yuki*; Adachi, Hiroto; Qiu, Z.*; Hou, D.*; Jin, X.-F.*; Maekawa, Sadamichi; Saito, Eiji

Physical Review B, 88(21), p.214403_1 - 214403_11, 2013/12

 Times Cited Count:89 Percentile:3.81(Materials Science, Multidisciplinary)

Journal Articles

Spin-wave spin current in magnetic insulators

Uchida, Kenichi*; Adachi, Hiroto; Kajiwara, Yosuke*; Maekawa, Sadamichi; Saito, Eiji

Solid State Physics, 64; Recent Advances in Magnetic Insulators; From Spintronics to Microwave Applications, p.1 - 27, 2013/11

 Times Cited Count:6 Percentile:87.82(Physics, Condensed Matter)

Journal Articles

Spin current; Experimental and theoretical aspects

Maekawa, Sadamichi; Adachi, Hiroto; Uchida, Kenichi*; Ieda, Junichi; Saito, Eiji

Journal of the Physical Society of Japan, 82(10), p.102002_1 - 102002_23, 2013/10

 Times Cited Count:65 Percentile:20(Physics, Multidisciplinary)

Journal Articles

Unidirectional spin-wave heat conveyer

An, Toshu*; Vasyuchka, V. I.*; Uchida, Kenichi*; Chumak, A. V.*; Yamaguchi, Kazuya*; Harii, Kazuya; Oe, Junichiro*; Jungfleisch, M. B.*; Kajiwara, Yosuke*; Adachi, Hiroto; et al.

Nature Materials, 12(6), p.549 - 553, 2013/06

 Times Cited Count:85 Percentile:4.1(Chemistry, Physical)

Journal Articles

Theory of the spin Seebeck effect

Adachi, Hiroto; Uchida, Kenichi*; Saito, Eiji; Maekawa, Sadamichi

Reports on Progress in Physics, 76(3), p.036501_1 - 036501_20, 2013/03

 Times Cited Count:250 Percentile:3.49(Physics, Multidisciplinary)

The spin Seebeck effect refers to the generation of a spin voltage caused by a temperature gradient in a ferromagnet, which enables the thermal injection of spin currents from the ferromagnet into an attached nonmagnetic metal over a macroscopic scale of several millimeters. The inverse spin Hall effect converts the injected spin current into a transverse charge voltage, thereby producing electromotive force as in the conventional charge Seebeck device. Recent theoretical and experimental efforts have shown that the magnon and phonon degrees of freedom play crucial roles in the spin Seebeck effect. In this paper, we present the theoretical basis for understanding the spin Seebeck effect and briefly discuss other thermal spin effects.

Journal Articles

Observation of the spin Seebeck effect in epitaxial Fe$$_{3}$$O$$_{4}$$ thin films

Ramos, R.*; Kikkawa, Takashi*; Uchida, Kenichi*; Adachi, Hiroto; Lucas, I.*; Aguirre, M.*; Algarabel, P.*; Morell$'o$n, L.*; Maekawa, Sadamichi; Saito, Eiji; et al.

Applied Physics Letters, 102(7), p.072413_1 - 072413_5, 2013/02

 Times Cited Count:120 Percentile:2.5(Physics, Applied)

Journal Articles

Spin Seebeck effect in antiferromagnets and compensated ferrimagnets

Onuma, Yuichi; Adachi, Hiroto; Saito, Eiji; Maekawa, Sadamichi

Physical Review B, 87(1), p.014423_1 - 014423_7, 2013/01

 Times Cited Count:86 Percentile:4.03(Materials Science, Multidisciplinary)

Journal Articles

Thermal spin pumping and magnon-phonon-mediated spin-Seebeck effect

Uchida, Kenichi*; Ota, Takeru*; Adachi, Hiroto; Xiao, J.*; Nonaka, Tatsumi*; Kajiwara, Yosuke*; Bauer, G. E. W.*; Maekawa, Sadamichi; Saito, Eiji

Journal of Applied Physics, 111(10), p.103903_1 - 103903_11, 2012/05

 Times Cited Count:99 Percentile:3.58(Physics, Applied)

Journal Articles

Acoustic spin pumping; Direct generation of spin currents from sound waves in Pt/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ hybrid structures

Uchida, Kenichi*; Adachi, Hiroto; An, Toshu*; Nakayama, Hiroyasu*; Toda, Masaya*; Hillebrands, B.*; Maekawa, Sadamichi; Saito, Eiji

Journal of Applied Physics, 111(5), p.053903_1 - 053903_8, 2012/03

 Times Cited Count:20 Percentile:32.03(Physics, Applied)

Using a Pt/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ (YIG) hybrid structure attached to a piezoelectric actuator, we demonstrate the generation of spin currents from sound waves. This "acoustic spin pumping" is caused by the sound wave generated by the piezoelectric actuator, which then modulates the distribution function of magnons in the YIG layer and results in a pure-spin-current injection into the Pt layer across the Pt/YIG interface. In the Pt layer, this injected spin current is converted into an electric voltage due to the inverse spin-Hall effect. The ISHE induced by the acoustic spin pumping is detected by measuring a voltage in the Pt layer at the piezoelectric resonance frequency of the actuator coupled with the Pt/YIG system. Our model calculation based on the linear response theory provides us with a qualitative and quantitative understanding of the acoustic spin pumping in the Pt/YIG system.

34 (Records 1-20 displayed on this page)