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Journal Articles

Unveiling the hidden risk: Cryo-TRLFS identifies critically elusive UO$$_{2}$$ alteration phases under chemically complex conditions

Mei, H.*; Aoyagi, Noboru; Takaki, Seiya; Saito, Takumi*

Journal of Hazardous Materials, 514, p.142804_1 - 142804_11, 2026/08

JAEA Reports

Irradiation test using foreign reactor, 2; Study of irradiation test with capsule temperature control system (Joint research)

Omori, Takazumi; Fuyushima, Takumi; Sayato, Natsuki; Saito, Nagatsuki; Takabe, Yugo; Endo, Yasuichi; Inoue, Shuichi; Wojtania, G.*; Migdal, M.*; Takeuchi, Tomoaki; et al.

JAEA-Technology 2026-006, 47 Pages, 2026/06

JAEA-Technology-2026-006.pdf:3.01MB

Japan Materials Testing Reactor (JMTR), which served as the core facility for neutron irradiation research including materials research and radioisotope production, has been decommissioned. As a result, it has become difficult to continue conducting irradiation tests domestically, as well as to transfer the operational expertise and irradiation technologies associated with test reactors, to address these challenges, it was decided to initiate JMTR alternative irradiation, in which foreign irradiation reactors are utilized to partially substitute for JMTR's irradiation capabilities. As a first step, based on the "Arrangement between the National Centre for Nuclear Research and the Japan Atomic Energy Agency for Cooperation in Research and Development on Testing Reactor". The MARIA reactor (30 MW) owned by the National Centre for Nuclear Research (NCBJ) was selected as the neutron irradiation facility, a temperature control system, which is one of JMTR's irradiation technologies, was introduced into the MARIA reactor, and irradiation tests were conducted. The results of this irradiation test confirmed that the combination of the newly introduced temperature control device and the JMTR irradiation test system operates without issues even after an irradiation period exceeding 150 days, it was also demonstrated that the tests could be conducted while continuously measuring the thermocouple temperature inside the capsule during irradiation, as well as the output of the LVDT and SPGD. Furthermore, regarding the constant temperature control of the irradiation capsule at 300$$^{circ}$$C constant temperature control test, which is highly demanded in materials irradiation testing, was conducted, during reactor power increases, when temperature fluctuations become significant, temperature control was maintained within $$pm$$6.3$$^{circ}$$C, while during power decreases, it was controlled within $$pm$$26.0$$^{circ}$$C. These results indicate that irradiation testing with irradiation temperature control system developed by JMTR, can also be performed in the MARIA reactor, it was confirmed that it can be offered as an alternative irradiation field.

JAEA Reports

Conceptual design of pilot ADS

Nishihara, Kenji; Fukushima, Masahiro; Abe, Takumi; Katano, Ryota; Yee-Rendon, B.; Iwamoto, Hiroki; Sugawara, Takanori; Obayashi, Hironari; Saito, Shigeru

JAEA-Research 2025-013, 125 Pages, 2026/03

JAEA-Research-2025-013.pdf:4.68MB

A conceptual design for a pilot Accelerator Driven subcritical System (ADS) was developed as a precursor to a commercial ADS aimed at partitioning and transmutation of minor actinides. The output of the pilot ADS was set at 200 MW. Based on safety assessment results, the design incorporates deep subcriticality and safety rods. Core design, accelerator design, target design, and in-vessel equipment design were performed, clarifying the specific concept.

Journal Articles

Diffusion of Cs$$^{+}$$, I$$^{-}$$ and HDO onto pre-Neogene sedimentary rocks

Hou, L.*; Fukatsu, Yuta; Okamoto, Shunichi*; Toda, Kanako*; Nakata, Kotaro*; Nohara, Shintaro*; Ishidera, Takamitsu; Saito, Takumi*

Journal of Nuclear Science and Technology, 62(11), p.1121 - 1134, 2025/11

 Times Cited Count:1 Percentile:50.28(Nuclear Science & Technology)

Journal Articles

Sorption mechanism of europium(III) onto metakaolin-based geopolymers

Yildirim, A. C.*; Mei, H.*; Toda, Kanako*; Aoyagi, Noboru; Saito, Takumi*

Applied Clay Science, 274, p.107853_1 - 107853_9, 2025/09

 Times Cited Count:1 Percentile:0.00(Chemistry, Physical)

Journal Articles

Bimodal pore size evolution of metakaolin-based geopolymers at the initial stage of curing; A Small-angle neutron scattering study

Toda, Kanako*; Motokawa, Ryuhei; Saito, Takumi*

Journal of Physical Chemistry C, 129(36), p.16261 - 16271, 2025/09

 Times Cited Count:1 Percentile:0.00(Chemistry, Physical)

Journal Articles

U(VI) adsorption on mudstone in the presence of carbonate; Batch experiments, modeling, cryo-TRLFS and PARAFAC analysis

Mei, H.; Aoyagi, Noboru; Saito, Takumi*; Tanaka, Kazuya; Sugiura, Yuki; Tachi, Yukio

Applied Clay Science, 276, p.107944_1 - 107944_8, 2025/07

 Times Cited Count:3 Percentile:78.65(Chemistry, Physical)

Journal Articles

Sorption of Cs$$^{+}$$ and Eu$$^{3+}$$ onto coherent and melange-type pre-neogene sedimentary rocks

Hou, L.*; Toda, Kanako*; Mei, H.; Aoyagi, Noboru; Saito, Takumi*

Journal of Nuclear Science and Technology, 61(11), p.1488 - 1498, 2024/11

 Times Cited Count:4 Percentile:66.28(Nuclear Science & Technology)

Journal Articles

Trivalent lanthanide sorption onto illite in the presence of carbonate; A Study combining thermodynamic sorption modeling, time-resolved laser fluorescence spectroscopy, and parallel factor analysis

Sugiura, Yuki; Ishidera, Takamitsu; Aoyagi, Noboru; Mei, H.; Saito, Takumi*; Tachi, Yukio

Applied Clay Science, 258, p.107476_1 - 107476_10, 2024/09

 Times Cited Count:4 Percentile:55.29(Chemistry, Physical)

Journal Articles

Application of diffusive gradients in thin films (DGT) for the dynamic speciation of radioactive cesium in Fukushima Prefecture, Japan

Tanaka, Takuro*; Fukuoka, Masafumi*; Toda, Kanako*; Nakanishi, Takahiro; Terashima, Motoki; Fujiwara, Kenso; Niwano, Yuma*; Kato, Hiroaki*; Kobayashi, Natsuko*; Tanoi, Keitaro*; et al.

ACS ES&T Water (Internet), 4(8), p.3579 - 3586, 2024/08

Journal Articles

Comprehensive extraction study using $$N,N$$-dioctylthiodiglycolamic acid; Effect of S donor on metal extraction

Shimojo, Kojiro; Fujiwara, Iori*; Saito, Takumi*; Oshima, Tatsuya*

Analytical Sciences, 40(8), p.1429 - 1436, 2024/08

 Times Cited Count:1 Percentile:8.87(Chemistry, Analytical)

Extraction ability of $$N,N$$-dioctylthiodiglycolamic acid (T-DODGAA), a soft-base sulfur donor ligand with an amide group and a carboxylic acid connected by a thioether chain, for 56 metal ions have been comprehensively investigated and compared with that of N,N-dioctyldiglycolamic acid (DODGAA) with an etheric oxygen atom, a hard-base donor. The p$$K_{a}$$ of the thiodiglycolamic acid framework was determined to be 3.71 $$pm$$ 0.06 in water (0.1 M LiCl, 25$$^{circ}$$C ) by potentiometric titration, indicating that T-DODGAA is a slightly weaker acid than DODGAA (p$$K_{a}$$ = 3.54 $$pm$$ 0.03). T-DODGAA can quantitatively extract various metal ions from the 56 metal ions through a proton-exchange reaction. T-DODGAA provided higher extraction performance than DODGAA for Hf(IV), Cr(III), Fe(III), Ni(II), Cu(II), Pd(II), Ag(I), Au(III), Hg(II), Al(III), and Ga(III), especially for soft metal ions. Furthermore, to demonstrate the practical feasibility of T-DODGAA for hydrometallurgy and metal recycling, we performed selective separation tests of rare metal ions such as Sc(III), Ni(II), Co(II), Pd(II), Au(III), In(III), and Ga(II) in metal-mixed extraction systems.

Journal Articles

Globular pattern formation of hierarchical ceria nanoarchitectures

Aoyagi, Noboru; Motokawa, Ryuhei; Okumura, Masahiko; Ueda, Yuki; Saito, Takumi*; Nishitsuji, Shotaro*; Taguchi, Tomitsugu*; Yomogida, Takumi; Sazaki, Gen*; Ikeda, Atsushi

Communications Chemistry (Internet), 7, p.128_1 - 128_13, 2024/06

 Times Cited Count:3 Percentile:28.33(Chemistry, Multidisciplinary)

Journal Articles

"Invisible" radioactive cesium atoms revealed; Pollucite inclusion in cesium-rich microparticles (CsMPs) from the Fukushima Daiichi Nuclear Power Plant

Miyazaki, Kanako*; Takehara, Masato*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Onuki, Toshihiko*; Takano, Masahide; Shiotsu, Hiroyuki; et al.

Journal of Hazardous Materials, 470(15), p.134104_1 - 134104_11, 2024/05

 Times Cited Count:4 Percentile:36.55(Engineering, Environmental)

Journal Articles

U(VI) sorption on illite in the presence of carbonate studied by cryogenic time-resolved laser fluorescence spectroscopy and parallel factor analysis

Mei, H.; Aoyagi, Noboru; Saito, Takumi*; Tanaka, Kazuya; Sugiura, Yuki; Tachi, Yukio

Applied Geochemistry, 162, p.105926_1 - 105926_8, 2024/02

 Times Cited Count:7 Percentile:66.51(Geochemistry & Geophysics)

Journal Articles

Origin of dissolved organic matter in deep groundwater of marine deposits and its implication for metal binding

Saito, Takumi*; Nishi, Shusaku*; Amano, Yuki; Beppu, Hikari*; Miyakawa, Kazuya

ACS ES&T Water (Internet), 3(12), p.4103 - 4112, 2023/12

Journal Articles

Heterogeneous aggregation of humic acids studied by small-angle neutron and X-ray scattering

Saito, Takumi*; Motokawa, Ryuhei; Okubo, Takahiro*; Miura, Daisuke*; Kumada, Takayuki

Environmental Science & Technology, 57(26), p.9802 - 9810, 2023/07

 Times Cited Count:4 Percentile:22.62(Engineering, Environmental)

Journal Articles

Hydration states of europium(III) adsorbed on silicas with nano-sized pores

Murota, Kento*; Aoyagi, Noboru; Mei, H.; Saito, Takumi*

Applied Geochemistry, 152, p.105620_1 - 105620_11, 2023/05

 Times Cited Count:6 Percentile:49.03(Geochemistry & Geophysics)

Journal Articles

Lanthanide and actinide ion complexes containing organic ligands investigated by surface-enhanced infrared absorption spectroscopy

Hirata, Sakiko*; Kusaka, Ryoji; Meiji, Shogo*; Tamekuni, Seita*; Okudera, Kosuke*; Hamada, Shoken*; Sakamoto, Chihiro*; Honda, Takumi*; Matsushita, Kosuke*; Muramatsu, Satoru*; et al.

Inorganic Chemistry, 62(1), p.474 - 486, 2023/01

 Times Cited Count:4 Percentile:27.55(Chemistry, Inorganic & Nuclear)

Journal Articles

High-temperature gaseous reaction of cesium with siliceous thermal insulation; The Potential implication to the provenance of enigmatic Fukushima cesium-bearing material

Rizaal, M.; Nakajima, Kunihisa; Saito, Takumi*; Osaka, Masahiko; Okamoto, Koji*

ACS Omega (Internet), 7(33), p.29326 - 29336, 2022/08

 Times Cited Count:7 Percentile:30.10(Chemistry, Multidisciplinary)

Journal Articles

Current status of Geological disposal by "all-Japan" activities, 6; Post-closure safety assessment (2)

Tachi, Yukio; Saito, Takumi*; Kirishima, Akira*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 64(5), p.290 - 295, 2022/05

no abstracts in English

159 (Records 1-20 displayed on this page)