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C control rods in Fukushima Daiichi nuclear reactors during meltdown; B-Li isotopic signatures in cesium-rich microparticlesFueda, Kazuki*; Takami, Ryu*; Minomo, Kenta*; Morooka, Kazuya*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Saito, Takumi*; Shiotsu, Hiroyuki; Onuki, Toshihiko*; et al.
Journal of Hazardous Materials, 428, p.128214_1 - 128214_10, 2022/04
Times Cited Count：6 Percentile：68.71(Engineering, Environmental)Kumazoe, Hiroyuki*; Igarashi, Yasuhiko*; Iesari, F.*; Shimizu, Ryota*; Komatsu, Yuya*; Hitosugi, Taro*; Matsumura, Daiju; Saito, Hiroyuki*; Iwamitsu, Kazunori*; Okajima, Toshihiko*; et al.
AIP Advances (Internet), 11(12), p.125013_1 - 125013_5, 2021/12
Times Cited Count：2 Percentile：7.86(Nanoscience & Nanotechnology)Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.
Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12
Times Cited Count：6 Percentile：51.19(Geosciences, Multidisciplinary)The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.
, Zn
+, and CoKato, Tomoaki*; Yu, Q.*; Tanaka, Kazuya; Kozai, Naofumi; Saito, Takumi*; Onuki, Toshihiko
Journal of Environmental Sciences, 86, p.78 - 86, 2019/12
Times Cited Count：2 Percentile：8.42(Environmental Sciences)This paper investigated the fate of the dissolved permanganate in aqueous solution after contact with bacterial cells and metal accumulation during precipitation of Mn oxides. When Mn(VII) was contacted with bacterial cells, cells were damaged and Mn(VII) was reduced by cells to lower valence and precipitated as Mn oxides (biomass Mn oxides). When Co ions were present, Co was incorporated into Mn oxides as Co
. These results suggest that Mn(VII) can be used to remove metal ions when introduced to wastewater as disinfectant.
Saito, Takumi; Terashima, Motoki; Aoyagi, Noboru; Nagao, Seiya*; Fujitake, Nobuhide*; Onuki, Toshihiko
Environmental Science; Processes & Impacts, 17(8), p.1386 - 1395, 2015/08
Times Cited Count：9 Percentile：32.46(Chemistry, Analytical)The deep groundwater HSs were different from surface HSs, having high aliphaticities, sulfur contents, and small molecular sizes. The amounts of their acidic functional groups were comparable to or slightly larger than those of surface HSs; however, the magnitude of Cu binding to the deep groundwater HSs was smaller. The NICA-Donnan model attributed this to the binding of Cu to chemically homogeneous carboxylic-type sites via mono-dentate coordination at relatively low pH. The binding mode tended to shift to multi-dentate coordination with carboxylic-type and probably more heterogeneous alcoholic hydroxide-type groups at higher pH. This study shows the particularity of the deep groundwater HSs in terms of their physicochemical and ion-binding properties, compared with surface HSs.
, Na, I
and HTO in granodiorite; Laboratory-scale results and their extrapolation to the in situ conditionTachi, Yukio; Ebina, Takanori*; Takeda, Chizuko*; Saito, Toshihiko*; Takahashi, Hiroaki*; Ouchi, Yuji*; Martin, A. J.*
Journal of Contaminant Hydrology, 179, p.10 - 24, 2015/08
Times Cited Count：29 Percentile：73.48(Environmental Sciences)Matrix diffusion and sorption are important processes in the assessment of radionuclide transport in crystalline rocks. Diffusion and sorption parameters for Cs, Na, I and HTO were determined by through-diffusion and batch sorption experiments using granodiorite samples from the Grimsel Test Site, Switzerland. The De values were in the order Cs, Na, HTO, I. The capacity factor and Kd values show the same trends. The dual depth profiles for Cs and Na can be interpreted by a near-surface Kd increment. The microscopic analysis indicated that this is caused by high porosity and sorption capacities in disturbed biotite minerals on the sample surface. The Kd values derived from the dual profiles are likely to correspond to Kd dependence on the grain sizes of crushed samples in the batch experiments. The results of the in situ LTD experiments were interpreted reasonably well by using transport parameters derived from laboratory data and extrapolating them to in situ conditions.
Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Usui, Aya; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Nara, Takayuki; et al.
JAEA-Review 2013-059, JAEA Takasaki Annual Report 2012, P. 179, 2014/03
Three electrostatic accelerators at TIARA were operated on schedule in fiscal year 2012 except changing its schedule by cancellations of users. The yearly operation time of the 3 MV tandem accelerator, the 400 kV ion implanter and the 3MV single-ended accelerator were in the same levels as the ordinary one, whose operation time totaled to 2,073, 1,847 and 2,389 hours, respectively. The tandem accelerator had no trouble, whereas the ion implanter and the single-ended accelerator stopped by any troubles for one day and four days, respectively. The molecular ion beam of helium hydride was generated by the ion implanter, because the users required irradiation of several cluster ions in order to study the effect of irradiation. As a result, its intensity of beam was 50 nA at 200 kV. The ion beam of tungsten (W) at 15 MeV was accelerated by the tandem accelerator, whose intensity was 20 nA at charge state of 4+, because of the request from a researcher in the field of nuclear fusion.
Isobe, Kanetsugu; Alimov, V. Kh.*; Taguchi, Akira*; Saito, Makiko; Torikai, Yuji*; Hatano, Yuji*; Yamanishi, Toshihiko
Journal of Plasma and Fusion Research SERIES, Vol.10, p.81 - 84, 2013/02
The distribution of hydrogen trapping sites on W surface exposed with D plasma was examined by the techniques of imaging plate and autoradiography. Recrystallized W specimens were exposed with D plasma at around 495 and 550 K to the same fluence of 10
D/m. Then, tritium was introduced into specimen by the exposure to tritium gaseous at 473 K. After that, the tritium distribution on W surface was examined by the techniques of imaging plate and autoradiography. From the results of the imaging plate, tritium was found to be highly concentrated within the area exposed with D plasma and the concentration of tritium was slightly varied even in that area. In the autoradiograph of W surface, it was found that tritium concentrated on the grain boundary and blisters.
Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Nara, Takayuki; Kitano, Toshihiko*; et al.
JAEA-Review 2012-046, JAEA Takasaki Annual Report 2011, P. 173, 2013/01
The three electrostatic accelerators at the TIARA had no mechanical damage when the Tohoku earthquake happened on March 11, 2011. But, they could not be operated during April, due to the influence of planned power outage by TEPCO. These accelerators additionally operated on Saturday for ten days in order to compensate for the lost experiment time. As a result, the yearly operation time had kept the same level as the ordinary one. The ion beam of erbium (Er) with 11.7MeV was accelerated newly by the tandem accelerator, whose intensity was 20nA at charge state of 3+. The sequential generation/irradiation of two different kinds of fullerene ions was achieved at the ion implanter by a mixed powder method without exchange of the Freeman type ion source by the user's request.
Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Nara, Takayuki; Kitano, Toshihiko*; et al.
Dai-7-Kai Takasaki Oyo Kenkyu Shimpojiumu Yoshishu, P. 119, 2012/10
The three electrostatic accelerators at TIARA had no damage when the Tohoku earthquake happened on March 11, 2011. But, they could not be operated until end of April, due to the influence of planned power outage and keep out into the controlled area for radiation. These accelerators additionally operated on Saturday for twelve days in order to compensate for the lost experiment time. Therefore, the yearly operation time had kept the same level as the ordinary one. The tandem accelerator has stopped leakage of the SF
gas from the base flange on the tank by the Viton gasket of rectangular cross section at the new type.
Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; Yamada, Naoto*; et al.
Dai-25-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.64 - 66, 2012/07
The three electrostatic accelerators at the TIARA had no damage when the Tohoku earthquake happened on March 11, 2011. But, they could not be operated until end of April, due to the influence of planned power outage and keep out into the controlled area for radiation. These accelerators additionally operated on Saturday for twelve days in order to compensate for the lost experiment time. Therefore, the yearly operation time had kept the same level as the ordinary one. The tandem accelerator has stopped leakage of the SF gas from the base flange on the tank by the Viton gasket of rectangular cross section at the new type. The ion implanter could generate two kinds of fullerene ions by a mixed material of ions and a controlled temperature of the oven without exchange of ion source.
Miura, Kuniaki*; Shibata, Akira; Nakamura, Jinichi; Ogasawara, Toshihiko*; Saito, Takashi; Tsuchiya, Kunihiko
JAEA-Conf 2011-003, p.193 - 195, 2012/03
In the Fukushima accident, measurement failure of water level was one of the most important factors which caused this serious situation. The differential pressure type water level indicators are widely used in various place of nuclear plant but after the accident of TMI-2, the need of other reliable method has been demanded. And the BICOTH type and the TRICOTH type water level indicator for light water power reactors had been developed for in-pile water level indicator but currently those are not adopted to a nuclear power plant. In this study, the development of new type water level indicator which composed of thermocouple and heater, and the demonstration test and characteristic evaluation of the water level indicator were described.
Agematsu, Takashi; Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Yokota, Wataru; et al.
JAEA-Review 2011-043, JAEA Takasaki Annual Report 2010, P. 173, 2012/01
Three electrostatic accelerators of TIARA were operated smoothly in FY 2010, and all the planned experiments were carried out except those canceled by users or the impact of Great East Japan Earthquake on March 11, 2011. On the other hand, Saturday operation for experiments was carried out after October on the Global Nuclear-Human Resource Development Initiative. The yearly operation time of the tandem accelerator, the single-ended accelerator and the ion implanter amounted to 2116, 2367 and 1800 hours, respectively, which were similar to those of usual years. Regarding the single-ended accelerator, the generator in the high-voltage terminal failed and was replaced with new one. A switching magnet was installed for a new branch beam line of the ion implanter. As to the tandem accelerator, In ion was generated and accelerated at intensity of 500 nA.
Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Agematsu, Takashi; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; et al.
Dai-24-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.125 - 128, 2011/07
The yearly operation time of three electrostatic accelerators at TIARA of Japan Atomic Energy Agency is keeping the same level since 2000, the tandem accelerator, the ion implanter and the single-ended accelerator amounted to about 2000, 1900 and 2500 hours, respectively. Three electrostatic accelerators did not have damage when the Tohoku Earthquake occurred on March 11, 2011. However, these accelerators were not able to operate during the planned power outage by Tokyo Electric Power Company (TEPCO). The tandem accelerator accelerated ion beam of In, which gave intensity of 500nA with stability. Additionally, the ion implanter generated maximum 400nA at ion beam of Gd, which was used in experiments for the users.
Agematsu, Takashi; Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Yokota, Wataru; et al.
JAEA-Review 2010-065, JAEA Takasaki Annual Report 2009, P. 181, 2011/01
Three electrostatic accelerators of TIARA were operated smoothly in FY 2009, and all the planned experiments were carried out except those canceled by users. The yearly operation time of the tandem accelerator, the single-ended accelerator and the ion implanter amounted to 2100, 2416 and 1866 hours, respectively. Regarding the single-ended accelerator, the radio frequency oscillator of the ion source mounted in high-voltage terminal and the sequencer for control of the SB beam line failed, and they were replaced. The oven controller of Freeman ion source of the ion implanter was renewed. As to the tandem accelerator, Mn ion was successfully generated and accelerated with intensity of 150 nA.
Chiba, Atsuya; Uno, Sadanori; Yamada, Keisuke; Yokoyama, Akihito; Agematsu, Takashi; Yokota, Wataru; Kitano, Toshihiko*; Takayama, Terumitsu*; Kanai, Shinji*; Orimo, Takao*; et al.
Dai-23-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.119 - 122, 2010/11
Operation times of each accelerator are keeping the same level as in recent 10 years, Tandem accelerator, Single-ended and Ion implanter amounted to about 2,000, 2,500 and 1,900 hours, respectively. In the last fiscal year, we succeeded in maintaining the terminal voltage of the tandem accelerator to high stability for long periods by exchanging the material of a corona-probe needle to the tungsten (NPS Co.). In the ion-implanter, the oven control system equipped with the Freeman ion source was renewed. There was no trouble to affect on the machine-time in the last fiscal year, so the all planned experiments were carried out.
Nakamura, Hirofumi; Kobayashi, Kazuhiro; Yokoyama, Sumi*; Saito, Shigeru; Yamanishi, Toshihiko; Kikuchi, Kenji*
Journal of Plasma and Fusion Research SERIES, Vol.9, p.326 - 331, 2010/08
Based on results of tritium measurement in the SS316 specimens irradiated up to 5.9 dpa in the SINQ target (580 MeV proton) using a thermal desorption (TDS) method, trap site density and trap energy in the materials induced by the high-energy proton irradiation have been evaluated by means of the numerical tritium transport analysis. The results indicate that almost residual tritium in the SS316 specimen exists in the trap site, whose trap density is maximum 238 appm (5.9 dpa) and trap energy is 
1.4 eV, and that tritium release by the TDS is mainly attributed to the disappearance of the trap sites by the specimen heating, whose activation energy is about 0.7 eV. The trap site density seems to be almost proportional to the irradiation dose (dpa). Additionally, irradiation conditions such as the dose or irradiation temperature do not affect on the trapping mechanism.
Sakaki, Hironao; Nishiuchi, Mamiko; Yogo, Akifumi; Bolton, P.; Hori, Toshihiko; Kondo, Kiminori; Saito, Fumihiro; Ueno, Masayuki; Takahashi, Hiroki; Iwase, Hiroshi*; et al.
Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.94 - 96, 2010/05
The concept of a compact ion particle accelerator has become attractive in view of recent progress in laser-driven hadrons acceleration. The Photo Medical Research Centre (PMRC) of JAEA was established to address the challenge of laser-driven ion accelerator development for hadrons therapeutic. In the development of the instrument, it is necessary to do the bench-mark of the amount of the different types of radiation by the simulation code for shielding. The Monte Carlo Particle and Heavy Ion Transport code (PHITS) was used for bench-mark the dose on laser-shot radiations of short duration. The code predicts reasonably well the observed total dose as measured with a glass dosimeter in the laser-driven radiations.
Chiba, Atsuya; Uno, Sadanori; Yamada, Keisuke; Yokoyama, Akihito; Agematsu, Takashi; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Koka, Masashi*; Aoki, Yuki*; et al.
Dai-22-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.104 - 106, 2010/01
no abstracts in English
Agematsu, Takashi; Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Yokota, Wataru; et al.
JAEA-Review 2009-041, JAEA Takasaki Annual Report 2008, P. 175, 2009/12
Three electrostatic accelerators of TIARA were operated smoothly in FY 2008, and all the planned experiments were carried out except those canceled by users. The yearly operation time of the tandem accelerator, the single-ended accelerator and the ion implanter amounted to 2009, 2426 and 1882 hours, respectively. Regarding the tandem accelerator, the control system was renewed, and the unstable acceleration voltage caused by mechanical vibration reduced by adjusting the driving mechanism of the pellet chains. The SF gas for the single-ended accelerator was purified, and its storage tank was repainted. As to the ion implanter, Bi
ion, which was requested by users, was successfully generated and accelerated with intensity of 0.5
A.
