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論文

Negative Te spin polarization responsible for ferromagnetic order in the doped topological insulator V $_{0.04}$ (Sb $_{1-x}$ Bi $_{x}$ ) $_{1.96}$ Te $_{3}$

Ye, M.*; Xu, T.*; Li, G.*; Qiao, S.*; 竹田幸治; 斎藤祐児; Zhu, S.-Y.*; Nurmamat, M.*; 角田一樹*; 石田行章*; et al.

Physical Review B, 99(14), p.144413_1 - 144413_7, 2019/04

https://doi.org/10.1103/PhysRevB.99.144413

パーセンタイル：100(Materials Science, Multidisciplinary)

We investigate the microscopic origin of ferromagnetism coupled with topological insulators in V-doped (Sb,Bi) $_{2}$ Te $_{3}$ employing X-ray magnetic circular dichroism and angle-resolved two-photon photoemission spectroscopies, combined with first-principles calculations. We found an magnetic moment at the Te site anti-parallel to that of the V and Sb sites, which plays a key role in the ferromagnetic order. We ascribe it to the hybridization between Te 5 and V 3 majority spin states at the Fermi energy, consistent with the Zener-type - exchange interaction scenario. The substitution of Bi for Sb suppresses the bulk ferromagnetism by introducing extra electron carriers in the majority spin channel of the Te states that compensates the antiparallel magnetic moment on the Te site. Our findings reveal important clues to designing magnetic topological insulators with higher Curie temperature that work under ambient conditions.

論文

Dirac gap opening and Dirac-fermion-mediated magnetic coupling in antiferromagnetic Gd-doped topological insulators and their manipulation by synchrotron radiation

Shikin, A. M.*; Estyunin, D. A.*; Surnin, Yu. I.*; Koroleva, A. V.*; Shevchenko, E. V.*; Kokh, K. A.*; Tereshchenko, O. E.*; Kumar, S.*; Schwier, E. F.*; 島田賢也*; et al.

Scientific Reports (Internet), 9(1), p.4813_1 - 4813_17, 2019/03

https://doi.org/10.1038/s41598-019-41137-w

パーセンタイル：100(Multidisciplinary Sciences)

A new kind of magnetically-doped antiferromagnetic (AFM) topological insulators (TIs), Bi $_{1.09}$ Gd $_{0.06}$ Sb $_{0.85}$ Te $_{3}$ , has been studied by angle-resolved photoemission, superconducting magnetometry (SQUID) and X-ray magnetic circular dichroism (XMCD). It has been shown that this TI is characterized by the Dirac gap at the Fermi level. In the paramagnetic phase, a surface magnetic layer is supposed to develop, where the coupling between the Gd magnetic moments is mediated by the topological surface states (TSSs). This assumption can be confirmed by opening a gap at the Dirac point indicated by the surface-sensitive ARPES, a weak hysteresis loop measured by SQUID, the XMCD showing a surface magnetic moment and the temperature dependence of electrical resistance demonstrating a mid-gap semiconducting behavior, which correlates with the temperature dependence of the surface magnetization and confirms the conclusion that only TSSs are located at the Fermi level.

論文

Manifestation of electron correlation effect in 5 states of uranium compounds revealed by 4-5 resonant photoelectron spectroscopy

藤森伸一; 小畠雅明; 竹田幸治; 岡根哲夫; 斎藤祐児; 藤森淳; 山上浩志; 芳賀芳範; 山本悦嗣; 大貫惇睦*

Physical Review B, 99(3), p.035109_1 - 035109_5, 2019/01

https://doi.org/10.1103/PhysRevB.99.035109

パーセンタイル：100(Materials Science, Multidisciplinary)

In the present study, we have elucidated the nature of the electron correlation effect in uranium compounds by imaging the partial density of states (pDOS) of typical itinerant, localized, and heavy fermion uranium compounds by using the 4-5 resonant photoemission spectroscopy. Obtained pDOS exhibit a systematic trend depending on the physical properties of compounds: Although the coherent peak at the Fermi level can be explained by the band-structure calculation, an incoherent peak emerges on the higher binding energy side () in the cases of localized and heavy fermion compounds. The intensity and energy position of the incoherent peak is increased and shifted to a higher binding energy as the localization of the state increases. These behaviors are consistent with the prediction of the Mott metal-insulator transition, suggesting that the Hubbard- type mechanism takes an essential role in the electronic structure of actinide materials.

論文

Electronic structure of URuSi studied by photoelectron spectroscopy (INVITED)

藤森伸一; 竹田幸治; 岡根哲夫; 斎藤祐児; 藤森淳; 山上浩志; 芳賀芳範; 山本悦嗣; 大貫惇睦*

Progress in Nuclear Science and Technology (Internet), 5, p.82 - 85, 2018/11

https://doi.org/10.15669/pnst.5.82

One of the most remarkable properties of actinide compounds is the coexistence of superconductivity and magnetic ordering which has been realized in several strongly-correlated uranium based compounds. In these compounds, both superconductivity and magnetic ordering originate from U 5f states. To understand the origin of the coexistence as well as the mechanism of the superconductivity, it is essential to reveal their U 5f electronic structures. In this presentation, the U 5f electronic structures of heavy Fermion superconductors UPdAl and URuSi studied by photoelectron spectroscopy using soft X-rays from SPring-8 BL23SU are presented. For UPdAl, U 4d-5f resonant photoemission experiment was performed, and its partial U 5f spectrum was revealed experimentally. Furthermore, we have applied the three-dimentional ARPES to the hidden order compound URuSi, and revealed its complete 3D electronic structure in the paramagnetic phase. Their electronic structures are discussed based on these results.

論文

Soft X-ray magnetic circular dichroism study on UGe $_{2}$

竹田幸治; 岡根哲夫; 斎藤祐児; 山上浩志; 山本悦嗣; 芳賀芳範

Progress in Nuclear Science and Technology (Internet), 5, p.171 - 174, 2018/11

In order to investigate the electronic and magnetic states of UGe $_{2}$ element-specifically, we have performed soft X-ray magnetic circular dichroism experiments at the U N $_{4,5}$ and Ge L $_{2,3}$ absorption edges. We have detected the XMCD signals at both the U and Ge sites and observed clear hysteresis loops in the ferromagnetic (FM) state at T = 5.5 K. From the branching ratio B, it is found that the occupation number of 5f electrons (n $^{5f}$ ) in UGe $_{2}$ is close to 3. In addition, applying the magneto-optical sum rules analysis to the XMCD spectrum at the U N $_{4,5}$ edges, the ratio of orbital magnetic moment to the spin magnetic moment (-M $_{L}$ /M $_{S}$ ) is estimated to be 2.17. These values of B and -M $_{L}$ /M $_{S}$ are comparable compared with the results of other FM superconductors: URhGe and UCoGe

論文

Local magnetic states of the weakly ferromagnetic iron-based superconductor Sr $_{2}$ VFeAsO $_{3-delta}$ studied by X-ray magnetic circular dichroism

堀尾眞史*; 竹田幸治; 並木宏允*; 片桐隆雄*; 若林勇希*; 坂本祥哉*; 野中洋亮*; 芝田悟朗*; 池田啓祐*; 斎藤祐児; et al.

Journal of the Physical Society of Japan, 87(10), p.105001_1 - 105001_2, 2018/10

https://doi.org/10.7566/JPSJ.87.105001

被引用回数：1 パーセンタイル：49.95(Physics, Multidisciplinary)

We have performed X-ray magnetic circular dichroism (XMCD) measurements on the iron-based superconductor Sr $_{2}$ VFeAsO $_{3-delta}$ to study the origin of weak ferromagnetism (WFM) reported for this compound. While Fe 3d electrons show a magnetic response similar to the other iron pnictides, signals from V 3d electrons remain finite at zero magnetic field and may be responsible for the WFM.

論文

Cation distribution and magnetic properties in ultrathin (Ni $_{1-x}$ Co $_{x}$ )Fe $_{2}$ O $_{4}$ (x=0-1) layers on Si(111) studied by soft X-ray magnetic circular dichroism

若林勇希*; 野中洋亮*; 竹田幸治; 坂本祥哉*; 池田啓祐*; Chi, Z.*; 芝田悟朗*; 田中新*; 斎藤祐児; 山上浩志; et al.

Physical Review Materials (Internet), 2(10), p.104416_1 - 104416_12, 2018/10

https://doi.org/10.1103/PhysRevMaterials.2.104416

We study the electronic structure and magnetic properties of epitaxial (Ni $_{1-x}$ Co $_{x}$ )Fe $_{2}$ O $_{4}$ (111) layers with thicknesses = 1.7 - 5.2 nm grown on Al $_{2}$ O $_{3}$ (111)/Si(111) structures. We revealed the crystallographic (octahedral $O_{h}$ or tetrahedral $T_{d}$ ) sites and the valences of the Fe, Co, and Ni cations using experimental soft X-ray absorption spectroscopy and X-ray magnetic circular dichroism spectra and configuration-interaction cluster-model calculation.

論文

Revising the 4 symmetry in CeCu $_{2}$ Ge $_{2}$ ; Soft X-ray absorption and hard X-ray photoemission spectroscopy

荒谷秀和*; 中谷泰博*; 藤原秀紀*; 川田萌樹*; 金井惟奈*; 山神光平*; 藤岡修平*; 濱本諭*; 久我健太郎*; 木須孝幸*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09

https://doi.org/10.1103/PhysRevB.98.121113

被引用回数：1 パーセンタイル：59.26(Materials Science, Multidisciplinary)

We present a detailed study on the ground state symmetry of the pressure-induced superconductor CeCuGe probed by soft X-ray absorption and hard X-ray photoemission spectroscopy. The revised Ce ground states are determined as $|{Gamma_7}rangle=sqrt{0.45}|{J_{z}=pm frac{5}{2}}rangle - sqrt{0.55}|{mp frac{3}{2}}rangle$ with in-plane rotational symmetry. This gives an in-plane magnetic moment consistent with the antiferromagnetic moment as reported in neutron measurements. Since the in-plane symmetry is the same as that for the superconductor CeCuSi, we propose that the charge distribution along the -axis plays an essential role in driving the system into a superconducting phase.

論文

Element-specific observation of the ferromagnetic ordering process in UCoAl via soft X-ray magnetic circular dichroism

竹田幸治; 斎藤祐児; 岡根哲夫; 山上浩志; 松田達磨*; 山本悦嗣; 芳賀芳範; 大貫惇睦*

Physical Review B, 97(18), p.184414_1 - 184414_7, 2018/05

https://doi.org/10.1103/PhysRevB.97.184414

パーセンタイル：100(Materials Science, Multidisciplinary)

We have performed soft X-ray magnetic circular dichroism (XMCD) experiments on the itinerant-electron metamagnet UCoAl at the U 4-5 ( $N_mathrm{4, 5}$ ) and Co 2-3 ( $L_mathrm{2, 3}$ ) absorption edges in order to investigate the magnetic properties of the U 5 and Co 3 electrons separately. From the line shape of the XMCD spectrum, it is deduced that the orbital magnetic moment of the Co 3 electrons is unusually large. Through the systematic temperature ()- and magnetic field ()-dependent XMCD measurements, we have obtained two types of the magnetization curve as a function of and (M-H curve and M-T curve, respectively). The metamagnetic transition from a paramagnetic state to a field-induced ferromagnetic state was observed clearly under 15 K at $H_mathrm{M}$ . The value of the $H_mathrm{M}$ and its -dependence agree well between the U and Co sites, and the bulk magnetization. Whereas, we have discovered the remarkable differences in the M-H and M-T curves between the U and Co sites. The present findings show clearly that the role of the Co 3 electrons should be considered more carefully in order to understand the origin of the magnetic ordering in UCoAl.

論文

Evidence for momentum-dependent heavy fermionic electronic structures; Soft X-ray ARPES for the superconductor CeNi $_{2}$ Ge $_{2}$ in the normal state

中谷泰博*; 荒谷秀和*; 藤原秀紀*; 森健雄*; 鶴田篤史*; 橘祥一*; 山口貴司*; 木須孝幸*; 山崎篤志*; 保井晃*; et al.

Physical Review B, 97(11), p.115160_1 - 115160_7, 2018/03

https://doi.org/10.1103/PhysRevB.97.115160

被引用回数：1 パーセンタイル：59.26(Materials Science, Multidisciplinary)

We present clear experimental evidence for the momentum-dependent heavy fermionic electronic structures of the 4-based strongly correlated system CeNi $_{2}$ Ge $_{2}$ by soft X-ray angle-resolved photoemission spectroscopy. A comparison between the experimental three-dimensional quasiparticle dispersion of LaNi $_{2}$ Ge $_{2}$ and CeNi $_{2}$ Ge $_{2}$ has revealed that heavy fermionic electronic structures are seen in the region surrounding at a specific momentum. Furthermore, the wave vectors between the observed "heavy spots" are consistent with a result of neutron scattering reflecting magnetic correlations, which could be a trigger of the superconductivity in CeNi $_{2}$ Ge $_{2}$ .

論文

Preferred site occupation of 3 atoms in Ni $_{x}$ Fe $_{4-x}$ N ( = 1 and 3) films revealed by X-ray absorption spectroscopy and magnetic circular dichroism

高田郁弥*; 伊藤啓太*; 竹田幸治; 斎藤祐児; 高梨弘毅*; 木村昭夫*; 末益崇*

Physical Review Materials (Internet), 2(2), p.024407_1 - 024407_5, 2018/02

https://doi.org/10.1103/PhysRevMaterials.2.024407

X-ray absorption spectroscopy (XAS) and X-ray magnetic circular dichroism measurements were performed at the Ni and Fe $L_{2,3}$ absorption edges for Ni $_{x}$ Fe $_{4-x}$ N ( = 1 and 3) epitaxial films. Shoulders at approximately 2 eV above the Ni $L_{2,3}$ main peaks in the XAS spectrum of Ni $_{3}$ FeN were interpreted to originate from hybridization of orbitals between Ni 3 at face-centered (II) sites and N 2 at body-centered sites, while such features were missing in NiFe $_{3}$ N film. Similar shoulders were observed at Fe $L_{2,3}$ edges in both films. Hence, Ni atoms preferentially occupied corner (I) sites, where the hybridization was weak because of the relatively long distance between Ni at I sites and N atoms. The relatively large magnetic moment deduced from sum-rule analysis of NiFe $_{3}$ N also showed a good agreement with the presence of Ni atoms at I sites.

論文

Electronic structure and magnetic properties of the half-metallic ferrimagnet Mn $_{2}$ VAl probed by soft X-ray spectroscopies

永井浩大*; 藤原秀紀*; 荒谷秀和*; 藤岡修平*; 右衛門佐寛*; 中谷泰博*; 木須孝幸*; 関山明*; 黒田文彬*; 藤井将*; et al.

Physical Review B, 97(3), p.035143_1 - 035143_8, 2018/01

https://doi.org/10.1103/PhysRevB.97.035143

被引用回数：1 パーセンタイル：59.26(Materials Science, Multidisciplinary)

フェリ磁性体Mn $_{2}$ VAl単結晶の電子構造を軟X線吸収磁気円二色性(XMCD)、軟X線共鳴非弾性散乱(RIX)によって調べた。全ての構成元素のXMCD信号を観測した。Mn L $_{2,3}$ XMCDの結果は、密度汎関数理論を基にしたスペクトル計算により再現でき、Mn 3状態の遍歴的性質が明らかとなった。V L $_{2,3}$ XMCDの結果はイオンモデル計算によって定性的に説明され、V 3電子はかなり局在的である。この描像は、V L $_{3}$ RIXSで明らかとなった局所的な遷移と矛盾しない。

論文

New precise measurement of muonium hyperfine structure interval at J-PARC

上野恭裕*; 青木正治*; 深尾祥紀*; 東芳隆*; 樋口嵩*; 飯沼裕美*; 池戸豊*; 石田啓一*; 伊藤孝; 岩崎雅彦*; et al.

Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11

https://doi.org/10.1007/s10751-016-1381-7

被引用回数：1 パーセンタイル：17.79

MuSEUM is an international collaboration aiming at a new precise measurement of the muonium hyperfine structure at J-PARC (Japan Proton Accelerator Research Complex). Utilizing its intense pulsed muon beam, we expect a ten-fold improvement for both measurements at high magnetic field and zero magnetic field. We have developed a sophisticated monitoring system, including a beam profile monitor to measure the 3D distribution of muonium atoms to suppress the systematic uncertainty.

論文

Electronic structure of ThRuSi studied by angle-resolved photoelectron spectroscopy; Elucidating the contribution of U 5 states in URu $_{2}$ Si $_{2}$

藤森伸一; 小畠雅明; 竹田幸治; 岡根哲夫; 斎藤祐児; 藤森淳; 山上浩志; 松本裕司*; 山本悦嗣; 立岩尚之; et al.

Physical Review B, 96(12), p.125117_1 - 125117_9, 2017/09

https://doi.org/10.1103/PhysRevB.96.125117

被引用回数：1 パーセンタイル：81.49(Materials Science, Multidisciplinary)

The Fermi surface and band structure of $mathrm{ThRu}_2mathrm{Si}_2$ have been studied by angle resolved photoelectron spectroscopy (ARPES) with the incident photon energies of = 665-735 eV. Detailed band structure and the three-dimensional shape of the Fermi surface were derived experimentally, and they are quantitatively explained by the band-structure calculation based on the density functional approximation. Comparison of the experimental ARPES spectra of $mathrm{ThRu}_2mathrm{Si}_2$ with those of $mathrm{URu}_2mathrm{Si}_2$ shows that they have considerably different spectral profiles particularly in the energy range of $E_mathrm{B} = E_mathrm{F}$ - 1 eV. Some energy bands with their energy dispersions of about 1 eV observed in $mathrm{URu}_2mathrm{Si}_2$ are missing in the ARPES spectra of $mathrm{ThRu}_2mathrm{Si}_2$ measured along the same high symmetry line of Brillouin zone, suggesting that U 5 states form these bands in $mathrm{URu}_2mathrm{Si}_2$ . The relationship between the ARPES spectra of $mathrm{URu}_2mathrm{Si}_2$ and $mathrm{ThRu}_2mathrm{Si}_2$ is very different from the case between $mathrm{CeRu}_2mathrm{Si}_2$ and $mathrm{LaRu}_2mathrm{Si}_2$ where their intrinsic difference is limited only in the very vicinity of the Fermi energy. The present result argues that the U 5 electrons in $mathrm{URu}_2mathrm{Si}_2$ have strong hybridization with ligand states, and essentially have an itinerant character.

論文

Electronic structures of U (=Al, Ga, and In) studied by photoelectron spectroscopy

藤森伸一; 小畠雅明; 竹田幸治; 岡根哲夫; 斎藤祐児; 藤森淳; 山上浩志; 芳賀芳範; 山本悦嗣; 大貫惇睦*

Physical Review B, 96(11), p.115126_1 - 115126_10, 2017/09

https://doi.org/10.1103/PhysRevB.96.115126

被引用回数：2 パーセンタイル：66.33(Materials Science, Multidisciplinary)

The electronic structures of U (=Al, Ga, and In) were studied by photoelectron spectroscopy to understand the the relationship between their electronic structure and magnetic properties. The band structures and Fermi surfaces of UAl and UGa were revealed experimentally by angle-resolved photoelectron spectroscopy (ARPES), and they were compared with the result of band structure calculations. The topologies of the Fermi surfaces and the band structures of UAl and UGa were explained reasonably well by the calculation, although bands near the Fermi level ( $E_mathrm{F}$ ) were renormalized owing to the finite electron correlation effect. The topologies of the Fermi surfaces of UAl and UGa are very similar to each other, except for some minor differences. Such minor differences in their Fermi surface or electron correlation effect might take an essential role in their magnetism.

論文

Experimental observation of temperature and magnetic-field evolution of the 4 states in CeFe $_{2}$ revealed by soft X-ray magnetic circular dichroism

斎藤祐児; 保井晃*; 渕本寛人*; 中谷泰博*; 藤原秀紀*; 今田真*; 鳴海康雄*; 金道浩一*; 高橋稔*; 海老原孝雄*; et al.

Physical Review B, 96(3), p.035151_1 - 035151_5, 2017/07

AA2017-0611.pdf:0.36MB

https://doi.org/10.1103/PhysRevB.96.035151

パーセンタイル：100(Materials Science, Multidisciplinary)

単結晶CeFeを用い、X線吸収(XAS)磁気円2色性(XMCD)の高精度実験により、その強磁性的秩序相におけるCe4状態を調べた。Ce $M_{4,5}$ XMCDスペクトルは、温度及び磁場に依存した形状変化を示す一方、Ce $M_{4,5}$ XAS、Fe $L_{2,3}$ XAS及びXMCDスペクトルでは変化が観測されないという通常の強磁性体とは異なる現象が観測された。このような振る舞いは、Ce 4配置の基底状態と状態が混ざり合ったことに由来すると解釈できる。外部摂動に対し非常に敏感なCe 4状態は、本物質での強磁性相と反強磁相が隣接する磁気不安定性と関連付けることができる。我々の実験データは、混成の強い強磁性Ce化合物の物性に対して、貴重な情報を与える。

論文

Circular dichroism in resonant angle-resolved photoemission spectra of LaNi $_{2}$ Ge $_{2}$

中谷泰博*; 藤原秀紀*; 荒谷秀和*; 森健雄*; 橘祥一*; 山口貴司*; 木須孝幸*; 山崎篤志*; 保井晃*; 山上浩志*; et al.

Journal of Electron Spectroscopy and Related Phenomena, 220, p.50 - 53, 2017/01

https://doi.org/10.1016/j.elspec.2017.01.008

被引用回数：1 パーセンタイル：72.38(Spectroscopy)

重い電子化合物CeNi $_{2}$ Ge $_{2}$ の非4バンド由来の電子構造を明らかにするため、LaNi $_{2}$ Ge $_{2}$ の軟X線角度分解光電子分光を行った。La M $_{4,5}$ 吸収端での光電子スペクトルで、価電子帯のLa 5成分の明瞭な強度の増大が観測された。さらに、軌道対称性に起因するバンドに依存した円二色性が観測された。

論文

Origin of the large positive magnetoresistance of Ge $_{1-x}$ Mn $_{x}$ granular thin films

若林勇希*; 秋山了太*; 竹田幸治; 堀尾眞史*; 芝田悟朗*; 坂本祥哉*; 伴芳祐*; 斎藤祐児; 山上浩志; 藤森淳*; et al.

Physical Review B, 95(1), p.014417_1 - 014417_6, 2017/01

https://doi.org/10.1103/PhysRevB.95.014417

被引用回数：6 パーセンタイル：30.1(Materials Science, Multidisciplinary)

Ge $_{1_x}$ Mn (GeMn) granular thin films are a unique and promising material for spintronic applications owing to their large positive magnetoresistance (MR). The microscopic origin of the MR has not yet been clarified. Here, we develop a method to separately investigate the magnetic properties of the nanoparticles and the matrix, utilizing the extremely high sensitivity of X-ray magnetic circular dichroism (XMCD) to the local magnetic state of each atom. We find that the MR ratio is proportional to the product of the magnetizations originating from the nanoparticles and the matrix. This result indicates that the spin-polarized holes in the nanoparticles penetrate into the matrix and that these holes undergo first order magnetic scattering by the paramagnetic Mn atoms in the matrix, which induces the large MR.

論文

New muonium HFS measurements at J-PARC/MUSE

Strasser, P.*; 青木正治*; 深尾祥紀*; 東芳隆*; 樋口嵩*; 飯沼裕美*; 池戸豊*; 石田啓一*; 伊藤孝; 岩崎雅彦*; et al.

Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12

https://doi.org/10.1007/s10751-016-1331-4

被引用回数：3 パーセンタイル：10.17

At the Muon Science Facility (MUSE) of J-PARC (Japan Proton Accelerator Research Complex), the MuSEUM collaboration is planning new measurements of the ground state hyperfine structure (HFS) of muonium both at zero field and at high magnetic field. The previous measurements were performed both at LAMPF (Los Alamos Meson Physics Facility) with experimental uncertainties mostly dominated by statistical errors. The new high intensity muon beam that will soon be available at MUSE H-Line will provide an opportunity to improve the precision of these measurements by one order of magnitude. An overview of the different aspects of these new muonium HFS measurements, the current status of the preparation, and the results of a first commissioning test experiment at zero field are presented.

論文

Electronic structures of ferromagnetic CeAgSb $_{2}$ ; Soft X-ray absorption, magnetic circular dichroism, and angle-resolved photoemission spectroscopies

斎藤祐児; 藤原秀紀*; 山口貴司*; 中谷泰博*; 森健雄*; 渕本寛人*; 木須孝幸*; 保井晃*; 宮脇淳*; 今田真*; et al.

Journal of the Physical Society of Japan, 85(11), p.114713_1 - 114713_7, 2016/11

https://doi.org/10.7566/JPSJ.85.114713

被引用回数：6 パーセンタイル：33.51(Physics, Multidisciplinary)

軟X線吸収(XAS)、磁気円二色性(XMCD)、角度分解光電子分光(ARPES)により強磁性体CeAgSb $_{2}$ の電子状態を調べた。Ce $M_{4,5}$ XASスペクトルのサテライト構造の強度が非常に小さいことから、Ce 4電子は非常に局在的であることが明らかとなった。Ce $M_{4,5}$ XASの線二色性効果から、Ce 4基底状態は軸方向を向いた $_{6}$ であることが分かった。XMCD結果は、CeAgSb $_{2}$ の局在磁性描像を支持する。さらに、ARPESで得られたバンド構造は、CeAgSb $_{2}$ では無くLaAgSb $_{2}$ に対するバンド計算結果とよく一致する。しかしながら、Ce 3-4共鳴ARPES結果では、ブリルアンゾーンの一部でCe 4 $f^{1}_{5/2}$ と4 $f^{1}_{7/2}$ ピーク強度比に波数依存性が観測され、Ce 4と伝導電子に無視できない混成効果が有ることが分かった。このことは、CeAgSb $_{2}$ のあまり大きくない電子比熱係数と関係づけることができる。