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Tokunaga, Yo; Suzuki, Michito*; Kr
mer, S.*; Sakai, Hironori; Kambe, Shinsaku; Harima, Hisatomo*; Aoki, Dai*; Horvati
, M.*; Sheikin, I.*
Physical Review B, 113(14), p.L140406_1 - L140406_7, 2026/04
Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)
Ge
probed by site-selective
Al NMRSakai, Hironori; Shin, S.*; Kambe, Shinsaku; Tokunaga, Yo; Harima, Hisatomo*; Pomjakushina, E.*; Park, T.*
Physical Review B, 112(23), p.235102_1 - 235102_9, 2025/12
Times Cited Count:1 Percentile:28.15(Materials Science, Multidisciplinary)
Vali
ka, M.*; Haidamak, T.*; Cabala, A.*; Posp
il, J.*; Bastien, G.*; Sechovsk
, V.*; Prokle
ka, J.*; Yanagisawa, Tatsuya*; Opletal, P.; Sakai, Hironori; et al.
Physical Review Materials (Internet), 8(9), p.094415_1 - 094415_9, 2024/09
Times Cited Count:2 Percentile:15.57(Materials Science, Multidisciplinary)
Eaton, A. G.*; Weinberger, T. I.*; Popiel, N. J. M.*; Wu, Z.*; Hickey, A. J.*; Cabala, A.*; Posp
il, J.*; Prokle
ka, J.*; Haidamak, T.*; Bastien, G.*; et al.
Nature Communications (Internet), 15, p.223_1 - 223_10, 2024/01
Times Cited Count:47 Percentile:98.44(Multidisciplinary Sciences)
Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori; Kitagawa, Shunsaku*; Ishida, Kenji*; Aoki, Dai*; Knebel, G.*; et al.
Physical Review Letters, 131(22), p.226503_1 - 226503_7, 2023/12
Times Cited Count:22 Percentile:88.47(Physics, Multidisciplinary)
10
W/cm
Skobelev, I. Yu.*; Ryazantsev, S. N.*; Kulikov, R. K.*; Sedov, M. V.*; Filippov, E. D.*; Pikuz, S. A.*; Asai, Takafumi*; Kanasaki, Masato*; Yamauchi, Tomoya*; Jinno, Satoshi; et al.
Photonics (Internet), 10(11), p.1250_1 - 1250_11, 2023/11
Times Cited Count:4 Percentile:37.56(Optics)It is challenging to clearly distinguish the impacts of the optical field and collisional ionization in the evolution of the charge state of a plasma produced when matter interacts with high-intensity laser pulses. In this work, time-dependent calculations of plasma kinetics are used to show that it is possible only when low-density gaseous targets with sufficiently small clusters are used. In the case of Ar plasma, the upper limit of the cluster radius was estimated to be
m.
Rh
Ga explored by
Ga nuclear quadrupole resonanceYamamoto, Shingo*; Fujii, Takuto*; Luther, S.*; Yasuoka, Hiroshi*; Sakai, Hironori; B
rtl, F.*; Ranjith, K. M.*; Rosner, H.*; Wosnitza, J.*; Strydom, A. M.*; et al.
Physical Review B, 106(11), p.115125_1 - 115125_5, 2022/09
Times Cited Count:1 Percentile:4.34(Materials Science, Multidisciplinary)We have studied the microscopic magnetic properties, the nature of the 130 K phase transition, and the ground state in the recently synthesized compound Ce
Rh
Ga by use of
Ga nuclear quadrupole resonance (NQR). The NQR spectra clearly show an unusual phase transition at
K, yielding a splitting of the high-temperature single NQR line into two well-resolved NQR lines, providing evidence for two crystallographically inequivalent Ga sites. The NQR frequencies are in good agreement with fully relativistic calculations of the band structure. Our NQR results indicate the absence of magnetic or charge order down to 0.3 K. The temperature dependence of the spin-lattice relaxation rate
shows three distinct regimes, with onset temperatures at
and 2 K. The temperature-independent
, observed between
and 2 K, crosses over to a Korringa process,
, below
2 K, which evidences a rare two-ion Kondo scenario: The system evolves into a dense Kondo coherent state below 2.0 and 0.8 K probed by the two different Ga sites.
;
In NQR/NMR and
Co NMR studySakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Ramakrishna, S. K.*; Reyes, A. P.*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.
Physical Review B, 104(8), p.085106_1 - 085106_12, 2021/08
Times Cited Count:5 Percentile:23.39(Materials Science, Multidisciplinary)Antiferromagnetism in a prototypical quantum critical metal CeCoIn
is known to be induced by slight substitutions of non-magnetic Zn atoms for In. In nominally 7% Zn substituted CeCoIn
, an antiferromagnetic (AFM) state coexists with heavy fermion superconductivity. Heterogeneity of the electronic states is investigated in Zn doped CeCoIn
by means of nuclear quadrupole and magnetic resonances (NQR and NMR). Site-dependent NQR relaxation rates
indicate that the AFM state is locally nucleated around Zn substituents in the matrix of a heavy fermion state, and percolates through the bulk at the AFM transition temperature
. At lower temperatures, an anisotropic superconducting (SC) gap below the SC transition temperature
, and the SC state permeates through the AFM regions via a SC proximity effect. Applying an external magnetic field induces a spin-flop transition near 5 T, reducing the volume of the AFM regions. Consequently, a short ranged inhomogeneous AFM state survives and coexists with a paramagnetic Fermi liquid state at high fields.

Park, J. S.*; Harada, Masahide; Hasegawa, Shoichi; Kasugai, Yoshimi; Meigo, Shinichiro; Sakai, Kenji; Suzuya, Kentaro; 55 of others*
Progress of Theoretical and Experimental Physics (Internet), 2021(6), p.063C01_1 - 063C01_12, 2021/06
Times Cited Count:2 Percentile:18.16(Physics, Multidisciplinary)
-Al
O
(0001)Entani, Shiro*; Honda, Mitsunori; Naramoto, Hiroshi*; Li, S.*; Sakai, Seiji*
Surface Science, 704, p.121749_1 - 121749_6, 2021/02
Times Cited Count:7 Percentile:30.40(Chemistry, Physical)Graphene is expected to be one of the most promising materials for nanoelectronics and spintronics. In most graphene-based devices, the graphene channel is placed on insulating substrates. Therefore, the study of inter-facial interactions between graphene and the insulator surface is of critical importance. In this study, the vertical arrangement of graphene which is transferred on
-Al
O
(0001) has been studied by normal incidence X-ray standing wave (NIXSW) technique. The analysis of the NIXSW profile reveals that the graphene layer is located at 3.57 (
) above the
-Al
O
(0001) surface, which is larger than the interlayer distance of graphite at 3.356 (
). Micro- Raman spectroscopy shows that the transferred graphene has a limited spatial distribution of hole concentration. The present study shows that transferred graphene on the sapphire substrate followed by vacuum-annealing has an atomically flat surface free from residual contaminations such as organic compounds and there occurs the hole-doping in graphene.
F from
O
?Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.
Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05
Times Cited Count:20 Percentile:70.10(Physics, Multidisciplinary)The structure of a neutron-rich
F nucleus is investigated by a quasifree (
) knockout reaction. The sum of spectroscopic factors of
orbital is found to be 1.0
0.3. The result shows that the
O core of
F nucleus significantly differs from a free
O nucleus, and the core consists of
35%
O
, and
65% excited
O. The result shows that the
O core of
F nucleus significantly differs from a free
O nucleus. The result may infer that the addition of the
proton considerably changes the neutron structure in
F from that in
O, which could be a possible mechanism responsible for the oxygen dripline anomaly.
S nuclear magnetic resonance spectra of uranium disulfide
-US
Sakai, Hironori; Tokunaga, Yo; Haga, Yoshinori; Kambe, Shinsaku; Ramakrishna, S. K.*; Reyes, A. P.*; Rosa, P. F. S.*; Ronning, F.*; Thompson, J. D.*; Fisk, Z.*; et al.
JPS Conference Proceedings (Internet), 30, p.011169_1 - 011169_6, 2020/03
Uranium disulfide
-US
showing a semimetal-to-semiconductor crossover has been investigated by the nuclear magnetic resonance (NMR) technique for
S nuclei with the nuclear spin of
. Since the natural concentration 0.76% of NMR active
S nuclei is too dilute, the isotopic enrichment to
50% has been carried out for the single crystal growth. The
S NMR spectra have been successfully obtained using a single crystal of
-US
with external fields along the crystallographic
axis. The S sites assignments have been made based on these NMR spectra.
Tokunaga, Yo; Aoki, Dai*; Mayaffre, H.*; Kr
mer, S.*; Julien, M.-H.*; Berthier, C.*; Horvati
, M.*; Sakai, Hironori; Kambe, Shinsaku; Hattori, Taisuke; et al.
JPS Conference Proceedings (Internet), 30, p.011037_1 - 011037_6, 2020/03
The field-angular dependence of Co-NMR spin-lattice relaxation rate
has been measured for a 10% Co-doped single crystal of URhGe. The experiment revealed that spin fluctuations in ferromagnetic (FM) state of URhGe are robust against magnetic field below about 4 T, applied along any direction in the
crystal plane. This is in clear contrast with the sister compound UCoGe, in which FM spin fluctuations are rapidly suppressed by a tiny applied field along the
axis. We show that such a difference in the character of the spin fluctuations is reflected in their two distinct phase diagrams for the upper critical field
, providing further support to the mechanism of superconductivity mediated by spin fluctuations in these materials.
Tanaka, Taiki*; Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Boll, R. A.*; Brewer, N. T.*; Van Cleve, S.*; Dean, D. J.*; Ishizawa, Satoshi*; et al.
Physical Review Letters, 124(5), p.052502_1 - 052502_6, 2020/02
Times Cited Count:43 Percentile:86.99(Physics, Multidisciplinary)
; Pulsed-field NMR study on single crystals up to 56 TTokunaga, Yo; Orlova, A.*; Bruyant, N.*; Aoki, Dai*; Mayaffre, H.*; Kr
mer, S.*; Julien, M.-H.*; Berthier, C.*; Horvati
, M.*; Higa, Nonoka; et al.
Physical Review B, 99(8), p.085142_1 - 085142_5, 2019/02
Times Cited Count:9 Percentile:34.93(Materials Science, Multidisciplinary)The heavy-fermion antiferromagnet CeIn
exhibits a field-induced anomaly associated with Fermi surface reconstruction at
45 T, well below the antiferromagnetic (AFM) critical field that exceeds 60 T. In order to explore the origin of this anomaly, we have measured
In NMR spectra in pulsed magnetic fields up to 56 T using high-quality single crystals. To within experimental resolution, we do not detect any change in the NMR spectra that could suggest a modification in either the character of the hyperfine field or the electric field gradient at In sites through
. This strongly suggests that the 45 T anomaly cannot be simply ascribed to a field-induced change in the magnetic structure of the AFM state.
Pu nuclear magnetic resonance in the candidate topological insulator PuB
Dioguardi, A. P.*; Yasuoka, Hiroshi*; Thomas, S. M.*; Sakai, Hironori; Cary, S. K.*; Kozimor, S. A.*; Albrecht-Schmitt, T. E.*; Choi, H. C.*; Zhu, J.-X.*; Thompson, J. D.*; et al.
Physical Review B, 99(3), p.035104_1 - 035104_6, 2019/01
Times Cited Count:12 Percentile:43.94(Materials Science, Multidisciplinary)We present a detailed nuclear magnetic resonance (NMR) study of
Pu in bulk and powdered single-crystal plutonium tetraboride (PuB
), which has recently been investigated as a potential correlated topological insulator. The
Pu NMR spectra are consistent with axial symmetry of the shift tensor showing for the first time that
Pu NMR can be observed in an anisotropic environment and up to room temperature. The temperature dependence of the
Pu shift, combined with a relatively long spin-lattice relaxation time (
), indicate that PuB
adopts a nonmagnetic state with gaplike behavior consistent with our density functional theory calculations. The temperature dependencies of the NMR Knight shift and
imply bulk gaplike behavior confirming that PuB
is a good candidate topological insulator.
Entani, Shiro*; Honda, Mitsunori; Shimoyama, Iwao; Li, S.*; Naramoto, Hiroshi*; Yaita, Tsuyoshi; Sakai, Seiji*
Japanese Journal of Applied Physics, 57(4S), p.04FP04_1 - 04FP04_4, 2018/04
Times Cited Count:4 Percentile:15.33(Physics, Applied)Sakai, Takaaki; Ren, L.*; Tsige-Tamirat, H.*; Vasile, A.*; Kang, S.-H.*; Ashurko, Y.*; Fanning, T.*
Proceedings of 24th International Conference on Nuclear Engineering (ICONE-24) (DVD-ROM), 7 Pages, 2016/06
Tokunaga, Yo; Aoki, Dai*; Mayaffre, H.*; Kr
mer, S.*; Julien, M.-H.*; Berthier, C.*; Horvati
, M.*; Sakai, Hironori; Hattori, Taisuke; Kambe, Shinsaku; et al.
Physical Review B, 93(20), p.201112_1 - 201112_5, 2016/05
Times Cited Count:18 Percentile:56.88(Materials Science, Multidisciplinary)The ferromagnetic superconductor URhGe has been known to exhibit an extremely large enhancement of the upper critical field when the field is confined and rotated in the (
) crystal plane. Our high-field
Co NMR measurements on 10% Co-doped URhGe up to 30 T prove that this unconventional behavior of the superconductivity (SC) is associated with a strong anisotropy of field-dependent quantum fluctuations near a tricritical point. These fluctuations are rapidly suppressed by the field component along the
axis, while being unaffected by any field component along the
axis. The observed close interplay between the SC and quantum fluctuations strongly supports a pairing mechanism mediated by these fluctuations in URhGe.
Tokunaga, Yo; Aoki, Dai*; Mayaffre, H.*; Kr
mer, S.*; Julien, M.-H.*; Berthier, C.*; Horvati
, M.*; Sakai, Hironori; Kambe, Shinsaku; Hattori, Taisuke; et al.
Journal of Physics; Conference Series, 683(1), p.012010_1 - 012010_6, 2016/02
Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)Metamagnetism is in itself quite interesting phenomena, especially in a system with itinerant f-electrons. Unconventional states observed in the vicinity of the metamagnetic transition have been the subject of a number of recent publications. The object of this study is to elucidate the interplay between superconductivity and metamagnetism in URhGe. The nature of the metamagnetism becomes particularly important in ferromagnetic superconductors URhGe and UCoGe, since it is likely related to the pairing mechanism for their unconventional superconductivity. Here we report the result of our Co-NMR study on URh
Co
Ge and discuss the origin of the field induced superconducting phenomenon observed in high fields around 12 T.