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Journal Articles

Odd-parity autoionizing levels of uranium observed by two-color two-step photoionization optogalvanic spectroscopy

Miyabe, Masabumi; Satou, Yukihiko; Wakaida, Ikuo; Terabayashi, Ryohei*; Sonnenschein, V.*; Tomita, Hideki*; Zhao, Y.*; Sakamoto, Tetsuo*

Journal of Physics B; Atomic, Molecular and Optical Physics, 54(14), p.145003_1 - 145003_8, 2021/07

 Times Cited Count:0 Percentile:0.01(Optics)

Two-color two-step photoionization optogalvanic spectroscopy was performed using high-repetition-rate titanium sapphire lasers and a uranium hollow cathode lamp to find the two-step resonance ionization schemes of uranium. Many ionization transitions were observed by exciting uranium atoms in a ground state into five, even parity, excited levels with the first-step laser and by scanning the second-step laser wavelengths. By blocking the first-step laser, single-color, two-photon ionization transitions were also identified. From these results, we have found more than 50 odd-parity autoionizing levels of uranium in the energy, ranging from the ionization potential (49958.4 cm$$^{-1}$$) to 51150 cm$$^{-1}$$. The determined energy levels are within 1 cm$$^{-1}$$ of previously reported values.

Journal Articles

Isotope-selective microscale imaging of radioactive Cs without isobaric interferences using sputtered neutral mass spectrometry with two-step resonant ionization employing newly-developed Ti:Sapphire lasers

Sakamoto, Tetsuo*; Morita, Masato*; Kanenari, Keita*; Tomita, Hideki*; Sonnenschein, V.*; Saito, Kosuke*; Ohashi, Masaya*; Kato, Kotaro*; Iguchi, Tetsuo*; Kawai, Toshihide*; et al.

Analytical Sciences, 34(11), p.1265 - 1270, 2018/11

 Times Cited Count:8 Percentile:31.98(Chemistry, Analytical)

Journal Articles

Spin and orbital magnetic moments of Fe in the $$n$$-type ferromagnetic semiconductor (In,Fe)As

Kobayashi, Masaki*; Anh, L. D.*; Hai, P. N.*; Takeda, Yukiharu; Sakamoto, Shoya*; Kadono, Toshiharu*; Okane, Tetsuo; Saito, Yuji; Yamagami, Hiroshi; Harada, Yoshihisa*; et al.

Applied Physics Letters, 105(3), p.032403_1 - 032403_4, 2014/07

AA2015-0418.pdf:0.82MB

 Times Cited Count:6 Percentile:26.85(Physics, Applied)

Journal Articles

Electronic configuration of Mn ions in the $$pi$$-$$d$$ molecular ferromagnetic $$beta$$-Mn phthalocyanine studied by soft X-ray magnetic circular dichroism

Kataoka, Takashi*; Sakamoto, Yuta*; Yamazaki, Yo*; Singh, V. R.*; Fujimori, Atsushi*; Takeda, Yukiharu; Okochi, Takuo*; Fujimori, Shinichi; Okane, Tetsuo; Saito, Yuji; et al.

Solid State Communications, 152(9), p.806 - 809, 2012/05

 Times Cited Count:20 Percentile:61.95(Physics, Condensed Matter)

no abstracts in English

Journal Articles

Electronic structure and magnetism of the diluted magnetic semiconductor Fe-doped ZnO nanoparticles

Kataoka, Takashi*; Kobayashi, Masaki*; Sakamoto, Yuta*; Song, G. S.*; Fujimori, Atsushi*; Chang, F.-H.*; Lin, H.-J.*; Huang, D. J.*; Chen, C. T.*; Okochi, Takuo*; et al.

Journal of Applied Physics, 107(3), p.033718_1 - 033718_7, 2010/02

AA2009-0977.pdf:1.0MB

 Times Cited Count:54 Percentile:86.13(Physics, Applied)

Journal Articles

Experimental observation of bulk band dispersions in the oxide semiconductor ZnO using soft X-ray angle-resolved photoemission spectroscopy

Kobayashi, Masaki*; Song, G.-S.*; Kataoka, Takashi*; Sakamoto, Yuta*; Fujimori, Atsushi; Okochi, Takuo*; Takeda, Yukiharu; Okane, Tetsuo; Saito, Yuji; Yamagami, Hiroshi; et al.

Journal of Applied Physics, 105(12), p.122403_1 - 122403_4, 2009/06

BB2009-1947.pdf:0.84MB

 Times Cited Count:12 Percentile:44.93(Physics, Applied)

Journal Articles

Report on ITPA meetings, 24

Idomura, Yasuhiro; Yoshida, Maiko; Yagi, Masatoshi*; Tanaka, Kenji*; Hayashi, Nobuhiko; Sakamoto, Yoshiteru; Tamura, Naoki*; Oyama, Naoyuki; Urano, Hajime; Aiba, Nobuyuki; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 84(12), p.952 - 955, 2008/12

no abstracts in English

Journal Articles

Report of meetings of ITPA (International Tokamak Physics Activity), 19

Sasao, Mamiko*; Kusama, Yoshinori; Kawano, Yasunori; Kawahata, Kazuo*; Mase, Atsushi*; Sugie, Tatsuo; Fujita, Takaaki; Fukuda, Takeshi*; Fukuyama, Atsushi*; Sakamoto, Yoshiteru; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 83(9), p.779 - 782, 2007/09

This is a report of highlights from 2007 spring meetings of seven Topical Groups (TG) of International Tokamak Physics Activity (ITPA). In each meeting, high priority issues in physics of International Thermonuclear Experimental Reactor (ITER) and other burning plasma experiments have been discussed and investigated. Twenty-seven scientists from Japan have participated in those meetings. Dates and places of the meetings are shown below. (1) Diagnostics TG: 26-30 March, Princeton (USA), (2) Transport Physics TG: 7-10 May, Lausanne (Switzerland), (3) Confinement Database and Modeling TG: 7-10 May, Lausanne (Switzerland), (4) Edge Pedestal Physics TG: 7-10 May, Garching (Germany) (5) Steady State Operation TG: 9-11 May, Daejeon (South Korea), (6)MHD TG: 21-24 May, San Diego (USA), (7) Scrape-off-layer and Divertor Physics TG: 7-10 May, Garching (Germany).

Journal Articles

Report on ITPA (International Tokamak Physics Activity) meeting, 18

Kawahata, Kazuo*; Kawano, Yasunori; Kusama, Yoshinori; Mase, Atsushi*; Sasao, Mamiko*; Sugie, Tatsuo; Fujita, Takaaki; Fukuda, Takeshi*; Fukuyama, Atsushi*; Sakamoto, Yoshiteru; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 83(2), p.195 - 198, 2007/02

no abstracts in English

Journal Articles

Report of ITPA (International Tokamak Physics Activity) meetings, 17

Asakura, Nobuyuki; Kato, Takako*; Nakano, Tomohide; Takamura, Shuichi*; Tanabe, Tetsuo*; Iio, Shunji*; Nakajima, Noriyoshi*; Ono, Yasushi*; Ozeki, Takahisa; Takechi, Manabu; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 82(7), p.448 - 450, 2006/07

no abstracts in English

Journal Articles

Report of ITPA (International Tokamak Physics Activity) meeting, 13

Kawano, Yasunori; Kawahata, Kazuo*; Kusama, Yoshinori; Sasao, Mamiko*; Sugie, Tatsuo; Mase, Atsushi*; Asakura, Nobuyuki; Kato, Takako*; Takamura, Shuichi*; Tanabe, Tetsuo*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 81(2), p.128 - 130, 2005/02

no abstracts in English

Journal Articles

Progress in physics and technology developments for the modification of JT-60

Tamai, Hiroshi; Matsukawa, Makoto; Kurita, Genichi; Hayashi, Nobuhiko; Urata, Kazuhiro*; Miura, Yushi; Kizu, Kaname; Tsuchiya, Katsuhiko; Morioka, Atsuhiko; Kudo, Yusuke; et al.

Plasma Science and Technology, 6(1), p.2141 - 2150, 2004/02

 Times Cited Count:2 Percentile:6.49(Physics, Fluids & Plasmas)

The dominant issue for the the modification program of JT-60 (JT-60SC) is to demonstrate the steady state reactor relevant plasma operation. Physics design on plasma parameters, operation scenarios, and the plasma control method are investigated for the achievement of high-$$beta$$. Engineering design and the R&D on the superconducting magnet coils, radiation shield, and vacuum vessel are performed. Recent progress in such physics and technology developments is presented.

Journal Articles

Objectives and design of the JT-60 superconducting tokamak

Ishida, Shinichi; Abe, Katsunori*; Ando, Akira*; Chujo, T.*; Fujii, Tsuneyuki; Fujita, Takaaki; Goto, Seiichi*; Hanada, Kazuaki*; Hatayama, Akiyoshi*; Hino, Tomoaki*; et al.

Nuclear Fusion, 43(7), p.606 - 613, 2003/07

no abstracts in English

Journal Articles

Objectives and design of the JT-60 superconducting tokamak

Ishida, Shinichi; Abe, Katsunori*; Ando, Akira*; Cho, T.*; Fujii, Tsuneyuki; Fujita, Takaaki; Goto, Seiichi*; Hanada, Kazuaki*; Hatayama, Akiyoshi*; Hino, Tomoaki*; et al.

Nuclear Fusion, 43(7), p.606 - 613, 2003/07

 Times Cited Count:33 Percentile:69.14(Physics, Fluids & Plasmas)

no abstracts in English

Oral presentation

Soft X-ray magnetic circular dichroism and photoemission spectroscopy study of ferromagnetic phthalocyanine

Kataoka, Takashi*; Sakamoto, Yuta*; Yamazaki, Yo*; Fujimori, Atsushi; Takeda, Yukiharu; Okochi, Takuo; Okane, Tetsuo; Saito, Yuji; Yamagami, Hiroshi

no journal, , 

Recently, transition-metal phthalocyanines (Pc) have attracted great interest in many fields of science and technology because of the structural similarities to bio-molecules, their remarkable thermal stability and chemical inertness. One of the most interesting investigations of transition-metal Pc involves their magnetic properties. At low temperature ($$sim$$10 K), the ferromagnetism in $$beta$$-type polycrystals of manganese phthalocyanine (MnPc) has been reported. We have investigated the electronic structure and magnetic interaction in $$beta$$-type polycrystals of the MnPc using X-ray magnetic circular dichroism (XMCD). The XMCD results suggest that the inter-molecular p-d hybridization occurs in the $$beta$$-type polycrystals of MnPc molecules. We will discuss correlation between the inter-molecular interaction and the ferromagnetic coupling in the MnPc molecules.

Oral presentation

Development of trace analysis of $$^{rm 93m}$$Nb by resonance ionization mass spectrometry in gas jet toward neutron dosimetry, 1; Resonance ionization mass spectroscopy on Nb by Ti:Sapphire laser

Sakamoto, Chika*; Takatsuka, Takaaki*; Sonnenchein, V.*; Tomita, Hideki*; Sonoda, Tetsu*; Mita, Koki*; Noto, Takuma*; Adachi, Yoshitaka*; Ito, Chikara; Maeda, Shigetaka; et al.

no journal, , 

no abstracts in English

Oral presentation

Resonant laser secondary neutral mass spectrometry for micro imaging of radioactive isotopes, 2

Tomita, Hideki*; Saito, Kosuke*; Ohashi, Masaya*; Sonnenschein, V.*; Kato, Kotaro*; Suzuki, So*; Iguchi, Tetsuo*; Morita, Masato*; Sakamoto, Tetsuo*; Kanenari, Keita*; et al.

no journal, , 

no abstracts in English

Oral presentation

Establishment of characterization method for small fuel debris using the world's first isotope micro imaging apparatus, 4; Development of resonance ionization scheme for highly sensitive and accurate isotope analysis

Iwata, Yoshihiro; Miyabe, Masabumi; Wakaida, Ikuo; Yoshimura, Shoki*; Matsumura, Tamaki*; Morita, Masato*; Sakamoto, Tetsuo*

no journal, , 

Information on the elemental and isotopic compositions of fuel debris is essential for the decommissioning of TEPCO's Fukushima Daiichi Nuclear Power Station. In this study, we have developed a double-resonance ionization scheme for highly sensitive and accurate isotope analysis of neodymium (Nd), which is a burnup indicator.

Oral presentation

Establishment of characterization method for small fuel debris using the world's first isotope micro imaging apparatus, 5; Micro-area isotope composition analysis of Fukushima Daiichi Nuclear Power Plant contaminant

Yoshida, Takeru; Sekio, Yoshihiro; Maeda, Koji; Morita, Masato*; Sakamoto, Tetsuo*; Mizokami, Masato*; Hirai, Mutsumi*

no journal, , 

In order to steadily carry out decommissioning of the Fukushima Daiichi Nuclear Power Plant (FDNPP), it is extremely important to understand the properties of fuel debris. In the past, analytical methods such as SEM-EDS, TEM and ICP-MS have been used to determine the properties of fuel debris. However, these analytical methods cannot obtain information on the local isotopic composition of the sample. FIB-TOF-SIMS, which the authors are developing, is expected to be a useful analytical method for determining the properties of fuel debris because it allows local isotopic composition analysis. In this study, we conducted analysis in a micro-area of FDNPP contaminated sample and succeeded in obtaining isotopic composition imaging of Li, B, and U from the measured particulates.

Oral presentation

Resonance ionization spectroscopy of Nd for isotope micro-imaging of particles

Miyabe, Masabumi; Iwata, Yoshihiro; Tomita, Hideki*; Morita, Masato*; Sakamoto, Tetsuo*

no journal, , 

The isotopic composition of Nd is used in a wide range of nuclear field, such as forensic analysis and fuel burnup evaluation, and the currently most used analytical methods include TIMS and ICP-MS. However, the analytical samples obtained in decommissioning of Fukushima's failed reactors contain a mixture of particles of different sources, and these analytical techniques which cannot distinguish individual particles lose the information on their origin and history. Conversely, if the origin can be determined from the burnup of each particle, it is important for clarifying accident progress and criticality safety assessment. For this reason, we have applied ion sputter mass spectrometry imaging, which can measure the distribution of nuclides in individual particles, and have developed laser resonance secondary neutral mass spectrometry as a countermeasure against the isobaric interference. In this study, we performed two-step ionization spectroscopy to obtain highly efficient ionization schemes of Nd. As a result, we found several schemes with higher ionization efficiency than previously reported one.

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