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Fuwa, Yasuhiro; Mizobata, Satoshi*; Nakano, Hideto; Shinozaki, Shinichi; Takayanagi, Tomohiro; Asano, Hiroyuki; Iwama, Yuhei*
Proceedings of 22nd Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 391, 2026/03
no abstracts in English
Nguyen, T. H. T.; Sanami, Toshiya*; Yamazaki, Hirohito*; Iwamoto, Nobuyuki; Itoga, Toshiro*; Kirihara, Yoichi; Lee, E.*; Sugihara, Kenta*; Miyamoto, Shuji*; Hashimoto, Satoshi*; et al.
Physics Letters B, 870, p.139900_1 - 139900_8, 2025/11
Times Cited Count:0 Percentile:0.00(Astronomy & Astrophysics)Hori, Junichi*; Sano, Tadafumi*; Takamiya, Koichi*; Fukutani, Satoshi*; Nakamura, Shoji; Nauchi, Yasushi*; 3 of others*; 10 of others*
KURNS-EKR-21, p.10 - 14, 2025/01
no abstracts in English
He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Sano, Asami; Abe, Jun*; Fukuyama, Ko*; Shimmei, Toru*; Nakano, Satoshi*
Inorganic Chemistry, 63(47), p.22349 - 22360, 2024/11
Times Cited Count:4 Percentile:37.51(Chemistry, Inorganic & Nuclear)Brucite, Mg(OH)
, is a key material for studying hydrogen bonds in solid hydroxides. This study explored how fluorine (F) substitution affects hydrogen-bonding in hydrogenated and deuterated brucite under ambient and high-pressure conditions using neutron powder diffraction, Raman, and IR spectroscopy. At ambient conditions, F substitution shortened donor- acceptor distances and elongated hydroxyl bonds, strengthening hydrogen bonds, as evidenced by red shifts in hydroxyl stretching modes. High-pressure experiments showed that F doping suppressed pressure-induced hydrogen-bond strengthening, reducing changes in hydroxyl bond length, bond angle, and cone angle. Spectroscopic measurements confirmed that F substitution limits pressure-induced hydroxyl elongation.
Machida, Shinichi*; Hattori, Takanori; Nakano, Satoshi*; Sano, Asami; Funakoshi, Kenichi*; Abe, Jun*
Koatsuryoku No Kagaku To Gijutsu, 34(3), p.134 - 142, 2024/09
A diamond anvil cell (DAC) for high-pressure neutron diffraction experiments has been developed at the PLANET beamline, Materials and Life Science Experimental Facility, in J-PARC. The conically supported diamond anvils were used for high-pressure generation. We succeeded in obtaining the neutron data for D
O ice up to 69.4 GPa. In addition, the gasket materials suitable for the neutron diffraction measurements were investigated. 11 kinds of alloys were tested and SUS304, Inconel718 and M2052 (73Mn-20Cu-5Ni-2Fe, at%) alloys showed excellent performance. Especially, M2052 null-matrix alloy has proven to be useful for neutron diffraction experiments where the beam inevitably hits the gasket. We then obtained refinable neutron diffraction profiles in Rietveld analysis from D
O ice at least up to 43.3 GPa.
He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Iizuka, Riko*; Okajima, Hajime*; Hattori, Takanori; Sano, Asami; Machida, Shinichi*; Abe, Jun*; Goto, Hirotada*; et al.
Journal of Molecular Structure, 1310, p.138271_1 - 138271_8, 2024/08
Times Cited Count:0 Percentile:0.00(Chemistry, Physical)High-pressure responses of the O-D
F hydrogen bonds in deuterated magnesium hydroxyfluoride were investigated using neutron powder diffraction and Raman spectroscopy. The Rietveld analysis at ambient conditions revealed a chemical formula of Mg(OD)
F
and hydroxyl group/fluorine disorder (OD/F disorder) in the crystal structure, which gave rise to two hydrogen-bonding configurations. The Rietveld analysis showed the hydrogen-bonding geometries remains up to 9.8 GPa, indicating no pressure-induced strengthening of hydrogen bonds. The Raman spectra at ambient conditions showed three hydroxyl stretching bands at 2613, 2694, and 2718 cm
. The high frequencies of the O-D stretching modes indicated that the hydroxyls should be involved in weak or none hydrogen-bonding interactions. Up to 20.2 GPa, the mode initially centered at 2694 cm
displayed a pressure-induced blue shift, revealing no strengthening of hydrogen bonds under compression. We discuss the existence of hydrogen bonds and the causes of the blue-shifting hydroxyls at ambient and at high pressures.

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G
mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.
Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03
Times Cited Count:6 Percentile:78.06(Physics, Nuclear)no abstracts in English
OKondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
Times Cited Count:55 Percentile:95.68(Multidisciplinary Sciences)no abstracts in English
Ca cast doubt on a doubly magic
CaChen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Chazono, Yoshiki*; Hagen, G.*; Holt, J. D.*; et al.
Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08
Times Cited Count:21 Percentile:93.22(Astronomy & Astrophysics)Gamma decays were observed in
Ca and
Ca following quasi-free one-proton knockout reactions from
Sc. For
Ca, a
ray transition was measured to be 1456(12) keV, while for
Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the
decays. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for
level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the
and
orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic
Ca and potentially drives the dripline of Ca isotopes to
Ca or even beyond.
Ne at the transition into the island of inversion; Detailed structure study of
NeWang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.
Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08
Times Cited Count:8 Percentile:73.64(Astronomy & Astrophysics)Detailed
-ray spectroscopy of the exotic neon isotope
Ne has been performed using the one-neutron removal reaction from
Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for
Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.
100 MeV/nucleonPohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G
mez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.
Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04
Times Cited Count:19 Percentile:86.92(Physics, Multidisciplinary)We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient
O nucleus with large Fermi-surface asymmetry at
100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.
island of inversion; First study of low-lying bound excited states in
V and
VElekes, Z.*; Juh
sz, M. M.*; Sohler, D.*; Sieja, K.*; Yoshida, Kazuki; Ogata, Kazuyuki*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; Baba, Hidetada*; et al.
Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12
Times Cited Count:6 Percentile:49.20(Physics, Nuclear)The low-lying level structure of
V and
V was investigated for the first time. The neutron knockout reaction and inelastic proton scattering were applied for
V while the neutron knock-out reaction provided the data for
V. Four and five new transitions were determined for
V and
V, respectively. Based on the comparison to our shell-model calculations using the Lenzi-Nowacki-Poves-Sieja (LNPS) interaction, three of the observed
rays for each isotope could be placed in the level scheme and assigned to the decay of the first 11/2
and 9/2
levels. The (
,
) excitation cross sections for
V were analyzed by the coupled-channels formalism assuming quadrupole plus hexadecapole deformations. Due to the role of the hexadecapole deformation,
V could not be unambiguously placed on the island of inversion.
neutron orbital and the
shell closure in
CaEnciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; Ogata, Kazuyuki*; Poves, A.*; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; et al.
Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12
Times Cited Count:28 Percentile:88.32(Physics, Multidisciplinary)The one-neutron knockout from
Ca was performed at
230 MeV/nucleon combined with prompt
spectroscopy. The momentum distributions corresponding to the removal of
and
neutrons were measured. The cross sections are consistent with a shell closure at the neutron number
, found as strong as at
and
in Ca isotopes from the same observables. The analysis of the momentum distributions leads to a difference of the root-mean-square radii of the neutron
and
orbitals of 0.61(23) fm, in agreement with the modified-shell-model prediction of 0.7 fm suggesting that the large root-mean-square radius of the
orbital in neutron-rich Ca isotopes is responsible for the unexpected linear increase of the charge radius with the neutron number.
Be produced by the strongest solar proton event during the holoceneSpiegl, T. C.*; Yoden, Shigeo*; Langematz, U.*; Sato, Tatsuhiko; Chhin, R.*; Noda, Satoshi*; Miyake, Fusa*; Kusano, Kanya*; Schaar, K.*; Kunze, M.*
Journal of Geophysical Research; Atmospheres, 127(13), p.e2021JD035658_1 - e2021JD035658_21, 2022/07
Times Cited Count:7 Percentile:35.17(Meteorology & Atmospheric Sciences)The abundance of cosmogenic isotopes in natural archives carries important information about the complex pathways from their source in the upper atmosphere to their deposition via atmospheric transport processes. Here, we use a new modelling framework to (a) estimate the
Be production yield for the 774 CE/775 event, (b) evaluate the performance of our model framework by comparing the model results to four ice core records and (c) investigate the atmospheric pathways with a state-of-the-art climate model in detail. The results give new constraints regarding the seasonal timing of the event, underpin the role of the background conditions in the stratosphere, and highlight regional variations in the cosmogenic surface flux.
Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.
Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07
This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.
Ca; Spectroscopy of
K,
Ca, and
CaKoiwai, Takuma*; Wimmer, K.*; Doornenbal, P.*; Obertelli, A.*; Barbieri, C.*; Duguet, T.*; Holt, J. D.*; Miyagi, Takayuki*; Navr
til, P.*; Ogata, Kazuyuki*; et al.
Physics Letters B, 827, p.136953_1 - 136953_7, 2022/04
Times Cited Count:12 Percentile:75.15(Astronomy & Astrophysics)no abstracts in English
Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.
Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12
Times Cited Count:7 Percentile:29.64(Geosciences, Multidisciplinary)The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.
Cl isotopesLinh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Chen, S.*; Chung, L. X.*; Duguet, T.*; G
mez-Ramos, M.*; et al.
Physical Review C, 104(4), p.044331_1 - 044331_16, 2021/10
Times Cited Count:13 Percentile:73.10(Physics, Nuclear)no abstracts in English
Sakamoto, Atsushi; Kibe, Satoshi*; Kawanobe, Kazunori*; Fujisaku, Kazuhiko*; Sano, Yuichi; Takeuchi, Masayuki; Suzuki, Hideya*; Tsubata, Yasuhiro; Ban, Yasutoshi; Matsumura, Tatsuro
JAEA-Research 2021-003, 30 Pages, 2021/06
Japan Atomic Energy Agency has been developing a solvent extraction process called SELECT to recover minor actinides (MA) from spent nuclear fuel. In the SELECT process, TDdDGA, HONTA, and ADAAM are used as the extractants for MA + Ln corecovery, MA/Ln separation and Am/Cm separation, respectively. These extractants do not contain phosphorus (P), and consist of carbon (C), hydrogen (H), oxygen (O), and nitrogen (N). In this study, in order to give beneficial information for designing flowsheet, the mass transfer coefficients of Ln between HNO
solution and TDdDGA or HONTA / n-dodecane solvent were evaluated by the single drop technique. Prior to the evaluation of mass transfer coefficient, we had optimized the structure of the single drop apparatus to improve accuracy of the measurement. Based on the mass transfer coefficients obtained in HNO
/ TDdDGA-n-dodecane system, Ln behaviors in the counter-current extraction and back-extraction using mixer-settlers and centrifugal contactors were estimated by simple calculation, and they had a good agreement with our previous experimental results. We also confirmed the mass transfer coefficients of Ln in HNO
/ HONTA - n-dodecane system are under 10
m/s.
Ca from direct reactionsBrowne, F.*; Chen, S.*; Doornenbal, P.*; Obertelli, A.*; Ogata, Kazuyuki*; Utsuno, Yutaka; Yoshida, Kazuki; Achouri, N. L.*; Baba, Hidetada*; Calvet, D.*; et al.
Physical Review Letters, 126(25), p.252501_1 - 252501_7, 2021/06
Times Cited Count:17 Percentile:69.14(Physics, Multidisciplinary)Direct proton-knockout reactions of
Sc were studied at the RIKEN Radioactive Isotope Beam Factory. Populated states of
Ca were investigated through
-ray and invariant-mass spectroscopy. Level energies were calculated from the nuclear shell model employing a phenomenological inter-nucleon interaction. Theoretical cross sections to states were calculated from distorted-wave impulse approximation estimates multiplied by the shell model spectroscopic factors. Despite the calculations showing a significant amplitude of excited neutron configurations in the ground-state of
Sc, valence proton removals populated predominantly the ground-state of
Ca. This counter-intuitive result is attributed to pairing effects leading to a dominance of the ground-state spectroscopic factor. Owing to the ubiquity of the pairing interaction, this argument should be generally applicable to direct knockout reactions from odd-even to even-even nuclei.