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Iwami, Satone*; Yamashita, Takuma*; Mitsuyasu, Yusuke*; Ono, Kenta*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2024-6, p.91 - 95, 2024/12
We aim to improve the detection limit of the ESR dosimetry method. In this study, the saturation behavior of each radical was investigated by varying the microwave power during ESR measurement. Based on the difference in spin relaxation time between carbonate radicals and native radicals, it is expected that the signal-to-noise ratio improves and the detection limit can be lowered when the microwave power is increased to 4.0 mW.
Yamashita, Takuma*; Iwami, Satone*; Mitsuyasu, Yusuke*; Ono, Kenta*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2024-6, p.85 - 90, 2024/12
To clarify the radiation effects of the accident at the TEPCO's Fukushima Daiichi NPP on living organisms, it is important to accurately estimate the dose to each individual. We have developed a multi-component analysis program using random number optimization to extract only the components derived from carbonate radicals from the ESR spectra.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
Radiation Protection Dosimetry, 199(14), p.1620 - 1625, 2023/09
Times Cited Count：1 Percentile：23.64(Environmental Sciences)We have been conducting dose assessments for Japanese macaques captured in Fukushima to reveal radiobiological effects on the low-dose expose animals. To accurately determine the external exposure dose, it is desirable to examine the analysis of the CO
radical intensity. We examined ESR spectra of teeth of 10 macaques captured in Fukushima by two spectrum-decomposition algorithms.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.
KEK Proceedings 2022-2, p.120 - 125, 2022/11
We investigate the effect of sample's anisotropy and measurement condition to obtain the higher reproducibility for the shape of the ESR spectrum and the intensity of CO radical.
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
KEK Proceedings 2021-2, p.91 - 96, 2021/12
We examined whether the ESR dose estimation method could be applied to wild Japanese macaque. In this work, we investigated the enamel preparation protocol and the analytical method of the ESR spectra.
Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometryKoarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.
Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08
Times Cited Count：7 Percentile：52.87(Chemistry, Analytical)Rapid analysis of Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of Sr in small bone and tooth samples derived from terrestrial animals.
Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.
Radiation Measurements, 134, p.106315_1 - 106315_4, 2020/06
Times Cited Count：9 Percentile：64.46(Nuclear Science & Technology)The relationship between the CO
radical intensity and the absorbed dose (dose response curve) of tooth enamel of Japanese macaque was observed by electron spin resonance and the detection limit of our system was estimated to be 33.5 mGy, which is comparable to the detection limit for human molar teeth. Using the dose response curve, external exposure dose for seven wild Japanese macaques captured in Fukushima prefecture were examined. The results suggest that the external exposure dose for the wild Japanese macaques were ranged between 45 mGy to 300 mGy.
Matsui, Hiroya; Sasaki, Manabu*
JAEA-Technology 2006-052, 101 Pages, 2006/11
JAEA-Technology-2006-052.pdf:9.64MB
Japan Atomic Energy Agency (JAEA) has been conducting the project with construction of the Underground Research Laboratory (URL) called "Horonobe URL Project" since FY2000/FY2001 in Horonobe-cho, Hokkaido in Japan. The project is divided into three major phase, such as surface-based investigation phase, construction phase and operation phase. Total duration of the project is about 20 years. In the surface-based investigation phase, the eleven deep borehole investigations, which were drilled until 1000m depth, have carried out to understand a geological environment in the selected URL area formed Neocence sedimentary formations in Horonobe-cho. This report describe summarized important experiences to perform the deep borehole investigations with max. 1000m depth. This information could be great helpful for future site investigations.
Sasaki, Akira; Jo, Kazuki*; Kashiwagi, Hiroe*; Watanabe, Chiemi*; Suzuki, Manabu*; Lucas, P.*; Oishi, Masatoshi*; Kato, Daiji*; Kato, Masatoshi*; Kato, Takako*
Journal of Plasma and Fusion Research SERIES, Vol.7, p.348 - 351, 2006/00
no abstracts in English
Hama, Katsuhiro; Takahashi, Kazuharu; Ishii, Eiichi; Takeuchi, Ryuji; Sasaki, Manabu; Kunimaru, Takanori; Matsui, Hiroya
JNC TN5400 2003-002, 61 Pages, 2003/08
JNC-TN5400-2003-002.pdf:5.42MBJNC-TN5400-2003-002(errata).pdf:0.08MB
The working program for deep borehole investigations (HDB-6,7,8 boreholes).
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reactions for 
=1.5-2.4 GeVZegers, R. G. T.*; Sumihama, Mizuki*; Ahn, D. S.*; Ahn, J. K.*; Akimune, Hidetoshi*; Asano, Yoshihiro; Chang, W. C.*; Dat
, S.*; Ejiri, Hiroyasu*; Fujimura, Hisako*; et al.
Physical Review Letters, 91(9), p.092001_1 - 092001_4, 2003/08
Times Cited Count：128 Percentile：94.59(Physics, Multidisciplinary)no abstracts in English
= +1 Baryon resonance in photoproduction from the neutronNakano, Takashi*; Ahn, D. S.*; Ahn, J. K.*; Akimune, Hidetoshi*; Asano, Yoshihiro; Chang, W. C.*; Date, S.*; Ejiri, Hiroyasu*; Fujimura, Hisako*; Fujiwara, Mamoru; et al.
Physical Review Letters, 91(1), p.012002_1 - 012002_4, 2003/07
Times Cited Count：1023 Percentile：99.84(Physics, Multidisciplinary)no abstracts in English
Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.
no journal, ,
Rapid analysis of Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. The ICP-MS method was improved by ICP-MS/MS and oxygen-ammonia mixed gas reaction.
Oka, Toshitaka; Suzuki, Masatoshi*; Takahashi, Atsushi*; Sato, Taku*; Mitsuyasu, Yusuke*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; et al.
no journal, ,
We examined ESR measurement to estimate the dose of wild Japanese macaque captured at the contaminated area of Fukushima Prefecture. The estimated doses were ranged from several mGy to ~270 mGy, which are comparable to the estimated dose reported in our previous work, suggesting that the maximum dose of wild Japanese macaques captured in this area is estimated to be about 300 mGy. The dose estimation using a novel deconvolution program developed by ourselves will be also discussed.
Hayashi, Teppei*; Yamashita, Takuma*; Mitsuyasu, Yusuke*; Ono, Kenta*; Iwami, Satone*; Kino, Yasushi*; Sekine, Tsutomu*; Oka, Toshitaka; Takahashi, Atsushi*; Shimizu, Yoshinaka*; et al.
no journal, ,
no abstracts in English
Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
no journal, ,
The improvement of the ESR dosimetry is required to apply that for the low-dose exposure of wild animals. We will report our progress of the improvement, and compare the external exposure dose estimated by the ESR dosimetry technique and the calculated result based on the external exposure dose rate of the captured point.
Sr in trace amount of bone; Application of inductively coupled plasma mass spectrometryKoarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.
no journal, ,
Rapid analysis of Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of Sr in small bone and tooth samples derived from terrestrial animals.
Koarai, Kazuma; Matsueda, Makoto; Fujiwara, Kenso; Ono, Takumi*; Kino, Yasushi*; Oka, Toshitaka; Okutsu, Kenichi*; Takahashi, Atsushi*; Suzuki, Toshihiko*; Shimizu, Yoshinaka*; et al.
no journal, ,
We have investigated incorporation of Sr and 
Cs in teeth of cattle and otoliths of fish. Specific activity of Sr in the dentin tissue was higher than that in the enamel tissue. The result shows change of Sr incorporation in cattle even within a tooth. Concentrations of stable Sr and Cs were 94 ppm and 3 ppb. Distributions of stable Sr and Cs were uniform in the otolith of fish. If distribution of Sr and Cs in the otolith was measured, change of Sr and Cs incorporation into the fish would be found. These findings suggest that distribution patterns of Sr and Cs in the environment could be estimated from distribution of the radionuclides in the tooth and otolith.
Oka, Toshitaka; Mitsuyasu, Yusuke*; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Sekine, Tsutomu*; Okutsu, Kenichi*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.
no journal, ,
Releases of the radioactive materials from the Fukushima Daiichi Nuclear Power Plant accident result in a low dose exposure to wild animals. The external dose of wild animals is commonly estimated by the external dose rate of the captured point, but the estimated exposure dose has huge uncertainties because the size of the habitat and/or the movement of the wild animals are not included in the estimation. To estimate the external dose precisely, we utilize electron spin resonance (ESR) dosimetry. In this work, we investigated the sample preparation procedure of wild animals. The ESR spectrum of enamel of racoon captured in Namie-town, Fukushima has a broad ESR signal due to metal components. The linear relationship between the Co intensity and the absorbed dose that we can apply ESR dosimetry for racoon teeth. Using this relationship, the external exposure dose was estimated.
Yamashita, Takuma*; Mitsuyasu, Yusuke*; Ono, Kenta*; Iwami, Satone*; Hayashi, Teppei*; Kino, Yasushi*; Sekine, Tsutomu*; Oka, Toshitaka; Takahashi, Atsushi*; Shimizu, Yoshinaka*; et al.
no journal, ,
no abstracts in English
