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Machida, Masahiko; Yamada, Susumu; Kim, M.; Okumura, Masahiko; Miyamura, Hiroko; Shikaze, Yoshiaki; Sato, Tomoki*; Numata, Yoshiaki*; Tobita, Yasuhiro*; Yamaguchi, Takashi; et al.
RIST News, (69), p.2 - 18, 2023/09
The contamination of radioactive materials leaked from the reactor has resulted in numerous hot spots in the Fukushima Daiichi Nuclear Power Station (1F) building, posing obstacles to its decommissioning. In order to solve this problem, JAEA has conducted research and development of the digital technique for inverse estimation of radiation source distribution and countermeasures against the estimated source in virtual space for two years from 2021 based on the subsidy program "Project of Decommissioning and Contaminated Water Management" performed by the funds from the Ministry of Economy, Trade and Industry. In this article, we introduce the results of the project and the plan of the renewal project started in April 2023. For the former project, we report the derivative method for LASSO method considering the complex structure inside the building and the character of the source and show the result of the inverse estimation using the method in the real reactor building. Moreover, we explain the platform software "3D-ADRES-Indoor" which integrates these achievements. Finally, we introduce the plan of the latter project.
OKondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
Times Cited Count：5 Percentile：92.64(Multidisciplinary Sciences)no abstracts in English
Ne at the transition into the island of inversion; Detailed structure study of NeWang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.
Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08
Times Cited Count：2 Percentile：68.16(Astronomy & Astrophysics)Detailed 
-ray spectroscopy of the exotic neon isotope Ne has been performed using the one-neutron removal reaction from Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.
Iwamoto, Osamu; Iwamoto, Nobuyuki; Kunieda, Satoshi; Minato, Futoshi; Nakayama, Shinsuke; Abe, Yutaka*; Tsubakihara, Kosuke*; Okumura, Shin*; Ishizuka, Chikako*; Yoshida, Tadashi*; et al.
Journal of Nuclear Science and Technology, 60(1), p.1 - 60, 2023/01
Times Cited Count：64 Percentile：99.99(Nuclear Science & Technology)Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.
Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09
Times Cited Count：6 Percentile：84.97(Nuclear Science & Technology)In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.
Senzaki, Tatsuya; Arai, Yoichi; Yano, Kimihiko; Sato, Daisuke; Tada, Kohei; Ogi, Hiromichi*; Kawanobe, Takayuki*; Ono, Shimpei; Nakamura, Masahiro; Kitawaki, Shinichi; et al.
JAEA-Testing 2022-001, 28 Pages, 2022/05
JAEA-Testing-2022-001.pdf:2.33MB
In preparation for the decommissioning of Laboratory B of the Nuclear Fuel Cycle Engineering Laboratory, the nuclear fuel material that had been stored in the glove box for a long time was moved to the Chemical Processing Facility (CPF). This nuclear fuel material was stored with sealed by a polyvinyl chloride (PVC) bag in the storage. Since it was confirmed that the PVC bag swelled during storage, it seems that any gas was generated by radiolysis of the some components contained in the nuclear fuel material. In order to avoid breakage of the PVC bag and keep it safety for long time, we began the study on the stabilization treatment of the nuclear fuel material. First, in order to clarify the properties of nuclear fuel material, radioactivity analysis, component analysis, and thermal analysis were carried out. From the results of thermal analysis, the existence of organic matter was clarified. Then, ion exchange resin with similar thermal characteristics was selected and the thermal decomposition conditions were investigated. From the results of these analyzes and examinations, the conditions for thermal decomposition of the nuclear fuel material contained with organic matter was established. Performing a heat treatment of a small amount of nuclear fuel material in order to confirm the safety, after which the treatment amount was scaled up. It was confirmed by the weight change after the heat treatment that the nuclear fuel material contained with organic matter was completely decomposed.
Komatsu, Yuya*; Shimizu, Ryota*; Sato, Ryuhei*; Wilde, M.*; Nishio, Kazunori*; Katase, Takayoshi*; Matsumura, Daiju; Saito, Hiroyuki*; Miyauchi, Masahiro*; Adelman, J. R.*; et al.
Chemistry of Materials, 34(8), p.3616 - 3623, 2022/04
Times Cited Count：9 Percentile：75.5(Chemistry, Physical)Sato, Tetsuya*; Tatsuno, Masahiro*; Matsuo, Mamoru; Kato, Takeo*
Journal of Magnetism and Magnetic Materials, 546, p.168814_1 - 168814_6, 2022/03
Times Cited Count：0 Percentile：0(Materials Science, Multidisciplinary)Kato, Chiaki; Yamagishi, Isao; Sato, Tomonori; Yamamoto, Masahiro*
Zairyo To Kankyo, 70(12), p.441 - 447, 2021/12
Zeolite particles have been used in a Cs adsorption vessel for purification of contaminated water in Fukushima Dai-ich Nuclear Power Station (1F). The used Cs adsorption vessels were kept in storage space on 1F site. The risk of localized corrosion of stainless steel used in the vessel was worried. To evaluate the risk of localized corrosion, using specially designed electrochemical testing apparatus was used under gamma-ray irradiation test. And, real size mock-up test conducted. The results showed the potential change caused by creation of H
O by water radiolysis decreased by zeolite particles and the enrichment of chloride ion concentration in the vessel do not propagate during dry up procedure of Cs adsorption vessel. These data indicate the risk of localized corrosion of Cs adsorption vessel may stay at considerably low level.
Chen, Y.*; Sato, Masahiro*; Tang, Y.*; Shiomi, Yuki*; Oyanagi, Koichi*; Masuda, Takatsugu*; Nambu, Yusuke*; Fujita, Masaki*; Saito, Eiji
Nature Communications (Internet), 12, p.5199_1 - 5199_7, 2021/08
Times Cited Count：8 Percentile：61.37(Multidisciplinary Sciences)
-state of a 
hypernucleus, 
Yoshimoto, Masahiro*; Fujita, Manami; Hashimoto, Tadashi; Hayakawa, Shuhei; Ichikawa, Yudai; Ichikawa, Masaya; Imai, Kenichi*; Nanamura, Takuya; Naruki, Megumi; Sako, Hiroyuki; et al.
Progress of Theoretical and Experimental Physics (Internet), 2021(7), p.073D02_1 - 073D02_19, 2021/07
Times Cited Count：13 Percentile：81.3(Physics, Multidisciplinary)Mori, Kazuhiro*; Okumura, Ryo*; Yoshino, Hirofumi*; Kanayama, Masaya*; Sato, Setsuo*; Oba, Yojiro; Iwase, Kenji*; Hiraka, Haruhiro*; Hino, Masahiro*; Sano, Tadafumi*; et al.
JPS Conference Proceedings (Internet), 33, p.011093_1 - 011093_6, 2021/03
no abstracts in English
Inoue, Rintaro*; Oda, Takashi*; Nakagawa, Hiroshi; Tominaga, Taiki*; Saio, Tomohide*; Kawakita, Yukinobu; Shimizu, Masahiro*; Okuda, Aya*; Morishima, Ken*; Sato, Nobuhiro*; et al.
Scientific Reports (Internet), 10, p.21678_1 - 21678_10, 2020/12
Times Cited Count：3 Percentile：13.48(Multidisciplinary Sciences)Incoherent quasielastic neutron scattering (iQENS) is a fascinating technique for investigating the internal dynamics of protein. However, both low flux of neutron beam and absence of analytical procedure for extracting the internal dynamics from iQENS profile have been obstacles for studying it under physiological condition (in solution). Thanks to the recent development of neutron source, spectrometer and computational technique, they enable us to decouple internal dynamics, translational and rotational diffusions from the iQENS profile. The internal dynamics of two proteins: globular domain protein (GDP) and intrinsically disordered protein (IDP) in solution were studied. It was found that the average relaxation rate of IDP was larger than that of GDP. Through the detailed analyses on their internal dynamics, it was revealed that the fraction of mobile H atoms in IDP was much higher than that in GDP. Interestingly, the fraction of mobile H atoms was closely related to the fraction of H atoms on highly solvent exposed surfaces. The iQENS study presented that the internal dynamics were governed by the highly solvent exposed amino acid residues depending upon protein molecular architectures.
H monitoring in radioactive gaseous wasteFurutani, Misa; Kometani, Tatsunari; Nakagawa, Masahiro; Ueno, Yumi; Sato, Junya; Iwai, Yasunori*
Hoken Butsuri (Internet), 55(2), p.97 - 101, 2020/06
Herein, an oxidation catalyst was introduced after heating it to 600
C to oxidize tritium gas (HT) existing in exhaust into tritiated water vapor (HTO). This study aims to establish a safer H monitoring system by lowering the heating temperature required for the catalyst. In these experiments, which were conducted in the Nuclear Science Research Institute, Japan Atomic Energy Agency, cupric oxide, hydrophobic palladium/silicon dioxide (Pd/SiO), and platinum/aluminum oxide (Pt/AlO
) catalysts were ventilated using standard hydrogen gas. After comparing the oxidation efficiency of each catalyst at different temperatures, we found that the hydrophobic Pd/SiO and Pt/AlO catalysts could oxidize HT into HTO at 25C.
Higashino, Ritsuko*; Sato, Yuji*; Masuno, Shinichiro*; Shobu, Takahisa; Funada, Yoshinori*; Abe, Nobuyuki*; Tsukamoto, Masahiro*
Laser 3D Manufacturing VII (Proceedings of SPIE Vol.11271), p.1127114_1 - 1127114_7, 2020/05
Times Cited Count：5 Percentile：95.2(Engineering, Manufacturing)-rays after neutron capture by 
La for a T-violation searchOkudaira, Takuya; Shimizu, Hirohiko*; Kitaguchi, Masaaki*; Hirota, Katsuya*; Haddock, C. C.*; Ito, Ikuya*; Yamamoto, Tomoki*; Endo, Shunsuke*; Ishizaki, Kohei*; Sato, Takumi*; et al.
EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12
Parity violating effects enhanced by up to 10
times have been observed in several neutron induced compound nuclei. There is a theoretical prediction that time reversal (T) violating effects can also be enhanced in these nuclei implying that T-violation can be searched for by making very sensitive measurements. However, the enhancement factor has not yet been measured in all nuclei. The angular distribution of the (n,) reaction was measured with La by using a germanium detector assembly at J-PARC, and the enhancement factor was obtained. From the result, the measurement time to achieve the most sensitive T-violation search was estimated as 1.4 days, and a 40% polarized La target and a 70% polarized 
He spin filter whose thickness is 70 atm
cm are needed. Therefore high quality He spin filter is developed in JAEA. The measurement result of the (n,) reaction at J-PARC and the development status of the He spin filter will be presented.
Hirobe, Daichi*; Sato, Masahiro*; Hagihara, Masato*; Shiomi, Yuki*; Masuda, Takatsugu*; Saito, Eiji
Physical Review Letters, 123(11), p.117202_1 - 117202_7, 2019/09
Times Cited Count：14 Percentile：65.02(Physics, Multidisciplinary)Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.
Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07
Times Cited Count：8 Percentile：56.2(Physics, Multidisciplinary)Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for 
Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.
Otani, Kyohei; Sato, Tomonori; Kaji, Yoshiyuki; Yamamoto, Masahiro
JAEA-Review 2019-007, 15 Pages, 2019/06
JAEA-Review-2019-007.pdf:2.35MB
Metallic pipes under solid-liquid two phase flow is damaged by collision of solid particle to the pipe walls, and this phenomenon is named "erosion". In the case of the liquid is corrosive solution, further damage is occurred on the pipe walls chemically, and this named "erosion-corrosion". In the Fukushima Daiichi decommissioning project, the fuel debris will be crushed during removal operation of the debris and micro debris particles would be generated. It is estimated that the pipes of the circulating cooling system would be damaged under the solid-liquid two phase flow containing fuel debris particles. For the reason, the previous study about erosion and erosion-corrosion of metallic materials under solid-liquid two phase flow was surveyed. The survey showed that the damage rate by erosion and erosion-corrosion is influence by a lot of parameter in comparison to the corrosion rate which occurred in no-flow solution. Therefore, it is necessary to pay attention to selecting the experimental method and condition before the investigation about erosion-corrosion of metallic materials under solid-liquid two phase flow is carried out.
Sato, Yuji*; Tsukamoto, Masahiro*; Shobu, Takahisa; Funada, Yoshinori*; Yamashita, Yorihiro*; Hara, Takahiro*; Sengoku, Masanori*; Sakon, Yu*; Okubo, Tomomasa*; Yoshida, Minoru*; et al.
Applied Surface Science, 480, p.861 - 867, 2019/06
Times Cited Count：30 Percentile：82.18(Chemistry, Physical)