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Journal Articles

Accumulation possibility of tritium released from the Fukushima Daiichi Nuclear Power Station in marine organisms

Sato, Yuhi*; Tani, Takashi*; Ikenoue, Tsubasa; Kawamura, Hideyuki; Omori, Yuko*

Environmental Science and Pollution Research, 33(13), p.5818 - 5826, 2026/04

Tokyo Electric Power Company Holdings began the oceanic release of treated water from the Fukushima Daiichi Nuclear Power Station (FDNPS) in August 2023, in which radioactive materials were effectively removed using the Advanced Liquid Processing System (ALPS). The environmental behavior of tritium, accounting for almost all radioactivity in ALPS-treated water, is of critical scientific and social concern. The accumulation possibility of tritium in marine organisms under the release conditions of ALPS-treated water was reviewed to ensure the safety of fishery products collected off the Fukushima coast and prevent unfounded reputation damages to the products. First, previous findings from actual measurements and numerical model estimations of the distribution of tritium derived from ALPS-treated water in seawater off the Fukushima coast are summarized to discuss the impact of oceanic release on tritium levels in seawater. As a result, the impact is suggested to be highly limited, which is indistinguishable from a natural level except for within 200 km from FDNPS. Second, the accumulation possibility of organically bound tritium (OBT) in marine organisms, such as phytoplankton, seaweed, and fish, was assessed using previous findings obtained from experimental and numerical studies, resulting in far smaller OBT accumulations in those organisms compared to the food-chain guideline proposed by FAO/WHO. Finally, the risks of internal exposure through the ingestion of fishery products collected off the Fukushima coast are discussed and quantitatively explained to be minimal especially in comparison with the food-chain guideline. However, continuous environmental monitoring of the oceanic release of ALPS-treated water is considered essential.

Journal Articles

Tailoring neutron-shielding boron-metakaolin geopolymers with B$$_{4}$$C filler; Surfactant-driven interfacial and microstructural control

Niu, X.*; Elakneswaran, Y.*; Kikuchi, Ryosuke*; Li, A.*; Seralathan, S.*; Hiraki, Yoshihisa; Sato, Junya; Osugi, Takeshi; Kamiyama, Takashi*; Walkley, B.*

Cement and Concrete Research, 200, p.108096_1 - 108096_17, 2026/02

 Times Cited Count:4 Percentile:38.01(Construction & Building Technology)

Journal Articles

Mechanical property evaluation of rocks around Tanakura Fault, 1; Applicability of impact and needle penetration tests

Asahina, Daisuke*; Takamura, Hiroaki*; Tsukamoto, Koji*; Honda, Fumito*; ITO, Takashi*; IWATA, Naoki*; Aydan, $"O$mer*; Sato, Toshinori

Dai-51-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koen Rombunshu(Internet), p.43 - 47, 2025/12

Fault zones commonly contain distinctive structures such as fault cores and damage zones, where physical properties vary locally. These zones are important for evaluating underground safety and groundwater flow in waste disposal, yet quantitative measurements near faults remain limited. We applied Schmidt hammer and needle penetration tests to assess the mechanical properties of the rocks near the Tanakura Fault, in a simple, non-destructive manner. The results showed a clear spatial variation in measured values with distance from the fault gouge boundary, suggesting that combining methods with different scales and sensitivities can provide a more comprehensive evaluation of rock mass properties near faults.

Journal Articles

Negligible tritium accumulation in Japanese flounder from treated water released from Fukushima Daiichi Nuclear Power Plant; A Numerical simulation study

Ikenoue, Tsubasa; Tani, Takashi*; Kawamura, Hideyuki; Sato, Yuhi*

Environmental Science & Technology, 59(38), p.20588 - 20594, 2025/09

 Times Cited Count:5 Percentile:68.17(Engineering, Environmental)

Since 2023, ALPS-treated water containing tritium from the Fukushima Daiichi Nuclear Power Plant (1F) accident has been released into the ocean. Monitoring of seafood collected near the Fukushima coast has shown negligible increases in the tritium concentration. However, this monitoring has limitations, including delayed data release and a limited sample size. Therefore, a predictive estimation is necessary to assess the potential for high tritium accumulation in seafood. This study estimated tritium concentrations in Japanese flounder near the Fukushima coast using numerical simulations. The estimation combined an oceanic dispersion model for tritiated water (HTO) with a tritium transfer model for the marine food web. Tritium accumulation was evaluated as organically bound tritium (OBT), the long-retaining chemical form of tritium in organisms. First, the dispersion model's ability to reproduce HTO concentrations in seawater was validated using actual measurement data from the Fukushima coast, showing good agreement. Subsequently, the OBT concentrations in flounder were estimated under the hypothetical maximum release scenario of the treated water. The estimation suggested that even within 100 km of 1F, the maximum concentration of the OBT was comparable with natural levels of tritium in environmental waters. Additionally, the maximum concentration in the flounder remained at a negligible level for internal radiation exposure through consumption.

Journal Articles

Large-scale experiment of floating seismic isolation system

Yamamoto, Tomohiko; Imai, Yoshiyuki; Marufuji, Takato; Akasaka, Naoaki; Yan, X.; Otani, Akihito*; Kai, Satoru*; Mori, Takashi*; Uoji, Tomoki*; Ueno, Tomohiro*; et al.

Proceedings of the ASME 2025 Pressure Vessels & Piping Conference (PVP2025) (Internet), 7 Pages, 2025/07

Journal Articles

Feasibility of individual dosimetry using RT-PHITS for patients with SPECT/CT imaging after $$^{177}$$Lu-DOTATATE peptide receptor radionuclide therapy

Miwa, Kenta*; Kakino, Ryo*; Sato, Tatsuhiko; Furuta, Takuya; Miyaji, Noriaki*; Yamao, Tensho*; Yamashita, Kosuke*; Terauchi, Takashi*

Physical and Engineering Sciences in Medicine, 48(2), p.949 - 957, 2025/06

 Times Cited Count:3 Percentile:73.58(Engineering, Biomedical)

Radiotherapy package based on Particle and Heavy Ion Transport code System (RT-PHITS) enables to calculate the 3-dimensional dose distribution inside patients using their individual SPECT/CT images coupled with the Monte Carlo radiation transport simulation. The objective of this study is to evaluate the feasibility of individual dosimetry based on RT-PHITS for patients after $$^{177}$$Lu-DOTATATE peptide receptor radionuclide therapy.

Journal Articles

Revealing an origin of temperature-dependent structural change in intrinsically disordered proteins

Inoue, Rintaro*; Oda, Takashi; Nakagawa, Hiroshi; Tominaga, Taiki*; Ikegami, Takahisa*; Konuma, Tsuyoshi*; Iwase, Hiroki*; Kawakita, Yukinobu; Sato, Mamoru*; Sugiyama, Masaaki*

Biophysical Journal, 124(3), p.540 - 548, 2025/02

 Times Cited Count:3 Percentile:53.37(Biophysics)

Journal Articles

Multiple metamagnetic transitions in the helical antiferromagnet CeVGe$$_{3}$$

Jin, H.*; Choi, E. S.*; Wu, H.-C.*; Curro, N. J.*; Nawa, Kazuhiro*; Sato, Taku*; Kiyanagi, Ryoji; Ohara, Takashi; Klavins, P.*; Taufour, V.*

Physical Review B, 111(3), p.035103_1 - 035103_7, 2025/01

 Times Cited Count:1 Percentile:0.00(Materials Science, Multidisciplinary)

Journal Articles

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer spectroscopy of Sm-based heavy fermion compounds

Tsutsui, Satoshi; Higashinaka, Ryuji*; Mizumaki, Masaichiro*; Kobayashi, Yoshio*; Nakamura, Jin*; Ito, Takashi; Yoda, Yoshitaka*; Matsuda, Tatsuma*; Aoki, Yuji*; Sato, Hideyuki*

Interactions (Internet), 245(1), p.9_1 - 9_10, 2024/12

Journal Articles

Single-shot laser-driven neutron resonance spectroscopy for temperature profiling

Lan, Z.*; Arikawa, Yasunobu*; Mirfayzi, S. R.*; Morace, A.*; Hayakawa, Takehito*; Sato, Hirotaka*; Kamiyama, Takashi*; Wei, T.*; Tatsumi, Yuta*; Koizumi, Mitsuo; et al.

Nature Communications (Internet), 15, p.5365_1 - 5365_7, 2024/07

 Times Cited Count:14 Percentile:85.90(Multidisciplinary Sciences)

Journal Articles

Production rates of long-lived radionuclides $$^{10}$$Be and $$^{26}$$Al under direct muon-induced spallation in granite quartz and its implications for past high-energy cosmic ray fluxes

Sakurai, Hirohisa*; Kurebayashi, Yutaka*; Suzuki, Soichiro*; Horiuchi, Kazuho*; Takahashi, Yui*; Doshita, Norihiro*; Kikuchi, Satoshi*; Tokanai, Fuyuki*; Iwata, Naoyoshi*; Tajima, Yasushi*; et al.

Physical Review D, 109(10), p.102005_1 - 102005_18, 2024/05

 Times Cited Count:0 Percentile:0.00(Astronomy & Astrophysics)

Secular variations of galactic cosmic rays (GCRs) are inseparably associated with the galactic activities and should reflect the environments of the local galactic magnetic field, interstellar clouds, and nearby supernova remnants. The high-energy muons produced in the atmosphere by high-energy GCRs can penetrate deep underground and generate radioisotopes in the rock. As long lived radionuclides such as $$^{10}$$Be and $$^{26}$$Al have been accumulating in these rocks, concentrations of $$^{10}$$Be and $$^{26}$$Al can be used to estimate the long-term variations in high-energy muon yields, corresponding to those in the high-energy GCRs over a few million years. This study measured the production cross sections for muon induced $$^{10}$$Be and $$^{26}$$Al by irradiating positive muons with the momentum of 160 GeV/c on the synthetic silica plates and the granite core at the COMPASS experiment line in CERN SPS. In addition, it the contributions of the direct muon spallation reaction and the nuclear reactions by muon-induced particles on the production of long lived radionuclides in the rocks were clarified.

Journal Articles

Development of an Fe$$^{rm II}$$ complex exhibiting intermolecular proton shifting coupled spin transition

Ji, T.*; Su, S.*; Wu, S.*; Hori, Yuta*; Shigeta, Yasuteru*; Huang, Y.*; Zheng, W.*; Xu, W.*; Zhang, X.*; Kiyanagi, Ryoji; et al.

Angewandte Chemie; International Edition, 63(25), p.e202404843_1 - e202404843_6, 2024/04

 Times Cited Count:4 Percentile:33.51(Chemistry, Multidisciplinary)

JAEA Reports

Analysis of deposits inside the reactor at Fukushima Daiichi Nuclear Power Station in JFY2021; The Subsidy program of "Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris)" starting FY2021

Ikeuchi, Hirotomo; Sasaki, Shinji; Onishi, Takashi; Nakayoshi, Akira; Arai, Yoichi; Sato, Takumi; Ohgi, Hiroshi; Sekio, Yoshihiro; Yamaguchi, Yukako; Morishita, Kazuki; et al.

JAEA-Data/Code 2023-005, 418 Pages, 2023/12

JAEA-Data-Code-2023-005-01.pdf:24.59MB
JAEA-Data-Code-2023-005-02.pdf:32.18MB

For safe and steady decommissioning of Tokyo Electric Power Company Holdings' Fukushima Daiichi Nuclear Power Station (1F), information concerning composition and physical/chemical properties of fuel debris generated in the reactors should be estimated and provided to other projects conducting the decommissioning work including the retrieval of fuel debris and the subsequent storage. For this purpose, in FY2021, samples of contaminants (the wiped smear samples and the deposits) obtained through the internal investigation of the 1F Unit 2 were analyzed to clarify the components and to characterize the micro-particles containing uranium originated from fuel (U-bearing particles) in detail. This report summarized the results of analyses performed in FY2021, including the microscopic analysis by SEM and TEM, radiation analysis, and elemental analysis by ICP-MS, as a database for evaluating the main features of each sample and the probable formation mechanism of the U-bearing particles.

JAEA Reports

Stabilization of post-experiment nuclear materials in Plutonium Fuel Research Facility

Sato, Takumi; Otobe, Haruyoshi; Morishita, Kazuki; Marufuji, Takato; Ishikawa, Takashi; Fujishima, Tadatsune; Nakano, Tomoyuki

JAEA-Technology 2023-016, 41 Pages, 2023/09

JAEA-Technology-2023-016.pdf:2.74MB

This report summarizes the results of the stabilization treatments of post-experiment nuclear materials in Plutonium Fuel Research Facility (PFRF) from August 2018 to March 2021. Based on the management standards for nuclear materials enacted after the contamination accident that occurred at PFRF on June 6, 2017, the post-experiment nuclear materials containing plutonium (Pu): samples mixed with organic substances that cause an increase in internal pressure due to radiolysis (including X-ray diffraction samples mixed with epoxy resin and plutonium powder which caused contamination accidents), carbides and nitrides samples which is reactive in air, and chloride samples which may cause corrosion of storage containers, were selected as targets of the stabilization. The samples containing organic materials, carbides and nitrides were heated in an air flow at 650 $$^{circ}$$C and 950 $$^{circ}$$C for 2 hours respectively to remove organic materials and convert uranium (U) and Pu into oxides. U and Pu chlorides in LiCl-KCl eutectic melt were reduced and extracted into liquid Cd metal by a reaction with lithium (Li) -cadmium (Cd) alloy and converted to U-Pu-Cd alloy at 500 $$^{circ}$$C or higher. All of the samples were stabilized and stored at PFRF. We hope that the contents of this report will be utilized to consider methods for stabilizing post experiment nuclear materials at other nuclear fuel material usage facilities.

Journal Articles

R&D of digital technology on inverse estimation of radioactive source distributions and related source countermeasures; R&D status of digital platform including 3D-ADRES-indoor

Machida, Masahiko; Yamada, Susumu; Kim, M.; Okumura, Masahiko; Miyamura, Hiroko; Shikaze, Yoshiaki; Sato, Tomoki*; Numata, Yoshiaki*; Tobita, Yasuhiro*; Yamaguchi, Takashi; et al.

RIST News, (69), p.2 - 18, 2023/09

The contamination of radioactive materials leaked from the reactor has resulted in numerous hot spots in the Fukushima Daiichi Nuclear Power Station (1F) building, posing obstacles to its decommissioning. In order to solve this problem, JAEA has conducted research and development of the digital technique for inverse estimation of radiation source distribution and countermeasures against the estimated source in virtual space for two years from 2021 based on the subsidy program "Project of Decommissioning and Contaminated Water Management" performed by the funds from the Ministry of Economy, Trade and Industry. In this article, we introduce the results of the project and the plan of the renewal project started in April 2023. For the former project, we report the derivative method for LASSO method considering the complex structure inside the building and the character of the source and show the result of the inverse estimation using the method in the real reactor building. Moreover, we explain the platform software "3D-ADRES-Indoor" which integrates these achievements. Finally, we introduce the plan of the latter project.

Journal Articles

A Terrestrial SER Estimation Methodology Based on Simulation Coupled With One-Time Neutron Irradiation Testing

Abe, Shinichiro; Hashimoto, Masanori*; Liao, W.*; Kato, Takashi*; Asai, Hiroaki*; Shimbo, Kenichi*; Matsuyama, Hideya*; Sato, Tatsuhiko; Kobayashi, Kazutoshi*; Watanabe, Yukinobu*

IEEE Transactions on Nuclear Science, 70(8, Part 1), p.1652 - 1657, 2023/08

 Times Cited Count:9 Percentile:71.24(Engineering, Electrical & Electronic)

Single event upsets (SEUs) caused by neutrons is a reliability problem for microelectronic devices in the terrestrial environment. Acceleration tests using white neutron beam provide realistic soft error rates (SERs), but only a few facilities can provide white neutron beam in the world. If single-source irradiation applicable to diverse neutron source can be utilized for the evaluation of the SER in the terrestrial environment, it contributes to solve the shortage of beam time. In this study, we investigated the feasibility of the SER estimation in the terrestrial environment by any one of these measured data with the SEU cross sections obtained by PHITS simulation. It was found that the SERs estimated by our proposed method are within a factor of 2.7 of that estimated by the Weibull function. We also investigated the effect of simplification which reduce the computational cost in simulation to the SER estimation.

Journal Articles

Development of an iron(II) complex exhibiting thermal- and photoinduced double proton-transfer-coupled spin transition in a short hydrogen bond

Nakanishi, Takumi*; Hori, Yuta*; Shigeta, Yasuteru*; Sato, Hiroyasu*; Kiyanagi, Ryoji; Munakata, Koji*; Ohara, Takashi; Okazawa, Atsushi*; Shimada, Rintaro*; Sakamoto, Akira*; et al.

Journal of the American Chemical Society, 145(35), p.19177 - 19181, 2023/08

 Times Cited Count:9 Percentile:49.45(Chemistry, Multidisciplinary)

Journal Articles

First observation of $$^{28}$$O

Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.

Nature, 620(7976), p.965 - 970, 2023/08

 Times Cited Count:57 Percentile:95.97(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

Intruder configurations in $$^{29}$$Ne at the transition into the island of inversion; Detailed structure study of $$^{28}$$Ne

Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.

Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08

 Times Cited Count:8 Percentile:72.63(Astronomy & Astrophysics)

Detailed $$gamma$$-ray spectroscopy of the exotic neon isotope $$^{28}$$Ne has been performed using the one-neutron removal reaction from $$^{29}$$Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $$^{28}$$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

Journal Articles

Factors regulating the concentration of particulate iodine in coastal seawater

Sato, Yuhi*; Otosaka, Shigeyoshi*; Suzuki, Takashi; Nakanishi, Takahiro

Limnology and Oceanography, 68(7), p.1580 - 1594, 2023/07

 Times Cited Count:8 Percentile:60.67(Limnology)

To investigate the factors regulating the concentration of particulate iodine (PI) in seawater, it was measured in two Pacific coastal areas adjacent to Japan in two seasons along with parameters such as particulate organic carbon (POC) and nitrogen (PON), dissolved iodine (DI), and phytoplankton pigments. The dataset was divided in three groups namely, lower (Group A), average (Group B), and higher (Group C) atomic ratios of PI to POC (I/C). The three groups were characterized by phytoplanktonic physiological states as highly productive, steady, and senescent states, respectively. Based on the finding that PI production is associated with the phytoplankton physiological state, the seasonal and regional differences in PI concentration and I/C in the observation areas were consistently explained. Finally, we suggest that the phytoplanktonic physiological state is one of the vital factors regulating the PI concentration in seawater.

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