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Journal Articles

Measurement of spent nuclear fuel burn-up using a new H$$(n,gamma)$$ method

Nauchi, Yasushi*; Sato, Shunsuke*; Hayakawa, Takehito*; Kimura, Yasuhiko; Suyama, Kenya; Kashima, Takao*; Futakami, Kazuhiro*

Nuclear Instruments and Methods in Physics Research A, 1050, p.168109_1 - 168109_9, 2023/05

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

Measurement of neutrons from spent nuclear fuel is performed in this study using the H$$(n,gamma)$$ method, which detects 2.223 MeV $$gamma$$ rays from neutron capture reaction of hydrogen using a highly pure germanium (HPGe) detector. The detection of the 2.223 MeV $$gamma$$ ray is affected by intense $$gamma$$ ray emission from fission products (FPs) because the emission rate of $$gamma$$ rays from the FP is seven orders of magnitude higher than the emission rate of neutrons. To shield the intense $$gamma$$ ray from the FP, the HPGe detector is placed off the axis of a collimator, whereas a polyethylene block is placed on the axis. In this geometry, the detector is shielded from the intense $$gamma$$ rays from the FP, but the detector can measure 2.223 MeV $$gamma$$ rays from the H$$(n,gamma)$$ reactions in the polyethylene block. The measured count rate of the 2.223 MeV $$gamma$$ rays is consistent with the expected rate within the statistical error, which is calculated based on the nuclide composition, which is primary $$^{244}$$Cm, estimated via depletion and decay calculations. Accordingly, the H$$(n,gamma)$$ method is considered feasible to quantify the number of neutron leakage from spent nuclear fuel assembly, which is applicable to certify burn up of the assembly.

Journal Articles

Role of resonance states of muonic molecule in muon catalyzed fusion

Okutsu, Kenichi*; Yamashita, Takuma*; Kino, Yasushi*; Miyashita, Konan*; Yasuda, Kazuhiro*; Oka, Toshitaka; Okada, Shinji*; Sato, Motoyasu*

JJAP Conference Proceedings (Internet), 9, p.011003_1 - 011003_7, 2023/00

Muon catalyzed fusion ($$mu$$CF) is a cyclic reaction where a negatively charged muon itself acts like a catalyst of nuclear fusion between hydrogen isotopes. In the $$mu$$CF reaction, muon transfer from deuteron to triton and muonic molecular formation are rate-limiting processes. In this work, we have investigated the role of resonance states of muonic molecule in the $$mu$$CF which affects the muonic deuterium atom population. Solving simultaneous rate equations numerically by the fourth-order Runge-Kutta method, we determined the muonic molecular formation rate so that the number of fusion events reproduces a latest experimental result. It is revealed that the resonance states play a role to enhance the fusion rate by accelerating the de-excitation of the muonic atoms.

Journal Articles

Spatial distribution and preferred orientation of crystalline microstructure of lead-bismuth eutectic

Ito, Daisuke*; Sato, Hirotaka*; Odaira, Naoya*; Saito, Yasushi*; Parker, J. D.*; Shinohara, Takenao; Kai, Tetsuya; Oikawa, Kenichi

Journal of Nuclear Materials, 569, p.153921_1 - 153921_6, 2022/10

 Times Cited Count:1 Percentile:31.61(Materials Science, Multidisciplinary)

Journal Articles

Absolute quantification of $$^{137}$$Cs activity in spent nuclear fuel with calculated detector response function

Sato, Shunsuke*; Nauchi, Yasushi*; Hayakawa, Takehito*; Kimura, Yasuhiko; Kashima, Takao*; Futakami, Kazuhiro*; Suyama, Kenya

Journal of Nuclear Science and Technology, 60(6), p.615 - 623, 2022/06

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A new non-destructive method for evaluating $$^{137}$$Cs activity in spent nuclear fuels was proposed and experimentally demonstrated for physical measurements in burnup credit implementation. $$^{137}$$Cs activities were quantified using gamma ray measurements and numerical detector response simulations without reference fuels, in which $$^{137}$$Cs activities are well known. Fuel samples were obtained from a lead use assembly (LUA) irradiated in a commercial pressurized water reactor (PWR) up to 53 GWd/t. Gamma rays emitted from the samples were measured using a bismuth germinate (BGO) scintillation detector through a collimator attached to a hot cell. The detection efficiency of gamma rays with the detector was calculated using the PHITS particle transport calculation code considering the measurement geometry. The relative activities of $$^{134}$$Cs, $$^{137}$$Cs, and $$^{154}$$Eu in the sample were measured with a high-purity germanium (HPGe) detector for more accurate simulations of the detector response for the samples. The absolute efficiency of the detector was calibrated by measuring a standard gamma ray source in another geometry. $$^{137}$$Cs activity in the fuel samples was quantified using the measured count rate and detection efficiency. The quantified $$^{137}$$Cs activities agreed well with those estimated using the MVP-BURN depletion calculation code.

Journal Articles

Design for detecting recycling muon after muon-catalyzed fusion reaction in solid hydrogen isotope target

Okutsu, Kenichi*; Yamashita, Takuma*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.

Fusion Engineering and Design, 170, p.112712_1 - 112712_4, 2021/09

 Times Cited Count:3 Percentile:45.99(Nuclear Science & Technology)

A muonic molecule which consists of two hydrogen isotope nuclei (deuteron (d) or tritium (t)) and a muon decays immediately via nuclear fusion and the muon will be released as a recycling muon, and start to find another hydrogen isotope nucleus. The reaction cycle continues until the muon ends up its lifetime of 2.2 $$mu$$s. Since the muon does not participate in the nuclear reaction, the reaction is so called a muon catalyzed fusion ($$mu$$CF). The recycling muon has a particular kinetic energy (KE) of the muon molecular orbital when the nuclear reaction occurs. Since the KE is based on the unified atom limit where distance between two nuclei is zero. A precise few-body calculation estimating KE distribution (KED) is also in progress, which could be compared with the experimental results. In the present work, we observed recycling muons after $$mu$$CF reaction.

Journal Articles

Time evolution calculation of muon catalysed fusion; Emission of recycling muons from a two-layer hydrogen film

Yamashita, Takuma*; Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.

Fusion Engineering and Design, 169, p.112580_1 - 112580_5, 2021/08

 Times Cited Count:3 Percentile:45.99(Nuclear Science & Technology)

A muon ($$mu$$) having 207 times larger mass of electron and the same charge as the electron has been known to catalyze a nuclear fusion between deuteron (d) and triton (t). These two nuclei are bound by $$mu$$ and form a muonic hydrogen molecular ion, dt$$mu$$. Due to the short inter-nuclear distance of dt$$mu$$, the nuclear fusion, d +t$$rightarrow alpha$$ + n + 17.6 MeV, occurs inside the molecule. This reaction is called muon catalyzed fusion ($$mu$$CF). Recently, the interest on $$mu$$CF is renewed from the viewpoint of applications, such as a source of high-resolution muon beam and mono-energetic neutron beam. In this work, we report a time evolution calculation of $$mu$$CF in a two-layered hydrogen isotope target.

Journal Articles

Magnetic fluctuation and first-order transition in trillium lattice of EuPtSi observed by $$^{151}$$Eu M$"o$ssbauer spectroscopy

Homma, Yoshiya*; Kakihana, Masashi*; Tokunaga, Yo; Yogi, Mamoru*; Nakashima, Miho*; Nakamura, Ai*; Shimizu, Yusei*; Li, D.*; Maurya, A.*; Sato, Yoshiki*; et al.

Journal of the Physical Society of Japan, 88(9), p.094702_1 - 094702_8, 2019/08

 Times Cited Count:9 Percentile:59.53(Physics, Multidisciplinary)

Journal Articles

Visualization of phase distribution in lead-bismuth eutectic during one-dimensional solidification process

Ito, Daisuke*; Sato, Hirotaka*; Saito, Yasushi*; Parker, J. D.*; Shinohara, Takenao; Kai, Tetsuya

Journal of Visualization, 22(5), p.889 - 895, 2019/06

 Times Cited Count:1 Percentile:7.41(Computer Science, Interdisciplinary Applications)

Journal Articles

Studies of high density baryon matter with high intensity heavy-ion beams at J-PARC

Sako, Hiroyuki; Harada, Hiroyuki; Sakaguchi, Takao*; Chujo, Tatsuya*; Esumi, Shinichi*; Gunji, Taku*; Hasegawa, Shoichi; Hwang, S.; Ichikawa, Yudai; Imai, Kenichi; et al.

Nuclear Physics A, 956, p.850 - 853, 2016/12

 Times Cited Count:12 Percentile:65.66(Physics, Nuclear)

JAEA Reports

The Second periodic safety review report of Tokai Reprocessing Plant

Shirai, Nobutoshi; Miura, Yasushi; Tachibana, Ikuya; Omori, Satoru; Wake, Junichi; Fukuda, Kazuhito; Nakano, Takafumi; Nagasato, Yoshihiko

JAEA-Technology 2016-007, 951 Pages, 2016/07

JAEA-Technology-2016-007-01.pdf:11.93MB
JAEA-Technology-2016-007-02.pdf:4.7MB

The periodic safety review of TRP is to confirm the safety activities and get effective additional measures the facility safety and its reliability. We implemented 4 items; for (1) evaluation of safety activity implementation, we confirmed we are adequately expanding its safety activities by the necessary documents and schemes. For (2) evaluation of status of safety activities reflecting the latest technical knowledges, we confirmed we reflect latest knowledges for improvement of safety and reliability. For (3) technical evaluation about aging degradation, we can keep the safety of the facilities important to safety and the sea discharge line, under assumption of the present maintenance, because of "focuses for aging degradation". For (4) planning measures about a 10-years-plan that the operator shall implement to keep the facility condition, by the technical evaluation, we found no additional safety plans into maintenance strategies.

JAEA Reports

Environmental remediation for the upstream of Yotsugi Mill Tailings Pond, Ningyo-toge Uranium Mine

Saito, Hiroshi; Sato, Yasushi*; Sakamoto, Atsushi*; Torikai, Kazuyoshi; Fukushima, Shigeru; Sakao, Ryota; Taki, Tomihiro

JAEA-Technology 2015-063, 119 Pages, 2016/03

JAEA-Technology-2015-063.pdf:86.2MB

Ningyo-toge Environmental Engineering Center has been conducting environmental remediation of the Ningyo-toge Uranium Mine, after decades of mine-related activities were terminated. Its purposes are to take measures to ensure safety and radiation protection from the exposure pathways to humans in future, and to prevent the occurrence of mining pollution. As part of the remediation, upstream part of the Yotsugi Mill Tailings Pond, the highest prioritized facility, has been remediated to fiscal year 2012. Multi-layered capping has been constructed using natural material, after specifications and whole procedure being examined in terms of long-term stability, radiation protection, economics, etc. Monitoring has been carried out to confirm the effectiveness of the capping, in terms of settlement, dose and radon exhalation rates, etc. Monitoring of drainage volume of penetrated rainwater is planned. Accumulated data will be examined and used for remediation of downstream part of the Pond.

JAEA Reports

Corroborative tests for Oarai Waste Reduction Treatment Facility using the in-can type high frequency induction heating method

Sakauchi, Hitoshi; Sato, Isamu*; Donomae, Yasushi; Kitamura, Ryoichi

JAEA-Technology 2015-059, 352 Pages, 2016/03

JAEA-Technology-2015-059.pdf:51.53MB

OWTF (Oarai Waste Reduction Treatment Facility) is constructed for volume reduction processing and stabilization treatment of $$alpha$$ solid waste, which was generated from hot facilities in Oarai Research and Develop Center of Japan Atomic Energy Agency, using in-can type high frequency induction heating by remote control. This report describes corroborative tests, in which incinerating and melting performance for OWTF is confirmed with a full-scale testing furnace. We have been carrying out the tests of incinerating and melting treatment with some kinds of simulated wastes, such as enclosure form of radioactive wastes, material and articles.

Journal Articles

Progress report of Japanese simulation research projects using the high-performance computer system Helios in the International Fusion Energy Research Centre

Ishizawa, Akihiro*; Idomura, Yasuhiro; Imadera, Kenji*; Kasuya, Naohiro*; Kanno, Ryutaro*; Satake, Shinsuke*; Tatsuno, Tomoya*; Nakata, Motoki*; Nunami, Masanori*; Maeyama, Shinya*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 92(3), p.157 - 210, 2016/03

The high-performance computer system Helios which is located at The Computational Simulation Centre (CSC) in The International Fusion Energy Research Centre (IFERC) started its operation in January 2012 under the Broader Approach (BA) agreement between Japan and the EU. The Helios system has been used for magnetised fusion related simulation studies in the EU and Japan and has kept high average usage rate. As a result, the Helios system has contributed to many research products in a wide range of research areas from core plasma physics to reactor material and reactor engineering. This project review gives a short catalogue of domestic simulation research projects. First, we outline the IFERC-CSC project. After that, shown are objectives of the research projects, numerical schemes used in simulation codes, obtained results and necessary computations in future.

Journal Articles

Femtosecond time-resolved dynamical Franz-Keldysh effect

Otobe, Tomohito; Shinohara, Yasushi*; Sato, Shunsuke*; Yabana, Kazuhiro*

Physical Review B, 93(4), p.045124_1 - 045124_9, 2016/01

 Times Cited Count:48 Percentile:86.99(Materials Science, Multidisciplinary)

We theoretically investigate the dynamical Franz-Keldysh effect in femtosecond time resolution, that is, the time-dependent modulation of a dielectric function at around the band gap under an irradiation of an intense laser field. We develop a pump-probe formalism in two distinct approaches: first-principles simulation based on real-time time-dependent density functional theory and analytic consideration of a simple two-band model. We find that, while time-average modulation may be reasonably described by the static Franz-Keldysh theory, a remarkable phase shift is found to appear between the dielectric response and the applied electric field.

Journal Articles

Time-dependent density functional theory of high-intensity short-pulse laser irradiation on insulators

Sato, Shunsuke*; Yabana, Kazuhiro*; Shinohara, Yasushi*; Otobe, Tomohito; Lee, K.-M.*; Bertsch, G. F.*

Physical Review B, 92(20), p.205413_1 - 205413_6, 2015/11

 Times Cited Count:46 Percentile:84.85(Materials Science, Multidisciplinary)

We calculate the energy deposition by very short laser pulses in SiO$$_{2}$$ ($$alpha$$-quartz) with a view to establishing systematics for predicting damage and nanoparticle production. The theoretical framework is time-dependent density functional theory, implemented by the real-time method in a multiscale representation. We find that the deposited energy in the medium can be accurately modeled as a function of the local electromagnetic pulse fluence. The energy deposition function can in turn be quite well fitted to the strong-field Keldysh formula. We find reasonable agreement between the damage threshold and the energy required to melt the substrate. The ablation threshold estimated by the energy to convert the substrate to an atomic fluid is higher than the measurement, indicating significance of nonthermal nature of the process. A fair agreement is found for the depth of the ablation.

Journal Articles

Numerical analysis of organ doses delivered during computed tomography examinations using Japanese adult phantoms with the WAZA-ARI dosimetry system

Takahashi, Fumiaki; Sato, Kaoru; Endo, Akira; Ono, Koji*; Ban, Nobuhiko*; Hasegawa, Takayuki*; Katsunuma, Yasushi*; Yoshitake, Takayasu*; Kai, Michiaki*

Health Physics, 109(2), p.104 - 112, 2015/08

 Times Cited Count:8 Percentile:56.13(Environmental Sciences)

A dosimetry system, named WAZA-ARI, is developed to assess accurately radiation doses to persons from Computed Tomography (CT) examination patients in Japan. Organ doses were prepared to application to dose calculations in WAZA-ARI by numerical analyses using average adult Japanese human models with the Particle and Heavy Ion Transport code System (PHITS). Experimental studies clarified the radiation configuration on the table for some multi-detector row CT (MDCT) devices. Then, a source model in PHITS could specifically take into account for emissions of X-ray in each MDCT device based on the experiment results. Numerical analyses with PHITS revealed a concordance of organ doses with human body size. The organ doses by the JM phantoms were compared with data obtained using previously developed systems. In addition, the dose calculation in WAZA-ARI were verified with previously reported results by realistic NUBAS phantoms and radiation dose measurement using a physical Japanese model. The results implied that analyses using the Japanese phantoms and PHITS including source models can appropriately give organ dose data with consideration of the MDCT device and physiques of typical Japanese adults.

Journal Articles

WAZA-ARI; A Dose assessment system for patients in CT scan

Sato, Kaoru; Takahashi, Fumiaki; Endo, Akira; Ono, Koji*; Hasegawa, Takayuki*; Katsunuma, Yasushi*; Yoshitake, Takayasu*; Ban, Nobuhiko*; Kai, Michiaki*

RIST News, (58), p.25 - 32, 2015/01

The Japan Atomic Energy Agency (JAEA) are now developing WAZA-ARI for improvement of management of exposure doses due to CT examination under the joint research with the Oita University of Nursing and Health Sciences. The trial version of WAZA-ARI has been released on 21 December 2012. In trial version, users can perform dose assessment by using organ dose database based on the average adult Japanese male (JM-103) and female (JF-103) voxel phantoms and a 4 years old female voxel phantom (UFF4). The homepage of WAZA-ARI has been accessed over 1000 times per month and 28421 times by the end of September 2014. We are developing WAZA-ARI version 2 as the extension version of dose calculation functions of WAZA-ARI. WAZA-ARI version 2 will be released by the end of March 2015. In WAZA-ARI version 2. Users can upload dose calculation results to WAZA-ARI version 2 server, and utilize improvement of the dose management of patients and the optimization of CT scan conditions.

Journal Articles

Dielectric response of laser-excited silicon at finite electron temperature

Sato, Shunsuke*; Shinohara, Yasushi*; Otobe, Tomohito; Yabana, Kazuhiro*

Physical Review B, 90(17), p.174303_1 - 174303_8, 2014/11

 Times Cited Count:39 Percentile:81.84(Materials Science, Multidisciplinary)

We calculate the dielectric response of excited crystalline silicon in electron thermal equilibrium by adiabatic time-dependent density functional theory (TDDFT) to model the response to irradiation by high-intensity laser pulses. We find that the extracted effective mass are in the range of 0.22-0.36 and lifetimes are in the range of 1-14 fs depending on the temperature.

Journal Articles

Cabling technology of Nb$$_3$$Sn conductor for ITER central solenoid

Takahashi, Yoshikazu; Nabara, Yoshihiro; Ozeki, Hidemasa; Hemmi, Tsutomu; Nunoya, Yoshihiko; Isono, Takaaki; Matsui, Kunihiro; Kawano, Katsumi; Oshikiri, Masayuki; Uno, Yasuhiro; et al.

IEEE Transactions on Applied Superconductivity, 24(3), p.4802404_1 - 4802404_4, 2014/06

 Times Cited Count:25 Percentile:72.88(Engineering, Electrical & Electronic)

Japan Atomic Energy Agency (JAEA) is procuring all amounts of Nb$$_3$$Sn conductors for Central Solenoid (CS) in the ITER project. Before start of mass-productions, the conductor should be tested to confirm superconducting performance in the SULTAN facility, Switzerland. The original design of cabling twist pitches is 45-85-145-250-450 mm, called normal twist pitch (NTP). The test results of the conductors with NTP was that current shearing temperature (Tcs) is decreasing due to electro-magnetic (EM) load cycles. On the other hand, the results of the conductors with short twist pitches (STP) of 25-45-80-150-450 mm show that the Tcs is stabilized during EM load cyclic tests. Because the conductors with STP have smaller void fraction, higher compaction ratio during cabling is required and possibility of damage on strands increases. The technology for the cables with STP was developed in Japanese cabling suppliers. The several key technologies will be described in this paper.

Journal Articles

First-principles simulation of the optical response of bulk and thin-film $$alpha$$-quartz irradiated with an ultrashort intense laser pulse

Lee, K.-M.*; Kim, C. M.*; Sato, Shunsuke*; Otobe, Tomohito; Shinohara, Yasushi*; Yabana, Kazuhiro; Jeong, T. M.*

Journal of Applied Physics, 115(5), p.053519_1 - 053519_8, 2014/02

 Times Cited Count:27 Percentile:72.71(Physics, Applied)

A computational method based on a first-principles multiscale simulation has been used for calculating the optical response and the ablation threshold of an optical material irradiated with an ultrashort intense laser pulse. The method was applied to investigate the changes in the optical reflectance of quartz bulk, half-wavelength thin-film and quarter-wavelength thin-film and to estimate their ablation thresholds. Despite the adiabatic local density approximation used in calculating the exchange-correlation potential, the reflectance and the ablation threshold obtained from our method agree well with the previous theoretical and experimental results. The method can be applied to estimate the ablation thresholds for optical materials in general.

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