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JAEA Reports

Structural investigation of borosilicate glasses by using XAFS measurement in soft X-ray region, 4 (Joint research)

Nagai, Takayuki; Okamoto, Yoshihiro; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*

JAEA-Research 2024-014, 54 Pages, 2025/02

JAEA-Research-2024-014.pdf:7.02MB

XAFS measurements in the soft X-ray region are suitable for evaluating the chemical state of the surface layer of a measurement sample because the X-ray transmittance is low. In this study, the purpose of the study was to confirm the difference between the coagulated surface layer and the inside of the simulated waste glasses by measuring the K-edge of the glass constituent elements boron, oxygen, sodium, and silicon, and the L$$_{3}$$ edge of the waste component cerium. As a result, the B K-edge XANES spectra showed that the proportion of B-O tetracoordinate sp$$^{3}$$ structures (BO$$_{4}$$) on the surface layer of the coagulated glass samples was higher than that on the cut surface inside the glass samples, which is expected to improve the water resistance of the coagulated surface. On the other hand, the O K-edge XANES spectra suggested that the O abundance in the coagulated surface layer was lower than that in the cut surface inside the glass samples, and that alkali metal elements may be concentrated in the coagulated surface layer. However, no difference was observed in the Na K-edge XANES spectra between the coagulated surface layer and the cut surface, and no difference was observed in the Si K-edge XANES spectra between the solidified surface and the inside of glass samples. In addition, the Ce L$$_{3}$$-edge XANES spectra confirmed that the Ce valence in the surface layer of coagulated glass samples were oxidized compared to the inside of glass samples.

Journal Articles

In-situ detection of high-energy beta ray emitter $$^{90}$$Sr/$$^{90}$$Y inside the Fukushima Daiichi Nuclear Power Station Unit 3 reactor building using a liquid light guide Cherenkov counter

Terasaka, Yuta; Sato, Yuki; Furuta, Yoshihiro*; Kubo, Shin*; Ichiba, Yuta*

Nuclear Instruments and Methods in Physics Research A, 1070(2), p.170021_1 - 170021_9, 2025/01

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Journal Articles

Surface structure of the 3$$times$$3-Si phase on Al(111), studied by the multiple usages of positron diffraction and core-level photoemission spectroscopy

Sato, Yusuke*; Fukaya, Yuki; 14 of others*

Physical Review Materials (Internet), 9(1), p.014002_1 - 014002_11, 2025/01

no abstracts in English

Journal Articles

Separating urban heat island circulation and convective cells through dynamic mode decomposition

Sato, Takuto; Hino, Hideitsu*; Kusaka, Hiroyuki*

Atmospheric Science Letters, 25(12), p.e1279_1 - e1279_10, 2024/12

 Times Cited Count:0 Percentile:0.00(Geochemistry & Geophysics)

This study applies dynamic mode decomposition (DMD) to three-dimensional simulation results of urban heat island circulation (UHIC, which is horizontal circulation) and thermals (vertical convections). The aim of this study is to revisit how these phenomena coexist based on the characteristics of temporal changes in the flow field. We used DMD to obtain the dominant spatial patterns and information on temporal changes. One of the modes of horizontal wind, which does not change temporally (no oscillation or amplification), exhibits a spatial UHIC pattern. The unique feature of this UHIC mode is that there are small-scale striated structures (150-200 m) and large-scale convergence. The other modes are time-varying (oscillating and decaying) and represent smaller spatial-scale phenomena (150-250 m), such as thermals. The frequency of each mode takes various values, some of which are lower than the lifetime of thermals in accordance with the Deardorff convective scale ($$sim$$10 min). These low-frequency modes showed striated structures similar to that observed in the UHIC modes. These results suggest that UHIC and thermals deform each other through components that vary in long temporal scales.

Journal Articles

Assessment of individual external exposure doses based on environmental radiation in areas affected by the Fukushima Daiichi Nuclear Power Station accident

Sato, Rina; Yoshimura, Kazuya; Sanada, Yukihisa; Mikami, Satoshi; Yamada, Tsutomu*; Nakasone, Takamasa*; Kanaizuka, Seiichi*; Sato, Tetsuro*; Mori, Tsubasa*; Takagi, Marie*

Environmental Science & Technology, 194, p.109148_1 - 109148_8, 2024/12

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Assessment of individual external doses from ambient dose equivalents is used for predictive and retrospective assessments where personal dosimeters are not applicable. However, it tends to contain more errors than assessment by personal dosimetry due to various parameters. Therefore, in order to accurately assess the individual dose from ambient dose equivalents, a model that estimates effective doses considering life patterns and the shielding effects by buildings and vehicles, were developed in this study. The model parameters were examined using robust datasets of environmental radiation measured in the areas affected by the Fukushima Daiichi Nuclear Power Station accident in 2020 to 2021. The accuracy of the model was validated by comparison with 106 daily personal doses measured in Fukushima Prefecture in 2020. The measured personal dose was well reproduced by the model-estimated effective dose, showing that the model can be used to assess the individual exposure dose, similar to personal dosimetry. Furthermore, this model is an effective tool for radiation protection, as it can estimate the individual dose predictively and retrospectively by using environmental radiation data.

Journal Articles

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer spectroscopy of Sm-based heavy fermion compounds

Tsutsui, Satoshi; Higashinaka, Ryuji*; Mizumaki, Masaichiro*; Kobayashi, Yoshio*; Nakamura, Jin*; Ito, Takashi; Yoda, Yoshitaka*; Matsuda, Tatsuma*; Aoki, Yuji*; Sato, Hideyuki*

Interactions (Internet), 245(1), p.9_1 - 9_10, 2024/12

Journal Articles

Forefront of development of next-generation innovative nuclear reactors (fast reactor and high-temperature gas-cooled reactor), 1; Latest trends of development of next-generation innovative nuclear reactors in Japan and foreign countries

Yamano, Hidemasa; Toyooka, Junichi; Sato, Hiroyuki; Sakaba, Nariaki

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 66(12), p.607 - 611, 2024/12

This report mainly introduces trends in fast reactor development in Japan in addition to introducing overseas development trends for major developing countries.

Journal Articles

Complete genome sequence of ${it Thiomicrospira}$ sp. strain V2501 isolated from 250 m below the ground level in Horonobe, Hokkaido, Japan

Ueno, Akio*; Sato, Kiyoshi*; Tamamura, Shuji*; Murakami, Takuma*; Inomata, Hidenori*; Tamazawa, Satoshi*; Amano, Yuki; Miyakawa, Kazuya; Naganuma, Takeshi*; Igarashi, Toshifumi*

Microbiology Resource Announcements (Internet), 13(11), p.e00108-24_1 - e00108-24_4, 2024/11

Journal Articles

Methodology development for explosion hazard evaluation in hydrogen production system using high temperature gas-cooled reactor

Morita, Keisuke; Aoki, Takeshi; Shimizu, Atsushi; Sato, Hiroyuki

Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 6 Pages, 2024/11

Journal Articles

Radioactivity estimation of radioactive hotspots using a Compton camera and derivation of dose rates in the surrounding environment

Sato, Yuki

Applied Radiation and Isotopes, 212, p.111421_1 - 111421_8, 2024/10

 Times Cited Count:0 Percentile:0.00(Chemistry, Inorganic & Nuclear)

Journal Articles

Dissolution of zirconium-cerium oxide solid solution in an aqueous system

Kobayashi, Taishi*; Sato, Yutaro*; Tonna, Ryutaro*; Matsumura, Daiju; Sasaki, Takayuki*; Ikeda, Atsushi

Dalton Transactions (Internet), 53(46), p.18616 - 18628, 2024/10

 Times Cited Count:0 Percentile:0.00(Chemistry, Inorganic & Nuclear)

Journal Articles

Development of a multi-scale meteorological Large-eddy simulation model for urban thermal environmental studies; The "City-LES" Model Version 2.0

Kusaka, Hiroyuki*; Ikeda, Ryosaku*; Sato, Takuto; Iizuka, Satoru*; Boku, Taisuke*

Journal of Advances in Modeling Earth Systems (Internet), 16(10), p.e2024MS004367_1 - e2024MS004367_38, 2024/10

 Times Cited Count:2 Percentile:64.04(Meteorology & Atmospheric Sciences)

To bridge the gaps between meteorological large-eddy simulation (LES) models and computational fluid dynamics (CFD) models for microscale urban climate simulations, the present study has developed a meteorological LES model for urban areas. This model simulates urban climates across both mesoscale (city scale) and microscale (city-block scale). The paper offers an overview of this LES model, which distinguishes itself from standard numerical weather prediction models by resolving buildings and trees at the microscale simulations. It also differs from standard CFD models by accounting for atmospheric stratification and physical processes. Noteworthy features of this model include: (a) the calculation of long- and short-wave radiations in three dimensions, incorporating multiple reflections within urban canopy layers using the radiosity method, and accounting for building and tree shadows in the simulations; (b) the provision of various heat stress indices (Universal Thermal Climate Index, Wet Bulb Globe Temperature, MRT, THI); (c) the assessment of the efficacy of heat stress mitigation measures such as dry-mist spraying, roadside trees, cool pavements, and green/cool roofs strategies; (d) the capability to run on supercomputers, with the code parallelized in a three-dimensional manner, and the model can also run on a graphics processing unit cluster. Following the introduction of this model, the study confirms its basic performance through various numerical experiments, including simulations of thermals in the convective boundary layer, coherent structure of turbulence over urban canopy, and thermal environment and heat stress indices in urban districts. The model developed in this study is intended to serve as a community tool for addressing both fundamental and applied studies in urban climatology.

Journal Articles

Addendum: Site occupancy of interstitial deuterium atoms in face-centred cubic iron

Machida, Akihiko*; Saito, Hiroyuki*; Sugimoto, Hidehiko*; Hattori, Takanori; Sano, Asami; Endo, Naruki*; Katayama, Yoshinori*; Iizuka, Riko*; Sato, Toyoto*; Matsuo, Motoaki*; et al.

Nature Communications (Internet), 15, p.8861_1 - 8861_2, 2024/10

 Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)

In our previous article (Nature Commun. 5, 5063 (2014)), the site occupancies of D atoms dissolved in an fcc Fe metal lattice were investigated via Rietveld refinement of neutron powder diffraction patterns collected at 988 K and 6.3 GPa. The fcc metal lattice has two interstitial sites available for accommodating D atoms: octahedral and tetrahedral sites. The Rietveld refinement revealed that D atoms occupied mainly the octahedral sites with occupancy of 0.532 and slightly the tetrahedral sites with occupancy of 0.056. Subsequent density-functional-theory (DFT) calculations by Antonov (Phys. Rev. Mater. 2019)) showed that the occupation energy on the tetrahedral site was significantly higher than that on the octahedral site; the tetrahedral site occupation was unlikely to occur even at temperatures as high as 988 K. We reexamined the site occupancies of D-atom by Rietveld refinement including extinction correction. As a result, the octahedral occupancy was increased to 0.60 and the tetrahedral occupancy was reduced to zero. The occupation of only the octahedral site for D atom is consistent with the DFT calculation, although in contrast to the previous results.

Journal Articles

Project plan of HTTR heat application test facility; Safety design and Safety analysis

Aoki, Takeshi; Hasegawa, Takeshi; Kurahayashi, Kaoru; Nomoto, Yasunobu; Shimizu, Atsushi; Sato, Hiroyuki; Sakaba, Nariaki

Proceedings of 11th International Topical Meeting on High Temperature Reactor Technology (HTR 2024), 6 Pages, 2024/10

Japan Atomic Energy Agency (JAEA) is planning to perform a test named HTTR heat application test coupling HTTR (High temperature engineering test reactor) and a hydrogen production plant. The present study reports results of the safety design and safety analysis for HTTR heat application test facility. As a safety design, safety classification of structures, systems, and components was defined in the test facility based on their safety functions. As a preliminary safety analysis, a thermal-hydraulic analysis was performed with RELAP5 code. The safety analysis revealed that newly identified events for HTTR heat application test facility except for the rupture of heat transfer tube of steam generator was enveloped by the licensing basis events in conventional HTTR. The preliminary analysis proved that the safety criteria is satisfied in the candidate of licensing basis event.

Journal Articles

Introduction to dismantling and decommissioning chemistry

Sato, Nobuaki*; Kameo, Yutaka; Sato, Soichi; Kumagai, Yuta; Sato, Tomonori; Yamamoto, Masahiro*; Watanabe, Yutaka*; Nagai, Takayuki; Niibori, Yuichi*; Watanabe, Masayuki; et al.

Introduction to Dismantling and Decommissioning Chemistry, 251 Pages, 2024/09

This book focuses on the dismantling and decommissioning of nuclear facilities and reactors that have suffered severe accidents. In Part 1, we introduce basic aspects ranging from fuel chemistry, analytical chemistry, radiation chemistry, corrosion, and decontamination chemistry to waste treatment and disposal. Then, Part 2 covers the chemistry involved in the decommissioning of various nuclear facilities, and discusses what chemical approaches are necessary and possible for the decommissioning of TEPCO's Fukushima Dai-ichi Nuclear Power Plants, how decommissioning should be carried out, and what kind of research and development and also human resource development are required for this.

Journal Articles

Missing-mass measurement of the $$^{12}$$C$$(K^-,K^+)$$ reaction at 1.8 GeV/$$c$$ with the Superconducting Kaon spectrometer

Ichikawa, Yudai; Fujita, Manami; Hasegawa, Shoichi; Imai, Kenichi*; Nanamura, Takuya; Naruki, Megumi; Sato, Susumu; Sako, Hiroyuki; Tamura, Hirokazu; Tanida, Kiyoshi; et al.

Progress of Theoretical and Experimental Physics (Internet), 2024(9), p.091D01_1 - 091D01_13, 2024/09

 Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)

Journal Articles

Current status of high temperature gas-cooled reactor development in Japan

Nagatsuka, Kentaro; Noguchi, Hiroki; Nagasumi, Satoru; Nomoto, Yasunobu; Shimizu, Atsushi; Sato, Hiroyuki; Nishihara, Tetsuo; Sakaba, Nariaki

Nuclear Engineering and Design, 425, p.113338_1 - 113338_11, 2024/08

 Times Cited Count:1 Percentile:75.38(Nuclear Science & Technology)

HTGR has a potential to contribute to decarbonization of hard-to-abate industries by supplying a large amount of hydrogen and high temperature heat or steam without carbon dioxide emission. JAEA has been conducting R&Ds for HTGR technologies with High Temperature Engineering Test Reactor (HTTR). This paper shows that HTTR's tests including the loss of core cooing test as a joint the OECD/NEA international research project and a HTTR heat application test plan which demonstrate hydrogen production by coupling the HTTR with a hydrogen production test facility. Additionally, aiming for operation start from the latter half of 2030s, the basic design of the HTGR demonstration reactor has been shown. The Japan's HTGR technology capabilities established by the HTTR project will be fully utilized for the construction of HTGR demonstration reactor.

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-2 and JRR-3 and Stored at the Waste Storage Facility L as compressed packages

Kinase, Akari; Goto, Katsunori*; Aono, Ryuji; Konda, Miki; Sato, Yoshiyuki; Haraga, Tomoko; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2024-004, 60 Pages, 2024/07

JAEA-Data-Code-2024-004.pdf:2.05MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed the samples generated from JRR-2 and JRR-3 and stored at the waste storage facility L. In this report, we summarized the radioactivity concentrations of 20 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{99}$$Tc, $$^{108m}$$Ag, $$^{129}$$I, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal year 2022.

Journal Articles

Investigation of chemical state of uranium included in simulated waste glass

Katsuoka, Nanako; Akiyama, Daisuke*; Kirishima, Akira*; Nagai, Takayuki; Okamoto, Yoshihiro; Sato, Nobuaki*

2023-Nendo "Busshitsu, Debaisu Ryoiki Kyodo Kenkyu Kyoten" Kenkyu Seika, Katsudo Hokokusho (Internet), 1 Pages, 2024/07

no abstracts in English

Journal Articles

Detailed visualization of radioactive hotspots inside the Unit 1 reactor building of the Fukushima Daiichi Nuclear Power Station using an integrated Radiation Imaging System mounted on a Mecanum wheel robot

Sato, Yuki; Terasaka, Yuta; Oura, Masatoshi*

Journal of Nuclear Science and Technology, 61(7), p.856 - 870, 2024/07

 Times Cited Count:4 Percentile:82.11(Nuclear Science & Technology)

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