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Terasaka, Yuta; Sato, Yuki; Uritani, Akira*
Nuclear Instruments and Methods in Physics Research A, 1062, p.169227_1 - 169227_6, 2024/05
Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Koike, Yuko; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; Nagai, Shinji; et al.
JAEA-Review 2023-046, 164 Pages, 2024/03
JAEA-Review-2023-046.pdf:4.2MB
The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2022 to March 2023 and the results of dose calculations for the surrounding public due to the release of radioactive materials into the atmosphere and ocean. In the results of the above environmental radiation monitoring, many items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.
C ions based on first-principles calculationsSekikawa, Takuya; Matsuya, Yusuke; Hwang, B.*; Ishizaka, Masato*; Kawai, Hiroyuki*; Ono, Yoshiaki*; Sato, Tatsuhiko; Kai, Takeshi
Nuclear Instruments and Methods in Physics Research B, 548, p.165231_1 - 165231_6, 2024/03
Times Cited Count：0 Percentile：0.44(Instruments & Instrumentation)One of the main causes of radiation effects on the human body is thought to be damage to DNA, which carries genetic information. However, it is not fully understood what kind of molecular structural changes DNA undergoes upon radiation damage. Since it has been reported that various types of DNA damage are formed when DNA is irradiated, our group has investigated the relationship between DNA damage and various patterns of radiation-induced ionization induced by radiation. Although we have so far analyzed DNA damage in a simple system using a rigid body model of DNA, more detailed calculations are required to analyze the molecular structural changes in DNA, which are considered to be important in considering the effects on the human body. In this study, we attempted to clarify the molecular conformational changes of DNA using OpenMX, a first-principles calculation software that can discuss electronic states based on molecular structures. Specifically, we calculated the most stable structure, band dispersion, and wave function of DNA under the assumption that one and two electrons are ionized by various radiation. In the presentation, we will discuss the relationship between the energy dependence of each incident radiation type and the molecular conformational change of DNA. In addition, the radiation-induced changes in the basic physical properties of DNA (corresponding to the initial stage of DNA damage) will be discussed from the viewpoints of both radiation physics and solid state physics.
Morishita, Yuki; Miyamura, Hiroko; Sato, Yuki; Oura, Masatoshi*
Radiation Measurements, 171, p.107064_1 - 107064_7, 2024/02
Times Cited Count：0The detection of alpha and beta contamination locations is important for decontaminating nuclear facilities. In the high radiation dose rate environment at the decommissioning sites, the contamination measurement by the workers is not effective. Thus, we developed a remote automatic contamination measurement system using a new scintillator-based detector. A 50 mm
100-
m-thick YAlO
(Ce)(YAP:Ce) scintillator was coupled with a flat panel-type multianode photomultiplier tube. The detector was installed downwards at the bottom of a robot. It has an energy measurement capability, and the energy measurement could discriminate the alpha particles from the beta and 
Rn alpha particles. With the energy information, alpha and beta particles could be identified and mapped simultaneously. In addition, a slow-moving robot could be used to obtain statistically sufficient counts in a single run measurement, allowing the evaluation of surface contamination density using only alpha particles. The remote automatic contamination measurement system will be useful in visualizing the contamination distribution in environments that are inaccessible to workers.
Re in the keV energy regionKatabuchi, Tatsuya*; Sato, Yaoki*; Takebe, Karin*; Igashira, Masayuki*; Umezawa, Seigo*; Fujioka, Ryo*; Saito, Tatsuhiro*; Iwamoto, Nobuyuki
Journal of Nuclear Science and Technology, 6 Pages, 2024/00
Times Cited Count：0 Percentile：0.18(Nuclear Science & Technology)
CMohamad, A. B.; Nemoto, Yoshiyuki; Furumoto, Kenichiro*; Okada, Yuji*; Sato, Daiki*
Corrosion Science, 224, p.111540_1 - 111540_15, 2023/11
Times Cited Count：0 Percentile：0(Materials Science, Multidisciplinary)Sato, Nobuaki*; Kirishima, Akira*; Sasaki, Takayuki*; Takano, Masahide; Kumagai, Yuta; Sato, Soichi; Tanaka, Kosuke
Current Location of Fuel Debris Chemistry, 178 Pages, 2023/11
Considerable efforts have been devoted to the decommissioning of the TEPCO's Fukushima Daiichi Nuclear Power Station (1F) and now the retrieval of fuel debris is being proceeded on a trial basis. It can be said that the succession of science and technology related to debris, that is, human resource development, is important and indispensable. For that reason, we thought that a specific textbook on decommissioning is necessary. Regarding the 1F fuel debris, we still do not know enough, and it would be difficult to describe the details. However, 12 years have passed since the accident, and we have come to understand the situation of 1F to a certain extent. At this stage, it is essential for future development to organize the current situation by combining examples of past severe accidents. Therefore, we presented in this book the current state of fuel debris chemistry research from the perspectives of solid chemistry, solution chemistry, analytical chemistry, radiochemistry, and radiation chemistry.
states in the electronic structure of the intermediate-valence superconductor CeIr
Fujimori, Shinichi; Kawasaki, Ikuto; Takeda, Yukiharu; Yamagami, Hiroshi; Sasabe, Norimasa*; Sato, Yoshiki*; Shimizu, Yusei*; Nakamura, Ai*; Maruya, A.*; Homma, Yoshiya*; et al.
Electronic Structure (Internet), 5(4), p.045009_1 - 045009_7, 2023/11
beam at J-PARC RCSSaha, P. K.; Harada, Hiroyuki; Yoneda, Hitoki*; Michine, Yurina*; Sato, Atsushi*; Shibata, Takanori*; Kinsho, Michikazu
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.59 - 63, 2023/11
Yoshimura, Nobuyuki*; Toyama, Takeshi*; Shobuda, Yoshihiro; Nakamura, Takeshi*; Omi, Kazuhito*; Kobayashi, Aine*; Okada, Masashi*; Sato, Yoichi*; Nakaya, Tsuyoshi*
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.260 - 264, 2023/11
The J-PARC main ring (MR) will be increased to 1.3 MW. To cope with the increase in beam intensity, the intra-bunch feedback system (IBFB) needs to be upgraded to handle higher frequencies up to about 200 MHz. To evaluate the performance and understand the optimal parameters after this upgrade, we are developing a particle tracking simulation that includes the necessary components. The recoherence period induced by chromaticity between tracking simulations and experiments are compared and it cannot be discribed by the simple simulations, and we investigate what mechanisms explain this result. The shift of synchrotron tune caused by longitudinal wakes using tracking simulations are calculated and it find that introducing the effect of longitudinal wakes only does not explain the recoherence period in the experimental results.
Nagayama, Shota; Harada, Hiroyuki; Shimogawa, Tetsushi*; Sato, Atsushi*; Yamada, Ippei; Chimura, Motoki; Kojima, Kunihiro; Yamamoto, Kazami; Kinsho, Michikazu
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.526 - 530, 2023/11
We have been developing "Non-destructive electrostatic septum" for a slow extraction. This septum has multiple electrodes placed around the region without the beam hitting and separate the beam by its electric field. To evaluate its electric field, we have built a prototype septum and a test machine, which consists of an electron gun and monitors. This test machine can measure the electric field indirectly by using a narrow electron beam. The experiment results of prototype septum is good agreement with the calculation one. However, this electric field distribution is not enough to separate the beam. A step function-like electric field distribution is ideal for the beam separation with minimal negative effect on the beam. We have studied to improve the electrode configuration to match the beam shape. In this paper, we present the result of the electric field measurements and the septum improvement. Additionally, we describe the future plan of this development.
Oikawa, Kenichi; Sato, Hirotaka*; Watanabe, Kenichi*; Su, Y. H.; Shinohara, Takenao; Kai, Tetsuya; Kiyanagi, Yoshiaki*; Hasemi, Hiroyuki
Journal of Physics; Conference Series, 2605, p.012013_1 - 012013_6, 2023/10
Sato, Takumi; Otobe, Haruyoshi; Morishita, Kazuki; Marufuji, Takato; Ishikawa, Takashi; Fujishima, Tadatsune; Nakano, Tomoyuki
JAEA-Technology 2023-016, 41 Pages, 2023/09
JAEA-Technology-2023-016.pdf:2.74MB
This report summarizes the results of the stabilization treatments of post-experiment nuclear materials in Plutonium Fuel Research Facility (PFRF) from August 2018 to March 2021. Based on the management standards for nuclear materials enacted after the contamination accident that occurred at PFRF on June 6, 2017, the post-experiment nuclear materials containing plutonium (Pu): samples mixed with organic substances that cause an increase in internal pressure due to radiolysis (including X-ray diffraction samples mixed with epoxy resin and plutonium powder which caused contamination accidents), carbides and nitrides samples which is reactive in air, and chloride samples which may cause corrosion of storage containers, were selected as targets of the stabilization. The samples containing organic materials, carbides and nitrides were heated in an air flow at 650 C and 950 C for 2 hours respectively to remove organic materials and convert uranium (U) and Pu into oxides. U and Pu chlorides in LiCl-KCl eutectic melt were reduced and extracted into liquid Cd metal by a reaction with lithium (Li) -cadmium (Cd) alloy and converted to U-Pu-Cd alloy at 500 C or higher. All of the samples were stabilized and stored at PFRF. We hope that the contents of this report will be utilized to consider methods for stabilizing post experiment nuclear materials at other nuclear fuel material usage facilities.
Nagai, Takayuki; Okamoto, Yoshihiro; Yamagishi, Hirona*; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2023-004, 45 Pages, 2023/09
JAEA-Research-2023-004.pdf:6.07MB
The local structure of glass-forming elements and waste elements in borosilicate glasses varies with its chemical composition. In this study, simulated waste glass samples were prepared and the chemical state regarding boron (B), silicon (Si) and waste elements of iron (Fe), cesium (Cs) were estimated by using XAFS measurement in soft X-ray region. To understand the chemical stability of simulated waste glasses, XANES spectra of B K-edge, Fe L, L
-edge, and Cs M
, M
-edge were measured on the glass surface exposed to the leachate. As a result, it was found that the glass surface exposed to the leachate was changed and it was difficult to obtain a clear XANES spectrum. From the B K-edge XANES spectra on glass surfaces exposed to the leachate, an increase in three-coordination of B-O (BO) and a decrease in four-coordination of B-O (BO) were observed compared to the glass surfaces before immersion. The XANES spectra of Fe L, L-edge, and Cs M, M-edge show that as the exposure time in the leachate increases, the Cs present on the glass surface dissolves into the leachate. The XANES spectra of Si K-edge were measured on simulated waste glass surfaces before immersion, and it was confirmed that the change in XANES spectra given by NaO concentration had a larger effect than the waste component concentration.
Yamashita, Susumu; Sato, Takumi; Nagae, Yuji; Kurata, Masaki; Yoshida, Hiroyuki
Journal of Nuclear Science and Technology, 60(9), p.1029 - 1045, 2023/09
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)Konno, Chikara; Ota, Masayuki*; Kwon, Saerom*; Onishi, Seiki*; Yamano, Naoki*; Sato, Satoshi*
Journal of Nuclear Science and Technology, 60(9), p.1046 - 1069, 2023/09
Times Cited Count：4 Percentile：98.08(Nuclear Science & Technology)JENDL-5 was validated from a viewpoint of shielding applications under the Shielding Integral Test Working Group of the JENDL Committee. The following benchmark experiments were selected: JAEA/FNS in-situ experiments, Osaka Univ./OKTAVIAN TOF experiments, ORNL/JASPER sodium experiments, NIST iron experiment and QST/TIARA experiments. These experiments were analyzed with MCNP and nuclear data libraries (JENDL-5, JENDL-4.0 or JENDL-4.0/HE, ENDF/B-VIII.0 and JEFF-3.3). The analysis results demonstrate that JENDL-5 is comparable to or better than JENDL-4.0 or JENDL-4.0/HE, ENDF/B-VIII.0 and JEFF-3.3.
Machida, Masahiko; Yamada, Susumu; Kim, M.; Okumura, Masahiko; Miyamura, Hiroko; Shikaze, Yoshiaki; Sato, Tomoki*; Numata, Yoshiaki*; Tobita, Yasuhiro*; Yamaguchi, Takashi; et al.
RIST News, (69), p.2 - 18, 2023/09
The contamination of radioactive materials leaked from the reactor has resulted in numerous hot spots in the Fukushima Daiichi Nuclear Power Station (1F) building, posing obstacles to its decommissioning. In order to solve this problem, JAEA has conducted research and development of the digital technique for inverse estimation of radiation source distribution and countermeasures against the estimated source in virtual space for two years from 2021 based on the subsidy program "Project of Decommissioning and Contaminated Water Management" performed by the funds from the Ministry of Economy, Trade and Industry. In this article, we introduce the results of the project and the plan of the renewal project started in April 2023. For the former project, we report the derivative method for LASSO method considering the complex structure inside the building and the character of the source and show the result of the inverse estimation using the method in the real reactor building. Moreover, we explain the platform software "3D-ADRES-Indoor" which integrates these achievements. Finally, we introduce the plan of the latter project.
Abe, Shinichiro; Hashimoto, Masanori*; Liao, W.*; Kato, Takashi*; Asai, Hiroaki*; Shimbo, Kenichi*; Matsuyama, Hideya*; Sato, Tatsuhiko; Kobayashi, Kazutoshi*; Watanabe, Yukinobu*
IEEE Transactions on Nuclear Science, 70(8, Part 1), p.1652 - 1657, 2023/08
Times Cited Count：0 Percentile：0.01(Engineering, Electrical & Electronic)Single event upsets (SEUs) caused by neutrons is a reliability problem for microelectronic devices in the terrestrial environment. Acceleration tests using white neutron beam provide realistic soft error rates (SERs), but only a few facilities can provide white neutron beam in the world. If single-source irradiation applicable to diverse neutron source can be utilized for the evaluation of the SER in the terrestrial environment, it contributes to solve the shortage of beam time. In this study, we investigated the feasibility of the SER estimation in the terrestrial environment by any one of these measured data with the SEU cross sections obtained by PHITS simulation. It was found that the SERs estimated by our proposed method are within a factor of 2.7 of that estimated by the Weibull function. We also investigated the effect of simplification which reduce the computational cost in simulation to the SER estimation.
Sato, Yuki; Terasaka, Yuta
Journal of Nuclear Science and Technology, 60(8), p.1013 - 1026, 2023/08
Times Cited Count：5 Percentile：98.92(Nuclear Science & Technology)
OKondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
Times Cited Count：5 Percentile：92.64(Multidisciplinary Sciences)no abstracts in English
