Study of the and shell gap for Ti and V by the first high-precision multireflection time-of-flight mass measurements at BigRIPS-SLOWRI

Iimura, Shun*; Rosenbusch, M.*; Takamine, Aiko*; Tsunoda, Yusuke*; Wada, Michiharu*; Chen, S.*; Hou, D. S.*; Xian, W.*; Ishiyama, Hironobu*; Yan, S.*; et al.

Physical Review Letters, 130(1), p.012501_1 - 012501_6, 2023/01

https://doi.org/10.1103/PhysRevLett.130.012501

First direct mass measurements of nuclides around = 100 with a multireflection time-of-flight mass spectrograph

Ito, Yuta*; Schury, P.*; Wada, Michiharu*; Arai, Fumiya*; Haba, Hiromitsu*; Hirayama, Yoshikazu*; Ishizawa, Satoshi*; Kaji, Daiya*; Kimura, Sota*; Koura, Hiroyuki; et al.

Physical Review Letters, 120(15), p.152501_1 - 152501_6, 2018/04

https://doi.org/10.1103/PhysRevLett.120.152501

Masses of Es, Fm and the transfermium nuclei Md, and No, produced by hot- and cold-fusion reactions, in the vicinity of the deformed neutron shell closure, have been directly measured using a multi-reflection time-of-flight mass spectrograph. The masses of Es and Md were measured for the first time. Using the masses of Md as anchor points for decay chains, the masses of heavier nuclei, up to Bh and Mt, were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter derived from three isotopic masses was updated with the new masses and corroborate the existence of the deformed neutron shell closure for Md and Lr.

First online multireflection time-of-flight mass measurements of isobar chains produced by fusion-evaporation reactions; Toward identification of superheavy elements via mass spectroscopy

Schury, P.*; Wada, Michiharu*; Ito, Yuta*; Kaji, Daiya*; Arai, Fumiya*; MacCormick, M.*; Murray, I.*; Haba, Hiromitsu*; Jeong, S.*; Kimura, Sota*; et al.

Physical Review C, 95(1), p.011305_1 - 011305_6, 2017/01

AA2016-0638.pdf:0.71MB

https://doi.org/10.1103/PhysRevC.95.011305

Using a multireflection time-of-flight mass spectrograph located after a gas cell coupled with the gas-filled recoil ion separator GARIS-II, the masses of several -decaying heavy nuclei were directly and precisely measured. The nuclei were produced via fusion-evaporation reactions and separated from projectilelike and targetlike particles using GARIS-II before being stopped in a helium-filled gas cell. Time-of-flight spectra for three isobar chains, Fr-Rn-At-Po, Fr- Rn-At-Po-Bi, and Fr-Rn-At, were observed. Precision atomic mass values were determined for Fr, Rn, and At. Identifications of Bi, Po, Rn, and At were made with N10 detected ions, representing the next step toward use of mass spectrometry to identify exceedingly low-yield species such as superheavy element ions.

A Multi-reflection time-of-flight mass spectrograph for short-lived and super-heavy nuclei

Schury, P. H.*; Wada, Michiharu*; Ito, Yuta*; Naimi, S.*; Sonoda, Tetsu*; Mita, Koki*; Takamine, Aiko*; Okada, Kunihiro*; Wollnik, H.*; Chon, S.*; et al.

Nuclear Instruments and Methods in Physics Research B, 317(Part B), p.537 - 543, 2013/12

https://doi.org/10.1016/j.nimb.2013.06.025

A multi-reflection time-of-flight (MRTOF) mass spectrograph has been implemented at RIKEN to provide high-precision mass measurements of very short-lived nuclei. Of particular interest are mass measurements of r-process nuclei and trans-uranium nuclei. In such nuclei, the MRTOF can perform on par with or better than traditional Penning trap systems. We demonstrate that the MRTOF-MS is capable of accurately attaining relative mass precision of m/m 10 and describe it's utility with heavy, short-lived nuclei.