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Journal Articles

Rapid analysis of $$^{90}$$Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometry

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.

Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08

 Times Cited Count:0 Percentile:0.02(Chemistry, Analytical)

Rapid analysis of $$^{90}$$Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of $$^{90}$$Sr in small bone and tooth samples derived from terrestrial animals.

Journal Articles

External exposure dose estimation by electron spin resonance technique for wild Japanese macaque captured in Fukushima Prefecture

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.

Radiation Measurements, 134, p.106315_1 - 106315_4, 2020/06

 Times Cited Count:1 Percentile:39.17(Nuclear Science & Technology)

The relationship between the CO$$_{2}$$ radical intensity and the absorbed dose (dose response curve) of tooth enamel of Japanese macaque was observed by electron spin resonance and the detection limit of our system was estimated to be 33.5 mGy, which is comparable to the detection limit for human molar teeth. Using the dose response curve, external exposure dose for seven wild Japanese macaques captured in Fukushima prefecture were examined. The results suggest that the external exposure dose for the wild Japanese macaques were ranged between 45 mGy to 300 mGy.

Journal Articles

Verification on recovery performance of repaired reinforced concrete using neutron beam technology

Sekine, Mariko*; Suzuki, Hiroshi; Kanematsu, Manabu*

Konkurito Kogaku Nenji Rombunshu (DVD-ROM), 40(1), p.1545 - 1550, 2018/07

no abstracts in English

Journal Articles

Deformation analysis of reinforced concrete using neutron imaging technique

Koyama, Taku*; Ueno, Kazuki*; Sekine, Mariko*; Matsumoto, Yoshihiro*; Kai, Tetsuya; Shinohara, Takenao; Iikura, Hiroshi; Suzuki, Hiroshi; Kanematsu, Manabu*

Materials Research Proceedings, Vol.4, p.155 - 160, 2018/05

 Times Cited Count:0 Percentile:0.2

JAEA Reports

Evaluation of irradiation behavior on oxide dispersion strengthened (ODS) steel claddings irradiated in Joyo/CMIR-6

Yano, Yasuhide; Otsuka, Satoshi; Yamashita, Shinichiro; Ogawa, Ryuichiro; Sekine, Manabu; Endo, Toshiaki; Yamagata, Ichiro; Sekio, Yoshihiro; Tanno, Takashi; Uwaba, Tomoyuki; et al.

JAEA-Research 2013-030, 57 Pages, 2013/11

JAEA-Research-2013-030.pdf:48.2MB

It is necessary to develop the fast reactor core materials, which can achieve high-burnup operation improving safety and economical performance. Ferritic steels are expected to be good candidate core materials to achieve this objective because of their excellent void swelling resistance. Therefore, oxide dispersion strengthened (ODS) ferritic steel and 11Cr-ferritic/martensitic steel (PNC-FMS) have been respectively developed for cladding and wrapper tube materials in Japan Atomic Energy Agency. In this study, the effects of fast neutron irradiation on mechanical properties and microstructure of 9Cr-and 12Cr-ODS steel claddings for fast reactor were investigated. Specimens were irradiated in the experimental fast reactor Joyo using the CMIR-6 at temperatures between 420 and 835$$^{circ}$$C to fast neutron doses ranging from 16 to 33 dpa. The post-irradiation ring tensile tests were carried out at irradiation temperatures.

Journal Articles

Effect of fine precipitate on void swelling behavior in heavily-irradiated modified SUS316 stainless steels for fast reactor application

Yamashita, Shinichiro; Sekine, Manabu*; Akasaka, Naoaki

Materia, 47(12), P. 624, 2008/12

no abstracts in English

Journal Articles

Neutron irradiation effects on $$^{11}$$B$$_{4}$$C and recovery by annealing

Donomae, Takako; Tachi, Yoshiaki; Sekine, Manabu*; Morohashi, Yuko; Akasaka, Naoaki; Onose, Shoji

Journal of the Ceramic Society of Japan, 115(1345), p.551 - 555, 2007/09

 Times Cited Count:4 Percentile:30.7(Materials Science, Ceramics)

Use of moderator materials in Fast Breeder Reactor (FBR) is effective for transmutation technology, and $$^{11}$$B$$_{4}$$C is one of the candidates. Up to now, the behavior of $$^{10}$$B$$_{4}$$C as the Control rod material is well known, but that of $$^{11}$$B$$_{4}$$C is hardly investigated. In this paper, the radiation effects of $$^{11}$$B$$_{4}$$C pellets, neutron irradiated in the experimental fast reactor JOYO were studied. From the experimental results, it was observed that no macro-cracks were recognized in the irradiated $$^{11}$$B$$_{4}$$C pellets. But, bubble nucleation was found in grain and along grain boundaries of $$^{11}$$B$$_{4}$$C. And, it was shown that the conductivity of $$^{11}$$B$$_{4}$$C was higher than that of $$^{10}$$B$$_{4}$$C. During the annealing from room temperature to 1400$$^{circ}$$C, three recovery stages were found on thermal conductivity. It was suggested that, the recovery of B$$_{4}$$C was related to the dispersion behavior of helium. Judging from these results, as $$^{11}$$B$$_{4}$$C was mechanically more stable compared with $$^{10}$$B$$_{4}$$C under irradiation, it was shown that $$^{11}$$B$$_{4}$$C had high applicability for a moderator.

Oral presentation

An Estimation of the applicability of $$^{11}$$B$$_{4}$$C for moderator

Donomae, Takako; Tachi, Yoshiaki; Onose, Shoji; Matsumoto, Shinichiro; Ito, Masahiko; Sekine, Manabu*

no journal, , 

no abstracts in English

Oral presentation

Microstructural evolutions of neutron-irradiated 11Cr ferritic and martensitic steels

Yamashita, Shinichiro; Tachi, Yoshiaki; Akasaka, Naoaki; Sekine, Manabu*

no journal, , 

no abstracts in English

Oral presentation

Microstructural change of PNC-FMS under neutron irradiation, 2

Yano, Yasuhide; Yamashita, Shinichiro; Sekine, Manabu*; Yoshitake, Tsunemitsu; Akasaka, Naoaki

no journal, , 

no abstracts in English

Oral presentation

Effect of fine precipitate on swelling behavior of heavily-irradiated PNC316 stainless steel

Yamashita, Shinichiro; Sekine, Manabu*; Tachi, Yoshiaki; Akasaka, Naoaki; Nishinoiri, Kenji; Takahashi, Heishichiro

no journal, , 

no abstracts in English

Oral presentation

Evaluation of deformation behavior of reinforced concrete using neutron beam techniques

Ueno, Kazuki*; Suzuki, Hiroshi; Koyama, Taku*; Sekine, Mariko*; Nishio, Yuhei*; Kanematsu, Manabu*

no journal, , 

no abstracts in English

Oral presentation

Experimental study on stress evaluation of rebar in repaired reinforced concrete by neutron diffraction

Sekine, Mariko*; Suzuki, Hiroshi; Koyama, Taku*; Ueno, Kazuki*; Nishio, Yuhei*; Kanematsu, Manabu*

no journal, , 

no abstracts in English

Oral presentation

External dose estimation of Japanese macaque and Procyon lotor using electron spin resonance spectroscopy

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Ono, Takumi*; Tamaki, Hiroaki*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.

no journal, , 

Releases of the radioactive materials from the Fukushima Daiichi Nuclear Power Plant accident result in an ionization exposure to people and animals, the precise dosimetry is required. To estimate the external dose due to the accident, we utilize electron spin resonance (ESR) spectroscopy which is a powerful tool for the dosimetry of external dose. The detection limit of this technique was 146 mGy, so that we have to improve the detection limit for the precise dosimetry. In this work, we developed a novel enamel-dentine separation technique and improved the detection limit down to 43 mGy, and estimated the external dose for Japanese macaque and Procyon lotor collected in Fukushima prefecture.

Oral presentation

Incorporation record of radionuclides in teeth and otoliths

Koarai, Kazuma; Matsueda, Makoto; Fujiwara, Kenso; Ono, Takumi*; Kino, Yasushi*; Oka, Toshitaka; Okutsu, Kenichi*; Takahashi, Atsushi*; Suzuki, Toshihiko*; Shimizu, Yoshinaka*; et al.

no journal, , 

We have investigated incorporation of $$^{90}$$Sr and $$^{137}$$Cs in teeth of cattle and otoliths of fish. Specific activity of $$^{90}$$Sr in the dentin tissue was higher than that in the enamel tissue. The result shows change of $$^{90}$$Sr incorporation in cattle even within a tooth. Concentrations of stable Sr and Cs were 94 ppm and 3 ppb. Distributions of stable Sr and Cs were uniform in the otolith of fish. If distribution of $$^{90}$$Sr and $$^{137}$$Cs in the otolith was measured, change of $$^{90}$$Sr and $$^{137}$$Cs incorporation into the fish would be found. These findings suggest that distribution patterns of $$^{90}$$Sr and $$^{137}$$Cs in the environment could be estimated from distribution of the radionuclides in the tooth and otolith.

Oral presentation

Sample preparation procedure for the estimation of external exposure dose of wild animals using elecron spin resonance spectroscopy

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Ono, Takumi*; Tamaki, Hiroaki*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

no journal, , 

Release of the radioactive materials from Fukushima Daiichi Nuclear Power Plant accident results in a long-term low dose rate ionization exposure to wild animals. The biological effects of the wild animal do not show a clear correlation with the external dose, which is estimated from the external dose rate of the captured point of the animal, a precise external dose estimation using ESR and tooth enamel is required instead of using the external dose rate. In this work, we attempted to estimate the external dose of wild Japanese macaque and Procyon lotor captured in the high dose rate area.

Oral presentation

External exposure dose of Japanese macaque captured in Fukushima prefecture

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.

no journal, , 

Due to the Fukushima Daiichi Nuclear Power Plant accident, the exposure dose estimation for human is examined by the whole body counter or by the Fukushima Health Management Survey, however, the precise estimated dose cannot obtained by such methods. We applied electron spin resonance (ESR) dosimetry for the external dose estimation using tooth enamel of human/animal. As we reported last year, we improved the detection limit of ESR dosimetry down to 43 mGy. We used this improved ESR dosimetry system and attempted to estimate the external dose of wild Japanese macaque capture in Fukushima prefecture, however, the metal component which may obstruct the ESR measurement was observed, so that we cannot estimate the external dose. In this work, we investigated how to remove such metal components, obtain the clear ESR spectrum, and estimate the external dose.

Oral presentation

Strontium-90 measurement in trace amount of hard tissues for distribution analysis

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Fujiwara, Kenso; Terashima, Motoki; Kino, Yasushi*; Oka, Toshitaka; Okutsu, Kenichi*; Yamashita, Takuma*; et al.

no journal, , 

We demonstrated a method of $$^{90}$$Sr measurement in small pieces of hard tissues with radioactivity measurement or ICP-MS measurement. Interference elements of the measurements were removed by chemical separation. We could determine $$^{90}$$Sr in 0.1 g of hard tissues by radioactivity measurement method and ICP-MS method. Limit of detection of the ICP-MS method was lower than that of the radioactivity measurement. The ICP-MS method is adequate method for distribution analysis of $$^{90}$$Sr in the hard tissues.

Oral presentation

Sample preparation procedure for ESR dosimetry using teeth of wild animal

Oka, Toshitaka; Mitsuyasu, Yusuke*; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Sekine, Tsutomu*; Okutsu, Kenichi*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

no journal, , 

Releases of the radioactive materials from the Fukushima Daiichi Nuclear Power Plant accident result in a low dose exposure to wild animals. The external dose of wild animals is commonly estimated by the external dose rate of the captured point, but the estimated exposure dose has huge uncertainties because the size of the habitat and/or the movement of the wild animals are not included in the estimation. To estimate the external dose precisely, we utilize electron spin resonance (ESR) dosimetry. In this work, we investigated the sample preparation procedure of wild animals. The ESR spectrum of enamel of racoon captured in Namie-town, Fukushima has a broad ESR signal due to metal components. The linear relationship between the Co$$_{2}$$ intensity and the absorbed dose that we can apply ESR dosimetry for racoon teeth. Using this relationship, the external exposure dose was estimated.

Oral presentation

Dose estimation for animals exposed low dose using their teeth

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

no journal, , 

The improvement of the ESR dosimetry is required to apply that for the low-dose exposure of wild animals. We will report our progress of the improvement, and compare the external exposure dose estimated by the ESR dosimetry technique and the calculated result based on the external exposure dose rate of the captured point.

Oral presentation

External exposure dose estimation using ESR dosimetry technique

Oka, Toshitaka; Takahashi, Atsushi*; Mitsuyasu, Yusuke*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Yamashita, Takuma*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

no journal, , 

Electron spin resonance (ESR) dosimetry technique is a powerful tool that has been used in the study of external exposure dose assessment of human by measuring CO$$_{2}$$ radicals of teeth. In this work, we applied this technique for wild monkey and wild racoon captured in Fukushima prefecture, and estimated the external exposure dose.

21 (Records 1-20 displayed on this page)