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Journal Articles

Utilizing nuclear data in delayed gamma-ray spectroscopy inverse Monte Carlo analysis

Rodriguez, D.; Abbas, K.*; Crochemore, J.-M.*; Koizumi, Mitsuo; Nonneman, S.*; Pedersen, B.*; Rossi, F.; Seya, Michio*; Takahashi, Toon

EPJ Web of Conferences, 239, p.17005_1 - 17005_5, 2020/09

Journal Articles

Utilizing PUNITA experiments to evaluate fundamental delayed gamma-ray spectroscopy interrogation requirements for nuclear safeguards

Rodriguez, D.; Koizumi, Mitsuo; Rossi, F.; Seya, Michio; Takahashi, Toon; Bogucarska, T.*; Crochemore, J.-M.*; Pedersen, B.*; Takamine, Jun

Journal of Nuclear Science and Technology, 57(8), p.975 - 988, 2020/08

Journal Articles

Journal Articles

Delayed gamma-ray spectroscopy for nuclear material analysis, 2; Design of a practical system with DD neutron generator

Rossi, F.; Rodriguez, D.; Takahashi, Toon; Seya, Michio; Koizumi, Mitsuo

Proceedings of INMM 60th Annual Meeting (Internet), 7 Pages, 2019/07

Journal Articles

Model design of a compact delayed gamma-ray moderator system using $$^{252}$$Cf for safeguards verification measurements

Rodriguez, D.; Rossi, F.; Takahashi, Toon; Seya, Michio; Koizumi, Mitsuo

Applied Radiation and Isotopes, 148, p.114 - 125, 2019/06

 Times Cited Count:3 Percentile:31.52(Chemistry, Inorganic & Nuclear)

Journal Articles

Delayed gamma-ray spectroscopy, 2; Design study of moderator for a practical system

Rossi, F.; Rodriguez, D.; Takahashi, Toon; Seya, Michio; Koizumi, Mitsuo

Nihon Kaku Busshitsu Kanri Gakkai Dai-39-Kai Nenji Taikai Rombunshu (CD-ROM), 3 Pages, 2018/11

This paper (presentation) reports on the design study for seeking compactness of moderator (and reflector) structure for the Delayed Gamma-ray Spectroscopy Non Destructive Assay system to be applied for verification of fissile isotopic (Pu-239, Pu-241 and U-235) composition ratio in High Radioactive Nuclear Material sample such as dissolved solution of reprocessing facility. We first investigated advantages and disadvantages of using different compact neutron sources as DT and DD neutron generators. This led us to the conclusion of using DD sources to achieve a compact (and practical) NDA system. Based on MCNP simulations, with the use of a DD neutron generator, a preliminary optimization study was performed and will be shown here.

Journal Articles

Delayed gamma-ray spectroscopy, 1; Phase-I summary, Phase-II preview, and continuous solution monitoring

Rodriguez, D.; Rossi, F.; Takahashi, Toon; Seya, Michio; Koizumi, Mitsuo

Nihon Kaku Busshitsu Kanri Gakkai Dai-39-Kai Nenji Taikai Rombunshu (Internet), 2 Pages, 2018/11

Safeguards verification of high-radioactivity nuclear material (HRNM) solution samples is performed by HKED analysis for Pu/U element masses and time-consuming destructive analysis for isotopic compositions. To reduce the composition verification time, we have been collaborating with the EC-JRC to develop Delayed Gamma-ray Spectroscopy (DGS), which utilizes fission product $$gamma$$ rays with $$>$$ 3 MeV energy, above the intense passive background. We present the DGS Phase-I development summary and the Phase-II development plan. Additionally, we report about the $$gamma$$ ray pipe monitoring demonstration we performed at TRP and our process monitoring concept that includes GR pipe monitoring and self-interrogation DGS technique in reprocessing facilities.

Journal Articles

Concepts for and demonstration of gamma-ray process monitoring for reprocessing facilities

Rodriguez, D.; Tanigawa, Masafumi; Seya, Michio; Nakamura, Hironobu

Proceeding IAEA Symposium on International Safeguards; Building Future Safeguards Capabilities (Internet), 6 Pages, 2018/11

Journal Articles

Development of differential die-away technique in an integrated active neutron NDA system for nuclear non-proliferation and nuclear security

Ozu, Akira; Maeda, Makoto; Komeda, Masao; Toh, Yosuke; Koizumi, Mitsuo; Seya, Michio

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 4 Pages, 2018/11

Journal Articles

Delayed gamma-ray spectroscopy inverse Monte Carlo analysis method for nuclear safeguards nondestructive assay applications

Rodriguez, D.; Rossi, F.; Seya, Michio; Koizumi, Mitsuo

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11

Journal Articles

Demonstration of $$gamma$$-ray pipe-monitoring capabilities for real-time process monitoring safeguards applications in reprocessing facilities

Rodriguez, D.; Tanigawa, Masafumi; Nishimura, Kazuaki; Mukai, Yasunobu; Nakamura, Hironobu; Kurita, Tsutomu; Takamine, Jun; Suzuki, Satoshi*; Sekine, Megumi; Rossi, F.; et al.

Journal of Nuclear Science and Technology, 55(7), p.792 - 804, 2018/07

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Nuclear material in reprocessing facilities is safeguarded by random sample verification with additional continuous monitoring applied to solution masses and volume in important tanks to maintain continuity-of-knowledge of process operation. Measuring the unique $$gamma$$ rays of each solution as the material flows through pipes connecting all tanks and process apparatuses could potentially improve process monitoring by verifying the compositions in real time. We tested this $$gamma$$ ray pipe-monitoring method using plutonium-nitrate solution transferred between tanks at the PCDF-TRP. The $$gamma$$ rays were measured using a lanthanum-bromide detector with a list-mode data acquisition system to obtain both time and energy of $$gamma$$-ray. The analysis and results of this measurement demonstrate an ability to determine isotopic composition, process timing, flow rate, and volume of solution flowing through pipes, introducing a viable capability for process monitoring safeguards verification.

Journal Articles

Development of detection and measurement technologies for Nuclear Non-proliferation and Security at JAEA

Koizumi, Mitsuo; Seya, Michio; Tomikawa, Hirofumi; Hori, Masato; Naoi, Yosuke

Proceedings of INMM 59th Annual Meeting (Internet), 8 Pages, 2018/07

no abstracts in English

Journal Articles

Development of delayed gamma-ray spectroscopy for nuclear material analysis

Rodriguez, D.; Rossi, F.; Takahashi, Toon; Seya, Michio; Koizumi, Mitsuo; Crochemore, J. M.*; Varasano, G.*; Bogucarska, T.*; Abbas, K.*; Pedersen, B.*

Proceedings of INMM 59th Annual Meeting (Internet), 7 Pages, 2018/07

Journal Articles

Delayed $$gamma$$-ray spectroscopy combined with active neutron interrogation for nuclear security and safeguards

Koizumi, Mitsuo; Rossi, F.; Rodriguez, D.; Takamine, Jun; Seya, Michio; Bogucarska, T.*; Crochemore, J.-M.*; Varasano, G.*; Abbas, K.*; Pedersen, B.*; et al.

EPJ Web of Conferences, 146, p.09018_1 - 09018_4, 2017/09

 Times Cited Count:2 Percentile:9.6

Journal Articles

Delayed gamma-ray spectroscopy, 1; Development and current status

Rodriguez, D.; Rossi, F.; Takamine, Jun; Koizumi, Mitsuo; Seya, Michio; Crochemore, J. M.*; Varasano, G.*; Bogucarska, T.*; Abbas, K.*; Pedersen, B.*

Proceedings of INMM 58th Annual Meeting (Internet), 6 Pages, 2017/07

The JAEA is collaborating with the EC-JRC to develop a NDA system combining four active techniques to improve safeguards verification. Delayed gamma-ray spectroscopy can determine nuclide ratios by correlating observed fission products' time-dependent, high-energy, $$gamma$$ rays to the sample's complex fission yield. To quantify fissile nuclides of significant interest, the fast neutrons from compact, transportable sources must be thermalized to where the fissile nuclides have large cross-sections while maintaining high fluxes to provide significant signals. Experiments are underway at some facilities to improve DGS, including the PUNITA system at JRC-Ispra. These neutron fluxes and measurement conditions are used to develop a Monte Carlo that will be used to analyze the DGS data by an inverse-MC method. The DGS program described here summarizes the 3-year development to optimize the moderator, perform experiments, and create the IMC in preparation for a demonstration of the technique.

Journal Articles

Delayed gamma-ray spectroscopy, 2; Experimental studies for determination of fissile materials ratios

Rossi, F.; Koizumi, Mitsuo; Rodriguez, D.; Takamine, Jun; Seya, Michio; Pedersen, B.*; Crochemore, J. M.*; Abbas, K.*; Bogucarska, T.*; Varasano, G.*

Proceedings of INMM 58th Annual Meeting (Internet), 7 Pages, 2017/07

In the field of nuclear safeguards, new and improved active-interrogation NDA technologies are needed for the independent verification of the fissile composition in HRNM. JAEA and the JRC are now collaborating to develop DGS to determine ratios of fissile nuclides present in the sample measuring the decay gamma rays from FP. Measurements of LRNM samples are underway using different facilities. To minimize the interference from the LLFP, it is important to use shielding and to consider those gamma rays above 3-MeV. Different compact neutron sources are available, but all of them need to be slowed down to the thermal energy region. We are optimizing moderator and reflector materials using MCNP. Optimization of the irradiation, transfer and measurement sequence is now underway. The experiments we are conducting using certified mono-elemental U/Pu samples allow us to associate observed DG to the proportional isotopic compositions. In this paper we will present the current status of the optimization process and the experimental campaign for the determination of the ratio of fissile materials of U and Pu in a sample.

Journal Articles

$$gamma$$-ray pipe monitoring for comprehensive safeguards process monitoring of reprocessing facilities

Rodriguez, D.; Tanigawa, Masafumi; Mukai, Yasunobu; Isomae, Hidemi; Nakamura, Hironobu; Rossi, F.; Koizumi, Mitsuo; Seya, Michio

Proceedings of INMM 58th Annual Meeting (Internet), 9 Pages, 2017/07

Safegaurding nuclear material at reprocessing facilities utilizes sampling to verify the quantity and process monitoring to maintain continuity-of-knowledge to reduce re-verification. Solution Monitoring and Measurement Systems that determine the solution density and volume are installed at solution tanks, though this only provides indirect verification. To offset this safeguards limitation we propose measuring $$gamma$$ rays from solutions passing through the pipes and at the tanks to provide improved continuous monitoring and direct verification. This can provide both real-time flow measurements and Pu isotopic composition quantification through passive nondestructive assay. This concept was tested by recent experimental studies performed at the Japan Atomic Energy Agency's Plutonium Conversion Development Facility of flowing Pu-nitrate $$gamma$$ rays. This presentation will describe the concept details and analysis of using $$gamma$$ ray pipe monitoring as a capability for real-time safeguards verification.

Journal Articles

A Proposal of secure non-destructive detection system of nuclear materials in heavily shielded objects and interior investigation system

Seya, Michio; Hajima, Ryoichi*; Kureta, Masatoshi

Proceedings of INMM 58th Annual Meeting (Internet), 10 Pages, 2017/07

Large size freight cargo containers are the most vulnerable items from nuclear security points of view because of their large volume and weight of cargo inside for hiding heavily shielded objects. For strengthening nuclear security, secure detection of NMs in heavily shielded objects, and safe handling (dismantlement) of detected (suspicious) objects, are essential. These require secure detection of NMs, inspection of detailed interior structures of detected objects, rough characterization of NMs (for nuclear bomb or RDD etc.) and confirmation of existence of explosives etc. By using information obtained by these inspections, safe dismantlement of objects is possible. In this paper, we propose a combination of X-ray scanning system with NRF-based NDD system using monochromatic $$gamma$$-ray beam for a secure detection and interior inspections. We also we propose active neutron NDA system using a DT source for interior inspection of NM part.

Journal Articles

Development of active neutron NDA techniques for nonproliferation and nuclear security, 6; Experimental studies for analyzing nuclear materials by High-Energy Delayed Gamma-ray Spectroscopy (HE-DGS)

Rossi, F.; Koizumi, Mitsuo; Rodriguez, D.; Takamine, Jun; Seya, Michio

Dai-37-Kai Kaku Busshitsu Kanri Gakkai Nippon Shibu Nenji Taikai Rombunshu (CD-ROM), 8 Pages, 2017/02

Journal Articles

Necessity (proposal) of secure detection system of nuclear materials and interior inspection systems of detected / suspicious objects in non-destructive manner for safe dismantling

Seya, Michio; Hajima, Ryoichi*; Kureta, Masatoshi

Dai-37-Kai Kaku Busshitsu Kanri Gakkai Nippon Shibu Nenji Taikai Rombunshu (CD-ROM), 10 Pages, 2017/02

Large size freight cargo containers are the most volunurable items from nuclear security points of view because of their large volume and weight of cargo inside for hiding heavily shielded objects. For strengthning nuclear security, secure detection of NMs in heavily shielded objects, and safe handling (dismatlement) of detected / suspicious objects for taking out of NMs, are essential. These require the following things, (1) Introduction of secure detection system of NMs, (2) Inspection of deteiled and interior structures of detected objects, (3) Rough chracterization of NMs (for nuclear bomb or RDD etc.) / Confirmation of existence of explosives etc.. By using information obtained by interior inspections, safe dismantlement of objects and taking NMs out are possible. In this papaer, we propose a combined system of X-ray scanning system with NRF-based NDD system using monochromatic $$gamma$$-ray beam not only as a secure detection system of NMs but also interior inspection system (covering (1) and (2)). Also we propose active neutron NDA system using a D-T source for interior inspection of NM part (covering (3)).

176 (Records 1-20 displayed on this page)