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Dei, Shuntaro; Shibata, Masahito*; Negishi, Kumi*; Sugiura, Yuki; Amano, Yuki; Bateman, K.*; Wilson, J.*; Yokoyama, Tatsunori; Kagami, Saya; Takeda, Masaki; et al.
Results in Earth Sciences (Internet), 3, p.100097_1 - 100097_16, 2025/12
Interactions between cement and host rock in geological repositories for radioactive waste will result in a chemically disturbed zone, which may potentially affect the long-term safety. This paper investigates the chemical evolution at the interface between cement (Ordinary Portland Cement: OPC and Low Alkaline Cement: LAC) and mudstone after 11 years of in situ reactions at the Horonobe Underground Research Laboratory. The study combines various analytical techniques to identify the key reactions at the cement-rock interface, including cement dissolution, precipitation of secondary minerals such as calcite and C-(A-)S-H phases, cation exchange in montmorillonite and reduced porosity in mudstone. The study also highlights the effects of cement-mudstone interactions on radionuclide migration, such as reduction of diffusivity due to reduced porosity and enhancement of sorption due to incorporation into secondary minerals in the altered mudstone.
-butadiene) reinforced by carbon blackWatanabe, Yuki*; Kumagawa, Daiki*; Karitani, Shu*; Inoue, Tadashi*; Iwabuki, Hitoshi*; Nakanishi, Yohei*; Shibata, Motoki*; Motokawa, Ryuhei; Sugita, Tsuyoshi; Ueda, Yuki; et al.
Macromolecules, 58(16), p.8641 - 8648, 2025/08
Times Cited Count：0 Percentile：0.00Nagai, Takayuki; Okamoto, Yoshihiro; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2024-014, 54 Pages, 2025/02
JAEA-Research-2024-014.pdf:7.02MB
XAFS measurements in the soft X-ray region are suitable for evaluating the chemical state of the surface layer of a measurement sample because the X-ray transmittance is low. In this study, the purpose of the study was to confirm the difference between the coagulated surface layer and the inside of the simulated waste glasses by measuring the K-edge of the glass constituent elements boron, oxygen, sodium, and silicon, and the L
edge of the waste component cerium. As a result, the B K-edge XANES spectra showed that the proportion of B-O tetracoordinate sp
structures (BO
) on the surface layer of the coagulated glass samples was higher than that on the cut surface inside the glass samples, which is expected to improve the water resistance of the coagulated surface. On the other hand, the O K-edge XANES spectra suggested that the O abundance in the coagulated surface layer was lower than that in the cut surface inside the glass samples, and that alkali metal elements may be concentrated in the coagulated surface layer. However, no difference was observed in the Na K-edge XANES spectra between the coagulated surface layer and the cut surface, and no difference was observed in the Si K-edge XANES spectra between the solidified surface and the inside of glass samples. In addition, the Ce L-edge XANES spectra confirmed that the Ce valence in the surface layer of coagulated glass samples were oxidized compared to the inside of glass samples.
Shinto, Katsuhiro; Okoshi, Kiyonori; Shibata, Takanori*; Nammo, Kesao*; Kawai, Isao*; Ikegami, Kiyoshi*; Ueno, Akira
Proceedings of 21st Annual Meeting of Particle Accelerator Society of Japan (Internet), p.525 - 528, 2024/10
A decade has elapsed since the radio frequency (RF)-driven negative hydrogen (H
) ion source initiated operation at J-PARC. In the 2023/2024 campaign, a single RF-driven H ion source has generated H beams with a beam current of 60 mA, which enabled the J-PARC linac to inject them into the 3 GeV rapid cycling synchrotron (RCS) with a beam current of 50 mA. The continuous operation time of the ion source reached exceeding 4,900 hours in this campaign, which signifies a notable enhancement in operational longevity in comparison to the preceding longest campaign in 2022/2023, which spanned 4,412 hours. This paper provides the operational status of the RF-driven H ion source during this campaign and the current status of the J-PARC-made antenna, which is currently under development.
Takeda, Takeshi; Shibata, Taiju
JAEA-Review 2024-040, 29 Pages, 2024/09
JAEA-Review-2024-040.pdf:1.33MB
An important theme of Japan's 6th strategic energy plan is to indicate the energy policy path towards carbon neutrality by 2050. Policy responses for Japan's nuclear energy research and development (R&D) towards 2030 contain the demonstrations of technologies for small modular reactors (SMRs) through international cooperation by 2030. In light of this energy plan, basic policy initiatives over the next 10 years have been compiled to realize Green Transformation (GX), which simultaneously achieves decarbonization and economic growth. Looking overseas, activities of SMR R&D are active internationally, mainly in the US, Canada, Europe, China, and Russia. These activities are not only by heavy industry manufactures and R&D institutes, but also by venture companies. Under these circumstances, the NEA CSNI has gathered an Expert Group on SMRs (EGSMR) to help estimate the safety effects of SMRs. The EGSMR efforts required the submission of responses to several questionnaires whose main purpose was to collect the latest information on the efforts of SMR deployment and research. The first author of this report responded to this based on information from Hitachi-GE Nuclear Energy, Ltd. and Mitsubishi Heavy Industries, Ltd. as well as JAEA. Most of the responses from Japan to the questionnaires are the information that serves as the basis of CSNI Technical Opinion Paper No. 21 (TOP-21). In this report, the Japan's publicly available responses to the questionnaires arranged and additional information are explained, which complements some of the content of the TOP-21. In this manner, the investigation results of R&D related to SMR in Japan, focusing on the EGSMR activities (2022-2023), are summarized. The target of this report is to provide useful information for future discussions on international cooperation concerning SMR as well as nuclear power field human resources development internationally and domestically.
Tamura, Koji; Nakanishi, Ryuzo; Oba, Hironori; Karino, Takahiro; Shibata, Takuya; Taira, Takunori*; Wakaida, Ikuo
Journal of Nuclear Science and Technology, 61(8), p.1109 - 1116, 2024/08
Times Cited Count：1 Percentile：18.87(Nuclear Science & Technology)Shibata, Hiroki; Saito, Hiroaki; Hayashi, Hirokazu; Takano, Masahide
Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 23(3), p.74 - 80, 2024/08
Partitioning and transmutation of minor actinides techniques have been developed to reduce the radiotoxicity and volume in the high-level radioactive wastes. Minor actinide nitride fuel has been chosen as a candidate for transmutation of long-lived nuclides by accelerator-driven system. Understanding irradiation behavior of nitride fuel is important for its design and development, however, experimental data on irradiation tests of actinide nitrides and these solid solutions are scarce. Recently, in JAEA, nitride fuel performance analysis module based on light water reactor fuel performance code, FEMAXI-7, has been developed to simulate irradiation behavior of the nitride fuel. In this study, performance analysis was carried out focusing on the pellet-cladding mechanical interaction (PCMI), which was pointed out as the most effective factor for the fuel safety during irradiation. Simulation results show that PCMI does not cause the creep rupture of the cladding.
ion sourceShibata, Takanori*; Okoshi, Kiyonori; Ueno, Akira; Ikegami, Kiyoshi*; Shinto, Katsuhiro; Nammo, Kesao*; Kawai, Isao*; Oguri, Hidetomo
Kasokuki, 21(2), p.94 - 100, 2024/07
In the recent J-PARC user operation from Nov. 10th, 2022 to Jun. 22nd, 2023, continuous operation of 4,412 hours with hydrogen negative ion (H ion) beam current up to 60 mA was achieved by J-PARC radio frequency (RF) H ion source. This was also the first time to supply H ion beam to the linac in the yearly J-PARC user operation term by a single ion source (w/o ion source exchange). To satisfy the requirements of the further upgrade in J-PARC, a soundness evaluation of the present ion source components has been performed. Furthermore, the RF ion source with a newly manufactured RF antenna coil has been under development.
Shibata, Takanori*; Shinto, Katsuhiro; Nakano, Haruhisa*; Hoshino, Kazuo*; Miyamoto, Kenji*; Okoshi, Kiyonori; Nammo, Kesao*; Ikegami, Kiyoshi*; Kawai, Isao*; Oguri, Hidetomo; et al.
Journal of Physics; Conference Series, 2743, p.012007_1 - 012007_5, 2024/05
Times Cited Count：0 Percentile：0.00(Physics, Particles & Fields)Oscillation of the negative hydrogen ion (H) beam phase space in Radio Frequency (RF) ion source is investigated by a simple 3D Particle-In-Cell (PIC) model which takes into account the transport processes of electron, proton and H in the extraction region. The calculation domain is in vicinity of the single beam aperture in J-PARC ion source configuration. In order to understand relation between the plasma density oscillation and the extracted H beam characteristics, the input electron and proton fluxes from the driver region are varied parametrically with the 1st and the 2nd harmonics of the J-PARC RF frequency (2 or 4 MHz). The numerical results give an idea to the main physical processes between the oscillations of the plasma parameters and the extracted H ion trajectories in the different RF phases. Countermeasures to reduce the oscillation mechanisms are also discussed in the presentation.
ion sourceShinto, Katsuhiro; Shibata, Takanori*; Okoshi, Kiyonori; Nammo, Kesao*; Kawai, Isao*; Ikegami, Kiyoshi*
Journal of Physics; Conference Series, 2743, p.012023_1 - 012023_5, 2024/05
Times Cited Count：0 Percentile：0.00(Physics, Particles & Fields)We have been conducting the test of a new J-PARC-made internal antenna for the J-PARC RF-driven cesiated H ion source. After the development of the first J-PARC-made antenna, the composition of the porcelain enamel coating of the antenna was changed because we were afraid of the outgassing of the impurities from the previous antenna coating. During the test of high-density plasma production by the new antenna, we monitored the outgassing characteristics of the new antenna by measuring mass spectrometry and optical spectrum analysis. It is confirmed that no remarkable impurities were emitted from the new antenna. We also carried out the H beam extraction and measured the H beam characteristics by using the new antenna. It is found that the emittances of the H beam extracted from the J-PARC RF-driven cesiated H ion source by using the new antenna were similar to those in the case by using the SNS-made antenna. To accelerate the endurance test of the new antenna, we applied the antenna for the high-density plasma production to the 5% duty factor (1 ms pulse width with 50 Hz repetition rate) with the 2 MHz RF input power of approximately 60 kW, whose values were much higher than those in the J-PARC nominal operation; 0.8 ms pulse width with 25 Hz repetition rate (the duty factor of 2%) with the RF input power of approximately 30 kW. This presentation shows the results of the characteristics of the new J-PARC-made antenna and discusses the feasibility of the new antenna for use in the J-PARC accelerator operation.
Fukaya, Yuji; Goto, Minoru; Shibata, Taiju
IAEA-TECDOC-2040, p.133 - 136, 2023/12
Japan has developed back-end technologies to establish a multi-recycling fuel cycle with fast breeder reactors (FBRs) to ensure energy resources. Even though the development of FBR has been retreated to one of fundamental research, the reprocessing technologies for uranium fuel and disposal technologies had been completed for Light Water Reactor (LWR) fuel cycle on the process. These technologies were inherited to utilities and are about to be practical. Now, Japan had been completed High Temperature Engineering Test Reactor (HTTR) a prototype and research reactor, a commercial High Temperature Gas-cooled Reactor (HTGR) design Gas Turbine High Temperature Reactor 300 (GTHTR300) with related reprocessing technologies, and is planning domestic demonstration reactor project. In this context, a representative fuel cycle policy is reprocessing in Japan. However, Japan has investigated various fuel cycle scenarios to expand the usage of the commercial HTGR. Then, we would like to introduce the scenarios and development status of related technologies in the present study.
Shibata, Ryodai; Amano, Tsukasa; Yamada, Hiroyuki; Miyaji, Noriko; Nakamura, Hironobu
Dai-44-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2023/11
In April 2020, JAEA has been introduced Physical Protection Corrective Action Program (PPCAP) with full-scale. It was needed to introduce unified operation for six sites with different business scales, and headquarters developed the common guideline. There was an impression that physical protection activities were carried out by a limited number of employees. Therefore, a problem was to root and activate PPCAP activities among all employees in order to make them effective. Five activities were implemented to solve this problem. As a result, more than 3,700 condition reports (CR) have been collected for 4 years. This paper reports on the activities related to the PPCAP that have been implemented at JAEA.
Koyama, Shinichi; Ikeuchi, Hirotomo; Mitsugi, Takeshi; Maeda, Koji; Sasaki, Shinji; Onishi, Takashi; Tsai, T.-H.; Takano, Masahide; Fukaya, Hiroyuki; Nakamura, Satoshi; et al.
Hairo, Osensui, Shorisui Taisaku Jigyo Jimukyoku Homu Peji (Internet), 216 Pages, 2023/11
In FY 2021 and 2022, JAEA perfomed the subsidy program for "the Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris (Development of Technologies for Enhanced Analysis Accuracy, Thermal Bahavior Estimation, and Simplified Analysis of Fuel Debris)" started in FY 2021. This presentation material summarized the results of the project, which will be available shortly on the website of Management Office for the Project of Decommissioning, Contaminated Water and Treated Water Management.
Shinto, Katsuhiro; Okoshi, Kiyonori; Shibata, Takanori*; Nammo, Kesao*; Kawai, Isao*; Ikegami, Kiyoshi*; Ueno, Akira
Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.928 - 931, 2023/11
J-PARC initiated the operation of the high-intensity rf-driven negative hydrogen (H) ion source in 2014 autumn. The ion source produces the H beam with the beam current of 60 mA and the beam energy of 50 keV in order to inject the H beam into the 3 GeV RCS with the beam current of 50 mA and the beam energy of 400 MeV from the J-PARC linac. We have achieved the longest continuous operation time of 4001 hours in the previous (2021/2022) campaign. The 2022/2023 campaign was the first time that the continuous operation of the H ion source without any exchanges of the ion source until the end of the campaign was examined. We present the operation status of the J-PARC H ion source in this campaign as well as the status of the J-PARC-made internal antenna test.
Kamide, Hideki; Kawasaki, Nobuchika; Hayafune, Hiroki; Kubo, Shigenobu; Chikazawa, Yoshitaka; Maeda, Seiichiro; Sagayama, Yutaka; Nishihara, Tetsuo; Sumita, Junya; Shibata, Taiju; et al.
Jisedai Genshiro Ga Hiraku Atarashii Shijo; NSA/Commentaries, No.28, p.14 - 36, 2023/10
Developments of next generation nuclear reactors, e.g., Fast Reactor, and High Temperature Gas cooled Reactor, are in progress. They can contribute to markets of electricity and industrial heat utilization in the world including Japan. Here, current status of reactor developments in Japan and also situation in the world are summarized, especially for activities of Generation IV International Forum (GIF), developments of Fast Reactor and High Temperature Gas cooled Reactor in Japan, and SMR movements in the world.
Nagai, Takayuki; Okamoto, Yoshihiro; Yamagishi, Hirona*; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2023-004, 45 Pages, 2023/09
JAEA-Research-2023-004.pdf:6.07MB
The local structure of glass-forming elements and waste elements in borosilicate glasses varies with its chemical composition. In this study, simulated waste glass samples were prepared and the chemical state regarding boron (B), silicon (Si) and waste elements of iron (Fe), cesium (Cs) were estimated by using XAFS measurement in soft X-ray region. To understand the chemical stability of simulated waste glasses, XANES spectra of B K-edge, Fe L, L
-edge, and Cs M
, M-edge were measured on the glass surface exposed to the leachate. As a result, it was found that the glass surface exposed to the leachate was changed and it was difficult to obtain a clear XANES spectrum. From the B K-edge XANES spectra on glass surfaces exposed to the leachate, an increase in three-coordination of B-O (BO) and a decrease in four-coordination of B-O (BO) were observed compared to the glass surfaces before immersion. The XANES spectra of Fe L, L-edge, and Cs M, M-edge show that as the exposure time in the leachate increases, the Cs present on the glass surface dissolves into the leachate. The XANES spectra of Si K-edge were measured on simulated waste glass surfaces before immersion, and it was confirmed that the change in XANES spectra given by NaO concentration had a larger effect than the waste component concentration.
Mao, W.; Gao, S.*; Gong, W.; Bai, Y.*; Harjo, S.; Park, M.-H.*; Shibata, Akinobu*; Tsuji, Nobuhiro*
Acta Materialia, 256, p.119139_1 - 119139_16, 2023/09
Times Cited Count：42 Percentile：98.37(Materials Science, Multidisciplinary)Transformation-induced plasticity (TRIP)-assisted steels exhibit an excellent combination of strength and ductility due to enhanced strain hardening rate associated with deformation-induced martensitic transformation (DIMT). Quantitative evaluation on the role of DIMT in strain hardening behavior of TRIP-assisted steels and alloys can provide guidance for designing advanced materials with strength and ductility synergy, which is, however, difficult since the phase composition keeps changing and both stress and plastic strain are dynamically partitioned among constituent phases during deformation. In the present study, tensile deformation with 
neutron diffraction measurement was performed on an Fe-24Ni-0.3C (wt.%) TRIP-assisted austenitic steel. The analysis method based on stress partitioning and phase fractions measured by neutron diffraction was proposed, by which the tensile flow stress and the strain hardening rate of the specimen were resolved into factors associated with each phase, i.e., the austenite matrix, deformation-induced martensite, and the transformation rate of DIMT after differentiation, and then the role of each factor in the global strain hardening behavior was discussed. In addition, the plastic strain partitioning between austenite and martensite was indirectly estimated using the dislocation density measured by diffraction profile analysis, which constructed the full picture of stress and strain partitioning between austenite and martensite in the material. The results suggested that both the transformation rate and the phase stress borne by the deformation-induced martensite played important roles in the global tensile properties of the material. The proposed decomposition analysis method could be widely applied to investigating mechanical behavior of multi-phase alloys exhibiting the TRIP phenomenon.
Takahatake, Yoko; Watanabe, So; Arai, Tsuyoshi*; Sato, Takahiro*; Shibata, Atsuhiro
Applied Radiation and Isotopes, 196, p.110783_1 - 110783_5, 2023/06
Times Cited Count：2 Percentile：37.43(Chemistry, Inorganic & Nuclear)
dynamics in the H conductors LaH
O
Tamatsukuri, Hiromu; Fukui, Keiga*; Iimura, Soshi*; Honda, Takashi*; Tada, Tomofumi*; Murakami, Yoichi*; Yamaura, Junichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Yamada, Takeshi*; et al.
Physical Review B, 107(18), p.184114_1 - 184114_8, 2023/05
Times Cited Count：1 Percentile：9.43(Materials Science, Multidisciplinary)Amano, Tsukasa; Shibata, Ryodai; Sato, Yoshiharu; Yamazaki, Katsuyuki; Shiromo, Hideo; Nakamura, Hironobu
Proceedings of INMM & ESARDA Joint Annual Meeting 2023 (Internet), 6 Pages, 2023/05
In Japan, about 10 years have passed since the law obligated nuclear operators to develop and maintain a nuclear security culture. During this period, the global nuclear situation has changed significantly, and it is becoming important to maintain a stance that emphasizes compliance with regulations and nuclear security culture. In JAEA, the policy of legal compliance and developing nuclear security culture is determined by the president of JAEA. For legal compliance and developing nuclear security culture, many activities are carried out based on that policy. Finally, these activities are evaluated and improved it every year. Case study is the one of activities that can obtain skills for legal compliance and developing nuclear security culture, such as sensitivity of nuclear security risks, correct understanding of the laws. The procedure for the case study was created with reference to a method called KY-Training which is often applied to safety training program in Japan. KY-Training is a training that participants (groups) can reach the conclusion how to respond to cases through four questions. Firstly, participants are given illustrations and descriptions which has potential of nuclear security risks. Then, participants make discussion according to four questions. Consequently, participants can effectively become aware of nuclear security risks. In the 2022 case study, we prepared 23 cases so that they can select choose freely according to role of participants such as in charge of nuclear security, guards, general employees. Finally, participants are asked to fill a questionnaire to evaluate effectiveness of case study. The result of questionnaires indicated that the case study was able to lead to improvement sensitivity of nuclear security risks and correct understanding of the laws. Overall, case study results suggested that JAEA's efforts were implying sufficiently to develop and maintain a nuclear security culture.
