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Journal Articles

Spin-nematic interaction in the multiferroic compound Ba$$_{2}$$CoGe$$_{2}$$O$$_{7}$$

Soda, Minoru*; Matsumoto, Masashige*; M$"a$nsson, M.*; Kawamura, Seiko; Nakajima, Kenji; Shiina, Ryosuke*; Masuda, Takatsugu*

Physical Review Letters, 112(12), p.127205_1 - 127205_5, 2014/03

https://doi.org/10.1103/PhysRevLett.112.127205
 Times Cited Count：42 Percentile：84.93(Physics, Multidisciplinary)

We demonstrate the existence of the spin-nematic interactions in an easy-plane type antiferromagnet Ba$$_{2}$$CoGe$$_{2}$$O$$_{7}$$ by exploring the magnetic anisotropy and spin dynamics. The combination of neutron scattering and magnetic susceptibility measurements reveals that the origin of the in-plane anisotropy is an antiferro-type interaction of the spin-nematic operator. The relation between the nematic operator and the electric polarization in the ligand symmetry of this compound is presented. The introduction of the spinnematic interaction is useful to understand the physics of spin and electric dipole in multiferroic compounds.

Journal Articles

Neutron scattering study on the field-induced $$O_{xy}$$-type antiferroquadrupolar ordering of the heavy-fermion superconductor PrOs$$_4$$Sb$$_{12}$$

Kaneko, Koji; Metoki, Naoto; Shiina, Ryosuke*; Matsuda, Tatsuma; Kogi, Masafumi*; Kuwahara, Keitaro*; Bernhoeft, N.*

Physical Review B, 75(9), p.094408_1 - 094408_7, 2007/03

https://doi.org/10.1103/PhysRevB.75.094408
 Times Cited Count：21 Percentile：63.87(Materials Science, Multidisciplinary)

Neutron scattering experiments have revealed a field-induced antiferroquadrupolar order parameter in the Pr-based heavy-fermion superconductor PrOs$$_4$$Sb$$_{12}$$. We observed the field-induced antiferromagnetic dipole moment with the propagation vector $$q$$ = (1 0 0) for the applied field direction both $$H parallel$$ [1 1 0] and [0 0 1]. For $$H parallel$$ [1 1 0] at 8 T, it should be noted that the induced antiferromagnetic moment of 0.16 $$mu_{rm B}$$/ Pr orients parallel to the field within our experimental accuracy. This observation is strong evidence that the $$O_{xy}$$ electric quadrupole to be the primary order parameter for $$H parallel$$ [1 1 0]. A mean-field calculation, based on $$Gamma_1$$ singlet and $${Gamma}_4^{(2)}$$ excited triplet with the $$O_{xy}$$ quadrupolar interaction, reproduces the induced moment direction and its field response. These facts indicate the predominance of $$O_{xy}$$-type antiferroquadrupolar interaction in PrOs$$_4$$Sb$$_{12}$$.

Journal Articles

Field-induced antiferroquadrupolar order in the heavy fermion superconductor PrOs$$_4$$Sb$$_{12}$$

Kaneko, Koji; Metoki, Naoto; Matsuda, Tatsuma; Kuwahara, Keitaro*; Kogi, Masafumi*; Shiina, Ryosuke*; Mignot, J.-M.*; Gukasov, A.*; Bernhoeft, N.*

Physica B; Condensed Matter, 378-380, p.189 - 191, 2006/05

https://doi.org/10.1016/j.physb.2006.01.349
 Times Cited Count：1 Percentile：6.20(Physics, Condensed Matter)

Neutron diffraction experiments under magnetic fields were carried out on the heavy fermion superconductor PrOs$$_4$$Sb$$_{12}$$ in order to reveal the origin of the field-induced ordered phase (FIOP) for $$H$$$$Vert$$[1,1,0]. The application of magnetic field induces the weak superlattice peaks with the ordering vector $$q$$=(1,0,0) in FIOP, which is the same as for $$H{parallel}$$[0,0,1]. The observed superlattice reflections for $$H$$$$Vert$$[1,1,0] result from the antiferromagnetic component of $$J_x$$+$$J_y$$; the induced tiny antiferromagnetic moments orient parallel to the applied field. This result cannot be explained by magnetic interactions and strongly evidences the underlying AFQ order with $$O_{xy}$$ as a primary order parameter. These facts clarify the dominant role of $$O_{xy}$$-type antiferroquadrupolar interaction in PrOs$$_4$$Sb$$_{12}$$.

Oral presentation

Neutron scattering study on field-induced ordered phase and rattling in PrOs$$_4$$Sb$$_{12}$$

Kaneko, Koji; Metoki, Naoto; Kimura, Hiroyuki*; Noda, Yukio*; Matsuda, Tatsuma; Shiina, Ryosuke*; Kuwahara, Keitaro*; Iwasa, Kazuaki*; Kogi, Masafumi*; Bernhoeft, N.*

no journal, , 

no abstracts in English

Oral presentation

Novel field-induced ordered state in heavy-fermion compound YbCo$$_2$$Zn$$_{20}$$

Kaneko, Koji; Raymond, S.*; Ressouche, E.*; Shiina, Ryosuke*; Takeuchi, Tetsuya*; Hirose, Yusuke*; Honda, Fuminori*; Onuki, Yoshichika; Lapertot, G.*

no journal, , 

no abstracts in English

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