Haba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.
Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08
Igarashi, Junya*; Zhang, Z. J.*; Ninomiya, Kazuhiko*; Shinohara, Atsushi*; Satou, Yukihiko; Minowa, Haruka*; Yoshikawa, Hideki
KEK Proceedings 2019-2, p.54 - 59, 2019/11
no abstracts in English
Igarashi, Junya*; Zheng, J.*; Zhang, Z.*; Ninomiya, Kazuhiko*; Satou, Yukihiko; Fukuda, Miho*; Ni, Y.*; Aono, Tatsuo*; Shinohara, Atsushi*
Scientific Reports (Internet), 9(1), p.11807_1 - 11807_10, 2019/08
Radioactive particles were released into the environment during the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. Many studies have been conducted to elucidate the chemical composition of released radioactive particles in order to understand their formation process. However, whether radioactive particles contain nuclear fuel radionuclides remains to be investigated. Here, we report the first determination of Pu isotopes in radioactive particles. To determine the Pu isotopes (Pu, Pu and Pu) in radioactive particles derived from the FDNPP accident which were free from the influence of global fallout, radiochemical analysis and inductively coupled plasma-mass spectrometry measurements were conducted. Radioactive particles derived from unit 1 and unit 2 or 3 were analyzed. For the radioactive particles derived from unit 1, activities of Pu and Pu were (1.70-7.06)10 Bq and (4.10-8.10)10 Bq, respectively and atom ratios of Pu/Pu and Pu/Pu were 0.330-0.415 and 0.162-0.178, respectively. These ratios were consistent with the simulation results from ORIGEN code and measurements from various environmental samples. In contrast, Pu was not detected in the radioactive particles derived from unit 2 or 3. The difference in Pu contents is clear evidence towards different formation processes of radioactive particles, and detailed formation processes can be investigated from Pu analysis.
Zhang, Z.*; Igarashi, Junya*; Satou, Yukihiko; Ninomiya, Kazuhiko*; Sueki, Keisuke*; Shinohara, Atsushi*
Environmental Science & Technology, 53(10), p.5868 - 5876, 2019/05
The Fukushima Daiichi Nuclear Power Plant (FDNPP) accident released abundant radioactive particles into the surrounding environment. Herein, we analyzed the activity of Sr in these particles to estimate the contribution of this radionuclide to the overall radiation exposure and shed light on the processes that occurred during the accident. Seven radioactive particles were isolated from the dust and soil samples collected from areas surrounding the FDNPP, and the minimum/maximum Cs activities were determined as 224/4,100 Bq. Based on the size, specific activity, and Cs/Cs activity ratios, we concluded that six of the seven radioactive particles were released from the Unit 1 reactor, while one particle was released from the Unit 3 reactor by a hydrogen explosion. Strontium-90 was detected in all radioactive particles, and the minimal/maximal Sr activities were determined as 0.046/1.4 Bq. Cs/Sr activity ratios above 1000 were observed for all seven particles, that is, compared to Cs, Sr had negligible contribution to the overall radiation exposure. The Cs/Sr activity ratios of the radioactive particles were similar to those of terrestrial environmental samples and were higher for particles released from the Unit 1 reactor than for samples collected from the Unit 1 reactor building, which indicates possibility of additional Sr -rich contamination after release of the particles.
Shigekawa, Yudai*; Kasamatsu, Yoshitaka*; Yasuda, Yuki*; Kaneko, Masashi; Watanabe, Masayuki; Shinohara, Atsushi*
Physical Review C, 98(1), p.014306_1 - 014306_5, 2018/07
The nuclear half-life of U has been reported to vary depending on the chemical environment. In this study, both the half-life and the internal-conversion (IC) electron energy spectrum were measured for U with identical chemical environments for the first time. U oxide and fluoride samples were subjected to these measurements, and clear differences in the half-life and the energy spectrum between these samples were observed. The peaks in the energy spectra were identified with the relativistic density functional theory calculation, and the molecular orbital states of the U oxide and fluoride estimated from the energy spectra and the calculation qualitatively explained the difference in the half-lives between the samples.
Sakurai, Hiroshi*; Shinohara, Atsushi*; Koura, Hiroyuki; Kamigaito, Osamu*; Morimoto, Koji*; Haba, Hiromitsu*; Enyo, Hideto*
Isotope News, (特別号2), p.2 - 14, 2018/01
no abstracts in English
Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.
Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12
The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.
Seki, Yoshichika; Shinohara, Takenao; Parker, J. D.*; Yashiro, Wataru*; Momose, Atsushi*; Kato, Kosuke*; Kato, Hidemi*; Sadeghilaridjani, M.*; Otake, Yoshie*; Kiyanagi, Yoshiaki*
Journal of the Physical Society of Japan, 86(4), p.044001_1 - 044001_5, 2017/03
For the effective phase imaging at pulsed neutron sources, we have designed and developed the multi-colored Talbot-Lau interferometer which works at several wavelengths. At the Energy Resolved Neutron Imaging System RADEN in J-PARC, we demonstrated its operation by observing the visibilities of moire fringes derived from different wavelengths (0.25, 0.50, and 0.75 nm). We also investigated the variation of moire fringes dependent on the wavelength resolution from 18% to 50% and showed the advantage of pulsed beams. At the central wavelength of 0.5 nm, we have succeeded in interferometric imaging for the samples of metal rods made of aluminum, lead, and copper. An absorption grating as an analyzer was fabricated by imprinting of metallic glass for the first time, and showed a clear moire fringe with the high visibility of 68% and a well-controlled shape in comparison with previous ones fabricated by oblique evaporation of gadolinium.
Seki, Yoshichika; Shinohara, Takenao; Ueno, Wakana; Parker, J. D.*; Samoto, Tetsuo*; Yashiro, Wataru*; Momose, Atsushi*
Physics Procedia, 88, p.217 - 223, 2017/00
Ono, Masato; Shimizu, Atsushi; Kondo, Makoto; Shimazaki, Yosuke; Shinohara, Masanori; Tochio, Daisuke; Iigaki, Kazuhiko; Nakagawa, Shigeaki; Takada, Shoji; Sawa, Kazuhiro
Journal of Nuclear Engineering and Radiation Science, 2(4), p.044502_1 - 044502_4, 2016/10
In the loss of forced core cooling test using High Temperature engineering Test Reactor (HTTR), the forced cooling of reactor core is stopped without inserting control rods into the core and cooling by Vessel Cooling System (VCS) to verify safety evaluation codes to investigate the inherent safety of HTGR be secured by natural phenomena to make it possible to design a severe accident free reactor. The VCS passively removes the retained residual heat and the decay heat from the core via the reactor pressure vessel by natural convection and thermal radiation. In the test, the local temperature was supposed to exceed the limit from the viewpoint of long-term use at the uncovered water cooling tube by thermal reflectors in the VCS, although the safety of reactor is kept. Through a cold test, which was carried out by non-nuclear heat input from gas circulators with stopping water flow in the VCS, the local higher temperature position was specified although the temperature was sufficiently lower than the maximum allowable working temperature, and natural circulation of water had insufficient cooling effect on the temperature of water cooling tube below 1C. Then, a new safe and secured procedure for the loss of forced core cooling test was established, which will be carried out soon after the restart of HTTR.
Ogawa, Kazuma*; Mizuno, Yoshiaki*; Washiyama, Koshin*; Shiba, Kazuhiro*; Takahashi, Naruto*; Kozaka, Takashi*; Watanabe, Shigeki; Shinohara, Atsushi*; Odani, Akira*
Nuclear Medicine and Biology, 42(11), p.875 - 879, 2015/11
Ninomiya, Kazuhiko*; Kubo, Kenya*; Nagatomo, Takashi*; Higemoto, Wataru; Ito, Takashi; Kawamura, Naritoshi*; Strasser, P.*; Shimomura, Koichiro*; Miyake, Yasuhiro*; Suzuki, Takao*; et al.
Analytical Chemistry, 87(9), p.4597 - 4600, 2015/05
Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05
A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived Nb and Ta were produced with nuclear reactions using a F beam whose energy was the same as that to produce Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the Nb and Ta to a chemistry device for Db without changing other experimental conditions.
Takada, Shoji; Shimizu, Atsushi; Kondo, Makoto; Shimazaki, Yosuke; Shinohara, Masanori; Seki, Tomokazu; Tochio, Daisuke; Iigaki, Kazuhiko; Nakagawa, Shigeaki; Sawa, Kazuhiro
Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 5 Pages, 2015/05
In the loss of forced core cooling test using High Temperature engineering Test Reactor (HTTR), the forced cooling of reactor core is stopped without inserting control rods into the core and cooling by Vessel Cooling System (VCS) to demonstrate the inherent safety of HTGR be secured by natural phenomena to make it possible to design a severe accident free reactor. In the test, the local temperature was supposed to exceed the limit from the viewpoint of long-term use at the uncovered water cooling tube by thermal reflectors in the VCS, although the safety of reactor is kept. The local higher temperature position was specified although the temperature was sufficiently lower than the maximum allowable working temperature, and natural circulation of water had insufficient cooling effect on the temperature of water cooling tube below 1C. Then, a new safe and secured procedure for the loss of forced core cooling test was established, which will be carried out soon after the restart of HTTR.
Yashima, Hiroshi*; Sekimoto, Shun*; Ninomiya, Kazuhiko*; Kasamatsu, Yoshitaka*; Shima, Tatsushi*; Takahashi, Naruto*; Shinohara, Atsushi*; Matsumura, Hiroshi*; Satoh, Daiki; Iwamoto, Yosuke; et al.
Radiation Protection Dosimetry, 161(1-4), p.139 - 143, 2014/10
The neutron activation cross sections up to GeV are important for the neutron dosimetry of the radiation field in high-energy and high-intensity accelerator facilities for a project of intense spallation neutron source. But the evaluation of neutron activation cross section data is not enough above 20 MeV because experimental data are still scarce. This study aimed to measure the neutron activation cross sections of Bi and Co by using a quasi-monoenergetic neutron field. In this symposium, we will present obtained experimental cross section data with the other experimental data (neutron-induced and proton-induced), the calculated data by PHITS code and the evaluated nuclear data.
Haba, Hiromitsu*; Huang, M.*; Kaji, Daiya*; Kanaya, Jumpei*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Murakami, Masashi*; Ozeki, Kazutaka*; Sakai, Ryutaro*; et al.
Physical Review C, 89(2), p.024618_1 - 024618_11, 2014/02
Toyoshima, Atsushi; Li, Z.*; Asai, Masato; Sato, Nozomi; Sato, Tetsuya; Kikuchi, Takahiro; Kaneya, Yusuke; Kitatsuji, Yoshihiro; Tsukada, Kazuaki; Nagame, Yuichiro; et al.
Inorganic Chemistry, 52(21), p.12311 - 12313, 2013/11
The reduction behavior of mendelevium (Md) was studied using a flow electrolytic chromatography apparatus. By applying appropriate potentials on the chromatography column, the more stable Md is reduced to Md. The reduction potential of the Md + e Md couple was determined to be -0.160.05 V vs. a normal hydrogen electrode.
Li, Z.*; Toyoshima, Atsushi; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Sato, Nozomi; Kikuchi, Takahiro; Nagame, Yuichiro; Schdel, M.; Pershina, V.*; et al.
Radiochimica Acta, 100(3), p.157 - 164, 2012/03
Ninomiya, Kazuhiko; Nagatomo, Takashi*; Kubo, Kenya*; Ito, Takashi; Higemoto, Wataru; Kita, Makoto*; Shinohara, Atsushi*; Strasser, P.*; Kawamura, Naritoshi*; Shimomura, Koichiro*; et al.
Bulletin of the Chemical Society of Japan, 85(2), p.228 - 230, 2012/02
Elemental analysis of bulk materials can be performed by detecting the high-energy X-rays emitted from muonic atoms. Muon irradiation of standard bronze samples was performed to determine the muon capture probabilities for the elemental components from muonic X-ray spectra. Nondestructive elemental analysis of an ancient Chinese coin was also performed.
Haba, Hiromitsu*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sakai, Ryutaro*; Sumita, Takayuki*; Yoneda, Akira*; Kasamatsu, Yoshitaka*; et al.
Physical Review C, 85(2), p.024611_1 - 024611_11, 2012/02
Two isomeric states in Sg, i.e, Sg and Sg were produced in the Cm(Ne,5) reaction. Decay properties of Sg were investigated with a rotating-wheel apparatus for and spontaneous fission (SF) spectrometry under low background condition attained by a gas-jet transport system coupled to the RIKEN gas-filled recoil ion separator. Based on genetically correlated - (-) and -SF decay chains, 18 and 24 events were assigned to Sg and Sg, respectively. The half-life and -particle energy of Sg were measured to be s and MeV, respectively, and those of Sg were s and MeV.