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Polyelectrolyte-protein synergism; pH-responsive polyelectrolyte/insulin complexes as versatile carriers for targeted protein and drug delivery

Murmiliuk, A.*; 岩瀬 裕希*; Kang, J.-J.*; Mohanakumar, S.*; Appavou, M.-S.*; Wood, K.*; Alm$'a$sy, L.*; Len, A.*; Schw$"a$rzer, K.*; Allgaier, J.*; et al.

Journal of Colloid and Interface Science, 665, p.801 - 813, 2024/07



Laser-induced creation of antiferromagnetic 180-degree domains in NiO/Pt bilayers

Meer, H.*; Wust, S.*; Schmitt, C.*; Herrgen, P.*; Fuhrmann, F.*; Hirtle, S.*; Bednarz, B.*; Rajan, A.*; Ramos, R.*; Ni$~n$o, M. A.*; et al.

Advanced Functional Materials, 33(21), p.2213536_1 - 2213536_6, 2023/05

 被引用回数:1 パーセンタイル:44.21(Chemistry, Multidisciplinary)

The antiferromagnetic order in heterostructures of NiO/Pt thin films can be modified by optical pulses. After the irradiation with laser light, the optically induced creation of antiferromagnetic domains can be observed by imaging the created domain structure utilizing the X-ray magnetic linear dichroism effect. The effect of different laser polarizations on the domain formation can be studied and used to identify a polarization-independent creation of 180$$^{circ}$$ domain walls and domains with 180$$^{circ}$$ different N$'e$el vector orientation. By varying the irradiation parameters, the switching mechanism can be determined to be thermally induced. This study demonstrates experimentally the possibility to optically create antiferromagnetic domains, an important step towards future functionalization of all optical switching mechanisms in antiferromagnets.


$$beta^-$$ decay of exotic P and S isotopes with neutron number near 28

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 106(6), p.064314_1 - 064314_14, 2022/12

 被引用回数:2 パーセンタイル:47.44(Physics, Nuclear)



Improved measurement of the $$0_2^+rightarrow0_1^+$$ $$E$$0 transition strength for $$^{72}$$Se using the SPICE spectrometer

Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.

Physical Review C, 106(1), p.014312_1 - 014312_9, 2022/07

 被引用回数:3 パーセンタイル:61.19(Physics, Nuclear)

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $$^{72}$$Se by internal conversion electron and $$gamma$$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $$0_2^+$$ state were performed yielding a determination of $$rho^2(E0; 0_2^+{rightarrow}0_1^+)=29(3)$$ milliunits. Two state mixing calculations were performed that highlighted the importance of interpretation of such $$E0$$ strength values in the context of shape-coexistence.


Multi-methodical study of the Ti, Fe$$^{2+}$$ and Fe$$^{3+}$$ distribution in chevkinite-subgroup minerals; X-ray diffraction, neutron diffraction, $$^{57}$$Fe M$"o$ssbauer spectroscopy and electron-microprobe analyses

永嶌 真理子*; Armbruster, T.*; 赤坂 正秀*; 佐野 亜沙美; 浜根 大輔*; Malsy, A.*; 今岡 照喜*; 中島 和夫*

Physics and Chemistry of Minerals, 47(6), p.29_1 - 29_18, 2020/06

 被引用回数:3 パーセンタイル:16.03(Materials Science, Multidisciplinary)

足摺岬(日本), タンギールバレー(パキスタン), ディアマル地区(パキスタン), スカルドゥ地区(パキスタン)の3つの非メタミックチェブキナイト亜族鉱物を結晶化学的手法により研究した。粉末X線回折及び透過電子顕微鏡観察の結果、結晶性の良い試料であることが確認された。また、電子顕微鏡分析の結果、チェブキナイト-(Ce)として一般的に知られている組成であることが確認された。単結晶X線構造の精密化により決定されたサイト散乱値から、八面体のM3とM4に従属Nbが、Ashizuri試料ではM1に従属Thが、パキスタン産の両試料ではM1に従属Mgが割り当てられていることが示唆された。中性子飛行時間粉末回折法を用いて、全試料の八面体サイト間のTi/Fe分布を決定し、メスバウアー分光法を用いて四つの八面体サイトの鉄価数を決定した。ハラモッシュ試料のM1の鉄価数は鉄が支配的であるのに対し、足摺岬とタンギールバレーの試料では鉄が支配的であった。


In-source laser spectroscopy of dysprosium isotopes at the ISOLDE-RILIS

Chrysalidis, K.*; Barzakh, A. E.*; Ahmed, R.*; Andreyev, A. N.; Ballof, J.*; Cubiss, J. G.*; Fedorov, D. V.*; Fedosseev, V. N.*; Fraile, L. M.*; Harding, R. D.*; et al.

Nuclear Instruments and Methods in Physics Research B, 463, p.472 - 475, 2020/01

 被引用回数:3 パーセンタイル:35.09(Instruments & Instrumentation)

放射壊変によって生成された多数のジスプロシウム同位体について、ISOLDEのレーザー共鳴イオン源(RILIS)を用いてイオン源内レーザー分光法によって研究した。$$^{152}$$Dyに対する相対的な同位体シフトを$$4f^{10}6s^{2}~^{5}I_{8}$$ (gs) $$rightarrow$$ $$4f^{10}6s6p~(8,1)^{o}_{8}$$共鳴遷移を用いて測定した。電子的因子Fとマスシフト因子Mを導出し、それらを使って$$^{rm 145m}$$Dyと$$^{rm 147m}$$Dyの平均自乗荷電半径の変化を初めて決定した。


$$alpha$$-decay properties of $$^{200,202}$$Fr

Ghys, L.*; Andreyev, A. N.; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; Cocolios, T. E.*; Cubiss, J.*; Derkx, X.*; et al.

Physical Review C, 100(5), p.054310_1 - 054310_13, 2019/11

 被引用回数:13 パーセンタイル:78.16(Physics, Nuclear)

The aim of this work was to investigate the $$alpha$$-decay properties of $$^{200,202}$$Fr and daughter products. Neutron-deficient francium nuclei are produced at ISOLDE-CERN bombarding a UCx target with 1.4 GeV protons. Due to the very high statistics and the high beam purity, improved decay data for $$^{202}$$Fr and its daughters were obtained. The observation of crossover transitions positioned the isomeric high-spin level of $$^{198}$$At at an excitation energy of 265(3) keV. Half-life values of 4.47(5) s and 1.28(10) s were extracted for the ground state and isomeric state of $$^{198}$$At and 52(3) ms for the ground-state decay of $$^{200}$$Fr.


Effects of the nuclear structure of fission fragments on the high-energy prompt fission $$gamma$$-ray spectrum in $$^{235}$$U($$n_{rm th},f$$)

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.; 小川 達彦; Soldner, T.*; K$"o$ster, U.*; Pollitt, A.*; Hambsch, F.-J.*; et al.

Physical Review C, 100(4), p.044610_1 - 044610_7, 2019/10

 被引用回数:12 パーセンタイル:76.08(Physics, Nuclear)

The prompt fission $$gamma$$-ray energy spectrum for cold-neutron induced fission of $$^{235}$$U was measured in the energy range $$E_{rm gamma}$$ = 0.8 - 20,MeV, by gaining a factor of about 10$$^{5}$$ in statistics compared to the measurements performed so far. The spectrum exhibits local bump structures at $$E_{rm gamma}approx$$4,MeV and $$approx$$6,MeV, and also a broad one at $$approx$$15,MeV. In order to understand the origins of these bumps, the $$gamma$$-ray spectra were calculated using a statistical Hauser-Feshbach model, taking into account the de-excitation of all the possible primary fission fragments. It is shown that the bump at $$approx$$4,MeV is created by the transitions between the discrete levels in the fragments around $$^{132}$$Sn, and the bump at $$approx$$6,MeV mostly comes from the complementary light fragments. It is also indicated that a limited number of nuclides, which have high-spin states at low excitation energies, can contribute to the bump structure around $$E_{rm gamma}approx$$15,MeV, induced by the transition feeding into the low-lying high-spin states.


Fine structure in the $$alpha$$ decay of $$^{218}$$At

Cubiss, J. G.*; Andreyev, A. N.; Barzakh, A. E.*; Andel, B.*; Antalic, S.*; Cocolios, T. E.*; Day Goodacre, T.*; Fedorov, D. V.*; Fedosseev, V. N.*; Ferrer, R.*; et al.

Physical Review C, 99(6), p.064317_1 - 064317_6, 2019/06

 被引用回数:6 パーセンタイル:52.65(Physics, Nuclear)



Inverse odd-even staggering in nuclear charge radii and possible octupole collectivity in $$^{217,218,219}$$At revealed by in-source laser spectroscopy

Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero$'n$, J.*; et al.

Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05

 被引用回数:12 パーセンタイル:76.08(Physics, Nuclear)

Hyperfine-structure parameters and isotope shifts for the 795-nm atomic transitions in $$^{217,218,219}$$At have been measured at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy technique. Magnetic dipole and electric quadrupole moments, and changes in the nuclear mean-square charge radii, have been deduced. A large inverse odd-even staggering in radii, which may be associated with the presence of octupole collectivity, has been observed. Namely, the radius of the odd-odd isotope $$^{218}$$At has been found to be larger than the average.


A New detector system for the measurement of high-energy prompt $$gamma$$-rays for low-energy neutron induced fission

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.*; 小川 達彦; Soldner, T.*; Hambsch, F.-J.*; A$"i$che, M.*; Astier, A.*; et al.

Nuclear Instruments and Methods in Physics Research A, 906, p.88 - 96, 2018/10

 被引用回数:3 パーセンタイル:29.51(Instruments & Instrumentation)



Quasiparticle phonon model description of low-energy states in $$^{152}$$Pr

Alexa, P.*; Ramdhane, M.*; Thiamova, G.*; Simpson, G. S.*; Faust, H. R.*; Genevey, J.*; K$"o$ster, U.*; Materna, T.*; Orlandi, R.; Pinston, J. A.*; et al.

Physical Review C, 97(3), p.034327_1 - 034327_6, 2018/03

 被引用回数:2 パーセンタイル:20.61(Physics, Nuclear)

Delayed $$gamma$$-ray and conversion-electron spectroscopy was performed on A = 152 fission fragments, at the Lohengrin spectrometer of the Institut Laue-Langevin, Grenoble, France. In this study, a new decay scheme was observed for the odd-odd nuclide $$^{158}$$Pr. The low-energy structure of this isotope was analysed by comparison with the quasiparticle phonon model and the particle-rotor model. The main configurations for the ($$3^+$$) ground state and for the 4.7(3)-$$mu$$s ($$1^+$$) isomer at 115 keV were assigned to, respectively, $$pi$$3/2[541]$$otimes$$$$nu$$3/2[521] and $$pi$$3/2[422]$$otimes$$$$nu$$5/2[642].


Detailed $$alpha$$-decay study of $$^{180}$$Tl

Andel, B.*; Andreyev, A. N.; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; Diriken, J.*; Elseviers, J.*; Fedorov, D. V.*; et al.

Physical Review C, 96(5), p.054327_1 - 054327_11, 2017/12

 被引用回数:3 パーセンタイル:26.98(Physics, Nuclear)

A detailed $$alpha$$-decay spectroscopy study of $$^{180}$$Tl has been performed at ISOLDE (CERN). Z-selective ionization by the Resonance Ionization Laser Ion Source (RILIS) coupled to mass separation provided a high-purity beam of $$^{180}$$Tl. Fine-structure $$alpha$$ decays to excited levels in the daughter $$^{176}$$Au were identified and an $$alpha$$-decay scheme of $$^{180}$$Tl was constructed based on an analysis of $$alpha$$-$$gamma$$ and $$alpha$$-$$gamma$$ -$$gamma$$ coincidences. Multipolarities of several $$gamma$$-ray transitions deexciting levels in $$^{176}$$Au were determined. Based on the analysis of reduced $$alpha$$-decay widths, it was found that all $$alpha$$ decays are hindered, which signifies a change of configuration between the parent and all daughter states.


EXILL; A High-efficiency, high-resolution setup for $$gamma$$-spectroscopy at an intense cold neutron beam facility

Jentschel, M.*; Blanc, A.*; de France, G.*; K$"o$ster, U.*; Leoni, S.*; Mutti, P.*; Simpson, G.*; Soldner, T.*; Ur, C.*; Urban, W.*; et al.

Journal of Instrumentation (Internet), 12(11), p.P11003_1 - P11003_33, 2017/11

 被引用回数:38 パーセンタイル:85.07(Instruments & Instrumentation)

A highly efficient array of high-purity germanium (HPGe) detectors was developed and operated at the cold neutron beam facility PF1B of the Institut Laue-Langevin (ILL) to carry out nuclear structure studies, via measurements of $$gamma$$-rays following neutron-induced capture and fission reactions. The setup consisted of a collimation system producing a pencil beam with a thermal capture equivalent flux of about 10$$^8$$ns$$^{-1}$$cm$$^{-2}$$ at the target position and negligible neutron halo. The target was surrounded by an array of eight to ten anti-Compton shielded EXOGAM Clover detectors, four to six anti-Compton shielded large coaxial GASP detectors and two standard Clover detectors. For a part of the campaign the array was combined with 16 LaBr$$_{3}$$:(Ce) detectors from the FATIMA collaboration.


Measurement of high-energy prompt $$gamma$$-rays from neutron induced fission of U-235

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.; 小川 達彦; Soldner, T.*; Hambsch, F.-J.*; Astier, A.*; Pollitt, A.*; et al.

EPJ Web of Conferences, 146, p.04036_1 - 04036_4, 2017/09

 被引用回数:4 パーセンタイル:90.42(Nuclear Science & Technology)



Changes in mean-squared charge radii and magnetic moments of $$^{179-184}$$Tl measured by in-source laser spectroscopy

Barzakh, A.*; Andreyev, A. N.; Cocolios, T. E.*; de Groote, R. P.*; Fedorov, D. V.*; Fedosseev, V. N.*; Ferrer, R.*; Fink, D. A.*; Ghys, L.*; Huyse, M.*; et al.

Physical Review C, 95(1), p.014324_1 - 014324_12, 2017/01

 被引用回数:26 パーセンタイル:88.25(Physics, Nuclear)

Hyperfine structure and isotope shifts have been measured for the ground and isomeric states in the neutron deficient isotopes $$^{179-184}$$Tl using the 276.9 nm transition. The experiment has been performed at the CERN Isotope Separator On-Line facility using the in-source resonance-ionization laser spectroscopy technique. Spins for the ground states in $$^{179,181,183}$$Tl have been determined as $$I$$ = 1/2. Magnetic moments and changes in the nuclear mean-square charge radii have been deduced. By applying the additivity relation for magnetic moments of the odd-odd Tl nuclei the leading configuration assignments were confirmed. A deviation of magnetic moments for isomeric states in $$^{182,184}$$Tl from the trend of the heavier Tl nuclei is observed. The charge radii of the ground states of the isotopes $$^{179-184}$$Tl follow the trend for isotonic (spherical) lead nuclei. The noticeable difference in charge radii for ground and isomeric states of $$^{183,184}$$Tl has been observed, suggesting a larger deformation for the intruder-based 9/2$$^{-}$$ and 10$$^{-}$$ states compared to the ground states. An unexpected growth of the isomer shift for $$^{183}$$Tl has been found.


Stability and synthesis of superheavy elements; Fighting the battle against fission - Example of $$^{254}$$No

Lopez-Martens, A.*; Henning, G.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; 浅井 雅人; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

EPJ Web of Conferences, 131, p.03001_1 - 03001_6, 2016/12

 被引用回数:1 パーセンタイル:43.58(Chemistry, Inorganic & Nuclear)



$$beta$$-delayed fission and $$alpha$$ decay of $$^{196}$$At

Truesdale, V. L.*; Andreyev, A. N.; Ghys, L.*; Huyse, M.*; Van Duppen, P.*; Sels, S.*; Andel, B.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; et al.

Physical Review C, 94(3), p.034308_1 - 034308_11, 2016/09

 被引用回数:10 パーセンタイル:59.81(Physics, Nuclear)

A nuclear-decay spectroscopy study of the neutron-deficient isotope $$^{196}$$At is reported where an isotopically pure beam was produced using the selective Resonance Ionization Laser Ion Source and On-Line Isotope Mass Separator (CERN). The fine-structure $$alpha$$ decay of $$^{196}$$At allowed the low-energy excited states in the daughter nucleus $$^{192}$$Bi to be investigated. A $$beta$$-delayed fission study of $$^{196}$$At was also performed. A mixture of symmetric and asymmetric fission-fragment mass distributions of the daughter isotope $$^{196}$$Po (populated by $$beta$$ decay of $$^{196}$$At) was deduced based on the measured fission-fragment energies. A $$beta$$DF probability $$P_{rm beta DF}$$($$^{196}$$At) = 9(1)$$times$$10$$^{-5}$$ was determined.


Population and decay of a $$K^{pi}$$ = 8$$^{-}$$ two-quasineutron isomer in $$^{244}$$Pu

Hota, S.*; Tandel, S.*; Chowdhury, P.*; Ahmad, I.*; Carpenter, M. P.*; Chiara, C. J.*; Greene, J. P.*; Hoffman, C. R.*; Jackson, E. G.*; Janssens, R. V. F.*; et al.

Physical Review C, 94(2), p.021303_1 - 021303_5, 2016/08

 被引用回数:6 パーセンタイル:44.13(Physics, Nuclear)

$$^{244}$$Puにおける$$K^{pi}$$ = 8$$^{-}$$アイソマーからの崩壊と集団的バンド構造が$$^{47}$$Tiと$$^{208}$$Pbのビームによる深部非弾性散乱実験によって調べられた。バンド内の正確な$$M1/E2$$分岐比の測定によって、偶$$Z$$, $$N$$=150アイソトーンにおける$$K^{pi}$$ = 8$$^{-}$$二準中性子アイソマーが9/2$$^-$$[734]$$_{nu}$$$$otimes$$7/2$$^+$$[624]$$_{nu}$$の配位であることを確かめた。$$N$$=152における変形シェルギャップ近傍のこれらのアイソマーは、超重核の一粒子エネルギーの理論的な予言において重要なベンチマークとなる。


The Martian surface radiation environment; A Comparison of models and MSL/RAD measurements

Matthi$"a$, D.*; Ehresmann, B.*; Lohf, H.*; K$"o$hler, J.*; Zeitlin, C.*; Appel, J.*; 佐藤 達彦; Slaba, T. C.*; Martin, C.*; Berger, T.*; et al.

Journal of Space Weather and Space Climate (Internet), 6, p.A13_1 - A13_17, 2016/03

 被引用回数:66 パーセンタイル:93.60(Astronomy & Astrophysics)

2012年8月6日以降、Mars Science Laboratory (MSL)に搭載された複合型放射線検出器(RAD)を用いて火星表面による放射線環境の測定が続けられている。本研究では、GEANT4, PHITS, HZETRN/OLTARISなど様々なコードを用いて火星表面における放射線環境を推定し、その結果とRADによる測定値を比較した。その結果、計算結果は測定値と概ねよい一致を示すものの、場合によっては大きく解離することが分かった。また、RADのデータは放射線輸送計算について、最適なインプットパラメータや物理モデルの最適な選択に役立つことも確認された。今回の解析結果は、今後、有人火星ミッションを計画する際、その被ばく線量評価や宇宙機遮へい設計などに活用することができる。

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