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Ru
O
and the possible formation of Haldane chains in three-dimensional crystalsLee, S.*; Park, J.-G.*; Adroja, D. T.*; Khomskii, D.*; Streltsov, S.*; McEwen, K. A.*; Sakai, Hironori; Yoshimura, Kazuyoshi*; Anisimov, V. I.*; Mori, Daisuke*; et al.
Nature Materials, 5(6), p.471 - 476, 2006/06
Times Cited Count:116 Percentile:94.54(Chemistry, Physical)Here we show that the three-dimensional cubic system of Tl
Ru
O
most probably evolves into a one-dimensional spin-one Haldane system with a spin gap below 120 K, accompanied by anomalies in the structure, resistivity, and susceptibility. We argue that these anomalies are due to an orbital ordering of Ru
electrons, with a strong coupling among three degrees of freedom: orbital, spin, and lattice. Our work provides a unique example of the spontaneous formation of Haldane system with an insight into the intriguing interplay of different degrees of freedom.
-electron systems; X-ray magnetic circular dichroism study of Ba
CaOsO
Shibata, Goro; Hayashi, Hiroaki*; Kawamura, Naomi*; Okamoto, Jun*; Huang, D. J.*; Tanaka, Arata*; Streltsov, S.*; Yamaura, Kazunari*; Fujimori, Atsushi*
no journal, ,
CaOsO
as a candidate material for magnetic octupole studied by hard X-ray magnetic circular dichroismShibata, Goro; Okamoto, Jun*; Hayashi, Hiroaki*; Kawamura, Naomi*; Tanaka, Arata*; Yamaura, Kazunari*; Streltsov, S.*; Huang, D. J.*; Fujimori, Atsushi*
no journal, ,
no abstracts in English
CaOsO
Shibata, Goro; Hayashi, Hiroaki*; Kawamura, Naomi*; Okamoto, Jun*; Huang, D.-J.*; Streltsov, S.*; Yamaura, Kazunari*; Fujimori, Atsushi*
no journal, ,
no abstracts in English