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Fujiwara, Hidenori*; Umetsu, Rie*; Kuroda, Fumiaki*; Miyawaki, Jun*; Kashiuchi, Toshiyuki*; Nishimoto, Kohei*; Nagai, Kodai*; Sekiyama, Akira*; Irizawa, Akinori*; Takeda, Yukiharu; et al.
Scientific Reports (Internet), 11(1), p.18654_1 - 18654_9, 2021/09
Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)Saito, Yuji; Fujiwara, Hidenori*; Yasui, Akira*; Kadono, Toshiharu*; Sugawara, Hitoshi*; Kikuchi, Daisuke*; Sato, Hideyuki*; Suga, Shigemasa*; Yamasaki, Atsushi*; Sekiyama, Akira*; et al.
Physical Review B, 102(16), p.165152_1 - 165152_8, 2020/10
Times Cited Count:1 Percentile:4.84(Materials Science, Multidisciplinary)Nagai, Kodai*; Fujiwara, Hidenori*; Aratani, Hidekazu*; Fujioka, Shuhei*; Yomosa, Hiroshi*; Nakatani, Yasuhiro*; Kiss, Takayuki*; Sekiyama, Akira*; Kuroda, Fumiaki*; Fujii, Hitoshi*; et al.
Physical Review B, 97(3), p.035143_1 - 035143_8, 2018/01
Times Cited Count:23 Percentile:69.62(Materials Science, Multidisciplinary)We have studied the electronic structure of ferrimagnetic MnVAl single crystals by means of soft X-ray absorption spectroscopy (XAS), X-ray absorption magnetic circular dichroism (XMCD), and resonant soft X-ray inelastic scattering (RIXS). We have successfully observed the XMCD signals for all the constituent elements. The Mn L XAS and XMCD spectra are reproduced by spectral simulations based on density-functional theory, indicating the itinerant character of the Mn 3 states. On the other hand, the V 3 electrons are rather localized since the ionic model can qualitatively explain the V L XAS and XMCD spectra. This picture is consistent with local excitations revealed by the V L RIXS.
Mori, Takeo*; Kitayama, Satoshi*; Kanai, Yuina*; Naimen, Sho*; Fujiwara, Hidenori*; Higashiya, Atsushi*; Tamasaku, Kenji*; Tanaka, Arata*; Terashima, Kensei*; Imada, Shin*; et al.
Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12
Times Cited Count:16 Percentile:67.56(Physics, Multidisciplinary)We show that the strongly correlated 4-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra, as we have discovered for YbRhSi and YbCuSi. Theoretical analysis shows us that the linear dichroism reflects the anisotropic charge distributions resulting from a crystalline electric field. We have successfully determined the ground-state 4 symmetry for both compounds from the polarization-dependent angle resolved core-level spectra at a temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measurement temperatures are on the order of the crystal-field-splitting energies.
Berner, G.*; Sing, M.*; Fujiwara, Hidenori*; Yasui, Akira*; Saito, Yuji; Yamasaki, Atsushi*; Nishitani, Yoshihito*; Sekiyama, Akira*; Pavlenko, N.*; Kopp, T.*; et al.
Physical Review Letters, 110(24), p.247601_1 - 247601_5, 2013/06
Times Cited Count:135 Percentile:96.30(Physics, Multidisciplinary)The interface between LaAlO and SrTiO hosts a two-dimensional electron system of itinerant carriers, although both oxides are band insulators. Interface ferromagnetism coexisting with superconductivity has been found and attributed to local moments. Experimentally, it has been established that Ti 3 electrons are confined to the interface. Using soft X-ray angle-resolved resonant photoelectron spectroscopy we have directly mapped the interface states in space. Our data demonstrate a charge dichotomy. A mobile fraction contributes to Fermi surface sheets, whereas a localized portion at higher binding energies is tentatively attributed to electrons trapped by O vacancies in the SrTiO.
Mo, S.-K.*; Kim, H.-D.*; Denlinger, J. D.*; Allen, J. W.*; Park, J.-H.*; Sekiyama, Akira*; Yamasaki, Atsushi*; Suga, Shigemasa*; Saito, Yuji; Muro, Takayuki*; et al.
Physical Review B, 74(16), p.165101_1 - 165101_12, 2006/10
Times Cited Count:49 Percentile:84.47(Materials Science, Multidisciplinary)We present high-resolution bulk-sensitive photoemission spectra of (V)O (=Cr,Ti). The measurements were made for the paramagnetic metal (PM), paramagnetic insulator (PI), and antiferromagnetic insulator (AFI) phases of (V)O. In the PM phase, we observe a prominent quasiparticle peak in general agreement with theory, which combines dynamical mean-field theory with the local density approximation. For both the PI and AFI phases, the vanadium 3 parts of the valence spectra are not simple one peak structures. For the PI phase, there is not yet a good theoretical understanding of these structures. Spectra taken in the same phases with different compositions show interesting monotonic changes as the dopant concentration increases, regardless of the dopant species. With increased Cr-doping, the AFI phase gap decreases and the PI phase gap increases.
Irizawa, Akinori*; Higashiya, Atsushi*; Kasai, Shuichi*; Sasabayashi, Takehisa*; Shigemoto, Akihiko*; Sekiyama, Akira*; Imada, Shin*; Suga, Shigemasa*; Sakai, Hironori; Ono, Hiroyuki*; et al.
Journal of the Physical Society of Japan, 75(9), p.094701_1 - 094701_5, 2006/09
Times Cited Count:6 Percentile:41.48(Physics, Multidisciplinary)Photoemission spectroscopy (PES) and O X-ray absorption spectroscopy (XAS) measurements have been performed for Cd Re O single crystals. Temperature variations of their spectra reveal that the phase transition at 120 K directly changes the band structure near the Fermi level compared with another transition near 200 K. The roles of the transitions are discussed in terms of the changes in the Re-O orbital hybridization.
Sato, Hitoshi*; Yoshikawa, Kunta*; Hiraoka, Koichi*; Arita, Masashi*; Fujimoto, Koji*; Kojima, Kenichi*; Muro, Takayuki*; Saito, Yuji; Sekiyama, Akira*; Suga, Shigemasa*; et al.
Physical Review B, 69(16), p.165101_1 - 165101_6, 2004/04
Times Cited Count:33 Percentile:77.37(Materials Science, Multidisciplinary)no abstracts in English
Kang, J.-S.*; Kim, J. H.*; Sekiyama, Akira*; Kasai, Shuichi*; Suga, Shigemasa*; Han, S. W.*; Kim, K. H.*; Choi, E. J.*; Kimura, Tsuyoshi*; Muro, Takayuki*; et al.
Physical Review B, 68(1), p.012410_1 - 012410_4, 2003/07
Times Cited Count:21 Percentile:67.72(Materials Science, Multidisciplinary)no abstracts in English
Mo, S.-K.*; Denlinger, J. D.*; Kim, H.-D.*; Park, J.-H.*; Allen, J. W.*; Sekiyama, Akira*; Yamasaki, Atsushi*; Kadono, Koji*; Suga, Shigemasa*; Saito, Yuji; et al.
Physical Review Letters, 90(18), p.186403_1 - 186403_4, 2003/05
Times Cited Count:143 Percentile:95.37(Physics, Multidisciplinary)no abstracts in English
Kang, J.-S.*; Kim, J. H.*; Sekiyama, Akira*; Kasai, Shuichi*; Suga, Shigemasa*; Han, S. W.*; Kim, K. H.*; Muro, Takayuki*; Saito, Yuji; Hwang, C.*; et al.
Physical Review B, 66(11), p.113105_1 - 113105_4, 2002/09
Times Cited Count:65 Percentile:89.93(Materials Science, Multidisciplinary)The electronic structures of SrFeMoO (SFMO) and BaFeMoO (BFMO) double perovskites have been investigated using Fe 2p-3d resonant photoemission spectroscopy (PES) and the Cooper minimum in the Mo 4d photoionization cross section. The states close to the Fermi level are found to have a strongly mixed Mo–Fe t character, indicating that the Fe valence is far from pure 3+. The Fe 2p x-ray absorption spectroscopy spectra reveal the mixed-valent Fe –Fe configurations, and a larger Fe component for BFMO than for SFMO, suggesting an operative double exchange interaction. The valence-band PES spectra reveal good agreement with the local-spin-density-approximation (LSDA+U) calculation.
Iwasaki, T.*; Sekiyama, Akira*; Yamasaki, Atsushi*; Okazaki, Makoto*; Kadono, Koji*; Utsunomiya, Hiroshi*; Imada, Shin*; Saito, Yuji; Muro, Takayuki*; Matsushita, Tomohiro*; et al.
Physical Review B, 65(19), p.195109_1 - 195109_9, 2002/05
Times Cited Count:24 Percentile:71.27(Materials Science, Multidisciplinary)no abstracts in English
Yamasaki, Atsushi*; Imada, Shin*; Arai, Ryuji*; Utsunomiya, Hiroshi*; Suga, Shigemasa*; Muro, Takayuki*; Saito, Yuji; Kanomata, Takeshi*; Ishida, Shoji*
Physical Review B, 65(10), p.104410_1 - 104410_6, 2002/03
Times Cited Count:61 Percentile:89.14(Materials Science, Multidisciplinary)The magnetic circular dichroism (MCD) of core-level absorption [x-ray absorption spectroscopy (XAS)] spectra in the soft x-ray region has been measured for the ferromagnetic Heusler alloys CoTiSn, CoZrSn, and CoNbSn. The many-peak structures which are clearly observed in the Co 2p-3d XAS-MCD spectra cannot be well explained by atomic multiplet calculations but are better explained by the Co 3d unoccupied states predicted by linear muffin-tin orbital atomic sphere approximation band structure calculations. The MCD spectra show an obvious contribution of the orbital angular momentum component to the magnetic moment in these alloys. The ratio between the orbital angular momentum and spin derived from the MCD spectra varies by more than a factor of 2 within these alloys. The mechanism of this variation is discussed in comparison with the band structure calculations.
Saito, Yuji; Kimura, Hiroaki*; Suzuki, Yoshio*; Nakatani, Takeshi*; Matsushita, Tomohiro*; Muro, Takayuki*; Miyahara, Tsuneaki*; Fujisawa, M.*; Soda, Kazuo*; Ueda, Shigenori*; et al.
Nuclear Instruments and Methods in Physics Research A, 467-468(Part.1), p.553 - 556, 2001/07
Times Cited Count:23 Percentile:81.84(Instruments & Instrumentation)no abstracts in English
Yamasaki, Atsushi*; Imada, Shin*; Utsunomiya, Hiroshi*; Muro, Takayuki*; Saito, Yuji; Negishi, H.*; Sasaki, M.*; Inoue, M.*; Suga, Shigemasa*
Physica E, 10(1-3), p.387 - 390, 2001/05
Times Cited Count:5 Percentile:32.03(Nanoscience & Nanotechnology)no abstracts in English
Ueda, Shigenori*; Imada, Shin*; Muro, Takayuki*; Saito, Yuji; Suga, Shigemasa*; Matsukura, F.*; Ohno, Hideo*
Physica E, 10(1-3), p.210 - 214, 2001/05
Times Cited Count:24 Percentile:73.43(Nanoscience & Nanotechnology)no abstracts in English
Saito, Yuji; Muro, Takayuki*; Kotsugi, Masato*; Iwasaki, T.*; Sekiyama, Akira*; Imada, Shin*; Suga, Shigemasa*
Journal of Synchrotron Radiation, 8(Part2), p.339 - 341, 2001/03
no abstracts in English
Saito, Yuji; Kimura, Hiroaki*; Suzuki, Yoshio*; Nakatani, Takeshi*; Matsushita, Tomohiro*; Muro, Takayuki*; Miyahara, Tsuneaki*; Fujisawa, M.*; Soda, Kazuo*; Ueda, Shigenori*; et al.
Review of Scientific Instruments, 71(9), p.3254 - 3259, 2000/09
Times Cited Count:187 Percentile:98.96(Instruments & Instrumentation)no abstracts in English
Sekiyama, Akira*; Iwasaki, T.*; Matsuda, K.*; Saito, Yuji; Onuki, Yoshichika*; Suga, Shigemasa*
Nature, 403(6768), p.396 - 398, 2000/01
Times Cited Count:257 Percentile:98.87(Multidisciplinary Sciences)no abstracts in English
Saito, Yuji; Nakatani, Takeshi*; Matsushita, T.*; Miyahara, Tsuneaki*; Fujisawa, M.*; ; ; ; ; ; et al.
Journal of Synchrotron Radiation, 5, p.542 - 544, 1998/00
Times Cited Count:62 Percentile:94.24(Instruments & Instrumentation)no abstracts in English