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JAEA Reports

Assessment of probability of aircraft crashes for Nuclear Science Research Institute

Kamikawa, Yutaka; Suzuki, Makoto; Agake, Toshiki; Murakami, Takahiko; Morita, Yusuke; Shiina, Hidenori; Fukushima, Manabu; Hirane, Nobuhiko; Ouchi, Yasuhiro

JAEA-Technology 2023-030, 57 Pages, 2024/03

JAEA-Technology-2023-030.pdf:1.93MB

Owing to the publication of the latest data about aircraft crashes by Nuclear Regulation Authority (NRA), it was necessary to re-evaluate the probabilities of aircraft crashes for Nuclear Science Research Institute (NSRI). By using of the assessment method provided in "Regulatory Guide of the Assessment Standard for Probability of Airplane Crash on a Nuclear Power Reactor Facility", we re-evaluated the probabilities of aircraft crashes against the nuclear facilities in NSRI. As a result of the evaluations, the sum of the probabilities of aircraft crashes against Waste Treatment Facilities (maximum probability among all nuclear facilities in NSRI) is 5.68$$times$$10$$^{-8}$$ (times/(reactor $$cdot$$ year)) which is lower than 10$$^{-7}$$ (times/(reactor $$cdot$$ year)) that is the assessment criterion whether aircraft crashes is considered to be "anticipated external human induced events" in design basis or not.

JAEA Reports

Model catchments for testing biosphere assessment models of geological disposal

Yamaguchi, Masaaki; Suzuki, Yuji*; Kabasawa, Satsuki; Kato, Tomoko

JAEA-Data/Code 2024-001, 21 Pages, 2024/03

JAEA-Data-Code-2024-001.pdf:3.45MB
JAEA-Data-Code-2024-001-appendix(CD-ROM).zip:8.0MB

Model catchments have developed for use in testing various assessment models that can consider specific surface environmental conditions such as topography, riverine systems, and land use in the biosphere assessment of HLW geological disposal. The model catchments consist of the topography and riverine system of the catchment area created using existing tools, as well as land use and population distribution, river discharge, sediment flux data set by algorithms from topographical data. Datasets of three types of model watersheds (Types 1 to 3, watershed area: 730 to 770 km$$^{2}$$) with different topographical characteristics have released as raster data that can be handled by geographic information systems (GIS). Since the model catchments were created virtually reflecting as much as possible the main characteristics of Japan's surface environment, they can be used as a test bed for conducting hydraulic/mass transport analysis to set the GBI and compartment model.

Journal Articles

Stress measurement of stainless steel piping welds by complementary use of high-energy synchrotron X-rays and neutrons

Miura, Yasufumi*; Suzuki, Kenji*; Morooka, Satoshi; Shobu, Takahisa

Quantum Beam Science (Internet), 8(1), p.1_1 - 1_14, 2024/03

Journal Articles

Intercalative and non-intercalative photo-recharge using all-solid-state cells for solar energy conversion and storage

Yoshimoto, Masataka*; Tamura, Kazuhisa; Watanabe, Kenta*; Shimizu, Keisuke*; Horisawa, Yuhei*; Kobayashi, Takeshi*; Tsurita, Hanae*; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

Sustainable Energy & Fuels (Internet), 8(6), p.1236 - 1244, 2024/03

Photo-rechargeable systems, which can efficiently convert and store solar energy into chemical energy within single devices, are essential to harness sunlight effectively. Photo-(de)intercalation plays a pivotal role in the functionality of photorechargeable systems. Nevertheless, the photo-(de)intercalation process has not been conclusively confirmed owing to potential interference from side reactions, such as the decomposition of liquid electrolytes and the elution of electrode materials. In this study, we successfully demonstrated photo-responsive Li$$^{+}$$-deintercalation using an all-solid-state thin-film battery comprised of epitaxially-grown anatase TiO$$_{2}$$ doped with Nb (a-TiO$$_{2}$$:Nb) as the cathode. Under light irradiation, Li$$^{+}$$-deintercalation occurred and was subsequently reversibly intercalated into a-TiO$$_{2}$$:Nb during discharge.

Journal Articles

Experimental visualization of water/ice phase distribution at cold start for practical-sized polymer electrolyte fuel cells

Higuchi, Yuki*; Yoshimune, Wataru*; Kato, Satoru*; Hibi, Shogo*; Setoyama, Daigo*; Isegawa, Kazuhisa*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Nozaki, Hiroshi*; Harada, Masashi*; et al.

Communications Engineering (Internet), 3, p.33_1 - 33_7, 2024/02

Journal Articles

Neutron transmission CB-KID imager using samples placed at room temperature

Ishida, Takekazu*; Vu, TheDang*; Shishido, Hiroaki*; Aizawa, Kazuya; Oku, Takayuki; Oikawa, Kenichi; Harada, Masahide; Kojima, Kenji M*; Miyajima, Shigeyuki*; Koyama, Tomio*; et al.

Journal of Low Temperature Physics, 214(3-4), p.152 - 157, 2024/02

Journal Articles

Japan Atomic Energy Agency; Contribution to the decommissioning of the Fukushima Daiichi Nuclear Power Station and the reconstruction of Fukushima Prefecture at the Naraha center for Remote Control technology development

Morimoto, Kyoichi; Ono, Takahiro; Kakutani, Satomi; Yoshida, Moeka; Suzuki, Soichiro

Journal of Robotics and Mechatronics, 36(1), p.125 - 133, 2024/02

The Naraha Center for Remote Control Technology Development was established for the purpose of developing and verifying remote control equipment for promoting the decommissioning of the Fukushima Daiichi Nuclear Power Station and the external use of this center was started in 2016. The mission of this center is to contribute to the decommissioning of the Fukushima Daiichi Nuclear Power Station and for the reconstruction of Fukushima Prefecture. In this review, we describe the equipment related to the full-scale mock-up test, the component test for a remote-control device and the virtual reality system in this center. In addition, the case examples for usage of these equipment are introduced.

Journal Articles

Stable photoelectrochemical reactions at solid/solid interfaces toward solar energy conversion and storage

Watanabe, Kenta*; Horisawa, Yuhei*; Yoshimoto, Masataka*; Tamura, Kazuhisa; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

Nano Letters, 24(6), p.1916 - 1922, 2024/02

Electrochemistry has extended from reactions at solid/liquid interfaces to those at solid/solid interfaces. In this study, we achieve the stable photoelectrochemical reaction at the semiconductor-electrode/solid-electrolyte interface in Nb-doped anatase-TiO$$_{2}$$ (a-TiO$$_{2}$$:Nb)/Li$$_{3}$$PO$$_{4}$$ (LPO)/Li all-solid-state cell. The oxidative currents of a-TiO$$_{2}$$:Nb/LPO/Li increase upon light irradiation when a-TiO$$_{2}$$:Nb is located at a potential that is more positive than its flat-band potential. The photoelectrochemical reaction at the semiconductor/solid-electrolyte interface is driven by the same principle as that at semiconductor/liquid-electrolyte interfaces. Thus, we extend photoelectrochemistry to all-solid-state systems composed of solid/solid interfaces.

Journal Articles

Development of 0.5 mm gauge size radial collimators for high-pressure neutron diffraction experiments at PLANET in J-PARC

Hattori, Takanori; Suzuki, Koji*; Miyo, Tatsuya*; Ito, Takayoshi*; Machida, Shinichi*

Nuclear Instruments and Methods in Physics Research A, 1059, p.168956_1 - 168956_9, 2024/02

Radial collimators (RC) with a 0.5 mm gauge size (GS) were specially designed for high-pressure neutron diffraction experiments and their performance and efficacy were investigated. The RCs with nominal GS of 0.75 mm, 1.5 mm, and 3.0 mm effectively exhibited GS of 0.50 mm, 1.07 mm, and 2.78 mm, respectively. The transmissions of all three RCs were almost equivalent. The assessment using a P-E press and a DAC revealed that the anvil scattering was considerably minimized and the sample-to-anvil signal ratio reached values of 0.5 and 2.0 for the PE press and DAC, respectively, when using the 0.5 mm-GS RCs. These results indicate that the 0.5mm-GS RCs have been fabricated as intended and exhibit efficacy for the high-pressure-neutron diffraction experiments, specifically those exceeding 30 GPa. Among those ever manufactured for neutron scattering experiments, the RCs display the smallest GS.

Journal Articles

A Demonstration test to separate minor actinides in high-level liquid waste by ${it N,N,N',N',N'',N''}$-hexaoctyl nitrilotriacetamide (HONTA) using mixer-settler extractors in a hot cell

Ban, Yasutoshi; Suzuki, Hideya*; Hotoku, Shinobu; Tsubata, Yasuhiro

Solvent Extraction Research and Development, Japan, 31(1), p.1 - 11, 2024/00

A demonstration test was performed to separate minor actinides (MA; Am and Cm) by ${it N,N,N',N',N'',N''}$-hexaoctyl nitrilotriacetamide (HONTA) as an extractant using mixer-settler extractors installed in a hot cell. A high-level liquid waste containing MA, and rare earths (RE; Y, La, Nd, and Eu) was used as the feed. HONTA diluted to 0.05 mol/dm$$^{3}$$ in ${it n}$-dodecane was fed as the organic phase, and a part of the organic phase was reused without solvent regeneration. HONTA effectively extracted MA, whereas RE were less extractable. Consequently, the Y, La, Nd, and Eu ratios distributed to a RE fraction were $$>$$ 99.9%, 99.2%, 61.8%, and 81.4%, respectively. The Am and Cm ratios distributed to an MA fraction were 86.8% and 74.7%, respectively, and a substantial amount of MA (0.12 g) was recovered in the MA fraction by the end of the cumulative duration of 40 h.

Journal Articles

Exhumation history of the Kurobe area, Hida Range, based on solidification ages and depths of the Pliocene-Quaternary plutons

Sueoka, Shigeru; Kawakami, Tetsuo*; Suzuki, Kota*; Kagami, Saya; Yokoyama, Tatsunori; Shibazaki, Bunichiro*; Nagata, Mitsuhiro; Yamazaki, Ayu*; Higashino, Fumiko*; King, G. E.*; et al.

Fisshion, Torakku Nyusureta, (36), p.1 - 3, 2023/12

no abstracts in English

Journal Articles

Dirac Kondo effect under magnetic catalysis

Hattori, Koichi*; Suenaga, Daiki*; Suzuki, Kei; Yasui, Shigehiro*

Physical Review B, 108(24), p.245110_1 - 245110_11, 2023/12

We develop a mean-field theory of a novel Kondo effect emerging in systems without a Fermi surface, which instead emerges under strong magnetic fields. We determine the magnitude of the Kondo condensate, which is a particle pairing composed of conducting Dirac fermions and localized impurities. We focus on the competition between the Kondo effect and the energy gap formation that stems from the pairing among the Dirac fermions leading to the dynamical chiral symmetry breaking. We find that this competition induces a quantum critical point. We also investigate finite-temperature effects. This system at vanishing fermion density can be studied with Monte Carlo lattice simulations, which do not suffer from the sign problem.

Journal Articles

Applicability confirmation experiment of DDSI method for quantification of plutonium in fuel debris

Mitsuboshi, Natsumi; Nagatani, Taketeru; Kosuge, Yoshihiro*; Suzuki, Risa; Okada, Toyofumi

Dai-44-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2023/11

This paper reports the applicability confirmation experiment of DDSI method for quantification of plutonium in fuel debris. We conducted passive neutron measurement for the samples which consist of un-irradiated MOX sample, Cf-252 neutron source, and B-10 neutron absorber to simulate the fuel debris. It was revealed that DDSI method has enough capability to evaluate the leakage multiplication of the sample with unknown amounts of fissile material and neutron absorbers.

Journal Articles

Mutual separation of Am and Cm using ADAAM (alkyl DiAmide AMine) and reduction of volumes for liquid waste generated via batch-wise multistage extractions

Sasaki, Yuji; Kaneko, Masashi; Ban, Yasutoshi; Suzuki, Hideya*

Journal of Nuclear Science and Technology, 11 Pages, 2023/11

The mutual separation of Am and Cm is conducted using an alkyl-diamide amine (ADAAM) extractant. ADAAM exhibits extremely high separation factor with respect to Am and Cm separation (5.9) in a nitric acid-$$n$$-dodecane system. The batch-wise multistage extractions are performed using a system containing 0.2 M ADAAM and 1.5 M nitric acid. In this multistage extraction, an organic solvent give 96.5% and 1.06% yields of Am and Cm. After the mutual separation of Am and Cm, an additional extraction step is included to reduce the volumes of these aqueous and organic phases. Taking these steps, Am and Cm can be recovered in just two or three stages in the aqueous phases.

Journal Articles

Application of Bayesian machine learning for estimation of uncertainty in forecasted plume directions by atmospheric dispersion simulations

Kadowaki, Masanao; Nagai, Haruyasu; Yoshida, Toshiya*; Terada, Hiroaki; Tsuzuki, Katsunori; Sawa, Hiroki*

Journal of Nuclear Science and Technology, 60(10), p.1194 - 1207, 2023/10

 Times Cited Count:2 Percentile:75.85(Nuclear Science & Technology)

This study develops an estimation method using machine learning for uncertainty in forecasted plume directions. Bayesian machine learning was used in the machine learning approach. A three-day forecast simulation was conducted every day from 2015-2020, considering a hypothetical release of $$^{137}$$Cs from a nuclear facility to create training and test datasets for the machine learning. The findings reveal that the rate of good predictability was greater than 50% even in the forecast 36 h later when investigating the effectiveness of the Bayesian model on uncertainty estimation. Additionally, the frequency of miss prediction of higher uncertainty was low (0.9%-7.9%) throughout the forecast period. However, the rate of over-prediction of uncertainty increased with forecast time up to 31.2%, which is acceptable as a conservative estimation. These results show that the Bayesian model used in this study effectively estimates the uncertainty of plume directions predicted through atmospheric dispersion simulations.

Journal Articles

Extraction of $$^{99}$$Mo hot atoms made by a neutron capture method from $$alpha$$-MoO$$_{3}$$ to water

Quach, N. M.*; Ngo, M. C.*; Yang, Y.*; Nguyen, T. B.*; Nguyen, V. T.*; Fujita, Yoshitaka; Do, T. M. D.*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Suematsu, Hisayuki*

Journal of Radioanalytical and Nuclear Chemistry, 332(10), p.4057 - 4064, 2023/10

Technetium-99m ($$^{99m}$$Tc) is the most widely used medical radioisotope in the world and is produced from molybdenum-99 ($$^{99}$$Mo). Production of $$^{99}$$Mo via the neutron capture method draws attention as an alternative to fission-derived $$^{99}$$Mo due to non-proliferation issues, but the specific radioactivity of $$^{99}$$Mo is extremely low. In this work, a porous $$alpha$$-MoO$$_{3}$$ wire was prepared as an irradiation target in order to improve the specific activity by extracting $$^{99}$$Mo. Porous $$alpha$$-MoO$$_{3}$$ wire is synthesized from Mo metal wire by a two-step heating procedure. The hot atom effect of $$^{99}$$Mo was confirmed by activity and isotope measurements of the porous $$alpha$$-MoO$$_{3}$$ wire after neutron irradiation and the water used for extraction. In term of the extraction effectiveness, the effectiveness of $$^{99}$$Mo extraction in the porous $$alpha$$-MoO$$_{3}$$ wire was comparable to that of commercial $$alpha$$-MoO$$_{3}$$ powder.

JAEA Reports

Annual report for FY2021 on the activities of Naraha Center for Remote Control Technology Development (April 1, 2021 - March 31, 2022)

Akiyama, Yoichi; Shibanuma, So; Yanagisawa, Kenichi*; Yamada, Taichi; Suzuki, Kenta; Yoshida, Moeka; Ono, Takahiro; Kawabata, Kuniaki; Watanabe, Kaho; Morimoto, Kyoichi; et al.

JAEA-Review 2023-015, 60 Pages, 2023/09

JAEA-Review-2023-015.pdf:4.78MB

Naraha Center for Remote Control Technology Development (NARREC) was established in Japan Atomic Energy Agency to promote a decommissioning work of Fukushima Daiichi Nuclear Power Station (Fukushima Daiichi NPS). NARREC consists of a Full-scale Mock-up Test Building and Research Management Building. Various test facilities are installed in these buildings for the decommissioning work of Fukushima Daiichi NPS. These test facilities are intended to be used for various users, such as companies engaged in the decommissioning work, research and development institutions, educational institutions and so on. The number of NARREC facility uses was 84 in FY2021. We participated booth exhibitions and presentations on the decommissioning related events. Moreover, we also contributed to the development of human resources by supporting the 6th Creative Robot Contest for Decommissioning. As a new project, "Narahakko Children's Classroom" was implemented for elementary school students in Naraha Town. This report summarizes the activities of NARREC in FY2021, such as the utilization of facilities and equipment of NARREC, the development of remote-control technologies for supporting the decommissioning work, arrangement of the remote-control machines for emergency response, and training for operators by using the machines.

JAEA Reports

Acquisition of saltwater infiltration behavior data in unsaturated compacted bentonite

Sato, Hisashi*; Takayama, Yusuke; Suzuki, Hideaki*; Sato, Daisuke*

JAEA-Data/Code 2023-010, 47 Pages, 2023/09

JAEA-Data-Code-2023-010.pdf:1.45MB

When a high-level radioactive waste repository is constructed in a coastal area, it is necessary to fully evaluate the impact of seawater-based groundwater on engineered barriers, including buffer materials. In this report, one-dimensional saltwater infiltration tests were conducted to obtain data to understand the impact of seawater-based groundwater on the migration phenomena of water and solutes in the buffer material during the transient period. As a result, it was confirmed that the infiltration rate increased as the NaCl concentration in the infiltration solution increased. And it was confirmed that the water content ratio distribution changed as the NaCl concentration in the infiltration solution increased. As a result of analysis of the chloride ion concentration of the post-test specimens confirmed that chloride ion enrichment was occurred with infiltration. As a result of verifying the mechanism by which chloride ion enrichment occurs, it was confirmed that the phenomenon of chloride ion enrichment due to infiltration depends on the initial water content ratio.

Journal Articles

In situ transmission electron microscopy observation of melted germanium encapsulated in multilayer graphene

Suzuki, Seiya; Nemoto, Yoshihiro*; Shiiki, Natsumi*; Nakayama, Yoshiko*; Takeguchi, Masaki*

Annalen der Physik, 535(9), p.2300122_1 - 2300122_12, 2023/09

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Deuterium content and site occupancy in iron sulfide at high pressure and temperature determined using in situ neutron diffraction measurements

Abeykoon, S.*; Howard, C.*; Dominijanni, S.*; Eberhard, L.*; Kurnosov, A.*; Frost, D. J.*; Boffa Ballaran, T.*; Terasaki, Hidenori*; Sakamaki, Tatsuya*; Suzuki, Akio*; et al.

Journal of Geophysical Research; Solid Earth, 128(9), p.e2023JB026710_1 - e2023JB026710_17, 2023/09

Small amounts of iron sulphide minerals are found in most rocks from the Earth's mantle and as inclusions trapped in natural diamonds. Hydrogen may dissolve into iron sulphide minerals under high pressures and temperature, but is most likely lost once pressure and temperature are removed. In this study, we determined deuterium contents in iron sulphide, held under high pressure and temperature conditions, using neutron diffraction measurements with 6-ram multi-anvil press at PLANET, J-PARC. Deuterium contents in iron sulphide were measured at high-P, up to 11.4 GPa and high-T to 1300 K in in situ neutron diffraction experiments. The total deuterium content increases with both P and T. The results are used to estimate hydrogen contents of iron sulphide minerals in the deep continental lithospheric mantle, which are found to be in the range 1700-2700 ppm. This corresponds to approximately 2-3 ppm of hydrogen in the bulk mantle.

5843 (Records 1-20 displayed on this page)