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Uchino, Seiko*; Narita, Hirokazu*; Kita, Keisuke*; Suzuki, Hideya*; Matsumura, Tatsuro; Naganawa, Hirochika*; Sakaguchi, Koichi*; Oto, Keisuke*
Solvent Extraction Research and Development, Japan, 30(1), p.39 - 46, 2023/00
The extraction of trivalent rare earth ions (RE
) from HNO
solution using a triamide amine, tris(N,N-di-2-ethylhexyl-ethylamide)amine (DEHTAA), was conducted, and the extraction mechanism was estimated from extraction behavior of HNO and RE and the relationship between atomic number and extraction percentages (E%) for RE. A DEHTAA molecule dominantly formed a DEHTAA HNO at 1.0 M HNO and a DEHTAA(HNO)
at 6.0 M HNO in the acid-equilibrated organic phase. This would provide the unique dependence of E% for the light RE on the HNO concentration, in which the E% value had a minimum and maximum at 
0.5 M and 2 M HNO, respectively. The results of the slope analyses for the distribution ratios for RE suggested that the dominant RE complex was RE(NO)DEHTAA(DEHTAA HNO) at 1.0 M HNO. The E% for RE decreased from La to Lu at 1.0 M HNO; on the other hand, those increased from La to Nd at 0.25 M and from La to Sm and 6.0 M HNO.
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count：43 Percentile：96.93(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 
C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
RuO
proved by spin resonanceIida, Kazuki*; Kofu, Maiko; Suzuki, Katsuhiro*; Murai, Naoki; Kawamura, Seiko; Kajimoto, Ryoichi; Inamura, Yasuhiro; Ishikado, Motoyuki*; Hasegawa, Shunsuke*; Masuda, Takatsugu*; et al.
Journal of the Physical Society of Japan, 89(5), p.053702_1 - 053702_5, 2020/05
Times Cited Count：19 Percentile：81.08(Physics, Multidisciplinary)
Sr
Cu
Al
O
Ikeuchi, Kazuhiko*; Nakajima, Kenji; Kawamura, Seiko; Kajimoto, Ryoichi; Wakimoto, Shuichi; Suzuki, Kensuke*; Fujita, Masaki*
AIP Advances (Internet), 8(10), p.101318_1 - 101318_5, 2018/10
Times Cited Count：0 Percentile：0(Nanoscience & Nanotechnology)By means of inelastic neutron scattering, we measured magnetic excitations in a sizable single crystal of LaSrCuAlO, which is an Al-substituted system of the heavily hole-doped cuprate system La
Sr
CuO with an effective concentration of holes of 
= 0.25.
Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.
Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12
The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.
Sakasai, Kaoru; Sato, Setsuo*; Seya, Tomohiro*; Nakamura, Tatsuya; To, Kentaro; Yamagishi, Hideshi*; Soyama, Kazuhiko; Yamazaki, Dai; Maruyama, Ryuji; Oku, Takayuki; et al.
Quantum Beam Science (Internet), 1(2), p.10_1 - 10_35, 2017/09
Neutron devices such as neutron detectors, optical devices including supermirror devices and 
He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF.
Koyama, Shinichi; Suzuki, Tatsuya*; Ozawa, Masaki*; Kurosawa, Kiyoko*; Fujita, Reiko*; Mimura, Hitoshi*; Okada, Ken*; Morita, Yasuji; Fujii, Yasuhiko*
Procedia Chemistry, 7, p.222 - 230, 2012/00
Times Cited Count：2 Percentile：71.08(Chemistry, Analytical)Adv.-ORIENT cycle strategy has been proposed as a basic concept for trinitarian research on separation, transmutation and utilization of nuclides and elements based on FBR fuel cycle. Validation of principal separation method and related safety research were performed from 2006 through 2011 as Phase I program. First, more than 90% of Cs could be recovered from the actual spent fuel [IXC(I) step]. The next is the adsorption of the platinum group metals (PGM), lanthanides, Am and Cm were separated by using a tertiary pyridine-type resin (TPR) as ion exchange steps [IXC(II, III, IV) steps]. The separated PGM metals will be supplied to the electrochemical extraction [CEE step]. As experiment for safety issues, Hastelloy-B at RT and Ta at 90C were confirmed their anti-corrosive in highly concentrated HCl media. Thermo-chemical stability for TPR was verified. Issues to be solved for next phase based on the final results of phase I program.
Koyama, Shinichi; Yamagishi, Isao; Suzuki, Tatsuya*; Ozawa, Masaki*; Fujita, Reiko*; Okada, Ken*; Tatenuma, Katsuyoshi*; Mimura, Hitoshi*; Fujii, Yasuhiko
Proceedings of International Conference on Toward and Over the Fukushima Daiichi Accident (GLOBAL 2011) (CD-ROM), 8 Pages, 2011/12
Effective separation of MA and LLFP, transmutation and utilization were the main directions of Advanced OREINT Cycle project. Study for each integrant technology was concluded as first trial of the project. TPR enabled to separate MA/Ln and then Am/Cm precisely from spent fuel in HCl and HNO media. CEE method could separate the light PGM and Tc by HCl media. Recovery of Cs from simulated HLLW coul be achieved more than 90 %. In addition, the perspective for next phase was proposed.
Koyama, Shinichi; Suzuki, Tatsuya*; Mimura, Hitoshi*; Fujita, Reiko*; Kurosawa, Kiyoko*; Okada, Ken*; Ozawa, Masaki
Progress in Nuclear Energy, 53(7), p.980 - 987, 2011/09
Times Cited Count：5 Percentile：38.65(Nuclear Science & Technology)Individual basic researches of separation step were performed in the Advanced ORIENT Cycle project. High separation selectivity for Cs and Sr by novel nano adsorbents AMP-SG (D) and D18C6-MC were confirmed, respectively. TPR well adsorbed Pd and Tc in dilute HCl condition. Formation of rare metal fission product RMFP-deposit Pt electrodes from SHLLW was verified, and it was confirmed that high catalytic reactivity on electrolytic production of hydrogen. As experiment for engineering feasibility, Hastelloy-B at RT and Ta at 90C were confirmed their anti-corrosive in highly concentrated HCl media. Thermo-chemical stability for TPR was verified in either HCl or HNO media toward its practical use in the separation process. Issues to be solved for optimization based on the results of lab-scale experiment have revealed in this study.
Ogino, Haruyuki*; Kono, Takahiko; Yamasoto, Kotaro; Fujiwara, Keiko*; Suzuki, Chihiro*
Nihon Genshiryoku Gakkai-Shi ATOMO
, 52(8), p.458 - 461, 2010/08
no abstracts in English
Ozawa, Masaki; Suzuki, Tatsuya*; Koyama, Shinichi; Yamagishi, Isao; Fujita, Reiko*; Okada, Ken*; Tatenuma, Katsuyoshi*; Mimura, Hitoshi*; Fujii, Yasuhiko*
Proceedings of International Conference on Advanced Nuclear Fuel Cycle; Sustainable Options & Industrial Perspectives (Global 2009) (CD-ROM), p.1117 - 1126, 2009/09
, induces the somatic mutationFurusawa, Toshiharu*; Fukamoto, Kana*; Sakashita, Tetsuya; Suzuki, Eiko*; Kakizaki, Takehiko*; Hamada, Nobuyuki*; Funayama, Tomoo; Suzuki, Hiromi*; Ishioka, Noriaki*; Wada, Seiichi*; et al.
Journal of Radiation Research, 50(4), p.371 - 375, 2009/07
Times Cited Count：9 Percentile：32.08(Biology)Using heavy-ion microbeam, we report target irradiation of selected compartments within the diapause-terminated egg and its mutational consequences in the silkworm, . On one hand, carbon-ion exposure of embryo to 0.5 - 6 Gy increased the somatic mutation frequency, suggesting targeted radiation effects. On the other, such increases were not observed when yolk was targeted, suggesting a lack of nontargeted bystander effect.
Furusawa, Toshiharu*; Suzuki, Eiko*; Nagaoka, Shunji*; Suzuki, Hiromi*; Ishioka, Noriaki*; Hamada, Nobuyuki*; Wada, Seiichi*; Kobayashi, Yasuhiko; Sakashita, Tetsuya; Kakizaki, Takehiko*; et al.
JAEA-Review 2007-060, JAEA Takasaki Annual Report 2006, P. 115, 2008/03
Using heavy ion microbeam, we investigated the somatic mutation arising on the larvae in embyro and yolk in the egg of silkworm, . The incidence of the somatic mutation was 12%, and the same level of mutation following the microbeam irradiation at the center of the egg. However, the microbeam irradiation to the abdomen of the silkworm larvae induced the increase of somatic mutation, 63% (3 Gy) and 80% (6 Gy).
Yamasaki, Chisato*; Murakami, Katsuhiko*; Fujii, Yasuyuki*; Sato, Yoshiharu*; Harada, Erimi*; Takeda, Junichi*; Taniya, Takayuki*; Sakate, Ryuichi*; Kikugawa, Shingo*; Shimada, Makoto*; et al.
Nucleic Acids Research, 36(Database), p.D793 - D799, 2008/01
Times Cited Count：51 Percentile：71.25(Biochemistry & Molecular Biology)Here we report the new features and improvements in our latest release of the H-Invitational Database, a comprehensive annotation resource for human genes and transcripts. H-InvDB, originally developed as an integrated database of the human transcriptome based on extensive annotation of large sets of fulllength cDNA (FLcDNA) clones, now provides annotation for 120 558 human mRNAs extracted from the International Nucleotide Sequence Databases (INSD), in addition to 54 978 human FLcDNAs, in the latest release H-InvDB. We mapped those human transcripts onto the human genome sequences (NCBI build 36.1) and determined 34 699 human gene clusters, which could define 34 057 protein-coding and 642 non-protein-coding loci; 858 transcribed loci overlapped with predicted pseudogenes.
Ozawa, Masaki; Koyama, Shinichi; Suzuki, Tatsuya*; Fujita, Reiko*; Mimura, Hitoshi*; Fujii, Yasuhiko*
Proceedings of International Conference on Advanced Nuclear Fuel Cycles and Systems (Global 2007) (CD-ROM), p.451 - 457, 2007/09
To minimize the ecological burden originating in nuclear fuel recycling, a new R&D strategy, Adv.-ORIENT (Advanced Optimization by Recycling Instructive ElemeNTs) cycle, was set forth. A key separation tool is ion exchange chromatography (IXC) by a tertiary pyridine resin having soft donor nitrogen atoms. This method has provided individual recovery of pure Am and Cm products with a Pu/U/Np fraction from irradiated fuel in just a 3-step separation. A catalytic electrolytic extraction (CEE) method by Pd
has been employed to separate, purify and fabricate RMFP catalysts. High separation efficiency of RMFP proved hydrochloric acid as a suitable media for their recovery. Different functioned ion exchangers, e.g., ammonium molybdophosphate (AMP), have been investigated for the separation of Cs
. Theoretical and laboratory studies on the isotope separation of LLFPs were begun for 
Se, 
Sn and 
Cs.
Sano, Tadashi*; Wada, Seiichi*; Suzuki, Keiko*; Natsuhori, Masahiro*; Kakizaki, Takehiko; Ito, Takashi*; Nakazawa, Konomi*; Kobayashi, Yasuhiko; Ito, Nobuhiko*
JAEA-Review 2006-042, JAEA Takasaki Annual Report 2005, P. 115, 2007/02
, egg by the incidence of somatic mutation appearing in the larvaeFurusawa, Toshiharu*; Suzuki, Eiko*; Nagaoka, Shunji*; Suzuki, Hiromi*; Ishioka, Noriaki*; Hamada, Nobuyuki*; Wada, Seiichi*; Kobayashi, Yasuhiko; Sakashita, Tetsuya; Kakizaki, Takehiko; et al.
JAEA-Review 2006-042, JAEA Takasaki Annual Report 2005, P. 118, 2007/02
no abstracts in English
Ozawa, Masaki; Fujita, Reiko*; Koyama, Shinichi; Suzuki, Tatsuya*; Fujii, Yasuhiko*
Proceedings of 9th OECD/NEA Information Exchange Meeting on Actinide and Fission Product Partitioning and Transmutation, p.315 - 324, 2007/00
Catalytic Electrolytic extraction method has been studied as a separation tool for rare metal fission products, RMFP in the spent nuclear fuel. In an employed CEE process, Pd
cation itself would not only be easily deposited from various nitric acid solutions, but enhance also the deposition of co-existing RuNO, ReO
and 
TcO by acting as a catalyst. The quaternary-, Pd-Ru-Rh-Re, deposit Pt or Ti electrode, fabricated by CEE, suggested the highest cathodic current corresponding to the hydrogen generation reaction in both alkaline solution and sea water. Advanced ORIENT Cycle, where ion exchange chromatography using tertiary pyridine resin and the CEE employ as mainstay separation technology, will enhance separation and utilization of actinide and fission product, and thus be expected to realize ultimate reducing radioactive wastes.
Motoya, Kiyoichiro*; Hioki, Keiko*; Suzuki, Junichi
Journal of the Physical Society of Japan, 70(Suppl.A), p.139 - 141, 2001/05
no abstracts in English
Moribayashi, Kengo; Zhidkov, A. J.*; Sasaki, Akira; Sudo, Keiko; Suzuki, Shingo*
Atomic Collision Research in Japan, No.27, p.1 - 3, 2001/00
no abstracts in English
