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JAEA Reports

Practical guide on soil sampling, treatment, and carbon isotope analysis for carbon cycle studies

Koarashi, Jun; Atarashi-Andoh, Mariko; Nagano, Hirohiko*; Sugiharto, U.*; Saengkorakot, C.*; Suzuki, Takashi; Kokubu, Yoko; Fujita, Natsuko; Kinoshita, Naoki; Nagai, Haruyasu; et al.

JAEA-Technology 2020-012, 53 Pages, 2020/10


There is growing concern that recent rapid changes in climate and environment could have a significant influence on carbon cycling in terrestrial ecosystems (especially forest ecosystems) and could consequently lead to a positive feedback for global warming. The magnitude and timing of this feedback remain highly uncertain largely due to a lack of quantitative understanding of the dynamics of organic carbon stored in soils and its responses to changes in climate and environment. The tracing of radiocarbon (natural and bomb-derived $$^{14}$$C) and stable carbon ($$^{13}$$C) isotopes through terrestrial ecosystems can be a powerful tool for studying soil organic carbon (SOC) dynamics. The primary aim of this guide is to promote the use of isotope-based approaches to improve our understanding of the carbon cycling in soils, particularly in the Asian region. The guide covers practical methods of soil sampling; treatment and fractionation of soil samples; preparation of soil samples for $$^{13}$$C (and stable nitrogen isotope, $$^{15}$$N) and $$^{14}$$C analyses; and $$^{13}$$C, $$^{15}$$N, and $$^{14}$$C measurements by the use of isotope ratio mass spectrometry and accelerator mass spectrometry (AMS). The guide briefly introduces ways to report $$^{14}$$C data, which are frequently used for soil carbon cycling studies. The guide also reports results of a case study conducted in a Japanese forest ecosystem, as a practical application of the use of isotope-based approaches. This guide is mainly intended for researchers who are interested but are not experienced in this research field. The guide will hopefully encourage readers to participate in soil carbon cycling studies, including field works, laboratory experiments, isotope analyses, and discussions with great interest.

Journal Articles

Comprehensive analysis and evaluation of Fukushima Daiichi Nuclear Power Station Unit 2

Yamashita, Takuya; Sato, Ikken; Honda, Takeshi*; Nozaki, Kenichiro*; Suzuki, Hiroyuki*; Pellegrini, M.*; Sakai, Takeshi*; Mizokami, Shinya*

Nuclear Technology, 206(10), p.1517 - 1537, 2020/10

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Journal Articles

Numerical simulation of liquid jet behavior in shallow pool by interface tracking method

Suzuki, Takayuki*; Yoshida, Hiroyuki; Horiguchi, Naoki; Yamamura, Sota*; Abe, Yutaka*

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 7 Pages, 2020/08

Journal Articles

Numerical simulation of two-phase flow in 4$$times$$4 simulated bundle

Ono, Ayako; Yamashita, Susumu; Suzuki, Takayuki*; Yoshida, Hiroyuki

Mechanical Engineering Journal (Internet), 7(3), p.19-00583_1 - 19-00583_12, 2020/06

JAEA is implementing the 3D detailed nuclear-thermal-coupled analysis code to analyze the transition state of the core and to reduce the likelihood of the design. In the development plan, the computational fluid dynamics code based on the VOF method, JUPITER, is applied for TH part of the 3D detailed nuclear-thermal-coupled analysis code.

Journal Articles

Devil's staircase transition of the electronic structures in CeSb

Kuroda, Kenta*; Arai, Yosuke*; Rezaei, N.*; Kunisada, So*; Sakuragi, Shunsuke*; Alaei, M.*; Kinoshita, Yuto*; Bareille, C.*; Noguchi, Ryo*; Nakayama, Mitsuhiro*; et al.

Nature Communications (Internet), 11, p.2888_1 - 2888_9, 2020/06

 Times Cited Count:1 Percentile:34.82(Multidisciplinary Sciences)

Journal Articles

Spallation and fragmentation cross sections for 168 MeV/nucleon $$^{136}$$Xe ions on proton, deuteron, and carbon targets

Sun, X. H.*; Wang, H.*; Otsu, Hideaki*; Sakurai, Hiroyoshi*; Ahn, D. S.*; Aikawa, Masayuki*; Fukuda, Naoki*; Isobe, Tadaaki*; Kawakami, Shunsuke*; Koyama, Shumpei*; et al.

Physical Review C, 101(6), p.064623_1 - 064623_12, 2020/06

 Times Cited Count:0 Percentile:100(Physics, Nuclear)

The spallation and fragmentation reactions of $$^{136}$$Xe induced by proton, deuteron and carbon at 168 MeV/nucleon were studied at RIKEN Radioactive Isotope Beam Factory via the inverse kinematics technique. The cross sections of the lighter products are larger in the carbon-induced reactions due to the higher total kinetic energy of carbon. The energy dependence was investigated by comparing the newly obtained data with previous results obtained at higher reaction energies. The experimental data were compared with the results of SPACS, EPAX, PHITS and DEURACS calculations. These data serve as benchmarks for the model calculations.

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri. A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:1 Percentile:30.13(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

Journal Articles

Corrosion monitoring in humidity-controlled environment simulating gamma ray irradiation

Omori, Atsushi*; Akiyama, Eiji*; Abe, Hiroshi*; Hata, Kuniki; Sato, Tomonori; Kaji, Yoshiyuki; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; et al.

Zairyo To Kankyo, 69(4), p.107 - 111, 2020/04

To evaluate the effect of oxidants, which are formed by radiolysis of water under gamma ray irradiation, on the corrosion of a carbon steel in humid environment, ozone was introduced as a model oxidant in to humidity-controlled air at 50$$^{circ}$$C in a thermo-hygrostat chamber. Corrosion monitoring was performed by using an Atmospheric Corrosion Monitor-type (ACM) sensor consisting of a carbon steel anode and an Ag cathode. The output current of the ACM sensor was increased with the increase in relative humidity and it was obviously increased with the increase in the introduced ozone concentration at each relative humidity. The results indicate that ozone accelerates the corrosion of the carbon steel. The effect of ozone on the corrosion acceleration is attributed to the fast reduction reaction and fast dissolution reaction in to water compared to that of oxygen.

Journal Articles

The $$f$$-electron state of the heavy fermion superconductor NpPd$$_5$$Al$$_2$$ and the isostructural family

Metoki, Naoto; Aczel, A. A.*; Aoki, Dai*; Chi, S.*; Fernandez-Baca, J. A.*; Griveau, J.-C.*; Hagihala, Masato*; Hong, T.*; Haga, Yoshinori; Ikeuchi, Kazuhiko*; et al.

JPS Conference Proceedings (Internet), 30, p.011123_1 - 011123_6, 2020/03

Rare earths (4$$f$$) and actinides (5$$f$$) provide variety of interesting states realized with competing interactions between the increasing number of $$f$$ electrons. Since crystal field splitting of many-body $$f$$ electron system is smaller than the bandwidth, (1) high resolution experiments are needed, (2) essentially no clear spectrum with well defined peaks is expected in itinerant Ce and U compounds, and (3) Np and Pu is strictly regulated. Therefore, systematic research on magnetic excitations by neutron scattering experiments of localized compounds and rare earth iso-structural reference is useful. We describe the $$f$$ electron states of heavy electron compounds NpPd$$_5$$Al$$_2$$ and actinide and rare earth based iso-structural family.

Journal Articles

The Deposition densities of radiocesium and the air dose rates in undisturbed fields around the Fukushima Dai-ichi nuclear power plant; Their temporal changes for five years after the accident

Mikami, Satoshi; Tanaka, Hiroyuki*; Matsuda, Hideo*; Sato, Shoji*; Hoshide, Yoshifumi*; Okuda, Naotoshi*; Suzuki, Takeo*; Sakamoto, Ryuichi*; Ando, Masaki; Saito, Kimiaki

Journal of Environmental Radioactivity, 210, p.105941_1 - 105941_12, 2019/12

 Times Cited Count:9 Percentile:12.04(Environmental Sciences)

The deposition densities of radiocesium and the air dose rates were repeatedly measured in a large number of undisturbed fields within the 80km zone that surrounds the Fukushima Dai-ichi Nuclear Power Plant site between 2011 and 2016, and features of their temporal changes were clarified. The average air dose rate excluding background radiation in this zone decreased to about 20% of the initial value during the period from June 2011 to August 2016, which was essentially a result of the radioactive decay of $$^{134}$$Cs with a half-life of 2.06y. The air dose rate reduction was faster than that expected from the decay of radiocesium by a factor of about two, with most of this reduction being attributed to the penetration of radiocesium into the soil. The average deposition densities of $$^{134}$$Cs and $$^{137}$$Cs in fields that were not decontaminated were found to have decreased nearly according to their expected radioactive decay, which indicated that the movement of radiocesium in the horizontal direction was relatively small. The effect of decontamination was apparently observed in the measurements of air dose rates and deposition densities. Nominally, the average air dose rates in the measurement locations were reduced by about 20% by decontamination and other human activities, of which accurate quantitative analysis is and continue to be a challenge.

Journal Articles

Conceptual study on parasitic low-energy RI beam production with in-flight separator BigRIPS and the first stopping examination for high-energy RI beams in the parasitic gas cell

Sonoda, Tetsu*; Katayama, Ichiro*; Wada, Michiharu*; Iimura, Hideki; Sonnenschein, V.*; Iimura, Shun*; Takamine, Aiko*; Rosenbusch, M.*; Kojima, Takao*; Ahn, D. S.*; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(11), p.113D02_1 - 113D02_12, 2019/11

 Times Cited Count:0 Percentile:100(Physics, Multidisciplinary)

An in-flight separator, BigRIPS, at RIBF in RIKEN provides each experiment with specific nuclides separated from many nuclides produced by projectile fragmentation or in-flight fission. In this process, nuclides other than separated ones are discarded on the slits in BigRIPS, although they include many nuclides interested from the view point of nuclear structure. In order to extract these nuclides for parasitic experiments, we are developing a method using laser ion-source (PALIS). A test experiment with $$^{78}$$Se beam from RIBF has been performed by using a gas cell set in BigRIPS. Unstable nuclides around $$^{67}$$Se were stopped in the gas cell in accordance with a calculation using LISE code. The stopping efficiency has been estimated to be about 30%. As a next step, we will establish the technique for extracting reaction products from the gas cell.

Journal Articles

Comparative study on performance of various environmental radiation monitors

Tamakuma, Yuki*; Yamada, Ryohei; Suzuki, Takahito*; Kuroki, Tomohiro*; Saga, Rikiya*; Mizuno, Hiroyuki*; Sasaki, Hiroyuki*; Iwaoka, Kazuki*; Hosoda, Masahiro*; Tokonami, Shinji*

Radiation Protection Dosimetry, 184(3-4), p.307 - 310, 2019/10

 Times Cited Count:0 Percentile:100(Environmental Sciences)

After the Fukushima Daiichi Nuclear Power Plant accident, the radiation dose for first responders was not evaluated accurately due to lack of the monitoring data. It has been important to evaluate a radiation dose for workers in emergency response at a nuclear accident. In this study, a new device which can evaluate both of external and internal exposure doses was developed and the performance of various environmental radiation monitors including commercially available monitors were tested and compared from the viewpoint of an environmental monitoring at emergency situation. Background counts of the monitors and the ambient dose equivalent rate were measured in Fukushima Prefecture. The detection limit for beta particles was evaluated by the method of ISO11929. The sensitivity for gamma-rays of the dust monitor using a ZnS(Ag) and a plastic scintillator was high, but that of the external exposure monitor using a silicon photodiode with CsI(Tl) crystal was relatively low. The detection limit ranged 190-280 Bq m$$^{-3}$$ at 100 $$mu$$Sv h$$^{-1}$$, exceeding the detection limit of 100 Bq m$$^{-3}$$ in the minimum requirement by the National Regulation Authority in Japan. Use of the shielding with lead is necessary to achieve the minimum requirement. These results indicate that the dust monitor using a ZnS(Ag) scintillator and a plastic scintillator is suitable for the external exposure monitor and the developed internal exposure monitor is for the internal exposure monitor at emergency situation among the evaluated monitors. In the future study, the counting efficiency, the relative uncertainty and the performance of the detection for alpha particles will be evaluated, and it will be considered which type of a monitor is suitable after taking the portability into account.

Journal Articles

Experimental study of Gamow-Teller transitions via the high-energy-resolution $$^{18}$$O($$^3$$He,$$t$$)$$^{18}$$F reaction; Identification of the low-energy "super" -Gamow-Teller state

Fujita, Hirohiko*; Fujita, Yoshitaka*; Utsuno, Yutaka; Yoshida, Kenichi*; Adachi, Tatsuya*; Algora, A.*; Csatl$'o$s, M.*; Deaven, J. M.*; Estevez-Aguado, E.*; Guess, C. J.*; et al.

Physical Review C, 100(3), p.034618_1 - 034618_13, 2019/09

 Times Cited Count:1 Percentile:63.02(Physics, Nuclear)

no abstracts in English

Journal Articles

Study on the two-phase flow in simulated LWR fuel bundle by CFD code

Ono, Ayako; Yamashita, Susumu; Suzuki, Takayuki*; Yoshida, Hiroyuki

Proceedings of 18th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-18) (USB Flash Drive), p.666 - 677, 2019/08

An evaluation methodology of critical heat fluxes (CHFs) based on a mechanism for fuel assemblies in light water reactors (LWRs) is needed in order to design and evaluate the safety for the fuel assemblies in LWRs. In our study, the numerical simulation with surface-tracking will be applied for the two-phase flow in fuel assemblies in order to obtain the detail data relating to the size and velocity of bubbles in the subchannel, which is needed to predict the CHF based on the mechanism. In this study, the numerical simulation of two-phase flow in 4$$times$$4 bundle was implemented by using JUPITER in order to establish the evaluation method of the size and velocity of bubbles by the numerical simulation, which is the multi-physics simulation code and enable to track the gas-liquid surface. The simulation results are validated by the curve of flow regime for air-water under the adiabatic condition. The bubble and velocity of bubbles obtained by simulation results are analyzed.

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:4 Percentile:25.43(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

JAEA Reports

Construction of the sodium test loop in advanced technology experiment sodium facility (AtheNa)

Imamura, Hiroaki; Suzuki, Masashi*; Shimoyama, Kazuhito; Miyakoshi, Hiroyuki

JAEA-Technology 2019-005, 163 Pages, 2019/06


For the R&D of safety enhance in future fast reactor development, the constructed the large sodium test loop (mother loop) in advanced technology experiment sodium facility (AtheNa) was completed. The sodium test loop possesses the largest capacity of about 240 tons of the world's largest sodium and can supply impurity-controlled high temperature sodium to large structural and technology demonstration test sections. It is greatly expected as R&D such as future international cooperation. For the purpose of future R&D tests, this report compiled the design specifications, fabrication and performance confirmation results of sodium test loop.

Journal Articles

Study on loss-of-cooling and loss-of-coolant accidents in spent fuel pool, 1; Overview

Kaji, Yoshiyuki; Nemoto, Yoshiyuki; Nagatake, Taku; Yoshida, Hiroyuki; Tojo, Masayuki*; Goto, Daisuke*; Nishimura, Satoshi*; Suzuki, Hiroaki*; Yamato, Masaaki*; Watanabe, Satoshi*

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05

In this research program, cladding oxidation model in SFP accident condition, and numerical simulation method to evaluate capability of spray cooling system which was deployed for spent fuel cooling during SFP accident, have been developed. These were introduced into the severe accident codes such as MAAP and SAMPSON, and SFP accident analyses were conducted. Analyses using Computational Fluid Dynamics (CFD) code were conducted as well for the comparison with SA code analyses and investigation of detail in the SFP accident. In addition, three-dimensional criticality analysis method was developed as well, and safer loading pattern of spent fuels in pool was investigated.

Journal Articles

Evaluation of electronic state of Cs-adsorbed clay minerals by NEXAFS analysis using DFT calculations

Suzuki, Chikashi; Yaita, Tsuyoshi; Suzuki, Shinichi; Pacold, J.*; Altman, A. B.*; Minasian, S. G.*; Tyliszczak, T.*; Shuk, D. K.*; Yoshida, Hiroyuki; Osaka, Masahiko

Journal of Physics and Chemistry of Solids, 127, p.169 - 177, 2019/04

 Times Cited Count:1 Percentile:77.71(Chemistry, Multidisciplinary)

A combined method of NEXAFS measurement and DFT-calculation was employed for Cs evaluation in clay minerals. The Cs M$$_{4,5}$$ NEXAFS spectra of Cs halides were analyzed using the DFT-calculations, and were well reproduced by incorporating the core-hole strength. The Cs M$$_{4,5}$$ NEXAFS spectrum of clay minerals was well-reproduced by the DFT-calculations including the major transitions and tail structures with the established method. The further evaluation of this spectrum by charge density suggests that these major transitions and the tail structures likely reflect bonding states and local environments around the Cs atoms. Comparison of electronic states of Cs in the clay mineral with those in the Cs halides by DFT-calculations has shown that the interaction between Cs and the nearest-neighbor atom is largest in the clay mineral, because the energy level of Cs-5s and 5p is closer to that of O-2s and 2p than the s and p orbitals of other alkali metal and alkali earth metal elements.

Journal Articles

Observation of a Be double-Lambda hypernucleus in the J-PARC E07 experiment

Ekawa, Hiroyuki; Ashikaga, Sakiko; Hasegawa, Shoichi; Hashimoto, Tadashi; Hayakawa, Shuhei; Hosomi, Kenji; Ichikawa, Yudai; Imai, Kenichi; Kimbara, Shinji*; Nanamura, Takuya; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(2), p.021D02_1 - 021D02_11, 2019/02

 Times Cited Count:1 Percentile:100(Physics, Multidisciplinary)

Journal Articles

Measurement of water-steam flow behavior and pressure distribution in venturi scrubber

Uesawa, Shinichiro; Horiguchi, Naoki; Suzuki, Takayuki*; Shibata, Mitsuhiko; Yoshida, Hiroyuki

Proceedings of 12th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation and Safety (NUTHOS-12) (USB Flash Drive), 11 Pages, 2018/10

401 (Records 1-20 displayed on this page)