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Chimura, Motoki; Watanabe, Kazuhiko*; Takahashi, Hiroki; Hirano, Koichiro; Shinto, Katsuhiro; Kitamura, Ryo; Kawase, Masato*; Suzuki, Takahiro*; Morishita, Takatoshi
Proceedings of 22nd Annual Meeting of Particle Accelerator Society of Japan (Internet), p.709 - 713, 2026/03
no abstracts in English
Nakazawa, Yuga*; Cicek, E.*; Ishida, Katsuhiko*; Futatsukawa, Kenta*; Shimomura, Koichiro*; Otani, Masashi*; Kimura, Masato*; Kamioka, Shusei*; Yamazaki, Takayuki*; Mibe, Tsutomu*; et al.
Proceedings of 16th International Particle Accelerator Conference (IPAC25) (Internet), p.1163 - 1166, 2025/11
At the Japan Proton Accelerator Research Complex (J-PARC), low-emittance muon beams with a linear accelerator (linac) are proposed as a new approach to precisely measure the anomalous magnetic moment and electric dipole moment of the muon. Low-emittance muon beams can also be employed as new probes for non-destructive imaging techniques to see through structures. In the low-velocity section of the muon linac, a radio-frequency quadrupole linac (RFQ) and an interdigital H-mode drift tube linac (IH-DTL) are used to accelerate muons to 
= v/c = 0.08 and 0.28, respectively, at an operating frequency of 324 MHz. To reduce construction costs, the IH-DTL employs the alternating phase focusing (APF) method, which uses the transverse focusing force derived from the RF electric field. Because the APF method limits the transverse and longitudinal acceptances simultaneously, careful beam diagnostics and commissioning are essential to suppress the emittance growth derived from beam mismatches. As a result of the beam simulation, by conducting appropriate beam matching, the normalized rms emittance of 0.3 
-mm-mrad and the transmission to the downstream detector of 97% was obtained. In this paper, the results of the tracking simulation and the development status of the diagnostic and transport beamlines in the low-velocity section are described.
-molybdenum trioxide particles into waterYang, Y.*; Ngo, M. C.*; Kitagawa, Taiga*; Fujita, Yoshitaka; Takahashi, Yukiko*; Suzuki, Tatsuya*; Nakayama, Tadachika*; Do, T. M. D.*; Niihara, Koichi*; Suematsu, Hisayuki*
RSC Advances (Internet), 15(22), p.17222 - 17229, 2025/05
Times Cited Count：1 Percentile：24.56(Chemistry, Multidisciplinary)no abstracts in English
Hattori, Koichi*; Suenaga, Daiki*; Suzuki, Kei; Yasui, Shigehiro*
Physical Review B, 108(24), p.245110_1 - 245110_11, 2023/12
Times Cited Count：2 Percentile：13.49(Materials Science, Multidisciplinary)We develop a mean-field theory of a novel Kondo effect emerging in systems without a Fermi surface, which instead emerges under strong magnetic fields. We determine the magnitude of the Kondo condensate, which is a particle pairing composed of conducting Dirac fermions and localized impurities. We focus on the competition between the Kondo effect and the energy gap formation that stems from the pairing among the Dirac fermions leading to the dynamical chiral symmetry breaking. We find that this competition induces a quantum critical point. We also investigate finite-temperature effects. This system at vanishing fermion density can be studied with Monte Carlo lattice simulations, which do not suffer from the sign problem.
-MoO
whiskers in 
Mo/
Tc radioisotope production and Mo/Tc extraction using hot atomsNgo, M. C.*; Fujita, Yoshitaka; Suzuki, Tatsuya*; Do, T. M. D.*; Seki, Misaki; Nakayama, Tadachika*; Niihara, Koichi*; Suematsu, Hisayuki*
Inorganic Chemistry, 62(32), p.13140 - 13147, 2023/08
Times Cited Count：6 Percentile：48.29(Chemistry, Inorganic & Nuclear)Technetium-99m (Tc) is one of the most important radioisotopes for diagnostic radio-imaging applications. Tc is a daughter product of the Mo isotope. There are two methods used to produce Mo/Tc: the nuclear fission (n,f) and the neutron capture (n,
) methods. Between them, the (n,f) method is the main route, used for approximately 90% of the world's production. However, the (n,f) method faces numerous problems, including the use of highly enriched uranium, the release of highly radioactive waste, and nonproliferation problems. Therefore, the (n,) method is being developed as a future replacement for the (n,f) method. In this work, -MoO whiskers prepared by the thermal evaporation method and 
-MoO particles were irradiated in a nuclear reactor to produce Mo/Tc via neutron capture. The irradiated targets were dispersed into water to extract the Mo/Tc. As a result, -MoO whisker yielded higher Mo extraction rate than that from -MoO. In addition, by comparing the dissolved 
Mo concentrations in water, we clarified a prominent hot-atom of -MoO whiskers. This research is the first demonstration of -MoO being used as an irradiation target in the neutron capture method. On the basis of the results, -MoO is considered a promising irradiation target for producing Mo/Tc by neutron capture and using water for the radioisotope extraction process in the future.
Hattori, Koichi*; Suenaga, Daiki*; Suzuki, Kei; Yasui, Shigehiro*
EPJ Web of Conferences, 276, p.01015_1 - 01015_5, 2023/03
Times Cited Count：0 Percentile：0.00(Physics, Atomic, Molecular & Chemical)We investigate the QCD phase diagram in strong magnetic fields with heavy-quark impurities and determine the ground state within the mean-field analysis. The ground state is characterized by magnitudes of the pairing not only between the light quark and antiquark, i.e., chiral condensate, but also between the light quark and heavy-quark impurity, dubbed the Kondo condensate. We propose signatures of the interplay and/or competition between those two pairing phenomena reflected in the magnitude of the chiral condensate that is saturated with respect to the magnetic-field strength and anomalously increases with increasing temperature.
Uchino, Seiko*; Narita, Hirokazu*; Kita, Keisuke*; Suzuki, Hideya*; Matsumura, Tatsuro; Naganawa, Hirochika*; Sakaguchi, Koichi*; Oto, Keisuke*
Solvent Extraction Research and Development, Japan, 30(1), p.39 - 46, 2023/00
The extraction of trivalent rare earth ions (RE
) from HNO solution using a triamide amine, tris(N,N-di-2-ethylhexyl-ethylamide)amine (DEHTAA), was conducted, and the extraction mechanism was estimated from extraction behavior of HNO and RE and the relationship between atomic number and extraction percentages (E%) for RE. A DEHTAA molecule dominantly formed a DEHTAA HNO at 1.0 M HNO and a DEHTAA(HNO)
at 6.0 M HNO in the acid-equilibrated organic phase. This would provide the unique dependence of E% for the light RE on the HNO concentration, in which the E% value had a minimum and maximum at 
0.5 M and 2 M HNO, respectively. The results of the slope analyses for the distribution ratios for RE suggested that the dominant RE complex was RE(NO)DEHTAA(DEHTAA HNO) at 1.0 M HNO. The E% for RE decreased from La to Lu at 1.0 M HNO; on the other hand, those increased from La to Nd at 0.25 M and from La to Sm and 6.0 M HNO.
Ishikawa, Ryoya*; Suzuki, Masatoshi*; Kino, Yasushi*; Endo, Satoru*; Nakajima, Hiroo*; Oka, Toshitaka; Takahashi, Atsushi*; Shimizu, Yoshinaka*; Suzuki, Toshihiko*; Shinoda, Hisashi*; et al.
KEK Proceedings 2022-2, p.61 - 66, 2022/11
The balance between oxidative stress and antioxidant activity, which is a defense mechanism against oxidative stress, was investigated in the liver and bladder of wild Japanese macaques captured in Fukushima Prefecture. No significant induction of oxidative stress by exposure to environmental radionuclides after the Fukushima nuclear accident was observed, suggesting that the stress defense mechanism of the organism is activated in some organs.
Kondo, Yasuhiro; Kitamura, Ryo; Fuwa, Yasuhiro; Morishita, Takatoshi; Moriya, Katsuhiro; Takayanagi, Tomohiro; Otani, Masashi*; Cicek, E.*; Ego, Hiroyasu*; Fukao, Yoshinori*; et al.
Proceedings of 31st International Linear Accelerator Conference (LINAC 2022) (Internet), p.636 - 641, 2022/09
The muon linac project for the precise measurement of the muon anomalous magnetic and electric dipole moments, which is currently one of the hottest issues of the elementary particle physics, is in progress at J-PARC. The muons from the J-PARC muon facility are once cooled to room temperature, then accelerated up to 212 MeV with a normalized emittance of 1.5 mm mrad and a momentum spread of 0.1%. Four types of accelerating structures are adopted to obtain the efficient acceleration with a wide beta range from 0.01 to 0.94. The project is moving into the construction phase. We already demonstrated the re-acceleration scheme of the decelerated muons using a 324-MHz RFQ in 2017. The high-power test of the 324-MHz Interdigital H-mode (IH) DTL using a prototype cavity was performed in 2021. The fabrication of the first module of 14 modules of the 1296-MHz Disk and Washer (DAW) CCL will be done to confirm the production process. Moreover, the final design of the travelling wave accelerating structure for the high beta region is also proceeding. In this paper, the recent progress toward the realization of the world first muon linac will be presented.
Li, Y.; Katsumata, Genshichiro*; Masaki, Koichi; Hayashi, Shotaro*; Itabashi, Yu*; Nagai, Masaki*; Suzuki, Masahide*; Kanto, Yasuhiro*
Journal of Pressure Vessel Technology, 143(4), p.041501_1 - 041501_8, 2021/08
Times Cited Count：5 Percentile：24.21(Engineering, Mechanical)Segawa, Tomoomi; Kawaguchi, Koichi; Ishii, Katsunori; Suzuki, Masahiro; Tachihara, Joji; Takato, Kiyoto; Okita, Takatoshi; Satone, Hiroshi*; Suzuki, Michitaka*
Mechanical Engineering Journal (Internet), 8(3), p.21-00022_1 - 21-00022_9, 2021/06
To reduce the hold-up of the nuclear fuel materials in the glove box and the external exposure dose, the technology of the MOX powder adhesion prevention by the nanoparticle coating to the acrylic panels of the glove box has been developed. The surface analysis by means of atomic force microscopy (AFM) showed that the acrylic test piece surface coated with nanoparticles had a higher root mean square roughness value than that non-coated with nanoparticles. Due to the formation of nano-sized tiny rugged surface, the nanoparticle coating reduced the minimum adhesion force between the UO particles and the acrylic test piece surface with the smallest particle size of about 5 
m where desorption was observed, by about one-tenth. Moreover, the nanoparticle coating reduced the amount of the MOX powder adhering to the acrylic test piece to about one-tenth. In this study, it was found that applying the nanoparticle coating to the acrylic panels of glove box can prevent the adhesion of nuclear fuel materials. This method is effective for reducing the hold-up of the nuclear fuel materials in the glove box, the external exposure dose and improving the visibility of the acrylic panels.
Ito, Michitane*; Mukai, Tomohisa*; Suzuki, Hiroshi; Nanbu, Yoshihito*; Suzuki, Junichi*; Matsuzawa, Koichi*; Kinugasa, Hideyuki*
Nihon Kenchiku Gakkai Gijutsu Hokokushu, 27(65), p.99 - 103, 2021/02
no abstracts in English
for production of 
Tc radioactive isotopeSuematsu, Hisayuki*; Sato, Soma*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Niihara, Koichi*; Nanko, Makoto*; Tsuchiya, Kunihiko
Journal of Asian Ceramic Societies (Internet), 8(4), p.1154 - 1161, 2020/12
Times Cited Count：5 Percentile：17.57(Materials Science, Ceramics)Pulsed electric current sintering of molybdenum trioxide (MoO) was carried out by one- and two-step pressuring methods for fabrication of irradiation target using production of Mo and Tc nuclear medicine. At 550
C by the two-step pressurizing method, a relative density of 93.1% was obtained while, by the one-step pressurization method, the relative density was 76.9%. Direct sample temperature measurements were conducted by inserting a thermocouple in a punch. By the two-step pressurizing method, the sample temperature was higher than that by the one-step pressurizing method even almost the same die temperature. From voltage and current waveforms, it was thought that the conductivity of the sample increased by the two-step pressurizing method to increase the sample temperature and the relative density. The two-step pressurization method enables us to prepare dense targets at a low temperature from recycled and coarse-grained Mo enriched MoO powder.
Segawa, Tomoomi; Kawaguchi, Koichi; Ishii, Katsunori; Suzuki, Masahiro; Fukasawa, Tomonori*; Fukui, Kunihiro*
Funtai Kogakkai-Shi, 57(9), p.485 - 494, 2020/09
In the spent fuel reprocessing process, a mixed solution of uranyl nitrate and plutonium nitrate is converted into mixed oxide powder by the microwave heating. To evaluate the applicability to the industrial-scale and acquire the characteristics data of the microwave heating denitration of various metal nitrate aqueous solutions based on the knowledge studied in the development of laboratory-scale basic experiments, the microwave heating characteristics and metal oxide powder properties were investigated using cerium nitrate, cobalt nitrate and copper nitrate aqueous solutions. The progress rate of the denitration reaction was depended on the position, and the denitration reaction proceeded faster at the periphery than at the center. The morphologies of the synthesized products were porous and hard dry solid with cerium nitrate aqueous solution, foamed dry solid with cobalt nitrate aqueous solution, and powdery particles with copper nitrate aqueous solution. The denitration ratio and average particle size of the synthesized products increased in the order of the cerium nitrate aqueous solution, the cobalt nitrate aqueous solution, and the copper nitrate aqueous solution. The numerical simulations revealed that the periphery of the bottom surface of the metal nitrate aqueous solution was heated by microwaves. This results consistent with the experimental results in which the denitration reaction started from the periphery of the metal nitrate aqueous solution.
Segawa, Tomoomi; Kawaguchi, Koichi; Ishii, Katsunori; Suzuki, Masahiro; Tachihara, Joji; Takato, Kiyoto; Okita, Takatoshi; Satone, Hiroshi*; Suzuki, Michitaka*
Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08
To reduce the hold-up of the nuclear fuel materials in the glove box and the external exposure dose, the technology of the MOX powder adhesion prevention by the nanoparticle coating to the acrylic panels of the glove box has been developed. Due to the formation of nano-sized tiny rugged surface, the nanoparticle coating reduced the minimum adhesion force between the UO particles and the acrylic test piece surface with the smallest particle size of about 5 m where desorption was observed, by about one-tenth. Moreover, the nanoparticle coating reduced the amount of the MOX powder adhering to the acrylic test piece to about one-tenth. In this study, it was found that applying the nanoparticle coating to the acrylic panels of glove box can prevent the adhesion of nuclear fuel materials. This method is effective for reducing the hold-up of the nuclear fuel materials in the glove box, the external exposure dose and improving the visibility of the acrylic panels.
Xe ions on proton, deuteron, and carbon targetsSun, X. H.*; Wang, H.*; Otsu, Hideaki*; Sakurai, Hiroyoshi*; Ahn, D. S.*; Aikawa, Masayuki*; Fukuda, Naoki*; Isobe, Tadaaki*; Kawakami, Shunsuke*; Koyama, Shumpei*; et al.
Physical Review C, 101(6), p.064623_1 - 064623_12, 2020/06
Times Cited Count：8 Percentile：53.94(Physics, Nuclear)The spallation and fragmentation reactions of Xe induced by proton, deuteron and carbon at 168 MeV/nucleon were studied at RIKEN Radioactive Isotope Beam Factory via the inverse kinematics technique. The cross sections of the lighter products are larger in the carbon-induced reactions due to the higher total kinetic energy of carbon. The energy dependence was investigated by comparing the newly obtained data with previous results obtained at higher reaction energies. The experimental data were compared with the results of SPACS, EPAX, PHITS and DEURACS calculations. These data serve as benchmarks for the model calculations.
OYamakawa, Koichiro; Nasu, Hirokazu*; Suzuki, Natsumi*; Shimizu, Genki*; Arakawa, Ichiro*
Journal of Chemical Physics, 152(17), p.174310_1 - 174310_13, 2020/05
Times Cited Count：2 Percentile：6.66(Chemistry, Physical)We have established an apparatus for terahertz and mid-infrared spectroscopy in an ultrahigh vacuum and have measured absorption spectra of DO clusters trapped in solid Ar. To assign terahertz absorption peaks due to the DO dimer, trimer, and tetramer, the dependence of the spectrum on the annealing temperature and DO dilution was analyzed. The assignment was also examined by ab initio calculations with use of the ONIOM method, where flexibility of surrounding Ar atoms was systematically incorporated. We identified all of the intermolecular fundamentals of the dimer and those with significant intensities of the trimer and tetramer, whose structural symmetries were revealed to be broken down. After isolating the DO clusters in solid Ar, we sublimated only Ar atoms to leave behind matrix-sublimation ice, which was found to be amorphous- or crystal-like depending on the formation conditions: the dilution and sublimation-temperature. Since the crystallinity got higher with raising the dilution and sublimation-temperature, the diffusion of the DO monomer on the surface of sublimating solid Ar was found to be crucial to the crystallization of the sublimation ice.
F from 
O
?Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.
Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05
Times Cited Count：20 Percentile：70.10(Physics, Multidisciplinary)The structure of a neutron-rich F nucleus is investigated by a quasifree (
) knockout reaction. The sum of spectroscopic factors of 
orbital is found to be 1.0 
0.3. The result shows that the O core of F nucleus significantly differs from a free O nucleus, and the core consists of 35% O
, and 65% excited O. The result shows that the O core of F nucleus significantly differs from a free O nucleus. The result may infer that the addition of the 
proton considerably changes the neutron structure in F from that in O, which could be a possible mechanism responsible for the oxygen dripline anomaly.
Sekine, Megumi; Matsuki, Takuya; Suzuki, Satoshi*; Tsutagi, Koichi; Nishida, Naoki; Kitao, Takahiko; Tomikawa, Hirofumi; Nakamura, Hironobu; LaFleur, A.*; Browne, M.*
JAEA-Technology 2019-023, 160 Pages, 2020/03
JAEA-Technology-2019-023.pdf:9.43MB
The International Atomic Energy Agency (IAEA) has proposed in its Research and Development plan (STR-385), the development of technology to enable real-time flow measurement of nuclear material as a part of an advanced approach to effective and efficient safeguards for reprocessing facilities. To address this, Japan Atomic Energy Agency (JAEA) has been tackling development of a new detector to enable monitoring of Pu in solutions with numerous FPs as a joint research program with U.S. DOE to cover whole reprocessing process. In this study, High Active Liquid Waste (HALW) Storage Facility in Tokai Reprocessing Plant was used as the test field. At first, the design information of HALW storage tank and radiation (type and intensity) were investigated to develop a Monte Carlo N-Particle Transport Code (MCNP) model. And then, dose rate distribution outside/ inside of the concrete cell where the HALW tank is located was measured to design new detectors and check MCNP model applicability. Using the newly designed detectors, gamma rays and neutron were continuously measured at the outside/ inside of the concrete cell to assess the radiation characteristics and to optimize detector position. Finally, the applicability for Pu monitoring technology was evaluated based on the simulation results and gamma-ray/neutron measurement results. We have found that there is possibility to monitor the change of Pu amount in solution by combination both of gamma-ray and neutron measurement. The results of this study suggested the applicability and capability of the Pu motoring to enhance safeguards for entire reprocessing facility which handles Pu with FP as a feasibility study. This is final report of this project.
Ikushima, Kazuki*; Shibahara, Masakazu*; Kawajiri, Yoshitaka*; Okimi, Yui*; Uchida, Tomoki*; Akita, Koichi*; Suzuki, Hiroshi; Morooka, Satoshi
Nihon Senpaku Kaiyo Kogakkai Rombunshu, (30), p.123 - 130, 2019/12
In this research, the contour method was applied to measure the residual stress distribution of a bead-on-plate specimen. The measured residual stress distribution was compared with those measured by neutron diffraction method and calculated by thermal elastic plastic finite element analysis. As a result, it was found that the residual stress distribution obtained by these three methods are in good agreement. In addition, the equilibrium of reaction force on cut plane was considered in the contour method to measure residual stresses in asymmetric cutting which is assumed in the measurement of real structures. The proposed method was applied to the measurement of the residual stress in the multi-pass welded joint. The measured results indicated that the proposed method can measure the residual stress distribution in multi-pass welded joint in asymmetric test specimen.
