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Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.
Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08
Times Cited Count：2 Percentile：20.55(Chemistry, Multidisciplinary)The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 
C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl
TaOCl
DbOCl. From the obtained experimental results, thermochemical data for DbOCl were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.
Mo-adsorption/
Tc-elution properties of alumina with different surface structuresFujita, Yoshitaka; Seki, Misaki; Sano, Tadafumi*; Fujihara, Yasuyuki*; Kitagawa, Tomoya*; Matsukura, Minoru*; Hori, Junichi*; Suzuki, Tatsuya*; Tsuchiya, Kunihiko
Journal of Radioanalytical and Nuclear Chemistry, 327(3), p.1355 - 1363, 2021/03
Times Cited Count：1 Percentile：21.98(Chemistry, Analytical)We prepared three types of Al
O
with different surface structures and investigated Mo-adsorption/Tc-elution properties using [Mo]MoO that was irradiated in the Kyoto University Research Reactor. AlO adsorbed [Mo]molybdate ions in solutions at different pH; the lower was the pH, the higher was the Mo-adsorption capacity of AlO. The Tc-elution properties of molybdate ion adsorbed AlO were elucidated by flowing saline. Consequently, it was suggested that Mo-adsorption/desorption properties are affected by the specific surface of AlO and Tc-elution properties are affected by the crystal structure of AlO.
Sonoda, Tetsu*; Katayama, Ichiro*; Wada, Michiharu*; Iimura, Hideki; Sonnenschein, V.*; Iimura, Shun*; Takamine, Aiko*; Rosenbusch, M.*; Kojima, Takao*; Ahn, D. S.*; et al.
Progress of Theoretical and Experimental Physics (Internet), 2019(11), p.113D02_1 - 113D02_12, 2019/11
Times Cited Count：1 Percentile：12.78(Physics, Multidisciplinary)An in-flight separator, BigRIPS, at RIBF in RIKEN provides each experiment with specific nuclides separated from many nuclides produced by projectile fragmentation or in-flight fission. In this process, nuclides other than separated ones are discarded on the slits in BigRIPS, although they include many nuclides interested from the view point of nuclear structure. In order to extract these nuclides for parasitic experiments, we are developing a method using laser ion-source (PALIS). A test experiment with 
Se beam from RIBF has been performed by using a gas cell set in BigRIPS. Unstable nuclides around 
Se were stopped in the gas cell in accordance with a calculation using LISE code. The stopping efficiency has been estimated to be about 30%. As a next step, we will establish the technique for extracting reaction products from the gas cell.
Suzuki, Minoru*; Sakai, Takaaki*; Takata, Takashi; Doda, Norihiro
Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 7 Pages, 2019/05
With an aim to establish a quantitative risk assessment of accident managements (AMs) for various external hazards, the plant dynamics analyses with Continuous Markov Chain Monte Carlo (CMMC) method were carried out to assess repeatedly occurred multi-failures by volcano ash in volcanic eruption event. AM repetition of the filter exchange to recover the cooling function of the air coolers were considered. The results showed that this method can evaluate the effectiveness of AM measures against volcanic ash fall events with respect to time progress.
Kumazaki, Yui; Suzuki, Satoru; Kanazawa, Masashi*; Kunii, Katsuhiko; Yonezawa, Minoru; Itabashi, Keizo*
The Grey Journal; An International Journal on Grey Literature, 15(1), p.45 - 50, 2019/04
JAEA Library focuses on collecting conference proceedings and technical reports which are very important and referred materials for our users in the field of nuclear science and technology. There are an increasing number of cases that they are published in electronic media such as CD-ROM and flash memories. There are problems as to manage such electronic media in a library. Largest problems for electronic media would be the long-term preservation and permanent access. Lifetime of electronic media are much shorter compared with paper and/or microfilm. In this regard, the JAEA library is struggling to preserve electronic media including related PCs and software for a long-term. One of the effective countermeasure should be preserving PCs and software to browse, emulation and migration to another media. However, our countermeasure is not good enough for users and preservation. The authors would like to present JAEA Library's current activities on long term preservation and use of electronic media, and it comes to the conclusion the fact that even published electronic media are becoming grey literature in certain environment.
Kumazaki, Yui; Suzuki, Satoru; Kanazawa, Masashi*; Kunii, Katsuhiko; Yonezawa, Minoru; Itabashi, Keizo
Proceedings of 20th International Conference on Grey Literature (GL-20), p.99 - 104, 2019/02
JAEA Library focuses on collecting conference proceedings and technical reports which are very important and referred materials for our users in the field of nuclear science and technology. There are an increasing number of cases that they are published in electronic media such as CD-ROM and flash memories. There are problems as to manage such electronic media in a library. Largest problems for electronic media would be the long-term preservation and permanent access. Lifetime of electronic media are much shorter compared with paper and/or microfilm. In this regard, the JAEA library is struggling to preserve electronic media including related PCs and software for a long-term. One of the effective countermeasure should be preserving PCs and software to browse, emulation and migration to another media. However, our countermeasure is not good enough for users and preservation. The authors would like to present JAEA Library's current activities on long term preservation and use of electronic media, and it comes to the conclusion the fact that even published electronic media are becoming grey literature in certain environment.
Mo/Tc generatorsSuzuki, Yoshitaka; Kitagawa, Tomoya*; Namekawa, Yoji*; Matsukura, Minoru*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko
Transactions of the Materials Research Society of Japan, 43(2), p.75 - 80, 2018/04
no abstracts in English
Suzuki, Yoshitaka; Ishida, Takuya*; Suzuki, Yumi*; Matsukura, Minoru*; Kurosaki, Fumio*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko
JAEA-Technology 2016-027, 24 Pages, 2016/12
JAEA-Technology-2016-027.pdf:4.15MB
The research and development (R&D) on the production of Mo/Tc by (n,
) method has been carried out in the Neutron Irradiation and Testing Reactor Center. The Mo production by (n,) reaction is a simple and easy method, and it also is advantageous from viewpoints of nuclear proliferation resistance and waste management. However, it is difficult to produce the Tc solution with high radioactive concentration because the specific radioactivity of Mo by this method is extremely low. Up to now, various Mo absorbents such as Polyzirconium Compound (PZC) and Polytitanium Compound (PTC) have been developed with high Mo adsorption efficiency. It is necessary for utilization to the generator of these absorbents to evaluate the effect of elements containing these absorbents and to assure the quality of Tc solution. In this report, the status of R&D of the Mo adsorbents was investigated. The alumina as Mo adsorbent, which uses in medical Mo/Tc generator, was focused and Mo adsorption/desorption properties of three kinds of alumina was evaluated by different properties such as crystal structure and specific surface.
pellets for Mo-99 production, 3Ishida, Takuya; Suzuki, Yoshitaka; Nishikata, Kaori; Yonekawa, Minoru; Kato, Yoshiaki; Shibata, Akira; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; et al.
KURRI Progress Report 2015, P. 64, 2016/08
no abstracts in English
Miyao, Tomoaki*; Miura, Akihiko; Kawane, Yusuke; Tamura, Jun; Nemoto, Yasuo; Ao, Hiroyuki*; Hayashi, Naoki; Oguri, Hidetomo; Ouchi, Nobuo; Mayama, Minoru*; et al.
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1338 - 1341, 2015/09
no abstracts in English
-phase and high-pressure 
-phase of pure group IV transition metalsAdachi, Nozomu*; Todaka, Yoshikazu*; Suzuki, Hiroshi; Umemoto, Minoru*
Scripta Materialia, 98, p.1 - 4, 2015/03
Times Cited Count：13 Percentile：53.2(Nanoscience & Nanotechnology)The deformation texture of the high-pressure -phase of pure group IV metals was investigated using neutron diffraction analysis. The 
0001
direction gradually aligned to the shear direction with an increase in the shear strain introduced by the high-pressure torsion process. The deformation texture suggested that the main slip system of the -phase was {11-20}0001. We experimentally observed the orientation relationships of the mechanically stabilized -phase with respect to the reverse-transformed -phase, and determined that the relationship was similar to that proposed by Silcock and Rabinkin.
Kimura, Hideo; Aoyagi, Tetsuo; Sato, Taiichi; Sakai, Manabu; Hikasa, Naoki*; Suzuki, Hitoshi; Tsuji, Minoru
JAEA-Technology 2011-027, 31 Pages, 2011/09
JAEA-Technology-2011-027.pdf:2.16MB
The financial accounting and contract management system of JAEA, built on a commercial ERP package, had suffered from serious problems of high lifecycle cost, poor response, and lack of extensibility, due to the too much customization to the ERP package, and disorganized software structure. To solve those problems, three approaches were applied; (1) conducting thorough analysis of business flow and fit/gap, which enabled removing all customization brought to the ERP package; (2) dividing the system into subsystems, and clearly defining interfaces between the subsystems, which increases the transparency, extensibility and performance of the system; (3) outsourcing the development of the subsystems to multiple venders to reduce the development cost. Those approaches can be useful for developing business information systems using commercial software to save time and cost, while meeting the unique requirements of an organization.
Iijima, Kazuki; Tomura, Tsutomu*; Tobita, Minoru*; Suzuki, Yasuyuki*
Radiochimica Acta, 98(9-11), p.729 - 736, 2010/11
Times Cited Count：2 Percentile：17.77(Chemistry, Inorganic & Nuclear)Distribution behavior of Cs and Am in the synthetic groundwater-bentonite colloids-granite ternary system was investigated. Radionuclide sorbed onto the bentonite colloids is desorbed by addition of granite, indicating that the sorption of Cs and Am onto the bentonite colloids are reversible. The sorption model based on cation exchange and surface complexation reaction considering high edge site density for bentonite colloids is applicable to explain the sorption behavior of Am and Cs in the ternary system.
Horiguchi, Hironori; Nakamura, Takemi; Kumada, Hiroaki*; Yanagie, Hironobu*; Suzuki, Minoru*; Sagawa, Hisashi
Proceedings of 14th International Congress on Neutron Capture Therapy (ICNCT-14) (CD-ROM), p.234 - 237, 2010/10
Recurrent breast cancer has been considered the application for boron neutron capture therapy using the JRR-4. The investigation of irradiation conditions for the recurrent breast cancer was performed by simulation with the JCDS. We performed the preliminary dosimetry of the model to verify the efficient irradiation conditions such as the neutron energy modes and multiple field technique. From the result, when the 30 Gy-Eq dose as minimum dose was delivered to the cancers, comparable dose distribution was delivered at the healthy tissues by both a one-port irradiation from anterior direction and a two-port irradiation from tangential direction. We revealed that the two-port irradiation was not valid to reduce the healthy tissues dose due to the isotopic scattering of neutrons in the body. We concluded that the optimal irradiation condition was the one-port irradiation with thermal neutron beam mode in terms of less healthy tissues dose and shorter irradiation time.
Yanagie, Hironobu*; Kumada, Hiroaki*; Nakamura, Takemi; Higashi, Shushi*; Ikushima, Ichiro*; Morishita, Yasuyuki*; Shinohara, Atsuko*; Fujiwara, Mitsuteru*; Suzuki, Minoru*; Sakurai, Yoshinori*; et al.
Proceedings of 14th International Congress on Neutron Capture Therapy (ICNCT-14) (CD-ROM), p.157 - 160, 2010/10
Kobayashi, Takayuki; Isayama, Akihiko; Fasel, D.*; Yokokura, Kenji; Shimono, Mitsugu; Hasegawa, Koichi; Sawahata, Masayuki; Suzuki, Sadaaki; Terakado, Masayuki; Hiranai, Shinichi; et al.
Journal of Plasma and Fusion Research SERIES, Vol.9, p.363 - 368, 2010/08
Improvements are required for expanding the pulse length of the JT-60 ECRF system (5s) for JT-60SA (100s). Newly developed power supplies will be fabricated and installed by EU. The conditioning operation of an improved gyrotron equipping a newly designed mode convertor has been started. The mode convertor will reduce heat flux on the internal components and therefore expected to enable long pulse operation at 1 MW. Pre-programmed and/or feedback control of the heater current and anode voltage, which was successfully demonstrated in JT-60U, will be key techniques because the beam current decreases during a shot. The evacuated transmission lines have a capability of 1 MW per line. Since maintenance of the components in the vacuum vessel is difficult, a linear motion antenna concept was proposed to reduce risks of water leakage and fault of the driving mechanism in the vacuum vessel. The detailed design and the low power test of a mock-up antenna have been started.
Sakakibara, Tetsuro; Aoyama, Yoshio; Yamaguchi, Hiromi; Sasaki, Naoto*; Nishikawa, Takeshi*; Murata, Minoru*; Park, J.*; Taniguchi, Shoji*; Fujita, Michiru*; Fukuda, Tomoyuki*; et al.
Proceedings of International Waste Management Symposium 2009 (WM '09) (CD-ROM), 15 Pages, 2009/03
The volume reduction treatment of solid waste system by ultra-high frequency induction furnace (UHFIF) was developed from FY2005 to FY2007. Basic data for melting performance were collected by non-radioactive experiments using the bench scale UHFIF with a crucible capacity of 10 liters. Based on the obtained data, engineering specifications were evaluated for a demonstration scale UHFIF with a crucible capacity of 30 liters. A new demonstration scale UHFIF was constructed and melting experiments of surrogate wastes were carried out by this furnace. It was confirmed that the demonstration scale UHFIF can melt ferrous metal, ceramics and aluminum all together and stabilize aluminum by oxidation to alumina. Density, chemical composition, and surface condition of the solidified substances were analyzed, and homogeneity of the solidified substances was confirmed. Melting behavior in the demonstration scale UHFIF was analyzed by computer simulation and simulation results agreed well with the experimental ones. From the design study for a full scale UHFIF with a crucible capacity of 100 liters, basic specifications were evaluated for the full scale UHFIF. Based on the obtained specification, melting behavior in the full scale UHFIF was analyzed by computer simulation.
Kawamata, Yoichi; Naito, Osamu; Kiyono, Kimihiro; Itami, Kiyoshi; Totsuka, Toshiyuki; Akasaka, Hiromi; Sueoka, Michiharu; Sato, Tomoki; Oshima, Takayuki; Sakata, Shinya; et al.
Fusion Engineering and Design, 83(2-3), p.198 - 201, 2008/04
Times Cited Count：3 Percentile：23.9(Nuclear Science & Technology)The design activity of JT-60SA (JT-60 Super Advanced) which is remodeled to a superconducting tokamak device has been starting under the JA-EU collaborative ITER-BA project. For the JT-60SA control system, the existing system should be reused as much as possible from the viewpoint of cost-effectiveness. We have just begun to discuss the configuration of the advanced Supervisory Control System (SVCS) including the following systems: (1) ultimately flexible real-time control system, (2) precise timing system enough to clarify cause and effect, and (3) safety shutdown control system. In this report, we present the design study of the JT-60SA SVCS with focusing on these systems.
Iba, Katsuyuki*; Ozeki, Takahisa; Totsuka, Toshiyuki; Suzuki, Yoshio; Oshima, Takayuki; Sakata, Shinya; Sato, Minoru; Suzuki, Mitsuhiro; Hamamatsu, Kiyotaka; Kiyono, Kimihiro
Fusion Engineering and Design, 83(2-3), p.495 - 497, 2008/04
Times Cited Count：4 Percentile：29.91(Nuclear Science & Technology)Fusion research grid is an environment of collaborative researches using a network that connects scientists far apart and let them collaborate effectively over the difference in time and distance in a nuclear fusion research. Fundamental technology of Fusion research grid has been developed at JAEA in the VizGrid project under the e-Japan project at Ministry of Education, Culture, Sports, Science and Technology (MEXT). Remote research environments of experiments, diagnostics, analyses and communications were developed on Fusion research grid. We have developed prototype systems that include a remote experiment system, a remote diagnostics system, and a remote analysis system. All users can access these systems from anywhere because Fusion research grid does not required closed network like Super SINet to maintain security. The prototype systems were verified in experiments at JT-60U and their availability was confirmed.
-FeSi grown using high-purity FeSi sourceGoto, Kohei*; Suzuki, Hirokazu*; Udono, Haruhiko*; Kikuma, Isao*; Esaka, Fumitaka; Uchikoshi, Masahito*; Isshiki, Minoru*
Thin Solid Films, 515(22), p.8263 - 8267, 2007/08
Times Cited Count：15 Percentile：56.32(Materials Science, Multidisciplinary)We have investigated the effect of FeSi source purity on the electrical property of -FeSi grown from solution. A high purity FeSi source avoided a contamination of Cu and W metals was synthesized by melting a high purity Fe (5N) and Si (5N-up) in a quartz ampoule. The -FeSi crystals grown using the high purity FeSi and Zn solvent showed n-type conduction, whereas those grown using the arc-melted FeSi showed p-type. From the SIMS analysis of the grown crystals, we found that dominant impurity concentrations in the p-type crystals were higher than those in the n-type ones.
