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Journal Articles

Intercalative and non-intercalative photo-recharge using all-solid-state cells for solar energy conversion and storage

Yoshimoto, Masataka*; Tamura, Kazuhisa; Watanabe, Kenta*; Shimizu, Keisuke*; Horisawa, Yuhei*; Kobayashi, Takeshi*; Tsurita, Hanae*; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

Sustainable Energy & Fuels (Internet), 8(6), p.1236 - 1244, 2024/03

Photo-rechargeable systems, which can efficiently convert and store solar energy into chemical energy within single devices, are essential to harness sunlight effectively. Photo-(de)intercalation plays a pivotal role in the functionality of photorechargeable systems. Nevertheless, the photo-(de)intercalation process has not been conclusively confirmed owing to potential interference from side reactions, such as the decomposition of liquid electrolytes and the elution of electrode materials. In this study, we successfully demonstrated photo-responsive Li$$^{+}$$-deintercalation using an all-solid-state thin-film battery comprised of epitaxially-grown anatase TiO$$_{2}$$ doped with Nb (a-TiO$$_{2}$$:Nb) as the cathode. Under light irradiation, Li$$^{+}$$-deintercalation occurred and was subsequently reversibly intercalated into a-TiO$$_{2}$$:Nb during discharge.

Journal Articles

Stable photoelectrochemical reactions at solid/solid interfaces toward solar energy conversion and storage

Watanabe, Kenta*; Horisawa, Yuhei*; Yoshimoto, Masataka*; Tamura, Kazuhisa; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

Nano Letters, 24(6), p.1916 - 1922, 2024/02

Electrochemistry has extended from reactions at solid/liquid interfaces to those at solid/solid interfaces. In this study, we achieve the stable photoelectrochemical reaction at the semiconductor-electrode/solid-electrolyte interface in Nb-doped anatase-TiO$$_{2}$$ (a-TiO$$_{2}$$:Nb)/Li$$_{3}$$PO$$_{4}$$ (LPO)/Li all-solid-state cell. The oxidative currents of a-TiO$$_{2}$$:Nb/LPO/Li increase upon light irradiation when a-TiO$$_{2}$$:Nb is located at a potential that is more positive than its flat-band potential. The photoelectrochemical reaction at the semiconductor/solid-electrolyte interface is driven by the same principle as that at semiconductor/liquid-electrolyte interfaces. Thus, we extend photoelectrochemistry to all-solid-state systems composed of solid/solid interfaces.

Journal Articles

Applicability confirmation experiment of DDSI method for quantification of plutonium in fuel debris

Mitsuboshi, Natsumi; Nagatani, Taketeru; Kosuge, Yoshihiro*; Suzuki, Risa; Okada, Toyofumi

Dai-44-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2023/11

This paper reports the applicability confirmation experiment of DDSI method for quantification of plutonium in fuel debris. We conducted passive neutron measurement for the samples which consist of un-irradiated MOX sample, Cf-252 neutron source, and B-10 neutron absorber to simulate the fuel debris. It was revealed that DDSI method has enough capability to evaluate the leakage multiplication of the sample with unknown amounts of fissile material and neutron absorbers.

Journal Articles

Preliminary measurement of prompt gamma-ray from nuclear material for the classification of fuel debris and waste

Shiba, Tomooki; Kaburagi, Masaaki; Nomi, Takayoshi; Suzuki, Risa; Kosuge, Yoshihiro*; Nauchi, Yasushi*; Takada, Akira*; Nagatani, Taketeru; Okumura, Keisuke

Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR2022) (Internet), 3 Pages, 2022/10

Journal Articles

Study on identification of materials in fuel debris and waste by neutron induced gamma ray spectroscopy

Nauchi, Yasushi*; Nomi, Takayoshi; Suzuki, Risa; Kosuge, Yoshihiro*; Shiba, Tomooki; Takada, Akira*; Kaburagi, Masaaki; Okumura, Keisuke

Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR2022) (Internet), 4 Pages, 2022/10

Journal Articles

Project management efforts in the decommissioning project of Tokai Reprocessing Plant

Taguchi, Shigeo; Taguchi, Katsuya; Makino, Risa; Yamanaka, Atsushi; Suzuki, Kazuyuki; Takano, Masato; Koshino, Katsuhiko; Ishida, Michihiko; Nakano, Takafumi; Yamaguchi, Toshiya

Nihon Hozen Gakkai Dai-17-Kai Gakujutsu Koenkai Yoshishu, p.499 - 502, 2021/07

In 2018, Tokai Reprocessing Plan (TRP) shifted to the decommissioning stage. In order to proceed with steady decommissioning work, TRP effort to enhance project management function. This paper describes the establishment and role of the Decommissioning Project Management Office, effectiveness of applying the project management tool and its utilization concept, and the method of materialize the equipment dismantling plan.

Journal Articles

Improvement of INVS measurement uncertainty for Pu nitrate solution

Makino, Risa; Swinhoe, M. T.*; Suzuki, Hisanori; Ikeda, Atsushi*; Menlove, H. O.*; Shimizu, Yasuyuki; Nakamura, Hironobu

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-35-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2015/01

The Inventory Verification Sample system (INVS) is a non-destructive assay system for samples to quantify the Pu amount in Pu nitrate solutions and MOX with 31.3% of counting efficiency. It has been used for IAEA verification measurement for many years at the Plutonium Conversion Development Facility for the samples taken at the timing of PIV etc. as a partial defects verification system (uncertainty: about 3-5%). If the measurement uncertainty can be improved (to $$sim$$1%), it is expected that the usage can be extended to the operator's own measurements in MC&A to reduce the number of destructive analyses. In order to improve the measurement uncertainty for solution samples, after optimization of detector parameter and sample position, we conducted 3 different types of calibration method that is passive calibration curve, known-$$alpha$$ and multiplicity method to achieve the target uncertainty. To perform calibration and control the measurement quality, MOX fuel pellets with known Pu amount are fabricated and used. In the range of concentration of typical solution samples, we could confirm good correlations between measured doubles and $$^{240}$$Pu effective mass in the three methods. Especially, it was confirmed that the conventional calibration curve method could meet our target uncertainty ($$sim$$1%).

Journal Articles

Improvement of INVS measurement uncertainty for Pu and U-Pu nitrate solution

Makino, Risa; Swinhoe, M. T.*; Suzuki, Yoshimasa; Mukai, Yasunobu; Menlove, H. O.*; Marlow, J. B.*; Nakamura, Hironobu

Proceedings of INMM 55th Annual Meeting (Internet), 9 Pages, 2014/07

The Inventory Verification Sample systems (INVS) is a non-destructive assay (NDA) system for small inventory samples to quantify the Pu amount in Pu and U-Pu nitrate solutions and MOX powder with 31.3% counting efficiency (for Cf). It has been used for IAEA safeguards measurement for many years at the Plutonium Conversion Development Facility (PCDF) for the samples taken at the time of Random Interim Inspection (RII) and Physical Inventory Verification (PIV), and is currently used as partial defects verification equipment with uncertainty about 3$$sim$$5% accuracy for solution samples. The INVS is a inline detector therefore it is very convenient to use since it can be used for a sample inside the glove box without bag-out. If the measurement uncertainty can be improved (to $$sim$$1%), it is expected that the usage can be extended to the operator's own measurements in MC&A to reduce effort and the number of destructive analyses (DA). In order to improve the measurement uncertainty, we have performed multiplicity measurements using a variety of solution samples (concentration, acidity and volume) to determine the Pu amount and uncertainty, although the multiplicity analysis is challenging. To control the measurement quality, a few MOX ceramic fuel pellets with known Pu amount are used. The results are evaluated by three kinds of methods (calibration curve, known-$$alpha$$ and multiplicity) to determine the best measurement method. In the range of concentration of typical samples, we could confirm good correlations between measured doubles and $$^{240}$$Pu effective mass in the three methods. Especially, the conventional calibration curve method showed a good performance with short measurement time and small uncertainty when the calibration standards were a good match to the unknown samples. In this paper, we present the INVS system design and measurement results with uncertainty using solution samples and comparison results among the three calibration methods.

Journal Articles

Expansion control for cementation of incinerated ash

Nakayama, Takuya; Suzuki, Shinji; Hanada, Keiji; Tomioka, Osamu; Sato, Junya; Irisawa, Keita; Kato, Jun; Kawato, Yoshimi; Meguro, Yoshihiro

Proceedings of 2nd International Symposium on Cement-based Materials for Nuclear Wastes (NUWCEM 2014) (CD-ROM), 12 Pages, 2014/06

Journal Articles

Safety design and evaluation in a large-scale Japan sodium-cooled fast reactor

Yamano, Hidemasa; Kubo, Shigenobu; Shimakawa, Yoshio*; Fujita, Kaoru; Suzuki, Toru; Kurisaka, Kenichi

Science and Technology of Nuclear Installations, 2012, p.614973_1 - 614973_14, 2012/00

 Times Cited Count:12 Percentile:71.39(Nuclear Science & Technology)

This paper describes safety requirements for JSFR conformed to the defense-in-depth principle in IAEA. The safety design accommodation in JSFR was validated by safety analyses for representative DBEs: primary pump seizure and long-term loss-of-offsite power accidents. The safety analysis also showed the effectiveness of the passive shutdown system and mitigation measures against a typical ATWS.

Journal Articles

Conceptual design for a large-scale Japan sodium-cooled fast reactor, 2; Safety design and evaluation in JSFR

Yamano, Hidemasa; Kubo, Shigenobu*; Shimakawa, Yoshio*; Fujita, Kaoru; Suzuki, Toru; Kurisaka, Kenichi

Proceedings of 2011 International Congress on Advances in Nuclear Power Plants (ICAPP '11) (CD-ROM), p.728 - 740, 2011/05

Journal Articles

29th report of ITPA topical group meeting

Isayama, Akihiko; Sakakibara, Satoru*; Furukawa, Masaru*; Matsunaga, Go; Yamazaki, Kozo*; Watanabe, Kiyomasa*; Idomura, Yasuhiro; Sakamoto, Yoshiteru; Tanaka, Kenji*; Tamura, Naoki*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 86(6), p.374 - 377, 2010/06

no abstracts in English

Journal Articles

27th report of ITPA topical group meeting

Osakabe, Masaki*; Shinohara, Koji; Toi, Kazuo*; Todo, Yasushi*; Hamamatsu, Kiyotaka; Murakami, Sadayoshi*; Yamamoto, Satoshi*; Idomura, Yasuhiro; Sakamoto, Yoshiteru; Tanaka, Kenji*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 85(12), p.839 - 842, 2009/12

no abstracts in English

Journal Articles

Report on ITPA meetings, 24

Idomura, Yasuhiro; Yoshida, Maiko; Yagi, Masatoshi*; Tanaka, Kenji*; Hayashi, Nobuhiko; Sakamoto, Yoshiteru; Tamura, Naoki*; Oyama, Naoyuki; Urano, Hajime; Aiba, Nobuyuki; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 84(12), p.952 - 955, 2008/12

no abstracts in English

JAEA Reports

Feasibility Study on Commercialization of Fast Breeder Reactor Cycle Systems Interim Report of Phase II; Technical Study Report for Reactor Plant Systems

Konomura, Mamoru; Ogawa, Takashi; Okano, Yasushi; Yamaguchi, Hiroyuki; Murakami, Tsutomu; Takaki, Naoyuki; Nishiguchi, Youhei; Sugino, Kazuteru; Naganuma, Masayuki; Hishida, Masahiko; et al.

JNC TN9400 2004-035, 2071 Pages, 2004/06

JNC-TN9400-2004-035.pdf:76.42MB

The attractive concepts for Sodium-, lead-bismuth-, helium- and water-cooled FBRs have been created through using typical plant features and employing advanced technologies. Efforts on evaluating technological prospects of feasibility have been paid for these concepts. Also, it was comfirmed if these concepts satisfy design requierments of capability and performance presumed in the feasibilty study on commertialization of Fast Breeder Reactor Systems. As results, it was concluded that the selection of sodium-cooled reactor was most rational for practical use of FBR technologies in 2015.

Journal Articles

Demonstration of a transient high gain soft X-ray laser for neon-like Argon

Lu, P.; Kawachi, Tetsuya; Suzuki, M.*; Sukegawa, Kota*; Namba, Shinichi; Tanaka, Momoko; Hasegawa, Noboru; Nagashima, Keisuke; Daido, Hiroyuki; Arisawa, Takashi; et al.

Japanese Journal of Applied Physics, Part 2, 41(2A), p.L133 - L135, 2002/02

 Times Cited Count:9 Percentile:38.09(Physics, Applied)

no abstracts in English

Journal Articles

Enhancement of ion extraction from a cold plasma with radio-frequency plasma heating

Ozu, Akira; Suzuki, Yoji; Maruyama, Yoichiro; Arisawa, Takashi

Applied Physics Letters, 76(14), p.1822 - 1824, 2000/04

 Times Cited Count:4 Percentile:31.47(Physics, Applied)

no abstracts in English

Journal Articles

Enhancement of electron temperature in a laser-induced plasma using a radio-frequency electric field

Ozu, Akira; Suzuki, Yoji; Maruyama, Yoichiro; Arisawa, Takashi

Physics of Plasmas, 7(2), p.770 - 772, 2000/02

 Times Cited Count:2 Percentile:10.91(Physics, Fluids & Plasmas)

no abstracts in English

Journal Articles

Laser isotope separation via the atomic method

Maruyama, Yoichiro; Suzuki, Yoji; Kato, Masaaki; Ozu, Akira; Sugiyama, Akira; Arisawa, Takashi

Laser Advanced Materials Processing,Vol. 2, p.1251 - 1256, 1992/06

no abstracts in English

Oral presentation

Change of "effective plasma boundary" due to beta value in LHD divertor discharges

Watanabe, Kiyomasa*; Suzuki, Yasuhiro*; Yamaguchi, Taiki; Narihara, Kazumichi*; Tanaka, Kenji*; Tokuzawa, Tokihiko*; Yamada, Ichihiro*; Sakakibara, Satoru*; Morisaki, Tomohiro*; Nakajima, Noriyoshi*; et al.

no journal, , 

no abstracts in English

30 (Records 1-20 displayed on this page)