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Yokochi, Masaru; Sasaki, Shunichi; Yanagibashi, Futoshi; Asada, Naoki; Komori, Tsuyoshi; Fujieda, Sadao; Suzuki, Hisanori; Takeuchi, Kenji; Uchida, Naoki
Nihon Hozen Gakkai Dai-20-Kai Gakujutsu Koenkai Yoshishu, p.1 - 4, 2024/08
Tokai Reprocessing Plant, which is shifted to decommissioning stage, stores large amount of high-level radioactive liquid waste (HLLW) generated by reprocessing of spent nuclear fuels in High-level Active Waste facility (HAW). Radioactive risk related to HLLW has been concentrated in HAW until the completion of vitrification. Natural disasters such as earthquake may damage cooling function of HAW. Therefore, HAW must improve earthquake resistance, as exchanging the ground around HAW facility and pipe trench by concrete. This earthquake resistance construction starts from July of 2020 and completed in March 2024. This report summarizes the construction work and describes the inspection results after the construction.
Asada, Naoki; Sasaki, Shunichi; Rachi, Reona; Komori, Tsuyoshi; Suzuki, Hisanori; Takeuchi, Kenji; Uchida, Naoki
Nihon Hozen Gakkai Dai-20-Kai Gakujutsu Koenkai Yoshishu, p.5 - 8, 2024/08
no abstracts in English
Sato, Tomonori; Hata, Kuniki; Kaji, Yoshiyuki; Taguchi, Mitsumasa*; Seito, Hajime*; Inoue, Hiroyuki*; Tada, Eiji*; Abe, Hiroshi*; Akiyama, Eiji*; Suzuki, Shunichi*
Isotope News, (782), p.40 - 44, 2022/08
The stagnant water in the reactor building at Fukushima Daiichi Nuclear Power Station (1F) is exposed to the radiation from fuel debris and radioactive species. This water contains much amounts of impurities from the seawater which was injected in the emergency cooling. The impurities will affect the radiolysis and corrosive conditions in the water under irradiation. So, the water radiolysis data, corrosion data of steels under irradiations, and the evaluated potential impacts of corrosion in the decommissioning process of 1F are arranged as the database for corrosion under irradiation. This paper introduces the outline of this database.
Omori, Kazuki; Yamauchi, Sho; Yanagibashi, Futoshi; Sasaki, Shunichi; Wada, Takuya; Suzuki, Hisanori; Domura, Kazuyuki; Takeuchi, Kenji
Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.245 - 248, 2022/07
Tokai Reprocessing Plant (TRP), which is shifted to decommissioning stage, stores large amount of high-level radioactive liquid waste (HLLW). Although TRP is implementing vitrification of HLLW to reduce the risks related to HLLW storage, additional 20 years are required to complete vitrification of HLLW. Therefore, TRP is implementing safety countermeasure related to seismic resistance of HLLW storage facility as one of the top priorities. The results of the seismic evaluation indicate that although the facility itself is seismically resistant, there is a risk of insufficient binding force acting between the facility and the surrounding ground. Thus, replacement of the surrounding ground with concrete is performed. Since the countermeasures, to protect existing buries structure and coordinate with the other construction projects around the site, are required, the dedicated team was setup to handle the process and safety management of the concrete replacement construction.
Sato, Tomonori; Hata, Kuniki; Kaji, Yoshiyuki; Ueno, Fumiyoshi; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; Abe, Hiroshi*; Akiyama, Eiji*; et al.
JAEA-Review 2021-001, 123 Pages, 2021/06
JAEA-Review-2021-001.pdf:10.33MB
In the implement of the decommissioning of Fukushima Daiichi Nuclear Power Station (1F), there are many problems to be solved. Specially, the mitigation of the aging degradation by the corrosion of the structural materials is important to implement the decommissioning safely and continuously. However, there are limited data for the environmental factors of corrosion in 1F, and the condition of 1F is continuously changing. So, the literature data for the water radiolysis and the corrosion under irradiation are listed as the database of corrosion under irradiation in this report. And the new obtained radiolysis and corrosion data, which have not been reported in the literature and will be required in the decommissioning of 1F, are reported.
Zhou, Q.*; Saito, Takumi*; Suzuki, Seiya; Yano, Kimihiko; Suzuki, Shunichi*
Journal of Nuclear Science and Technology, 58(4), p.461 - 472, 2021/04
Times Cited Count：6 Percentile：69.63(Nuclear Science & Technology)Nakajima, Kunihisa; Nishioka, Shunichiro*; Suzuki, Eriko; Osaka, Masahiko
Mechanical Engineering Journal (Internet), 7(3), p.19-00564_1 - 19-00564_14, 2020/06
A large amount of cesium (Cs) chemisorbed onto stainless steel is predicted to be present especially in the upper region of reactor pressure vessel (RPV) during light water reactor severe accident (LWR SA) and a chemisorption model was developed for estimation of such amounts of Cs for stainless steel type 304 (SS304). However, this existing chemisorption model cannot accurately reproduce experimental results. Therefore, in this study, a modified Cs chemisorption model which accounts for silicon content in SS304 and concentration of cesium hydroxide (CsOH) in gaseous phases was constructed by combining penetration theory for gas-liquid mass transfer with chemical reaction and mass action law for CsOH decomposition at interface between gaseous and solid phases. As a result, it was found that the modified model was able to reproduce the experimental data more accurately than the existing model.
Miwa, Shuhei; Nakajima, Kunihisa; Miyahara, Naoya; Nishioka, Shunichiro; Suzuki, Eriko; Horiguchi, Naoki; Liu, J.; Miradji, F.; Imoto, Jumpei; Afiqa, B. M.; et al.
Mechanical Engineering Journal (Internet), 7(3), p.19-00537_1 - 19-00537_11, 2020/06
We constructed the fission product (FP) chemistry database named ECUME for LWR severe accident. This version of ECUME is equipped with dataset of the chemical reactions and their kinetics constants for the reactions of cesium(Cs)-iodine(I)-boron(B)-molybdenum(Mo)-oxygen(O)-hydrogen(H) system in gas phase, the elemental model for the high temperature chemical reaction of Cs with stainless steel applied as the structural material in a reactor, and thermodynamic data for CsBO
vapor species and solids of CsSi
O
and CsFeSiO for these chemical reactions. The ECUME will provide estimation of Cs distribution due to the evaluation of effects of interaction with BWR control material B and stainless steel on Cs behavior in the Fukushima Daiichi Nuclear Power Station.
Omori, Atsushi*; Akiyama, Eiji*; Abe, Hiroshi*; Hata, Kuniki; Sato, Tomonori; Kaji, Yoshiyuki; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; et al.
Zairyo To Kankyo, 69(4), p.107 - 111, 2020/04
To evaluate the effect of oxidants, which are formed by radiolysis of water under gamma ray irradiation, on the corrosion of a carbon steel in humid environment, ozone was introduced as a model oxidant in to humidity-controlled air at 50
C in a thermo-hygrostat chamber. Corrosion monitoring was performed by using an Atmospheric Corrosion Monitor-type (ACM) sensor consisting of a carbon steel anode and an Ag cathode. The output current of the ACM sensor was increased with the increase in relative humidity and it was obviously increased with the increase in the introduced ozone concentration at each relative humidity. The results indicate that ozone accelerates the corrosion of the carbon steel. The effect of ozone on the corrosion acceleration is attributed to the fast reduction reaction and fast dissolution reaction in to water compared to that of oxygen.
Nishioka, Shunichiro; Nakajima, Kunihisa; Suzuki, Eriko; Osaka, Masahiko
Journal of Nuclear Science and Technology, 56(11), p.988 - 995, 2019/11
Times Cited Count：12 Percentile：79.16(Nuclear Science & Technology)In order to contribute to improvement of Cs chemisorption model used in severe accident analysis codes, the influence of chemical factors (temperature, atmosphere, concentration of affecting chemical elements etc.) on the Cs chemisorption behaviour onto stainless steel was investigated experimentally. It was found that the surface reaction rate constant used in the current Cs-chemisorption model was influenced by not only temperature, as already known, but also atmosphere, cesium hydroxide (CsOH) concentration in the gas phase and silicon content in SS304. Such chemical factors should be considered for the construction of the improved Cs-chemisorption model. Another important finding is that the chemisorption behavior at lower temperatures, around 873 K, could differ from those above 1073 K. Namely, Cs-Fe-O compounds would form as the main Cs-chemisorbed compounds at 873 K while Cs-Si-Fe-O compounds at more than 1073 K.
Washiya, Tadahiro; Suzuki, Shunichi*
Nihon Kikai Gakkai-Shi, 122(1211), p.13 - 15, 2019/10
International Topical Workshop on Fukushima Decommissioning Research (FDR 2019) was held in last May. In this report, the out-line of Track-2: Debris Removal Strategy, Risk, Debris Characterization was described. In this Task-2, "1F decommissioning strategy plan 2019" was introduced by NDF, and challenging tasks are explained. As 1F's R&D issues, debris cutting technologies, dust generation behavior analysis and risk evaluation was reported. In this paper, the out-line of Track 2 will be reported.
Nakajima, Kunihisa; Nishioka, Shunichiro; Suzuki, Eriko; Osaka, Masahiko
Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05
Cesium chemisorption models were developed for estimation of amount of cesium chemisorbed onto stainless steel type 304 (SS304) during light water reactor severe accident. However, existing chemisorption models cannot accurately reproduce experimental results. In this study, a modified cesium chemisorption model was constructed based on a penetration theory for gas-liquid mass transfer with chemical reaction and was able to adequately describe effects on concentration of cesium hydroxide in gaseous phase and silicon content in SS304. It was found that the modified model can more accurately reproduce the experimental data than the existing model.
Miwa, Shuhei; Miyahara, Naoya; Nakajima, Kunihisa; Nishioka, Shunichiro; Suzuki, Eriko; Horiguchi, Naoki; Liu, J.; Miradji, F.; Imoto, Jumpei; Afiqa, B. M.; et al.
Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 8 Pages, 2019/05
We constructed the first version of fission product (FP) chemistry database named ECUME for LWR severe accident. The first version of ECUME is equipped with dataset of the chemical reactions and their kinetics constants for the reactions of cesium(Cs)-iodine(I)-boron(B)-molybdenum(Mo)-oxygen(O)-hydrogen(H) system in gas phase, the elemental model for the high temperature chemical reaction of Cs with stainless steel, and thermodynamic data for CsBO vapor species and solids of CsSiO and CsFeSiO. The ECUME will provide more accurate estimation of Cs distribution due to the evaluation of effects of interaction with BWR control material B and stainless steel on Cs behavior in the Fukushima Daiichi Nuclear Power Station.
Suzuki, Eriko; Takase, Gaku; Nakajima, Kunihisa; Nishioka, Shunichiro; Hashimoto, Naoyuki*; Isobe, Shigehito*; Osaka, Masahiko
Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR 2019) (Internet), 4 Pages, 2019/05
In order to acquire the knowledge of the Cs chemisorption behaviour in the lower temperature region, the Cs chemisorbed compounds and the surface reaction rates were investigated by conducting the Cs chemisorption tests onto stainless steel at 873 and 973 K. As a result, The cesium ferrate compounds were revealed to be formed at this temperatures. It was seen that the dependences of surface reaction rate constant on this temperature were different from that at the higher temperature region. This behaviour leads to the conclusion that the Cs chemisorption model in the low temperature region should be newly constructed.
Miradji, F.; Suzuki, Chikashi; Nishioka, Shunichiro; Suzuki, Eriko; Nakajima, Kunihisa; Osaka, Masahiko; Barrachin, M.*; Do, T. M. D.*; Murakami, Kenta*; Suzuki, Masahide*
Proceedings of 9th Conference on Severe Accident Research (ERMSAR 2019) (Internet), 21 Pages, 2019/03
Takahashi, Naoki; Suzuki, Soju; Saito, Hiroto; Ueno, Takashi; Abe, Sadayoshi; Yamanaka, Atsushi; Tanigawa, Masafumi; Nakamura, Daishi; Sasaki, Shunichi; Mine, Tadaharu
Nihon Genshiryoku Gakkai Homu Peji (Internet), 20 Pages, 2017/05
no abstracts in English
Takahashi, Satoru*; Nota, Yoshiki*; Matsuda, Asahi*; Kawabata, Kuniaki; Suzuki, Tsuyoshi*; Takemura, Fumiaki*; Ogasawara, Kei*; Kaneko, Shunichi*
Journal of Signal Processing, 21(1), p.15 - 24, 2017/01
In recent years, many researchers try to observe the state of the global environment from marine information for the understanding of the global environment change. First, we introduce the recording system of underwater environment which is made by the authors. By using this system, we want to observe the change of global environment from the coral bleaching. In this paper, especially, we propose the generation method of underwater landmark which is used to measure the position of robot of oceanographic observation based on the dynamic image processing. In here, underwater landmark means the feature point in underwater image.
Suzuki, Hideya; Tsubata, Yasuhiro; Kurosawa, Tatsuya; Shibata, Mitsunobu; Kawasaki, Tomohiro; Urabe, Shunichi*; Matsumura, Tatsuro
Analytical Sciences, 32(4), p.477 - 479, 2016/04
Times Cited Count：24 Percentile：67.95(Chemistry, Analytical)An impeccable, high-performance new reagent called alkyl diamide amine (ADAAM) was examined from the viewpoint of mutual separation of Am(III) and Eu(III). ADAAM has three donor atoms, one soft N-donor atom and two hard O-donor atoms, in the central frame. The combination of soft and hard atoms affords a tridentate donor set of atoms that ensures remarkable extractability and selectivity of Am(III) and Eu(III) in highly acidic media.
Mitamura, Hiroyuki*; Watanuki, Ryuta*; Kaneko, Koji; Onozaki, Norimichi*; Amo, Yuta*; Kittaka, Shunichiro*; Kobayashi, Riki*; Shimura, Yasuyuki*; Yamamoto, Isao*; Suzuki, Kazuya*; et al.
Physical Review Letters, 113(14), p.147202_1 - 147202_5, 2014/10
Times Cited Count：23 Percentile：75.83(Physics, Multidisciplinary)Yokota, Hideharu; Amano, Kenji; Maekawa, Keisuke; Kunimaru, Takanori; Naemura, Yumi*; Ijiri, Yuji*; Motoshima, Takayuki*; Suzuki, Shunichi*; Teshima, Kazufumi*
JAEA-Research 2013-002, 281 Pages, 2013/06
JAEA-Research-2013-002.pdf:13.03MB
To evaluate permeable heterogeneity in a fracture and scale effects which are problems to be solved based on the 
mass transportation data of fractures in hostrock, a number of tracer tests are simulated in a fictitious single plate fracture generated on computer in this study. And the transport parameters, e.g. longitudinal dispersion length, true velocity and dilution rate, are identified by fitting one- and two-dimensional models to the breakthrough curves obtained from the simulations in order to investigate the applicability of these models to the evaluation of tracer test. As a result, one-dimensional model yields larger longitudinal dispersion length than two-dimensional model in the both cases of homogeneous and heterogeneous hydraulic conductivity fields of the fictitious fracture. And, the longitudinal dispersion length identified from a tracer test is smaller and/or larger than the macroscopic longitudinal dispersion length identified from whole fracture. It is clarified that these are occurred by shorter or longer distance between boreholes compare to the correlation length of geostatistical heterogeneity of fictitious fracture.
