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I seawater concentrations off Fukushima and potential of 129I as an oceanographic tracer for ALPS-treated waterSuzuki, Takashi; Otosaka, Shigeyoshi*; Takata, Hyoe*; Kuwabara, Jun; Nakanishi, Takahiro; Ikenoue, Tsubasa
Environmental Science & Technology, 60(17), p.13123 - 13131, 2026/05
Times Cited Count:0 Percentile:0.00(Engineering, Environmental)As a results of the 2011 Fukushima Daiichi Nuclear Power Plant accident, long-lived radioactive
I has been released into the environment, with additional releases beginning in 2023 through ALPS-treated water. To study its long-term variation and potential as an oceanographic tracer,
I concentrations in seawater off Fukushima were measured from 2012 to 2024. The highest concentration, 445
10
Bq/L, was observed in 2013 near the plant. Levels have since declined toward the pre-accident value of 1.76
10
Bq/L. Spatial and temporal changes in the
I/
Cs ratio indicate the influence of small water masses and support its use as a tracer in areas with complex ocean circulation.
Sekine, Megumi; Ishikawa, Yuki; Kai, Sachiyo*; Sukegawa, Hidetoshi; Motokawa, Risa*; Kato, Akane; Obata, Takashi; Motome, Yuiko; Siregar, V.; Hayakawa, Tsuyoshi*; et al.
Dai-46-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 3 Pages, 2025/12
no abstracts in English
Wada, Kazuma*; Kazama, Hiroyuki*; Abe, Chikage*; Onishi, Takashi; Yamamoto, Masahiko; Taguchi, Shigeo; Kuno, Takehiko; Maeda, Koji; Idemitsu, Kazuya*; Suzuki, Tatsuya*
Journal of Radioanalytical and Nuclear Chemistry, 334(11), p.8961 - 8968, 2025/11
Times Cited Count:0 Percentile:0.00(Chemistry, Analytical)The feasibility of using commercially available polyvinylpolypyrrolidone (PVPP) as a pretreatment for mass spectrometry to separate actinides was investigated. Uranium, thorium, and plutonium were used as actinides in the study. Adsorption data for An(IV) and An(VI) were obtained by adsorption experiments in nitric acid. In addition, An(III)/An(IV)/An(VI) mutual separation was successfully performed by a column separation method using PVPP. Furthermore, the elution efficiency of U(VI) was improved by the introduction of carbonate ions. This method may be applicable as a mutual separation for actinide mass spectrometry.
Iketani, Shotaro; Suzuki, Takeshi; Yokobori, Tomohiko; Sugawara, Satoshi; Yokota, Akira; Kikuchi, Genta; Muraguchi, Yoshinori; Kitahara, Masaru; Seya, Manato; Kurosawa, Tsuyoshi; et al.
JAEA-Technology 2025-001, 169 Pages, 2025/08
The radioactive waste treatment facilities at the Nuclear Science Research Institute includes the Radioactive Waste Treatment Facility No. 3, Waste Size Reduction and Storage Facility, and Waste Volume Reduction Facility. These three facilities come under the purview of the Act on the Regulation of Nuclear Source Material, Nuclear Fuel Material and Reactors, and are included under Class C of the act based on the seismic requirements specified in the Act. We assessed the seismic capacity of these three radioactive waste treatment facilities based on the current Building Standards Act, to verify whether they comply with the new regulatory requirements enforced by the Nuclear Regulation Authority (NRA) in the aftermath of the 2011 nuclear accident at the Fukushima Daiichi Nuclear Power Station operated by the Tokyo Electric Power Company. We found that the allowable stress of a few structural members used in the construction of the facilities did not meet the regulatory requirements. After studying the approval granted by the NRA for the construction plans, including the design and construction methods (design and construction plans) of the three facilities on March 5, 2021, we made aseismic reinforcement at these facilities between 2021 and 2022. This report presents an overview of the seismic design of these facilities and an outline of the aseismic reinforcement conducted, management system existing, safety measures adopted, and the preoperational inspections conducted at these facilities.
Komatsu, Seiji; Nishida, Tetsuro; Kawasaki, Ichio; Gunji, Hikaru; Nishino, Shohei; Kambara, Takashi*; Miura, Hirohito*; Suzuki, Takaichi*; Kinoshita, Masato*; Kanei, Tatsuya*
Nihon Hozen Gakkai Dai-21-Kai Gakujutsu Koenkai Yoshishu, 5 Pages, 2025/07
Steam used for process and air conditioning in each facility at the Nuclear Fuel Cycle Engineering Institute is generated by a water tube boiler installed in the Institute's central control room and supplied to each facility via underground trenches. There are three steam supply pipelines (A, B, and C) to each facility, with two of these (A and B) designated for the reprocessing facility. The steam pipelines, including expansion joints and steam traps, are covered with insulation. The two steam pipelines for the reprocessing facility (A and B) are laid parallel, creating a structure that makes inspection and maintenance difficult. In particular, the expansion joints are spaced very closely between the A and B lines, making insulation removal difficult, which has been a challenge in performing visual inspections of the expansion joint bodies. This paper reports on the features and effects of an improved insulation system designed to allow for easy removal and installation.
Toyota, Kodai; Imagawa, Yuya; Onizawa, Takashi; Suzuki, Akihiro*
Proceedings of the ASME 2025 Pressure Vessels & Piping Conference (PVP2025) (Internet), 8 Pages, 2025/07
He neutron spin filter at J-PARCTakahashi, Shingo; Kiyanagi, Ryoji; Okudaira, Takuya*; Takada, Shusuke*; Kobayashi, Ryuju; Okuizumi, Mao; Ino, Takashi*; Asai, Kanta*; Tsuchikawa, Yusuke; Oikawa, Kenichi; et al.
Nuclear Instruments and Methods in Physics Research A, 1075, p.170410_1 - 170410_8, 2025/06
Times Cited Count:2 Percentile:51.17(Instruments & Instrumentation)Yuguchi, Takashi*; Endo, Kyoka*; Suzuki, Satoshi*; Ogita, Yasuhiro; Sakata, Shuhei*; Yokoyama, Tatsunori; Imura, Takumi*; Ono, Takeshi*; Sasao, Eiji
Lithos, 494-495, p.107909_1 - 107909_14, 2025/02
Times Cited Count:1 Percentile:13.86(Geochemistry & Geophysics)This study described the growth characteristics of zircon crystals in the Kuki granite from the Kitakami Mountains in northeastern Japan as the key for elucidating granitic magma chamber processes. Using two approaches, analyses based on multiple sections of separated zircon crystals and thin-section-based zircon crystal analyses, we determined the characteristics of the 3D internal structure of the crystals, variations in U-Pb age, Ti concentrations, and Th/U in relation to crystal texture, and the crystallization sequence between zircon crystals and other minerals within the magma chamber. The textures, which occupy a large proportion of zircon, comprise low luminescence homogeneous cores (LLCs) and oscillatory zoning (OZ). The 3D distribution of the zircon internal structure can be classified into three types: Type 1 zircon comprising LLCs and the surrounding OZ and Types 2 and 3 zircon crystals composed entirely of OZ from the cores to the rims and characterized by brightness and darkness cores, respectively. LLC and OZ grew at temperatures from approximately 900 to 800
C and 850 to 700
C, respectively, and LLC has a higher Th/U than that of OZ, indicating that fractional crystallization progression as the magma chamber cooled resulted in the transition from LLC to OZ. In the progression of fractional crystallization, the diffusion rate deceleration with decreasing magma temperatures triggered the transition from interfacial reaction-controlled growth producing LLC to diffusion-controlled growth producing OZ. In the thin-section analysis, zircon crystals which contained in different minerals are characterized by different Th/U values. The variation in Th/U and the crystallization temperature of zircon crystals considering the surrounding minerals can be used to elucidate the differentiation and mineral crystallization in magma chamber processes over a wide range of temperature conditions.

Yamamoto, Hajime*; Ikeda, Osamu*; Honda, Takashi*; Kimura, Kenta*; Aoyama, Takuya*; Ogushi, Kenya*; Suzuki, Akio*; Ishii, Kenji*; Matsumura, Daiju; Tsuji, Takuya; et al.
Physical Review Materials (Internet), 8(9), p.094402_1 - 094402_6, 2024/09
Times Cited Count:5 Percentile:34.77(Materials Science, Multidisciplinary)Machida, Masahiko; Yamada, Susumu; Kim, M.; Tanaka, Satoshi*; Tobita, Yasuhiro*; Iwata, Ayako*; Aoki, Yuto; Aoki, Kazuhisa; Yanagisawa, Kenichi*; Yamaguchi, Takashi; et al.
RIST News, (70), p.3 - 22, 2024/09
Inside the Fukushima Daiichi Nuclear Power Plant (1F), there are many locations with high radiation levels due to contamination by radioactive materials that leaked from the reactor. These pose a significant obstacle to the smooth progress of decommissioning work. To help solve this issue, the Japan Atomic Energy Agency (JAEA), under a subsidy from the Ministry of Economy, Trade, and Industry's decommissioning and contaminated water management project, is conducting research and development on digital technologies to improve the radiation environment inside the decommissioning site. This project, titled "Development of Technology to Improve the Environment Inside Reactor Buildings (Enhancing Digital Technology for Environment and Source Distribution to Reduce Radiation Exposure)," began in April of FY 2023. In this project, the aim is to develop three interconnected systems: FrontEnd, Pro, and BackEnd. The FrontEnd system, based on the previously developed 3D-ADRES-Indoor (prototype) from FY 2021-2022, will be upgraded to a high-speed digital twin technology usable on-site. The Pro system will carry out detailed analysis in rooms such as the new office building at 1F, while the BackEnd system will serve as a database to centrally manage the collected and analyzed data. This report focuses on the FrontEnd system, which will be used on-site. After point cloud measurement, the system will quickly create a 3D mesh model, estimate the radiation source from dose rate measurements, and refine the position and intensity of the estimated source using recalculation techniques (re-observation instructions and re-estimation). The results of verification tests conducted on Unit 5 are also presented. Furthermore, the report briefly discusses the future research and development plans for this project.
Kawabata, Kuniaki; Imabuchi, Takashi; Shirasaki, Norihito*; Suzuki, Soichiro; Ito, Rintaro; Aoki, Yuto; Omori, Takazumi
ROBOMECH Journal (Internet), 11, p.11_1 - 11_11, 2024/09
I in riverbank sediment after the Fukushima accidentNakanishi, Takahiro; Sakuma, Kazuyuki; Oyama, Takuya; Hagiwara, Hiroki; Suzuki, Takashi
Environmental Pollution, 355, p.124213_1 - 124213_7, 2024/08
Times Cited Count:8 Percentile:63.99(Environmental Sciences)This study investigated the transport behavior of
I by riverbank surveys conducted from 2013 to 2015 in a watershed where the
I/
Cs activity ratio is low in the mountainous area and high in the plain as of 2011. Until 2015, the
I/
Cs activity ratio of the levee crown in the studied watershed was similar to that of the surrounding area in 2011. However, the
I/
Cs ratios of the surface riverbank sediments were all low, indicating that radionuclides transported from the mountainous area were deposited on the riverbank in the plain. The vertical distribution of the
I/
Cs ratio in the riverbank sediments indicated that some
I and
Cs deposited during the accident remained in the lower layers, but most were eroded immediately after the accident. Based on the
I/
Cs ratios of sediments deposited on the riverbank, which remained constant until 2015 after the accident, the amount of
I discharged to the ocean was determined from the previously evaluated
Cs discharge. It was calculated that 1.8
10
Bq and 1.2
10
Bq of
I were discharged with sediment from the studied watershed and the contaminated river watersheds (Abukuma River and Fukushima coastal rivers, including the study river), respectively. The results of this study indicate that the continuous
I discharge from the river contribute little to their amount in the seafloor sediments along the Fukushima coast.
Nishino, Shohei; Nishida, Tetsuro; Kawasaki, Ichio; Motohashi, Masahiro; Kambara, Takashi*; Suzuki, Takaichi*; Kinoshita, Masato*
Nihon Hozen Gakkai Dai-20-Kai Gakujutsu Koenkai Yoshishu, p.14 - 21, 2024/08
Steam is used to a process and air conditioning in Nuclear fuel Cycle engineering Laboratories (NCL). The steam is used mainly in Reprocessing Plant, and it is supplied by two steam plumbing. A leak occurred from the steam plumbing in November, 2022. As a result of cause investigation, I estimated that it had leaked by a water hammer caused for the trouble of the steam trap.
CNguyen, B. V. C.*; Murakami, Kenta*; Chena, L.*; Phongsakorn, P. T.*; Chen, X.*; Hashimoto, Takashi; Hwang, T.*; Furusawa, Akinori; Suzuki, Tatsuya*
Nuclear Materials and Energy (Internet), 39, p.101639_1 - 101639_9, 2024/06
Times Cited Count:6 Percentile:80.76(Nuclear Science & Technology)
Be and
Al under direct muon-induced spallation in granite quartz and its implications for past high-energy cosmic ray fluxesSakurai, Hirohisa*; Kurebayashi, Yutaka*; Suzuki, Soichiro*; Horiuchi, Kazuho*; Takahashi, Yui*; Doshita, Norihiro*; Kikuchi, Satoshi*; Tokanai, Fuyuki*; Iwata, Naoyoshi*; Tajima, Yasushi*; et al.
Physical Review D, 109(10), p.102005_1 - 102005_18, 2024/05
Times Cited Count:0 Percentile:0.00(Astronomy & Astrophysics)Secular variations of galactic cosmic rays (GCRs) are inseparably associated with the galactic activities and should reflect the environments of the local galactic magnetic field, interstellar clouds, and nearby supernova remnants. The high-energy muons produced in the atmosphere by high-energy GCRs can penetrate deep underground and generate radioisotopes in the rock. As long lived radionuclides such as
Be and
Al have been accumulating in these rocks, concentrations of
Be and
Al can be used to estimate the long-term variations in high-energy muon yields, corresponding to those in the high-energy GCRs over a few million years. This study measured the production cross sections for muon induced
Be and
Al by irradiating positive muons with the momentum of 160 GeV/c on the synthetic silica plates and the granite core at the COMPASS experiment line in CERN SPS. In addition, it the contributions of the direct muon spallation reaction and the nuclear reactions by muon-induced particles on the production of long lived radionuclides in the rocks were clarified.
Suzuki, Satoshi*; Yuguchi, Takashi*; Ishiguro, Keito*; Endo, Kyoka*; Kato, Asuka*; Yokoyama, Kosuke*; Ogita, Yasuhiro; Yokoyama, Tatsunori; Sakata, Shuhei*; Ono, Takeshi*; et al.
Journal of Mineralogical and Petrological Sciences (Internet), 119(1), p.230807_1 - 230807_18, 2024/02
Times Cited Count:2 Percentile:29.85(Mineralogy)Understanding the crustal evolutionary dynamics of island arc-trench systems requires a thorough evaluation of magma chamber processes, and especially of shallow crustal granitic magma intrusion and emplacement processes. To address this, we studied the petrography and geochronology of the Kuki granite, Kitakami Mountains, northeast Japan, as an example of a non-adakitic granite at the magmatic flare-up stage. Granitic borehole samples reflect vertical variation within a magma chamber. Whole-rock chemical composition and mode data reveal a vertical transition from felsic to mafic composition with increasing depth, potentially due to gravitational fractionation of crystals in the magma chamber. The pressure and temperature history of the Kuki granite indicates no change in the magma depth with cooling from 800 to 730
C, and geobarometric calculations indicate the emplacement of magma at a depth of approximately10 km. Simultaneous determination of the zircon U Pb age, Ti concentration, and Th/U yields 1) the time temperature history of granitic magma before its solidification, and 2) the correlation between temperature and Th/U in the magma. The magma chamber cooled from ca. 900 to 700
C at approximately 125 Ma. The change in Th/U with temperature indicates greater fractional crystallization in the magma chamber at temperatures above 800
C than below 800
C. Samples from different depth exhibit common tendencies in terms of the relationship between Th/U and temperature, indicating the same system of fractional crystallization throughout the cooling magma chamber.
Be ground-state molecular structure using
Be(
)
He triple differential reaction cross-section measurementsLi, P. J.*; Beaumel, D.*; Lee, J.*; Assi
, M.*; Chen, S.*; Franchoo, S.*; Gibelin, J.*; Hammache, F.*; Harada, T.*; Kanada-En'yo, Yoshiko*; et al.
Physical Review Letters, 131(21), p.212501_1 - 212501_7, 2023/11
Times Cited Count:36 Percentile:94.69(Physics, Multidisciplinary)The cluster structure of the neutron-rich isotope
Be has been probed via the (
) reaction. The triple differential cross-section was extracted and compared to distorted-wave impulse approximation reaction calculations performed in a microscopic framework using the Tohsaki-Horiuchi-Schuck-R
pke wave function and the wave function deduced from Antisymmetrized Molecular Dynamics calculations. The remarkable agreement between calculated and measured cross-sections in both shape and magnitude validates the description of the
Be ground-state as a rather compact nuclear molecule.
Machida, Masahiko; Yamada, Susumu; Kim, M.; Okumura, Masahiko; Miyamura, Hiroko; Shikaze, Yoshiaki; Sato, Tomoki*; Numata, Yoshiaki*; Tobita, Yasuhiro*; Yamaguchi, Takashi; et al.
RIST News, (69), p.2 - 18, 2023/09
The contamination of radioactive materials leaked from the reactor has resulted in numerous hot spots in the Fukushima Daiichi Nuclear Power Station (1F) building, posing obstacles to its decommissioning. In order to solve this problem, JAEA has conducted research and development of the digital technique for inverse estimation of radiation source distribution and countermeasures against the estimated source in virtual space for two years from 2021 based on the subsidy program "Project of Decommissioning and Contaminated Water Management" performed by the funds from the Ministry of Economy, Trade and Industry. In this article, we introduce the results of the project and the plan of the renewal project started in April 2023. For the former project, we report the derivative method for LASSO method considering the complex structure inside the building and the character of the source and show the result of the inverse estimation using the method in the real reactor building. Moreover, we explain the platform software "3D-ADRES-Indoor" which integrates these achievements. Finally, we introduce the plan of the latter project.
and O
in a reaction cell in triple quadrupole inductively coupled plasma mass spectrometryKazama, Hiroyuki; Konashi, Kenji*; Suzuki, Tatsuya*; Koyama, Shinichi; Maeda, Koji; Sekio, Yoshihiro; Onishi, Takashi; Abe, Chikage*; Shikamori, Yasuyuki*; Nagai, Yasuyoshi*
Journal of Analytical Atomic Spectrometry, 38(8), p.1676 - 1681, 2023/07
Times Cited Count:5 Percentile:50.66(Chemistry, Analytical)Sato, Yuhi*; Otosaka, Shigeyoshi*; Suzuki, Takashi; Nakanishi, Takahiro
Limnology and Oceanography, 68(7), p.1580 - 1594, 2023/07
Times Cited Count:8 Percentile:64.53(Limnology)To investigate the factors regulating the concentration of particulate iodine (PI) in seawater, it was measured in two Pacific coastal areas adjacent to Japan in two seasons along with parameters such as particulate organic carbon (POC) and nitrogen (PON), dissolved iodine (DI), and phytoplankton pigments. The dataset was divided in three groups namely, lower (Group A), average (Group B), and higher (Group C) atomic ratios of PI to POC (I/C). The three groups were characterized by phytoplanktonic physiological states as highly productive, steady, and senescent states, respectively. Based on the finding that PI production is associated with the phytoplankton physiological state, the seasonal and regional differences in PI concentration and I/C in the observation areas were consistently explained. Finally, we suggest that the phytoplanktonic physiological state is one of the vital factors regulating the PI concentration in seawater.