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G
tz, M.*; Yakushev, A.*; Gtz, S.*; Di Nitto, A.*; D
llmann, Ch. E.*; Asai, Masato; Kindler, B.*; Krier, J.*; Lommel, B.*; Nagame, Yuichiro*; et al.
Radiochimica Acta, 110(2), p.75 - 86, 2022/02
Times Cited Count：2 Percentile：31.78(Chemistry, Inorganic & Nuclear)The study of volatile superheavy element carbonyl complexes requires more efficient methods because the yield of transactinide elements decreases with increasing atomic number. This is achieved by using a newly developed double chamber system to separate the recoil chamber and the reaction one, thereby avoiding the decomposition of reactive molecules by the projectile ion beam, which hinders the synthesis of carbonyl complexes. The feasibility of this method was verified by synthesizing 5d metal short-lived isotopes as homologous element isotopes of the light transactinide elements Sg, Bh, Hs, and Mt at the Japan Atomic Energy Agency tandem accelerator and conducting model experiments.
Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.
Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08
Times Cited Count：2 Percentile：14.88(Chemistry, Multidisciplinary)The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 
C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl
TaOCl
DbOCl. From the obtained experimental results, thermochemical data for DbOCl were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.
Harada, Masahide; Sekijima, Mitsuaki*; Morikawa, Noriyuki*; Masuda, Shiho; Kinoshita, Hidetaka; Sakai, Kenji; Kai, Tetsuya; Kasugai, Yoshimi; Muto, Giichi*; Suzuki, Akio*; et al.
JPS Conference Proceedings (Internet), 33, p.011099_1 - 011099_6, 2021/03
In MLF at J-PARC, a unified mercury radioactivity monitor (UHAM) is installed to find an indication of failure of the mercury target and loop system by detecting radioactive materials leaked from the system with a 
-ray energy analysis with Germanium semi-conductor detectors (Ge detectors). It is composed of three units of sampling port and radiation monitors: (1) HAM for interstitial helium gas layer between the mercury vessel and surrounding water shroud of the mercury target, (2) CAM for atmosphere in the hot cell where the target loop is operated and (3) VAM for helium gas in the helium vessel where the target vessel is installed. Once any leakages of radioactive materials are detected, an alarm signal is issued immediately to the accelerator control system to stop beam operation. Software and hardware have been upgraded yearly. For example, two Ge detectors are used for HAM for redundancy, NaI Scintillation detectors are also used as supplemental for the Ge detector to keep availability of the system for high counting rate event. In April 2015, the UHAM activated when a small water coolant leakage from the water shroud of the mercury target occurred. VAM detected an abnormal increase of the counting rate in the helium vessel. It was also indicated that the measured radioactive nuclides were generated from the activation of the coolant (water) in the water shroud and not from the mercury.
Hosoda, Masahiro*; Nugraha, E. D.*; Akata, Naofumi*; Yamada, Ryohei; Tamakuma, Yuki*; Sasaki, Michiya*; Kelleher, K.*; Yoshinaga, Shinji*; Suzuki, Takahito*; Rattanapongs, C. P.*; et al.
Science of the Total Environment, 750, p.142346_1 - 142346_11, 2021/01
Times Cited Count：23 Percentile：86.19(Environmental Sciences)The biological effects of low dose-rate radiation exposures on humans remains unknown. In fact, the Japanese nation still struggles with this issue after the Fukushima Dai-ichi Nuclear Power Plant accident. Recently, we have found a unique area in Indonesia where naturally high radiation levels are present, resulting in chronic low dose-rate radiation exposures. We aimed to estimate the comprehensive dose due to internal and external exposures at the particularly high natural radiation area, and to discuss the enhancement mechanism of radon. A car-borne survey was conducted to estimate the external doses from terrestrial radiation. Indoor radon measurements were made in 47 dwellings over three to five months, covering the two typical seasons, to estimate the internal doses. Atmospheric radon gases were simultaneously collected at several heights to evaluate the vertical distribution. The absorbed dose rates in air in the study area vary widely between 50 nGy h
and 1109 nGy h. Indoor radon concentrations ranged from 124 Bq m
to 1015 Bq m. That is, the indoor radon concentrations measured exceed the reference levels of 100 Bq m recommended by the World Health Organization. Furthermore, the outdoor radon concentrations measured were comparable to the high indoor radon concentrations. The annual effective dose due to external and internal exposures in the study area was estimated to be 27 mSv using the median values. It was found that many residents are receiving radiation exposure from natural radionuclides over the dose limit for occupational exposure to radiation workers. This enhanced outdoor radon concentration might be as a result of the stable atmospheric conditions generated at an exceptionally low altitude. Our findings suggest that this area provides a unique opportunity to conduct an epidemiological study related to health effects due to chronic low dose-rate radiation exposure.
Takahashi, Osamu*; Shibui, Yohei*; Xu, P. G.; Harjo, S.; Suzuki, Tetsuya*; Tomota, Yo*
Quantum Beam Science (Internet), 4(1), p.16_1 - 16_15, 2020/03
Shoji, Eita*; Isogai, Shosei*; Suzuki, Rikuto*; Kubo, Masaki*; Tsukada, Takao*; Kai, Tetsuya; Shinohara, Takenao; Matsumoto, Yoshihiro*; Fukuyama, Hiroyuki*
Scripta Materialia, 175, p.29 - 32, 2020/01
Times Cited Count：19 Percentile：78.21(Nanoscience & Nanotechnology)Iwasaki, Sachio; Oka, Makoto; Suzuki, Kei*; Yoshida, Tetsuya*
AIP Conference Proceedings 2130, p.050001_1 - 050001_8, 2019/07
Times Cited Count：0 Percentile：0.09(Physics, Nuclear)We find a novel phenomenon induced by the interplay between a strong magnetic field and finite orbital angular momenta in hadronic systems, which is analogous to the Paschen-Back effect observed in the field of atomic physics. This effect allows the wave functions to drastically deform. We discuss anisotropic decay from the deformation as a possibility to measure the strength of the magnetic field in heavy-ion collision at LHC, RHIC and SPS, which has not experimentally been measured. As an example we investigate charmonia with finite orbital angular momentum in a strong magnetic field. We calculate the mass spectra and mixing rate. To obtain anisotropic wave functions, we apply the cylindrical Gaussian expansion method, where the Gaussian bases to expand the wave functions have different widths along transverse and longitudinal directions in the cylindrical coordinate.
Iwasaki, Sachio; Oka, Makoto; Suzuki, Kei*; Yoshida, Tetsuya*
International Journal of Modern Physics; Conference Series (Internet), 49, p.1960002_1 - 1960002_6, 2019/07
Times Cited Count：0 Percentile：0.09(Astronomy & Astrophysics)The hadronic Paschen-Back effects in P-wave charmonia are analyzed using the constituent quark models in strong magnetic field.
Chiera, N. M.; Sato, Tetsuya; Tomitsuka, Tomohiro; Asai, Masato; Ito, Yuta; Shirai, Kaori*; Suzuki, Hayato; Tokoi, Katsuyuki; Toyoshima, Atsushi; Tsukada, Kazuaki; et al.
Journal of Radioanalytical and Nuclear Chemistry, 320(3), p.633 - 642, 2019/06
Times Cited Count：1 Percentile：11.15(Chemistry, Analytical)An isothermal gas-chromatographic (IGC) device has been developed and tested for on-line gas phase studies of volatile oxychlorides of short-lived group-5 transition metals. Radioisotopes of niobium and tantalum, produced in nuclear fusion evaporation reactions, are directly flushed into the IGC setup by an inert gas-jet. Oxychloride compounds are formed by the addition of SOCl
and O. Parameters influencing the formation and transport of NbOCl and TaOCl are investigated. For nuclides with half-lives (
) of about 30 s, an overall efficiency of 7% is obtained, rendering the IGC setup suitable for the chemical exploration of 
Db( = 34s).
Iwasaki, Sachio; Oka, Makoto; Suzuki, Kei*; Yoshida, Tetsuya*
Physics Letters B, 790, p.71 - 76, 2019/03
Times Cited Count：10 Percentile：71.88(Astronomy & Astrophysics)We find a novel phenomenon induced by the interplay between a strong magnetic field and finite orbital angular momenta in hadronic systems, which is analogous to the Paschen-Back effect observed in the field of atomic physics. This effect allows the wave functions to drastically deform. We discuss anisotropic decay from the deformation as a possibility to measure the strength of the magnetic field in heavy-ion collision at LHC, RHIC and SPS, which has not experimentally been measured. As an example we investigate charmonia with finite orbital angular momentum in a strong magnetic field. We calculate the mass spectra and mixing rate. To obtain anisotropic wave functions, we apply the cylindrical Gaussian expansion method, where the Gaussian bases to expand the wave functions have different widths along transverse and longitudinal directions in the cylindrical coordinate.
Chiera, N. M.; Sato, Tetsuya; Tomitsuka, Tomohiro; Asai, Masato; Suzuki, Hayato*; Tokoi, Katsuyuki; Toyoshima, Atsushi; Tsukada, Kazuaki; Nagame, Yuichiro
Inorganica Chimica Acta, 486, p.361 - 366, 2019/02
Times Cited Count：3 Percentile：18.6(Chemistry, Inorganic & Nuclear)The formation of NbOCl and TaOCl and their adsorption behavior on quartz surfaces was explored by applying an isothermal gas-chromatographic method. Trace amounts of short-lived Nb and Ta isotopes were used. Adsorption enthalpy values (
) at zero surface coverage of -(NbOCl) = 102 
4 kJ/mol and -(TaOCl) = 128 5 kJ/mol were determined by analyzing the chromatographic behavior of the Nb andTa complexes with a Monte-Carlo simulation method based on an adsorption-desorption kinetic model.By applying an empirical correlation, the experimental values were successively related to the macroscopic standard sublimation enthalpy, 
, as a measure of the volatility of each substance. The inferred sublimation enthalpies are in agreement with tabulated thermochemical values. Thus, the linear empirical correlation between and for metal-oxychlorides was updated with the inclusion of the present data. According to the predicted (DbOCl), a (DbOCl) value of 135 2 kJ/mol was extrapolated. The future accomplishment of comparative studies with DbOCl under the same experimental conditions will provide valuable information on the volatility trend in Group-5 elements, together with an indication on the magnitude of relativistic effects on the electronic structure of dubnium.
Koyama, Taku*; Ueno, Kazuki*; Sekine, Mariko*; Matsumoto, Yoshihiro*; Kai, Tetsuya; Shinohara, Takenao; Iikura, Hiroshi; Suzuki, Hiroshi; Kanematsu, Manabu*
Materials Research Proceedings, Vol.4, p.155 - 160, 2018/05
Times Cited Count：0 Percentile：0.18(Materials Science, Characterization & Testing)Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.
Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12
The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.
Yokota, Yuichiro; Funayama, Tomoo; Ikeda, Hiroko; Sakashita, Tetsuya; Suzuki, Michiyo; Kobayashi, Yasuhiko
JAEA-Review 2015-022, JAEA Takasaki Annual Report 2014, P. 67, 2016/02
The role of nitric oxide (NO) in bystander effect was investigated. Human fibroblasts were irradiated with -rays (LET: 0.2 keV/
m) or carbon-ion beam (108 keV/m), and then, co-cultured with the non-irradiated cells. After 24 h culture, the survival rates of non-irradiated cells and the concentrations of nitrate, an oxide of NO, in the medium were measured. The survival rates of non-irradiated cells decreased in dose-dependent and radiation quality-independent manners. Negative relationships between survival rates and nitrite concentrations existed, indicating the amounts of produced NO are an important determinant of bystander effects. Next, a reagent producing two molecules of NO in a half-life of 100 min was added in the culture medium. After incubation of 24 h the survival rates of treated cells did not decrease, suggesting NO produced intracellularly has an important role to lead the bystander effect but is not the signal molecule for intercellular communication.
-tetrafluoroethylene) films using different mediaNuryanthi, N.*; Yamaki, Tetsuya; Kitamura, Akane; Koshikawa, Hiroshi; Yoshimura, Kimio; Sawada, Shinichi; Hasegawa, Shin; Asano, Masaharu; Maekawa, Yasunari; Suzuki, Akihiro*; et al.
Transactions of the Materials Research Society of Japan, 40(4), p.359 - 362, 2015/12
The ion-track grafting of a vinylbenzyl chloride (VBC) into a poly(ethylene-co-tetrafluoroethylene) (ETFE) film is necessary for preparing nanostructured hydroxide-ion-conductive electrolyte membranes. A key for success here is to obtain as high graft levels as possible (for higher conductivity) in a smaller number of tracks (for improving the other membrane properties). To this end, therefore, the effect of the medium for the VBC grafting was investigated as part of our continuing effort to optimize the experimental conditions. A 25 m-thick ETFE film was irradiated in a vacuum chamber with 560 MeV 
Xe at different fluences, and then the grafting was performed by immersing the irradiated films in a 20vol% VBC monomer at 60
C. A medium was a mixture of water (H
O) and isopropyl alcohol (iPrOH) at different volume ratios. The degree of grafting increased as the HO content became higher, and reached a maximum in pure HO. These results can be explained by considering the well-known Trommsdorff effect, in which poor solubility of the grafted polymer in polar media leads to an increased polymerization rate probably due to a lower termination rate.
Dinh, T.-H.*; Suzuki, Yuhei*; Arai, Goki*; Li, B.*; Dunne, P.*; O'Sullivan, G.*; Fujioka, Shinsuke*; Hasegawa, Noboru; Kawachi, Tetsuya; Nishikino, Masaharu; et al.
Applied Physics Letters, 107(12), p.121101_1 - 121101_5, 2015/09
Times Cited Count：5 Percentile：22.94(Physics, Applied)Xu, P. G.; Harjo, S.; Ito, Takayoshi*; Morii, Yukio*; Gong, W.; Suzuki, Hiroshi; Akita, Koichi; Suzuki, Tetsuya*; Tomota, Yo; Lutterotti, L.*
JPS Conference Proceedings (Internet), 8, p.031022_1 - 031022_6, 2015/09
Doshida, Tomoki*; Suzuki, Hiroshi*; Takai, Kenichi*; Hirade, Tetsuya; Oshima, Nagayasu*
NanotechJapan Bulletin (Internet), 8(3), 5 Pages, 2015/07
Studying the creation and time evolution of defects is an important issue for interpreting the hydrogen embrittlement mechanism of steels. We have been studied the relationship between hydrogen embrittlement of high strength steel and lattice defects associated with hydrogen by thermal desorption analysis (TDA) and positron probe microanalyzer (PPMA).
Yamaguchi, Hiroshi*; Ijichi, Ryo*; Suzuki, Yoshiyuki*; Ooka, Sachiyo*; Shimada, Keiji*; Takahashi, Naoki*; Washio, Hidetoshi*; Nakamura, Kazuyo*; Takamoto, Tatsuya*; Imaizumi, Mitsuru*; et al.
Proceedings of 42nd IEEE Photovoltaic Specialists Conference (PVSC-42) (CD-ROM), p.2407 - 2411, 2015/06
mutants to microbeam irradiationSakashita, Tetsuya; Suzuki, Michiyo; Hattori, Yuya; Ikeda, Hiroko; Muto, Yasuko*; Yokota, Yuichiro; Funayama, Tomoo; Hamada, Nobuyuki*; Shirai, Kana*; Kobayashi, Yasuhiko
JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 74, 2015/03
An increasing body of data indicates that ionizing radiation affects the nervous system and alters its function. Recently, we reported that chemotaxis of during the salt chemotaxis learning (SCL), that is conditioned taste aversion to NaCl, was modulated by carbon ion irradiation, i.e. accelerated decrease in chemotaxis to NaCl during the SCL. However, we had no direct evidence for the interaction of ionizing radiation with the central neuronal tissue (nerve ring) in . Microbeam irradiation is useful to analyze direct radiation effects at a cellular or tissue level. Thus, we applied the microbeam irradiation of the nerve ring and examined the effect on the SCL.
