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Journal Articles

Experimental study of Gamow-Teller transitions via the high-energy-resolution $$^{18}$$O($$^3$$He,$$t$$)$$^{18}$$F reaction; Identification of the low-energy "super" -Gamow-Teller state

Fujita, Hirohiko*; Fujita, Yoshitaka*; Utsuno, Yutaka; Yoshida, Kenichi*; Adachi, Tatsuya*; Algora, A.*; Csatl$'o$s, M.*; Deaven, J. M.*; Estevez-Aguado, E.*; Guess, C. J.*; et al.

Physical Review C, 100(3), p.034618_1 - 034618_13, 2019/09

no abstracts in English

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{99m}$$Tc generator by (n,$$gamma$$) method

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Kimura, Akihiro; Shibata, Akira; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2018, P. 155, 2019/08

no abstracts in English

Journal Articles

Template-free fabrication of mesoporous alumina nanospheres using post-synthesis water-ethanol treatment of monodispersed aluminium glycerate nanospheres for molybdenum adsorption

Saptiama, I.*; Kaneti, Y. V.*; Suzuki, Yoshitaka; Tsuchiya, Kunihiko; Fukumitsu, Nobuyoshi*; Sakae, Takeji*; Kim, J.*; Kang, Y.-M.*; Ariga, Katsuhiko*; Yamauchi, Yusuke*

Small, 14(21), p.1800474_1 - 1800474_14, 2018/05

no abstracts in English

Journal Articles

Molybdenum adsorption and desorption properties of alumina with different surface structures for $$^{99}$$Mo/$$^{99m}$$Tc generators

Suzuki, Yoshitaka; Kitagawa, Tomoya*; Namekawa, Yoji*; Matsukura, Minoru*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko

Transactions of the Materials Research Society of Japan, 43(2), p.75 - 80, 2018/04

no abstracts in English

Journal Articles

Molybdenum adsorption properties of alumina-embedded mesoporous silica for medical radioisotope production

Saptiama, I.*; Kaneti, Y. V.*; Oveisi, H.*; Suzuki, Yoshitaka; Tsuchiya, Kunihiko; Takai, Kimiko*; Sakae, Takeji*; Pradhan, S.*; Hossain, M. S. A.*; Fukumitsu, Nobuyoshi*; et al.

Bulletin of the Chemical Society of Japan, 91(2), p.195 - 200, 2018/02

 Times Cited Count:13 Percentile:4.41(Chemistry, Multidisciplinary)

no abstracts in English

JAEA Reports

Establishment of experimental equipments in irradiation technology development building, 2

Shibata, Hiroshi; Nakano, Hiroko; Suzuki, Yoshitaka; Otsuka, Noriaki; Nishikata, Kaori; Takeuchi, Tomoaki; Hirota, Noriaki; Tsuchiya, Kunihiko

JAEA-Testing 2017-002, 138 Pages, 2017/12

JAEA-Testing-2017-002.pdf:9.3MB

From the viewpoints of utilization improvement of the Japan Materials Testing Reactor (JMTR), the experimental devices have been established for the out-pile tests in the irradiation technology development building. The devices for the irradiation capsule assembly, material tests and inspections were established at first and experimental data were accumulated before the neutron irradiation tests. On the other hand, after the Great East Japan Earthquake, the repairs and earthquake-resistant measures of the existing devices were carried out. New devices and equipments were also established for the R&D program for power plant safety enhancement of the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry (METI) and $$^{99}$$Mo/$$^{99m}$$Tc production development under the Tsukuba International Strategic Zone. This report describes the outline and basic operation manuals of the devices established from 2011 to 2016 and the management points for the safety works in the irradiation technology development building.

Journal Articles

Mesoporous alumina as an effective adsorbent for molybdenum (Mo) toward Instant production of radioisotope for medical use

Saptiama, I.*; Kaneti, Y. V.*; Suzuki, Yumi*; Suzuki, Yoshitaka; Tsuchiya, Kunihiko; Sakae, Takeji*; Takai, Kimiko*; Fukumitsu, Nobuyoshi*; Alothman, Z. A.*; Hossain, M. S. A.*; et al.

Bulletin of the Chemical Society of Japan, 90(10), p.1174 - 1179, 2017/10

 Times Cited Count:23 Percentile:7.51(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

Radioactive strontium measurement using ICP-MS following cascade preconcentration and separation system

Takagai, Yoshitaka*; Furukawa, Makoto*; Kameo, Yutaka; Matsueda, Makoto; Suzuki, Katsuhiko*

Bunseki Kagaku, 66(4), p.223 - 231, 2017/04

 Times Cited Count:2 Percentile:70.83(Chemistry, Analytical)

no abstracts in English

JAEA Reports

Preliminary tests on adsorption / desorption of alumina adsorbents

Suzuki, Yoshitaka; Ishida, Takuya*; Suzuki, Yumi*; Matsukura, Minoru*; Kurosaki, Fumio*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko

JAEA-Technology 2016-027, 24 Pages, 2016/12

JAEA-Technology-2016-027.pdf:4.15MB

The research and development (R&D) on the production of $$^{99}$$Mo/$$^{99m}$$Tc by (n,$$gamma$$) method has been carried out in the Neutron Irradiation and Testing Reactor Center. The $$^{99}$$Mo production by (n,$$gamma$$) reaction is a simple and easy method, and it also is advantageous from viewpoints of nuclear proliferation resistance and waste management. However, it is difficult to produce the $$^{99m}$$Tc solution with high radioactive concentration because the specific radioactivity of $$^{99}$$Mo by this method is extremely low. Up to now, various Mo absorbents such as Polyzirconium Compound (PZC) and Polytitanium Compound (PTC) have been developed with high Mo adsorption efficiency. It is necessary for utilization to the generator of these absorbents to evaluate the effect of elements containing these absorbents and to assure the quality of $$^{99m}$$Tc solution. In this report, the status of R&D of the Mo adsorbents was investigated. The alumina as Mo adsorbent, which uses in medical $$^{99}$$Mo/$$^{99m}$$Tc generator, was focused and Mo adsorption/desorption properties of three kinds of alumina was evaluated by different properties such as crystal structure and specific surface.

Journal Articles

Neutron irradiation effect of high-density MoO$$_{3}$$ pellets for Mo-99 production, 3

Ishida, Takuya; Suzuki, Yoshitaka; Nishikata, Kaori; Yonekawa, Minoru; Kato, Yoshiaki; Shibata, Akira; Kimura, Akihiro; Matsui, Yoshinori; Tsuchiya, Kunihiko; Sano, Tadafumi*; et al.

KURRI Progress Report 2015, P. 64, 2016/08

no abstracts in English

JAEA Reports

Decommissioning activities and R&D of nuclear facilities in the second midterm plan

Terunuma, Akihiro; Mimura, Ryuji; Nagashima, Hisao; Aoyagi, Yoshitaka; Hirokawa, Katsunori*; Uta, Masato; Ishimori, Yuu; Kuwabara, Jun; Okamoto, Hisato; Kimura, Yasuhisa; et al.

JAEA-Review 2016-008, 98 Pages, 2016/07

JAEA-Review-2016-008.pdf:11.73MB

Japan Atomic Energy Agency formulated the plan to achieve the medium-term target in the period of April 2010 to March 2015(hereinafter referred to as "the second medium-term plan"). JAEA determined the plan for the business operations of each year (hereinafter referred to as "the year plan"). This report is that the Sector of Decommissioning and Radioactive Waste Management has summarized the results of the decommissioning technology development and decommissioning of nuclear facilities which were carried out in the second medium-term plan.

Journal Articles

Technical estimation for mass production of highly-concentrated $$^{rm 99m}$$Tc solution from $$^{99}$$Mo to be obtained by ($$n,gamma$$) reaction; A Preliminary study using inactive Re instead of $$^{rm 99m}$$Tc

Tanase, Masakazu*; Fujisaki, Saburo*; Ota, Akio*; Shiina, Takayuki*; Yamabayashi, Hisamichi*; Takeuchi, Nobuhiro*; Tsuchiya, Kunihiko; Kimura, Akihiro; Suzuki, Yoshitaka; Ishida, Takuya; et al.

Radioisotopes, 65(5), p.237 - 245, 2016/05

no abstracts in English

Journal Articles

Real-time observation of rotational twin formation during molecular-beam epitaxial growth of GaAs on Si (111) by X-ray diffraction

Suzuki, Hidetoshi*; Nakata, Yuka*; Takahashi, Masamitsu; Ikeda, Kazuma*; Oshita, Yoshio*; Morohara, Osamu*; Geka, Hirotaka*; Moriyasu, Yoshitaka*

AIP Advances (Internet), 6(3), p.035303_1 - 035303_6, 2016/03

 Times Cited Count:3 Percentile:66.57(Nanoscience & Nanotechnology)

JAEA Reports

Performance tests of radiation detectors for inspection of $$^{99}$$Mo/$$^{99m}$$Tc solution, 1

Suzuki, Yumi*; Nakano, Hiroko; Suzuki, Yoshitaka; Ishida, Takuya; Shibata, Akira; Kato, Yoshiaki; Kawamata, Kazuo; Tsuchiya, Kunihiko

JAEA-Technology 2015-031, 58 Pages, 2015/11

JAEA-Technology-2015-031.pdf:14.57MB

Technetium-99m ($$^{99m}$$Tc) is one of the most commonly used radioisotopes in the field of nuclear medicine. In the Japan Atomic Energy Agency (JAEA), the research and development (R&D) have been carried out for production of molybdenum-99 ($$^{99}$$Mo) by (n, $$gamma$$) method, a parent nuclide of $$^{99m}$$Tc, with the Japan Material Testing Reactor (JMTR). On the other hand, the new project as "Domestic Production of Medical Radioisotope (Technetium preparation) in Japan" was adopted in the Tsukuba International Strategic Zone on October, 2013 and the demonstration tests will be planned for the domestic production of $$^{99}$$Mo/$$^{99m}$$Tc with the JMTR. Thus, new facilities and analysis devices were equipped in the JMTR hot laboratory in 2014 as the part of this project. As the part of the analytical device equipment, the $$gamma$$-TLC analyzer and the radiation detector connected with the High Performance Liquid Chromatography (HPLC) were installed for quality inspection of the $$^{99}$$Mo/$$^{99m}$$Tc solution and the extracted $$^{99m}$$Tc solution in the JMTR hot laboratory. The performance tests of these devices such as detection sensitivity, resolution, linearity and selectivity of energy range were carried out with $$^{137}$$Cs and $$^{152}$$Eu as alternative radionuclides of $$^{99}$$Mo and $$^{99m}$$Tc, respectively. In the results, bright prospects were obtained concerning the quality inspection of the $$^{99}$$Mo/$$^{99m}$$Tc and $$^{99m}$$Tc solutions using these devices. This report describes the results of those performance tests.

Journal Articles

Effects of thermal aging on microstructure and hardness of stainless steel weld-overlay claddings of nuclear reactor pressure vessels

Takeuchi, Tomoaki; Kakubo, Yuta*; Matsukawa, Yoshitaka*; Nozawa, Yasuko*; Toyama, Takeshi*; Nagai, Yasuyoshi*; Nishiyama, Yutaka; Katsuyama, Jinya; Yamaguchi, Yoshihito; Onizawa, Kunio; et al.

Journal of Nuclear Materials, 452(1-3), p.235 - 240, 2014/09

 Times Cited Count:19 Percentile:5.58(Materials Science, Multidisciplinary)

Microstructures and hardness of stainless steel weld overlay cladding of reactor pressure vessels subjected to the thermal aging at 400 $$^{circ}$$C for 100-10,000 h were investigated using atom probe tomography and nanoindentation technique. The Cr concentration fluctuation in the $$delta$$-ferrite phase caused by spinodal decomposition rapidly progressed by the 100 h aging while NiSiMn clusters increased in number density at 2,000 h and coarsened at 10,000 h. The hardness of the $$delta$$-ferrite phase also rapidly increased at the short aging time. The Cr concentration fluctuation and the hardness were in good correlation with the degree of the Cr concentration fluctuation rather than the formation of the NiSiMn clusters. These results strongly suggested that the dominant factor of the hardening of the $$delta$$-ferrite phase by the thermal aging was Cr spinodal decomposition.

Journal Articles

Comparative study on annual $$^{137}$$Cs discharge rates after the Fukushima Dai-ichi Nuclear Power Plant accident from two distinct watershed simulation models

Kitamura, Akihiro; Imaizumi, Yoshitaka*; Yamaguchi, Masaaki; Yui, Mikazu; Suzuki, Noriyuki*; Hayashi, Seiji*

Kankyo Hoshano Josen Gakkai-Shi, 2(3), p.185 - 192, 2014/09

Annual discharge rates of radioactive cesium through selected rivers due to the Fukushima Dai-ichi Nuclear Power Plant accident were simulated by two different watershed models. One is the Soil and Cesium Transport, SACT, model which was developed by Japan Atomic Energy Agency and the other one is the Grid-Catchment Integrated Modeling System, G-CIEMS, which was developed by National Institute of Environmental Studies. We choose the Abukuma, the Ukedo, and the Niida rivers for the present study. Comparative results showed that while components and assumptions adopted in two models differ, both methods predicted the same order of magnitude estimates.

Journal Articles

Rapid analysis of radioactive strontium by induction coupled plasma mass spectrometry

Takagai, Yoshitaka*; Furukawa, Makoto*; Kameo, Yutaka; Suzuki, Katsuhiko*

Isotope News, (721), p.2 - 7, 2014/05

no abstracts in English

JAEA Reports

Disassembly of JT-60 tokamak device and ancillary facilities for JT-60 tokamak

Okano, Fuminori; Ichige, Hisashi; Miyo, Yasuhiko; Kaminaga, Atsushi; Sasajima, Tadayuki; Nishiyama, Tomokazu; Yagyu, Junichi; Ishige, Yoichi; Suzuki, Hiroaki; Komuro, Kenichi; et al.

JAEA-Technology 2014-003, 125 Pages, 2014/03

JAEA-Technology-2014-003.pdf:13.32MB

The disassembly of JT-60 tokamak device and its peripheral equipments, where the total weight was about 5400 tons, started in 2009 and accomplished in October 2012. This disassembly was required process for JT-60SA project, which is the Satellite Tokamak project under Japan-EU international corroboration to modify the JT-60 to the superconducting tokamak. This work was the first experience of disassembling a large radioactive fusion device based on Radiation Hazard Prevention Act in Japan. The cutting was one of the main problems in this disassembly, such as to cut the wielded parts together with toroidal field coils, and to cut the vacuum vessel into two. After solving these problems, the disassembly completed without disaster and accident. This report presents the outline of the JT-60 disassembly, especially tokamak device and ancillary facilities for tokamak device.

Journal Articles

Sequential inductively coupled plasma quadrupole mass-spectrometric quantification of radioactive strontium-90 incorporating cascade separation steps for radioactive contamination rapid survey

Takagai, Yoshitaka*; Furukawa, Makoto*; Kameo, Yutaka; Suzuki, Katsuhiko*

Analytical Methods, 6(2), p.355 - 362, 2014/01

 Times Cited Count:32 Percentile:3.26(Chemistry, Analytical)

Radioactive strontium-90 ($$^{90}$$Sr) scattered by nuclear power plant accident was specifically determined by conventional inductively coupled plasma quadrupole mass-spectrometry (ICP-QMS) preceded by on-line chelate column separation and oxygen reaction. After implementing the cascade-step, the detection limit (DL) of quantitative ICP-QMS of $$^{90}$$Sr from spiked water samples was 2.85 Bq/L (equivalent to 0.56 ppq). Analysis of microwave-digested soil yielded a DL of 4.73 Bq/kg (equivalent to 0.93 ppq). The $$^{90}$$Sr from environmental contaminated soil samples ranged from 63 Bq/kg to 89 Bq/kg, with no statistical difference between the proposed and general methods at 98% confidence level.

JAEA Reports

Disassembly of JT-60 tokamak device

Okano, Fuminori; Ikeda, Yoshitaka; Sakasai, Akira; Hanada, Masaya; Ichige, Hisashi; Miyo, Yasuhiko; Kaminaga, Atsushi; Sasajima, Tadayuki; Nishiyama, Tomokazu; Yagyu, Junichi; et al.

JAEA-Technology 2013-031, 42 Pages, 2013/11

JAEA-Technology-2013-031.pdf:18.1MB

The disassembly of JT-60 tokamak device and its peripheral equipments, where the total weight was about 6200 tons, started in 2009 and accomplished in October 2012. This disassembly was required process for JT-60SA project, which is the Satellite Tokamak project under Japan-EU international corroboration to modify the JT-60 to the superconducting tokamak. This work was the first experience of disassembling a large radioactive fusion device based on Radiation Hazard Prevention Act in Japan. The cutting was one of the main problems in this disassembly, such as to cut the wielded parts together with toroidal field coils, and to cut the vacuum vessel into two. After solving these problems, the disassembly completed without disaster and accident. This report presents the outline of the JT-60 disassembly, especially tokamak device.

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