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Journal Articles

Quasielastic neutron scattering probing H$$^{-}$$ dynamics in the H$$^{-}$$ conductors LaH$$_{3-2x}$$O$$_{x}$$

Tamatsukuri, Hiromu; Fukui, Keiga*; Iimura, Soshi*; Honda, Takashi*; Tada, Tomofumi*; Murakami, Yoichi*; Yamaura, Junichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Yamada, Takeshi*; et al.

Physical Review B, 107(18), p.184114_1 - 184114_8, 2023/05

https://doi.org/10.1103/PhysRevB.107.184114
 Times Cited Count：0 Percentile：0(Materials Science, Multidisciplinary)

Journal Articles

Electrical and magnetic properties of a single crystal UCu$$_2$$Si$$_2$$

Matsuda, Tatsuma; Haga, Yoshinori; Ikeda, Shugo; Galatanu, A.; Yamamoto, Etsuji; Shishido, Hiroaki*; Yamada, Mineko*; Yamaura, Junichi*; Hedo, Masato*; Uwatoko, Yoshiya*; et al.

Journal of the Physical Society of Japan, 74(5), p.1552 - 1556, 2005/05

https://doi.org/10.1143/JPSJ.74.1552
 Times Cited Count：24 Percentile：72.16(Physics, Multidisciplinary)

We have succeeded in growing a high-quality single crystal of UCu$$_2$$Si$$_2$$ with the tetragonal structure by the Sn-flux method and measured the electrical resistivity, magnetic susceptibility, magnetization and specific heat. UCu$$_2$$Si$$_2$$ is found to order antiferromagnetically below $$T_{rm N}$$ = 106 K, and follows a successive ferromagnetic ordering at $$T_{rm C}$$ = 100 K. The magnetic properties are highly anisotropic, reflecting the crystal structure. An easy-axis of magnetization is found to be the [001] direction ($$c$$-axis) both in the antiferromagnetic and ferromagnetic phases, while the [100] direction ($$a$$-axis) corresponds to the hard-axis in magnetization. The magnetization curve in the antiferromagnetic phase indicates a clear metamagnetic transition at a low field of about 1 kOe and changes smoothly into a ferromagnetic magnetization curve below $$T_{rm C}$$ = 100 K. The saturation moment is determined as 1.75$$mu_{rm B}$$/U at 2 K. The electronic specific heat coefficient is also determined as 20 mJ/K$$^2$$$$cdot$$mol.

Oral presentation

Quasielastic neutron scattering probing H$$^{-}$$ dynamics in the H$$^{-}$$ conductors LaH$$_{3-2x}$$O$$_{x}$$

Tamatsukuri, Hiromu; Fukui, Keiga*; Iimura, Soshi*; Honda, Takashi*; Tada, Tomofumi*; Murakami, Yoichi*; Yamaura, Junichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Yamada, Takeshi*; et al.

no journal, , 

no abstracts in English

Oral presentation

Quasielastic neutron scattering probing H$$^{-}$$ dynamics in the H$$^{-}$$ conductors LaH$$_{3-2x}$$O$$_{x}$$

Tamatsukuri, Hiromu; Fukui, Keiga*; Iimura, Soshi*; Honda, Takashi*; Tada, Tomofumi*; Murakami, Yoichi*; Yamaura, Junichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Yamada, Takeshi*; et al.

no journal, , 

no abstracts in English

Oral presentation

Quasielastic neutron scattering probing H$$^{-}$$ dynamics in the H$$^{-}$$ conductors LaH$$_{3-2x}$$O$$_{x}$$

Tamatsukuri, Hiromu; Fukui, Keiga*; Iimura, Soshi*; Honda, Takashi*; Tada, Tomofumi*; Murakami, Yoichi*; Yamaura, Junichi*; Kuramoto, Yoshio*; Sagayama, Hajime*; Yamada, Takeshi*; et al.

no journal, , 

A series of oxyhydrides LaH$$_{3-2x}$$O$$_{x}$$ exhibits characteristic high H$$^{-}$$ conductivity. In this study, we performed the incoherent quasielastic neutron scattering measurements to investigate H$$^{-}$$ dynamics in LaH$$_{3-2x}$$O$$_{x}$$. We successfully identify two kinds of microscopic H$$^{-}$$ dynamics in the end member LaH$$_{3}$$; the jump diffusion and the localized back and forth jump between neighboring tetrahedral and octahedral sites. These dynamics have the common elementary jump process between the Tet and adjacent Oct sites, and become more conspicuous with increasing a concentration of H$$^{-}$$. Based on these results, we discuss that the origin of the high H$$^{-}$$ conductivity in this system is explained by a so-called concerted migration model.

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