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Journal Articles

Transverse asymmetry of individual $$gamma$$ rays in the $$^{139}$$La($$overrightarrow{n},gamma$$)$$^{140}$$La reaction

Okuizumi, Mao*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ino, Takashi*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; et al.

Physical Review C, 111(3), p.034611_1 - 034611_6, 2025/03

JAEA Reports

Analysis work on flush-out of plutonium and uranium for decommissioning of main plant in Tokai Reprocessing Plant

Sato, Hinata; Mori, Amami; Kuno, Sorato; Horigome, Kazushi; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo

JAEA-Technology 2024-011, 56 Pages, 2024/10

JAEA-Technology-2024-011.pdf:2.5MB

Flush-out, which recovers remaining nuclear materials in the process and transfer it to a highly radioactive liquid waste storage tank, has been performed at main plant of Tokai Reprocessing Plant. The flush-out has been composed from three steps: first step is to remove of spent fuel sheared powder, second step is to collect plutonium solution stored in the process, and third step is to convert uranium solution into uranium trioxide powder. The first step of flush-out activity has been completed in 2022. Second and third steps of flush-out have been completed from March 2023 to February 2024. Process control analysis has been performed for operation of the facility, and material accountancy analysis has been performed to control the accountancy of nuclear materials. In addition, related analytical work such as pretreatment for transporting inspection samples for safeguards analysis laboratories in IAEA has been also performed. This report describes results of analytical work performed in collections of plutonium and uranium solutions in second and third steps of the flush-out, including calibration of analytical equipment, waste generation, and education and training of analytical operator.

Journal Articles

Analysis of nuclear materials in process solution during flush-out activities for decommissioning of reprocessing plant

Yamamoto, Masahiko; Horigome, Kazushi; Goto, Yuichi; Taguchi, Shigeo

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

Flush-out activities of Tokai Reprocessing Plant were completed in February, 2024. Since it contained remaining nuclear materials in main process of the facility, purpose of activities was to flush-out them and to rinse with nitric acid solution. This paper describes analysis of nuclear materials related to flush-out activities.

Journal Articles

Circular polarization measurement for individual gamma rays in capture reactions with intense pulsed neutrons

Endo, Shunsuke; Abe, Ryota*; Fujioka, Hiroyuki*; Ino, Takashi*; Iwamoto, Osamu; Iwamoto, Nobuyuki; Kawamura, Shiori*; Kimura, Atsushi; Kitaguchi, Masaaki*; Kobayashi, Ryuju*; et al.

European Physical Journal A, 60(8), p.166_1 - 166_10, 2024/08

 Times Cited Count:0 Percentile:0.00(Physics, Nuclear)

Journal Articles

Globular pattern formation of hierarchical ceria nanoarchitectures

Aoyagi, Noboru; Motokawa, Ryuhei; Okumura, Masahiko; Ueda, Yuki; Saito, Takumi*; Nishitsuji, Shotaro*; Taguchi, Tomitsugu*; Yomogida, Takumi; Sazaki, Gen*; Ikeda, Atsushi

Communications Chemistry (Internet), 7, p.128_1 - 128_13, 2024/06

 Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)

Journal Articles

Spin dependence in the $$p$$-wave resonance of $$^{139}$$$overrightarrow{textrm{La}}$+$overrightarrow{n}$

Okudaira, Takuya*; Nakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.

Physical Review C, 109(4), p.044606_1 - 044606_9, 2024/04

 Times Cited Count:0 Percentile:0.00(Physics, Nuclear)

Journal Articles

High sensitivity of a future search for effects of $$P$$-odd/$$T$$-odd interactions on the 0.75 eV $$p$$-wave resonance in $$overrightarrow{n}$$+$$^{139}overrightarrow{textrm{La}}$$ forward transmission determined using a pulsed neutron beam

Nakabe, Rintaro*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Gudkov, V.*; Hirota, Katsuya*; Ide, Ikuo*; Ino, Takashi*; Ishikado, Motoyuki*; Kambara, Wataru*; et al.

Physical Review C, 109(4), p.L041602_1 - L041602_4, 2024/04

 Times Cited Count:0 Percentile:0.00(Physics, Nuclear)

Journal Articles

Hot cell equipment improvement effortsat Analytical Laboratory in Tokai Reprocessing Plant

Ishibashi, Atsushi; Masui, Kenji; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo; Ishikawa, Satoshi*; Ishikawa, Tomoya*

Nihon Hozen Gakkai Dai-19-Kai Gakujutsu Koenkai Yoshishu, p.18 - 21, 2023/08

An inner-box typed hot cell for analysis of highly radioactive samples has been operated for about 40 years in Tokai Reprocessing Plant since its installation in 1980. During the operation of analytical hot cell, improvement and upgrades including auxiliary equipment have been performed, in addition to keep the equipment in proper condition through periodic inspections and maintenance. This paper describes about these efforts for analytical hot cell and its results.

JAEA Reports

Analysis work report on removal of spent fuel sheared powder for decommissioning of main plant

Aoya, Juri; Mori, Amami; Sato, Hinata; Kono, Soma; Morokado, Shiori; Horigome, Kazushi; Goto, Yuichi; Yamamoto, Masahiko; Taguchi, Shigeo

JAEA-Technology 2023-008, 34 Pages, 2023/06

JAEA-Technology-2023-008.pdf:1.92MB

Flush-out, by which nuclear materials in the Tokai Reprocessing Plant process are recovered, has been started in June 2022 as the first step of decommissioning. Flush-out consists of removal of spent fuel sheared powder, plutonium solution, uranium solution, and the other nuclear materials. Removal of spent fuel sheared powder has been completed in September 2022. During removal of spent fuel sheared powder, uranium concentration, plutonium concentration, acid concentration, radioactivity concentration, and solution density have been analyzed for process control. For nuclear material accountancy, uranium concentration, plutonium concentration, isotope ratio, and solution density have been analyzed. Analysis work including sample pretreatment before transportation to IAEA analytical facility for safeguards, and the other operations related to Flush-out such as calibration of analytical instruments, education, and training of operators are reported.

Journal Articles

Angular distribution of $$gamma$$ rays from a neutron-induced $$p$$-wave resonance of $$^{132}$$Xe

Okudaira, Takuya*; Tani, Yuika*; Endo, Shunsuke; Doskow, J.*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kameda, Kento*; Kimura, Atsushi; Kitaguchi, Masaaki*; Luxnat, M.*; et al.

Physical Review C, 107(5), p.054602_1 - 054602_7, 2023/05

 Times Cited Count:4 Percentile:73.33(Physics, Nuclear)

no abstracts in English

Journal Articles

Estimation of the total angular momentum of resonances using low-energy gamma-rays in $$^{181}$$Ta(n,$$gamma$$)$$^{182}$$Ta reaction

Kawamura, Shiori*; Endo, Shunsuke; Iwamoto, Osamu; Iwamoto, Nobuyuki; Kimura, Atsushi; Kitaguchi, Masaaki*; Nakamura, Shoji; Okudaira, Takuya*; Rovira Leveroni, G.; Shimizu, Hirohiko*; et al.

JAEA-Conf 2023-001, p.115 - 120, 2023/02

no abstracts in English

Journal Articles

Measurement of the transverse asymmetry of $$gamma$$ rays in the $$^{117}$$Sn($$n,gamma$$)$$^{118}$$Sn reaction

Endo, Shunsuke; Okudaira, Takuya*; Abe, Ryota*; Fujioka, Hiroyuki*; Hirota, Katsuya*; Kimura, Atsushi; Kitaguchi, Masaaki*; Oku, Takayuki; Sakai, Kenji; Shima, Tatsushi*; et al.

Physical Review C, 106(6), p.064601_1 - 064601_7, 2022/12

 Times Cited Count:5 Percentile:64.05(Physics, Nuclear)

no abstracts in English

Journal Articles

Evaluation of analyzing power of gamma-ray polarimeter

Endo, Shunsuke; Shizuma, Toshiyuki*; Zen, H.*; Taira, Yoshitaka*; Omer, M.; Kawamura, Shiori*; Abe, Ryota*; Okudaira, Takuya*; Kitaguchi, Masaaki*; Shimizu, Hirohiko*

UVSOR-49, P. 38, 2022/08

Journal Articles

Development of a local exhaust device for removal of radioactive waste from glove-box for handling nuclear fuel materials

Ishibashi, Atsushi; Saegusa, Yu; Aoya, Juri; Yamamoto, Masahiko; Taguchi, Shigeo; Kuno, Takehiko

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.241 - 244, 2022/07

no abstracts in English

Journal Articles

Surface nanostructures on Nb-doped SrTiO$$_{3}$$ irradiated with swift heavy ions at grazing incidence

Ishikawa, Norito; Fujimura, Yuki; Kondo, Keietsu; Szabo, G. L.*; Wilhelm, R. A.*; Ogawa, Hiroaki; Taguchi, Tomitsugu*

Nanotechnology, 33(23), p.235303_1 - 235303_10, 2022/06

 Times Cited Count:7 Percentile:57.43(Nanoscience & Nanotechnology)

A single crystal of SrTiO$$_{3}$$ doped with niobium (Nb-STO) was irradiated with 200 MeV Au ions at grazing incidence. Atomic force microscopy (AFM) and scanning electron microscopy (SEM) are used to study the relation between irradiation-induced change of surface topography and corresponding material property changes. As expected, multiple hillocks as high as 5-6 nm are imaged by AFM observation. It is also found that the region in between the adjacent hillocks is slightly elevated rather than depressed. Line-like contrasts along the ion paths are found in both AFM phase images and SEM images, indicating the formation of continuous ion tracks in addition to multiple hillocks. Cross-sectional transmission electron microscopy (TEM) observation shows that the ion tracks in the near-surface region are found to be relatively large, whereas buried ion tracks in the deeper region are relatively small. The results suggest that recrystallization plays an important role in the formation of small ion tracks in the deep region, whereas formation of large ion tracks in the near-surface region is likely due to the absence of recrystallization.

Journal Articles

Angular distribution of $$gamma$$ rays from the $$p$$-wave resonance of $$^{118}$$Sn

Koga, Jun*; Takada, Shusuke*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Niinomi, Yudai*; Okudaira, Takuya*; et al.

Physical Review C, 105(5), p.054615_1 - 054615_5, 2022/05

 Times Cited Count:6 Percentile:69.74(Physics, Nuclear)

no abstracts in English

Journal Articles

Project management efforts in the decommissioning project of Tokai Reprocessing Plant

Taguchi, Shigeo; Taguchi, Katsuya; Makino, Risa; Yamanaka, Atsushi; Suzuki, Kazuyuki; Takano, Masato; Koshino, Katsuhiko; Ishida, Michihiko; Nakano, Takafumi; Yamaguchi, Toshiya

Nihon Hozen Gakkai Dai-17-Kai Gakujutsu Koenkai Yoshishu, p.499 - 502, 2021/07

In 2018, Tokai Reprocessing Plan (TRP) shifted to the decommissioning stage. In order to proceed with steady decommissioning work, TRP effort to enhance project management function. This paper describes the establishment and role of the Decommissioning Project Management Office, effectiveness of applying the project management tool and its utilization concept, and the method of materialize the equipment dismantling plan.

Journal Articles

Energy-dependent angular distribution of individual $$gamma$$ rays in the $$^{139}$$La($$n, gamma$$)$$^{140}$$La$$^{ast}$$ reaction

Okudaira, Takuya*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; Niinomi, Yudai*; Sakai, Kenji; et al.

Physical Review C, 104(1), p.014601_1 - 014601_6, 2021/07

 Times Cited Count:6 Percentile:60.24(Physics, Nuclear)

Journal Articles

Radiation dose rate effects on the properties of a laser-induced breakdown spectroscopy system developed using a ceramics micro-laser for fiber-optic remote analysis

Tamura, Koji; Oba, Hironori; Saeki, Morihisa; Taguchi, Tomitsugu*; Lim, H. H.*; Taira, Takunori*; Wakaida, Ikuo

Journal of Nuclear Science and Technology, 58(4), p.405 - 415, 2021/04

 Times Cited Count:15 Percentile:83.18(Nuclear Science & Technology)

Radiation dose rate effects on the properties of a compact fiber-optic laser-induced breakdown spectroscopy (LIBS) system with a monolithic Nd:YAG/Cr:YAG composite ceramics were investigated for remote analysis in hazardous environment. To investigate radiation effects on the LIBS signal, properties related to the Nd:YAG laser operation such as oscillation threshold, output energy, oscillation timing, temporal pulse shape, and beam profile were measured as a function of the radiation dose rate from 0 to 10 kGy/hr in view of their influences to the signal. LIBS spectra of zirconium metal were measured under irradiation. Although signal intensity decreased considerably by irradiation, informative spectra were well obtained even at the maximum radiation dose rate. From the comparison of the LIBS-related parameters among the laser properties, signal reduction was mainly ascribed to the pulse energy reduction. Scintillation emission spectra were also measured from the ceramics during the irradiation, where the signal intensity increased linearly with the dose rate. The results show that the developed system.

Journal Articles

Determination of alkali and alkaline earth elements in radioactive waste generated from reprocessing plant by liquid electrode plasma optical emission spectrometry

Yamamoto, Masahiko; Do, V. K.; Taguchi, Shigeo; Kuno, Takehiko; Takamura, Yuzuru*

Journal of Radioanalytical and Nuclear Chemistry, 327(1), p.433 - 444, 2021/01

 Times Cited Count:0 Percentile:0.00(Chemistry, Analytical)

A simple, practical, and reliable analytical method for determination of Na, K, Ca, Sr, and Ba by liquid electrode plasma optical emission spectrometry is developed. Appropriate emission lines for quantification, interferences from co-existing elements, and effect of measurement conditions with cell damage have been investigated. The spike and recovery tests using actual sample have been performed for method validation, and negligible sample matrix effect has been observed. Consequently, the method is successfully applied to several radioactive wastes. The obtained data have been agreed well with data from computer calculation and inductively coupled plasma optical emission spectrometry within 10% difference.

424 (Records 1-20 displayed on this page)