Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
-ray beam measurementsOmer, M.; Shizuma, Toshiyuki*; Koizumi, Mitsuo; Taira, Yoshitaka*; Zen, H.*; Ogaki, Hideaki*; Hajima, Ryoichi*
Radiation Physics and Chemistry, 240, p.113467_1 - 113467_8, 2026/03
Times Cited Count:1 Percentile:50.28(Chemistry, Physical)Yang, Y.*; Taira, Yoshitaka*; Shizuma, Toshiyuki*; Omer, M.
Proceedings of 16th International Particle Accelerator Conference (IPAC25) (Internet), p.194 - 196, 2025/11
Taira, Yoshitaka*; Yang, Y.*; Shizuma, Toshiyuki*; Omer, M.
Physical Review Research (Internet), 7(3), p.033130_1 - 033130_17, 2025/08
Endo, Shunsuke; Abe, Ryota*; Fujioka, Hiroyuki*; Ino, Takashi*; Iwamoto, Osamu; Iwamoto, Nobuyuki; Kawamura, Shiori*; Kimura, Atsushi; Kitaguchi, Masaaki*; Kobayashi, Ryuju*; et al.
European Physical Journal A, 60(8), p.166_1 - 166_10, 2024/08
Times Cited Count:5 Percentile:73.54(Physics, Nuclear)Omer, M.; Shizuma, Toshiyuki*; Koizumi, Mitsuo; Taira, Yoshitaka*; Zen, H.*; Ogaki, Hideaki*; Hajima, Ryoichi
UVSOR-50, P. 37, 2023/08
no abstracts in English
Taira, Yoshitaka*; Endo, Shunsuke; Kawamura, Shiori*; Nambu, Taro*; Okuizumi, Mao*; Shizuma, Toshiyuki*; Omer, M.; Zen, H.*; Okano, Yasuaki*; Kitaguchi, Masaaki*
Physical Review A, 107(6), p.063503_1 - 063503_10, 2023/06
Times Cited Count:10 Percentile:71.80(Optics)no abstracts in English
Endo, Shunsuke; Shizuma, Toshiyuki*; Zen, H.*; Taira, Yoshitaka*; Omer, M.; Kawamura, Shiori*; Abe, Ryota*; Okudaira, Takuya*; Kitaguchi, Masaaki*; Shimizu, Hirohiko*
UVSOR-49, P. 38, 2022/08
Al
Ga
O
scintillators by gamma-ray-induced positron annihilation lifetime spectroscopyFujimori, Kosuke*; Kitaura, Mamoru*; Taira, Yoshitaka*; Fujimoto, Masaki*; Zen, H.*; Watanabe, Shinta*; Kamada, Kei*; Okano, Yasuaki*; Kato, Masahiro*; Hosaka, Masahito*; et al.
Applied Physics Express, 13(8), p.085505_1 - 085505_4, 2020/08
Times Cited Count:7 Percentile:29.72(Physics, Applied)To clarify the existence of cation vacancies in Ce-doped Gd
Al
Ga
O
(Ce:GAGG) scintillators, we performed gamma-ray-induced positron annihilation lifetime spectroscopy (GiPALS). GiPAL spectra of GAGG and Ce:GAGG comprised two exponential decay components, which were assigned to positron annihilation at bulk and defect states. By an analogy with Ce:Y
Al
O
, the defect-related component was attributed to Al/Ga-O divacancy complexes. This component was weaker for Ce, Mg:GAGG, which correlated with the suppression of shallow electron traps responsible for phosphorescence. Oxygen vacancies were charge compensators for Al/Ga vacancies. The lifetime of the defect-related component was significantly changed by Mg co-doping. This was understood by considering aggregates of Mg
ions at Al/Ga sites with oxygen vacancies, which resulted in the formation of vacancy clusters.
Yamamoto, Ryohei*; Sugita, Kento*; Taira, Yoshitaka*; Hirade, Tetsuya
no journal, ,
Age-Momentum Correlation (AMOC) can observe the Doppler broadening of time-resolved annihilation gamma rays. The annihilation rate depends on the positron state, and it is possible to know if positrons are trapped in structural defects in a sample. Moreover, the Doppler broadening gives the information of impurities around the defects. Positrons from radioactive isotopes cannot penetrate a deep region of bulk material. The application of radioisotopes is difficult for the measurements under severe conditions such as in high pressure or a high temperature. Therefore, we have developed a GiAMOC (Gamma-ray induced AMOC) system, which is a measurement method for generating positrons in a sample using inverse Thomson scattered gamma rays in UVSOR-III. In addition, the developed measurement system was used to measure the reference material for positron lifetime measurement.
Taira, Yoshitaka*; Sugita, Kento*; Okano, Yasuaki*; Fujimoto, Masaki*; Hirade, Tetsuya
no journal, ,
Positron annihilation spectroscopy is a powerful analytical method that can observe single-atom vacant defects in crystals and micro voids in insulating materials. UVSOR-III installed at the Institute of Molecular Science is promoting the development and user use of Gamma-ray induced positron annihilation spectroscopy (GiPAS) by ultrashort pulse gamma rays. Since the ultrashort pulse gamma rays generate positrons inside the material by pair production, positron annihilation experiments of bulk materials with a thickness of several cm can be performed non-destructively. We have succeeded in the generation of ultrashort pulse gamma rays and positron annihilation experiments such as the lifetime measurement and the positron age-momentum correlation measurement.
Taira, Yoshitaka*; Sugita, Kento*; Yamamoto, Ryohei*; Okano, Yasuaki*; Hirade, Tetsuya
no journal, ,
Positron annihilation spectroscopy is a powerful analytical method to observe single-atom vacant defects in crystals and microvoids in insulating materials. UVSOR-III installed at the Institute of Molecular Science promotes the development and user use of Gamma-ray induced positron annihilation spectroscopy (GiPAS) by ultrashort pulse gamma rays. Since the ultrashort pulse gamma rays generate positrons inside the material by pair production, positron annihilation experiments of bulk materials with a thickness of several cm can be performed non-destructively. In addition, since the sample is irradiated with gamma rays from the outside, measurement can be performed in an environment such as high temperature, high pressure, and immersion. We report on the generation of ultrashort pulse gamma rays and the development status of the positron lifetime measurement, and the positron age-momentum correlation measurement.
-ray beamOmer, M.; Shizuma, Toshiyuki*; Koizumi, Mitsuo; Hajima, Ryoichi*; Zen, H.*; Taira, Yoshitaka*
no journal, ,
Taira, Yoshitaka*; Fujimoto, Masaki*; Fujimori, Kosuke*; Kitaura, Mamoru*; Zen, H.*; Okano, Yasuaki*; Hosaka, Masahito*; Yamazaki, Junichiro*; Kato, Masahiro*; Hirade, Tetsuya; et al.
no journal, ,
For general positron sources, radioisotopes such as
Na are often used. However, there is a problem that positrons cannot probe the deep region of metal materials with a thickness of 1 mm or more. Gamma-ray induced positron annihilation lifetime measurement (GiPALS) is a method for generating positrons in bulk samples with a thickness of several centimeters and samples placed in vessels such as high temperature and/or pressure furnaces. The annihilation lifetime of positrons is about 200 ps for metal materials, so it is important to use gamma rays with a shorter pulse width for GiPALS in order to accurately measure the positron lifetime. We have succeeded in the proof-of-principle experiment for GiPALS of ultra-short pulse gamma rays with a pulse width of 2 ps, which was originally developed using 90
collision laser Compton scattering at UVSOR.
Shizuma, Toshiyuki*; Omer, M.; Hajima, Ryoichi*; Koizumi, Mitsuo; Zen, H.*; Ogaki, Hideaki*; Taira, Yoshitaka*
no journal, ,
Kitaura, Mamoru*; Fujimori, Kosuke*; Taira, Yoshitaka*; Fujimoto, Masaki*; Zen, H.*; Hirade, Tetsuya; Kamada, Kei*; Watanabe, Shinta*; Onishi, Akimasa*
no journal, ,
Positron annihilation spectroscopy is the only way to investigate the properties of cation vacancies because they are negatively charged. We generated high-energy pulsed gamma rays by the vertical collision of an ultrashort pulse laser and electron beam. In this study, we investigated the vacancy-type defects present in the crystals of GAGG(Gd
Al
Ga
O
), GAGG: Ce and GAGG: Ce, Mg by positron annihilation lifetime spectroscopy using the high-energy gamma rays. The lifetime of the defect-related component was significantly changed by Mg co-doping. This was understood by considering aggregates of Mg
ions at Al/Ga sites with oxygen vacancies, which resulted in the formation of vacancy clusters.
Al
Ga
O
crystals revealed by gamma-ray induced positron annihilation lifetime spectroscopyFujimori, Kosuke*; Kitaura, Mamoru*; Taira, Yoshitaka*; Fujimoto, Masaki*; Zen, H.*; Hirade, Tetsuya; Kamada, Kei*; Watanabe, Shinta*; Onishi, Akimasa*
no journal, ,
We generated high-energy pulsed gamma rays by the vertical collision of an ultrashort pulse laser and electron beam. In this study, we investigated the vacancy-type defects present in the crystals of GAGG(Gd
Al
Ga
O
), GAGG: Ce and GAGG: Ce, Mg by positron annihilation lifetime spectroscopy using the high-energy gamma rays. The lifetime of the defect-related component was significantly changed by Mg co-doping. This indicates that the Al/Ga vacancies disappear. This fact corresponds well with the suppression of the phosphorescence component and is an important result showing that the Mg co-doping is effective in suppressing the shallow electron capture center.
Yang, Y.*; Taira, Yoshitaka*; Shizuma, Toshiyuki*; Omer, M.
no journal, ,
Taira, Yoshitaka*; Yang, Y.*; Shizuma, Toshiyuki*; Omer, M.
no journal, ,
Shizuma, Toshiyuki*; Omer, M.; Hajima, Ryoichi*; Koizumi, Mitsuo; Zen, H.*; Ogaki, Hideaki*; Taira, Yoshitaka*
no journal, ,
no abstracts in English
Taira, Yoshitaka*; Okano, Yasuaki*; Hirade, Tetsuya
no journal, ,
We are developing gamma-ray-induced positron annihilation spectroscopy (GiPAS) using ultra-short pulsed gamma rays at the UVSOR synchrotron facility in Japan. The gamma rays with the pulse width of picosecond range are generated by 90-degree inverse Compton scattering between a 750 MeV electron beam and an 800 nm laser. As the energy of the gamma rays is 6.6 MeV, gamma-ray irradiation produces positrons by pair production inside the material. Generated positrons localize on atomic-scale defects in solid crystals, such as vacancies, dislocations, and vacancy clusters. Positronium, the bound state of an electron-positron pair, localizes in vacant space caused by the free volume in polymers. Therefore, positrons are excellent probes of the nanostructure of these materials. Furthermore, the circularly polarized gamma rays generated by a circularly polarized laser can produce spin polarized positrons. The spin polarized positrons provide additional information about the electron spins around defects. GiPAS is currently available for users in UVSOR-III.