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Murai, Naoki; Fukuda, Tatsuo; Nakajima, Masamichi*; Kawamura, Mitsuaki*; Ishikawa, Daisuke*; Tajima, Setsuko*; Baron, A. Q. R.*
Physical Review B, 101(3), p.035126_1 - 035126_6, 2020/01
Times Cited Count：0 Percentile：100(Materials Science, Multidisciplinary)We report an inelastic X-ray scattering investigation of phonons in FeSe superconductor. Comparing the experimental phonon dispersion with density functional theory (DFT) calculations in the non-magnetic state, we found a significant disagreement between them. A better overall agreement was obtained by allowing for spin-polarization in DFT calculations, despite the absence of magnetic order in FeSe. This calculation gives a realistic approximation, at DFT level, of the disordered paramagnetic state of FeSe, in which strong spin fluctuations are present.
As using high-resolution inelastic X-ray scatteringMurai, Naoki*; Fukuda, Tatsuo; Kobayashi, Tatsuya*; Nakajima, Masamichi*; Uchiyama, Hiroshi*; Ishikawa, Daisuke*; Tsutsui, Satoshi*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.
Physical Review B, 93(2), p.020301_1 - 020301_5, 2016/01
Times Cited Count：6 Percentile：55.15(Materials Science, Multidisciplinary)Hirata, Yasuyuki*; Kojima, Kenji*; Uchida, Shinichi*; Ishikado, Motoyuki; Iyo, Akira*; Eisaki, Hiroshi*; Tajima, Setsuko*
Physica C, 470(Suppl.1), p.S44 - S46, 2010/12
Times Cited Count：2 Percentile：86.1(Physics, Applied)Infrared reflectivity spectra of the multilayered HgBa
Ca
Cu
O
(
= 2, 3, 4, and 5) are measured. Optical plasma modes associated with the Josephson coupling between CuO planes within a multilayer appear below 
in the c-axis component of the reflectivity spectrum. For the bilayer and trilayer compound an optical Josephson plasma mode appears at unprecedentedly high frequency, 
700-800 cm
, below . The plasma frequencies appreciably decrease in four- and five-layer compounds which indicates the suppression of superconducting order in the inner CuO planes, consistent with the result of NMR experiment.
cuprates studied by resonant inelastic X-ray scatteringIshii, Kenji; Hoesch, M.*; Inami, Toshiya; Kuzushita, Kaori*; Owada, Kenji; Tsubota, Masami; Murakami, Yoichi; Mizuki, Junichiro; Endo, Yasuo; Tsutsui, Kenji*; et al.
Journal of Physics and Chemistry of Solids, 69(12), p.3118 - 3124, 2008/12
Times Cited Count：3 Percentile：79.94(Chemistry, Multidisciplinary)Cu
O
studied by resonant inelastic X-ray scatteringIshii, Kenji; Tsutsui, Kenji*; Endo, Yasuo*; Toyama, Takami*; Kuzushita, Kaori; Inami, Toshiya; Owada, Kenji; Maekawa, Sadamichi*; Masui, Takahiko*; Tajima, Setsuko*; et al.
AIP Conference Proceedings 850, p.445 - 446, 2006/09
Mott gap excitations in the optimally doped high-
superconductor YBaCuO ( = 93 K) have been studied by the resonant inelastic X-ray scattering method. Anisotropic spectra in the 
-plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the 
direction, while the excitation from the CuO plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculation based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO plane site.
CuO ( = 93 K) studied by resonant inelastic X-ray scatteringIshii, Kenji; Tsutsui, Kenji*; Endo, Yasuo*; Toyama, Takami*; Kuzushita, Kaori; Inami, Toshiya; Owada, Kenji; Maekawa, Sadamichi*; Masui, Takahiko*; Tajima, Setsuko*; et al.
Physical Review Letters, 94(18), p.187002_1 - 187002_4, 2005/05
Times Cited Count：38 Percentile：18.06(Physics, Multidisciplinary)Mott gap excitations in the optimally doped high- superconductor YBaCuO ( = 93 K) have been studied by the resonant inelastic X-ray scattering method. Anisotropic spectra in the -plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the direction, while the excitation from the CuO plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculation based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO plane site.
Ishii, Kenji; Tsutsui, Kenji*; Endo, Yasuo*; Toyama, Takami*; Inami, Toshiya; Owada, Kenji; Kuzushita, Kaori*; Hoesch, M.; Tsubota, Masami; Mizuki, Junichiro; et al.
no journal, ,
Resonant inelastic X-ray scattering studies on high-
superconductors Nd
Ce
CuO
and YBaCuO
are presented. In NdCuO and YBaCuO
, which are Mott insulators, an excitation across the Mott gap is observed around 2 eV. The spectral weight of this excitation shifts to higher energy with increasing the momentum transfer and the dispersion of the excitation is larger along the ![$$[pi,pi]$$](/search/images/ERNVY2DJFROHA0K3EQ.gif)
direction than the ![$$[pi,0]$$](/search/images/ERNVY2DJFQYF0JA.gif)
direction. An intraband excitation in the upper Hubbard band emerges in the spectra of electron-doped Nd
Ce
CuO. As a function of the momentum transfer in the CuO plane, the excitation shifts to higher energy up to 2-2.5 eV at the zone boundary, accompanied by an increase of the spectral width. On the other hand, excitations from two inequivalent Cu sites in hole-doped YBaCuO
are distinguished by the momentum dependence and the Mott gap of the CuO chain site is found to be much smaller than that of the CuO plane site.
As via inelastic X-ray scatteringMurai, Naoki*; Fukuda, Tatsuo; Uchiyama, Hiroshi*; Tsutsui, Satoshi*; Ishikawa, Daisuke*; Kobayashi, Tatsuya*; Nakamura, Hiroki; Machida, Masahiko; Nakajima, Masamichi*; Miyasaka, Shigeki*; et al.
no journal, ,
no abstracts in English
Co)As by inelastic X-ray scatteringMurai, Naoki*; Fukuda, Tatsuo; Nakajima, Masamichi*; Kobayashi, Tatsuya*; Uchiyama, Hiroshi*; Tsutsui, Satoshi*; Ishikawa, Daisuke*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.
no journal, ,
As via high-resolution inelastic X-ray scatteringMurai, Naoki; Fukuda, Tatsuo; Kobayashi, Tatsuya*; Nakajima, Masamichi*; Uchiyama, Hiroshi*; Ishikawa, Daisuke*; Tsutsui, Satoshi*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.
no journal, ,
We report the first IXS study of single crystals of SrFeAs that have been detwinned via application of in-plane uniaxial stress. Our results clearly show anisotropy in phonon structure below 
= 
characterized by mode splitting at tetragonally-equivalent momentum transfers. To the best of our knowledge, this is the first observation of phonon anisotropy in iron-pnictides at finite momentum transfers. We obtain good agreement with our results using calculations that are modified to account for a reduced magnetic moment and fluctuating magnetism. Previous efforts using either non-magnetic calculations or static magnetism tend to either get the dispersion wrong from non-magnetic calculations or strongly over-estimate the phonon mode splitting when static magnetism is included. Our model for the response below incorporates a phenomenological reduction in force constant anisotropy, by about 65%, that can be attributed to residual fast magnetic fluctuations. Above , all fluctuations are assumed to be fast and the response becomes the average of the results from the static magnetism. This serves as a starting point for a general model of phonons in iron-pnictides applicable to both non-magnetic and magnetic phases.
