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Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Koike, Yuko; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; Nagai, Shinji; et al.
JAEA-Review 2023-046, 164 Pages, 2024/03
JAEA-Review-2023-046.pdf:4.2MB
The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2022 to March 2023 and the results of dose calculations for the surrounding public due to the release of radioactive materials into the atmosphere and ocean. In the results of the above environmental radiation monitoring, many items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.
Nakada, Akira; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Futagawa, Kazuo; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; et al.
JAEA-Review 2022-078, 164 Pages, 2023/03
JAEA-Review-2022-078.pdf:2.64MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2021 to March 2022. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
-ray discrimination based on the property and thickness controls of scintillators using Li glass and LiCAF(Ce) in a -ray fieldKaburagi, Masaaki; Shimazoe, Kenji*; Terasaka, Yuta; Tomita, Hideki*; Yoshihashi, Sachiko*; Yamazaki, Atsushi*; Uritani, Akira*; Takahashi, Hiroyuki*
Nuclear Instruments and Methods in Physics Research A, 1046, p.167636_1 - 167636_8, 2023/01
Times Cited Count：3 Percentile：90.12(Instruments & Instrumentation)We focus on the thickness and property controls of inorganic scintillators used for thermal neutron detection in intense -ray fields without considering pulse shape discrimination techniques. GS20
(a lithium glass) and LiCaAlF
:Ce(LiCAF:Ce) cintillators with thicknesses of 0.5 and 1.0 mm, respectively, have been employed. Pulse signals generated by photomultiplier tubes, to which the scintillators were coupled, were inserted into a digital pulse processing unit with 1 Gsps, and the areas of waveforms were integrated for 360 ns. In a 
Co -ray field, the neutron detection for GS20 with a 0.5-mm thickness was possible at dose rates of up to 0.919 Gy/h; however, for LiCAF:Ce, neutron detection was possible at 0.473 Gy/h, and it failed at 0.709 Gy/h. Threfore, in a Co -ray field, the neutron/-ray discrimination of GS20 was better than that of LiCAF:Ce due to its better energy resolution and higher detection efficiency.
-edge to assess the U(V) electronic structure in FeUO
Yomogida, Takumi; Akiyama, Daisuke*; Ouchi, Kazuki; Kumagai, Yuta; Higashi, Kotaro*; Kitatsuji, Yoshihiro; Kirishima, Akira*; Kawamura, Naomi*; Takahashi, Yoshio*
Inorganic Chemistry, 61(50), p.20206 - 20210, 2022/12
Times Cited Count：2 Percentile：36.89(Chemistry, Inorganic & Nuclear)FeUO was studied to clarify the electronic structure of U(V) in a metal monouranate compound. We obtained the peak splitting of HERFD-XANES spectra utilizing high-energy-resolution fluorescence detection-X-ray absorption near edge structure (HERFD-XANES) spectroscopy at the U L-edge, which is a novel technique in the U(V) compounds. Theoretical calculations revealed that the peak splitting was caused by splitting the 6d orbital of U(V). Such distinctive electronic states are of major interest to researchers and engineers working in various fields, from fundamental physics to the nuclear industry and environmental sciences for actinide elements.
Sasada, Seiji*; Takahashi, Yoshihito*; Takeuchi, Keisuke*; Hiroi, Kosuke; Su, Y. H.; Shinohara, Takenao; Watanabe, Kenichi*; Uritani, Akira*
Japanese Journal of Applied Physics, 61(4), p.046004_1 - 046004_8, 2022/03
Times Cited Count：0 Percentile：0(Physics, Applied)Nakada, Akira; Nakano, Masanao; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Nemoto, Masashi; Tobita, Keiji; Futagawa, Kazuo; Yamada, Ryohei; Uchiyama, Rei; et al.
JAEA-Review 2021-062, 163 Pages, 2022/02
JAEA-Review-2021-062.pdf:2.87MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2020 to March 2021. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
-ray spectrometer and its performance under intense 
Cs and Co radiation fieldsKaburagi, Masaaki; Shimazoe, Kenji*; Kato, Masahiro*; Kurosawa, Tadahiro*; Kamada, Kei*; Kim, K. J.*; Yoshino, Masao*; Shoji, Yasuhiro*; Yoshikawa, Akira*; Takahashi, Hiroyuki*
Nuclear Instruments and Methods in Physics Research A, 1010, p.165544_1 - 165544_9, 2021/09
Times Cited Count：0 Percentile：0.02(Instruments & Instrumentation)The number of nuclear facilities being decommissioned has been increasing worldwide, in particular following the accident of the Tokyo Electric Power Company Holdings' Fukushima Daiichi Nuclear Power Station in 2011. In these nuclear facilities, proper management of radioactive materials is required. Then, A -ray spectrometer with four segmentations using small volume CeBr scintillators with a dimension of 
was developed. The four scintillators were coupled to a multi-anode photomultiplier tube specific to intense radiation fields. We performed the -ray exposure study under Cs and Co radiation fields. Under the Cs radiation field, the relative energy resolution at 1375 mSv/h was the relative energy resolution at 1375 mSv/h was 9.2
0.05%, 8.00.08%, 8.0
0.03%, and 9.00.04% for the four channels, respectively.
Takahashi, Atsushi*; Chiba, Mirei*; Tanahara, Akira*; Aida, Jun*; Shimizu, Yoshinaka*; Suzuki, Toshihiko*; Murakami, Shinobu*; Koarai, Kazuma; Ono, Takumi*; Oka, Toshitaka; et al.
Scientific Reports (Internet), 11(1), p.10355_1 - 10355_11, 2021/05
Times Cited Count：6 Percentile：41.49(Multidisciplinary Sciences)Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count：43 Percentile：96.93(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 
C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
scintillator under intense -ray fields for nuclear decommissioningKaburagi, Masaaki; Shimazoe, Kenji*; Kato, Masahiro*; Kurosawa, Tadahiro*; Kamada, Kei*; Kim, K. J.*; Yoshino, Masao*; Shoji, Yasuhiro*; Yoshikawa, Akira*; Takahashi, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research A, 988, p.164900_1 - 164900_8, 2021/02
Times Cited Count：11 Percentile：89.29(Instruments & Instrumentation)An increasing number of nuclear facilities have been decommissioned worldwide following the 2011 accident of the TEPCO' Fukushima Daiichi Nuclear Power Station. During the decommissioning, radioactive materials have to be retrieved under proper management. In this study, a small cubic CeBr spectrometer with dimensions of 5 mm 
5 mm 5 mm was manufactured to perform -ray spectroscopy under intense -ray fields. Furthermore, thanks to a fast digital process unit and a customized photomultiplier, the device could perform -ray spectroscopy at dose rates of over 1 Sv/h. The energy resolution (FWHM) at 662 keV ranged from 4.4% at 22 mSv/h to 5.2% at 1407 mSv/h for a Cs radiation field. Correspondingly, at 1333 keV, it ranged from 3.1% at 26 mSv/h to 4.2% at 2221 mSv/h for a Co radiation field, which suggested to realize -ray assessment of 
Cs, Cs, Co, and 
Eu at dose rates of over 1 Sv/h.
gamma-ray spectrometer suitable for the decommissioning of the Fukushima Daiichi Nuclear Power StationKaburagi, Masaaki; Shimazoe, Kenji*; Otaka, Yutaka*; Uenomachi, Mizuki*; Kamada, Kei*; Kim, K. J.*; Yoshino, Masao*; Shoji, Yasuhiro*; Yoshikawa, Akira*; Takahashi, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research A, 971, p.164118_1 - 164118_8, 2020/08
Times Cited Count：7 Percentile：66.68(Instruments & Instrumentation)
states in CeFe
revealed by soft X-ray magnetic circular dichroismSaito, Yuji; Yasui, Akira*; Fuchimoto, Hiroto*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Imada, Shin*; Narumi, Yasuo*; Kindo, Koichi*; Takahashi, Minoru*; Ebihara, Takao*; et al.
Physical Review B, 96(3), p.035151_1 - 035151_5, 2017/07
Times Cited Count：3 Percentile：17.1(Materials Science, Multidisciplinary)We revisit the delocalized character of the 4
states of CeFe
in the ferromagnetically ordered phase by X-ray magnetic circular dichroism (XMCD) in X-ray absorption spectroscopy (XAS) with improved data quality using single crystals. Surprisingly, the Ce 
XMCD spectral shape changes significantly as a function of temperature and applied magnetic field, with no concomitant changes in the spectral shape of the Ce XAS as well as the Fe 
XAS and XMCD. This unusual behavior is characterized by the 
states in a 4
configuration mixed into the 
ground state. Such extreme sensitivity of the Ce 4 states to the external perturbations can be related to the magnetic instability toward an antiferromagnetic phase in CeFe. Our experimental data presented here provide valuable insights into the underlying physics in strongly-hybridized ferromagnetic Ce compounds.
(Al,Ga)
O
scintillator Compton camera mounted on an unmanned helicopterShikaze, Yoshiaki; Nishizawa, Yukiyasu; Sanada, Yukihisa; Torii, Tatsuo; Jiang, J.*; Shimazoe, Kenji*; Takahashi, Hiroyuki*; Yoshino, Masao*; Ito, Shigeki*; Endo, Takanori*; et al.
Journal of Nuclear Science and Technology, 53(12), p.1907 - 1918, 2016/12
Times Cited Count：37 Percentile：96.48(Nuclear Science & Technology)The Compton camera was improved for use with the unmanned helicopter. Increase of the scintillator array from 44 to 88 and expanse of the distance between the two layers contributed to the improvements of detection efficiency and angular resolution, respectively. Measurements were performed over the riverbed of the Ukedo river of Namie town in Fukushima Prefecture. By programming of flight path and speed, the areas of 65 m 60 m and 65 m 180 m were measured during about 20 and 30 minutes, respectively. By the analysis the air dose rate maps at 1 m height were obtained precisely with the angular resolution corresponding to the position resolution of about 10 m from 10 m height. Hovering flights were executed over the hot spot areas for 10-20 minutes at 5-20 m height. By using the reconstruction software the -ray images including the hot spots were obtained with the angular resolution same as that evaluated in the laboratory (about 10).
Sasaki, Akira; Kato, Susumu*; Takahashi, Eiichi*; Kishimoto, Yasuaki*; Fujii, Takashi*; Kanazawa, Seiji*
Japanese Journal of Applied Physics, 55(2), p.026101_1 - 026101_10, 2016/02
Times Cited Count：2 Percentile：9.68(Physics, Applied)A percolation model of discharge, which can reproduce stochastic behaviors of initial partial discharge to the growth of a stepped leader, is presented. The model uses macroscopic cells, from which a network of electric circuits is defined, and the spatial and temporal evolutions of the electric field and current in the discharge medium are calculated. For each cell, one of two states, either insulator or conductor, which corresponds to neutral gas or ionized plasmas, respectively, is decided. The decision is made on the basis of probability for each calculation cell at each time step, taking the effects of local electric field and current, which enhance ionization and sustain the discharge channel, respectively, into account. The stochastic behavior of discharge is discussed, in conjunction with the characteristic feature of ionization, that is, the ionization occurs not only ahead of the streamer tip where the electric field is enhanced but randomly in the discharge medium.
Okumura, Yoshikazu; Gobin, R.*; Knaster, J.*; Heidinger, R.*; Ayala, J.-M.*; Bolzon, B.*; Cara, P.*; Chauvin, N.*; Chel, S.*; Gex, D.*; et al.
Review of Scientific Instruments, 87(2), p.02A739_1 - 02A739_3, 2016/02
Times Cited Count：7 Percentile：35.23(Instruments & Instrumentation)IFMIF is an accelerator based neutron facility having two set of linear accelerators each producing 125mA/CW deuterium ion beams (250mA in total) at 40MeV. The LIPAc (Linear IFMIF Prototype Accelerator) being developed in the IFMIF-EVEDA project consists of an injector, a RFQ accelerator, and a part of superconducting Linac, whose target is to demonstrate 125mA/CW deuterium ion beam acceleration up to 9MeV. The injector has been developed in CEA Saclay and already demonstrated 140mA/100keV deuterium beam. The injector was disassembled and delivered to the International Fusion Energy Research Center (IFERC) in Rokkasho, Japan, and the commissioning has started after its reassembly 2014; the first beam production has been achieved in November 2014. Up to now, 100keV/120mA/CW hydrogen ion beam has been produced with a low beam emittance of 0.2 
.mm.mrad (rms, normalized).
/D ion source for IFMIF (International Fusion Materials Irradiation Facility)Shinto, Katsuhiro; Sen
e, F.*; Ayala, J.-M.*; Bolzon, B.*; Chauvin, N.*; Gobin, R.*; Ichimiya, Ryo; Ihara, Akira; Ikeda, Yukiharu; Kasugai, Atsushi; et al.
Review of Scientific Instruments, 87(2), p.02A727_1 - 02A727_3, 2016/02
Times Cited Count：8 Percentile：39.15(Instruments & Instrumentation)Satoh, Daiki; Furuta, Takuya; Takahashi, Fumiaki; Endo, Akira; Lee, C.*; Bolch, W. E.*
Journal of Nuclear Science and Technology, 53(1), p.69 - 81, 2016/01
Times Cited Count：18 Percentile：85.7(Nuclear Science & Technology)To estimate effective doses for the public exposed to external radiation from radioactive cesium (Cs and Cs) deposited on the ground by the Fukushima nuclear accident, we calculate the conversion coefficients for converting activity concentration to effective dose rate by using the Particle and Heavy Ion Transport code System (PHITS). The data were produced from different age groups within the public (newborns; 1-, 5-, 10-, and 15-year-old children; and adults) for the situations in which radioactive cesium is distributed uniformly in the soil over a planar area and at specific depths of 0.0, 0.5, 2.5, 5.0, 10.0, and 50.0 g/cm
. On the basis of the results, we also derive the conversion coefficients for exponentially distributed volumetric sources. In addition, we obtain the conversion coefficients that give the effective dose accumulated over the first and second months, the first year, and over a lifetime (50 years) because of the contamination remaining on the ground. These calculations indicate that the conversion coefficients to obtain the effective dose rate are higher for the younger ages compared with adults but do not exceed the ambient dose equivalent rate. Furthermore, we find that the difference between the calculated effective dose rates according to the International Commission on Radiological Protection (ICRP) 1990 and 2007 Recommendations is small (7% maximum) for a ground contamination of radioactive cesium.
Tsukuda, Satoshi*; Takahashi, Ryota*; Seki, Shuhei*; Sugimoto, Masaki; Idesaki, Akira; Yoshikawa, Masahito; Tanaka, Shunichiro*
Radiation Physics and Chemistry, 118, p.16 - 20, 2016/01
Times Cited Count：1 Percentile：10.71(Chemistry, Physical)Polyvinylpyrrolidone (PVP)-Pt nanoparticles (NPs) hybrid nanowires were fabricated by high energy ion beam irradiation to PVP thin films including HPtCl
. Single ion hitting caused crosslinking reactions of PVP and reduction of Pt ions within local cylindrical area along an ion trajectory (ion track); therefore, the PVP nanowires including Pt NPs were formed and isolated on Si substrate after wet-development procedure. The number of Pt NPs was easily controlled by the mixed ratio of PVP and HPtCl. However, increasing the amount of HPtCl led to decreasing the radial size and separation of the hybrid nanowires during the wet-development. Additional electron beam irradiation after ion beam improved separation of the nanowires and controlled radial sizes due to an increase in the density of crosslinking points inner the nanowires.
radionuclide therapyOgawa, Kazuma*; Mizuno, Yoshiaki*; Washiyama, Koshin*; Shiba, Kazuhiro*; Takahashi, Naruto*; Kozaka, Takashi*; Watanabe, Shigeki; Shinohara, Atsushi*; Odani, Akira*
Nuclear Medicine and Biology, 42(11), p.875 - 879, 2015/11
Times Cited Count：23 Percentile：70.83(Radiology, Nuclear Medicine & Medical Imaging)Okumura, Yoshikazu; Ayala, J.-M.*; Bolzon, B.*; Cara, P.*; Chauvin, N.*; Chel, S.*; Gex, D.*; Gobin, R.*; Harrault, F.*; Heidinger, R.*; et al.
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.203 - 205, 2015/09
Under the framework of Broader Approach (BA) agreement between Japan and Euratom, IFMIF/EVEDA project was launched in 2007 to validate the key technologies to realize IFMIF. The most crucial technology to realize IFMIF is two set of linear accelerator each producing 125mA/CW deuterium ion beams up to 40MeV. The prototype accelerator, whose target is 125mA/CW deuterium ion beam acceleration up to 9MeV, is being developed in International Fusion Research Energy Center (IFERC) in Rokkasho, Japan. The injector developed in CEA Saclay was delivered in Rokkasho in 2014, and is under commissioning. Up to now, 100keV/120mA/CW hydrogen ion beams and 100keV/90mA/CW duty deuterium ion beams are successfully produced with a low beam emittance of 0.21 .mm.mrad (rms, normalized). Delivery of RFQ components will start in 2015, followed by the installation of RF power supplies in 2015.
