Development of hydrogen behavior integrated analysis system

Terada, Atsuhiko; Thwe Thwe, A.; Hino, Ryutaro*; Harai, Yasutaka*; Sasaki, Gaku*; Shingeya, Hideshi*; Yamashita, Toshiyuki*; Yoneda, Jiro*; Okabayashi, Kazuki*; Sakamoto, Hiroyuki*; et al.

JAEA-Data/Code 2025-012, 151 Pages, 2025/12

JAEA-Data-Code-2025-012.pdf:9.69MB

Based on the lessons learned from the Fukushima Daiichi Nuclear Power Station accident, we have highly paid attention to the advancement of the fundamental technologies which are indispensable in timely response to hydrogen safety measures and assessments especially in both nuclear reactors and decommissioning. Focusing on this attention, we developed an analysis system that predicts the behavior of hydrogen from generation to diffusion, combustion and explosion. The system utilizes the commercial computational fluid dynamics software (FLUENT, AUTODYN), and incorporates new modules and pre/post-processors in order to withstand the general practical use. We also developed a system by utilizing open-source code (OpenFOAM) that can be used in hydrogen disaster prevention plans for nuclear facilities. So far, we have expanded the system to deal with the phenomena that should be considered from the practical point of view for PWR (Pressurized Water Reactor) in nuclear power plants. This report summarizes the overview of the integrated analysis system for hydrogen behavior, the handling method, and real scale analysis examples.

A Study for establishment of passive creep-fatigue test techniques using the difference of thermal expansion coefficients of the materials

Wakai, Takashi; Ando, Masanori; Okajima, Satoshi; Toyota, Kodai; Onuma, Terumitsu*; Takahashi, Ryoya*; Asayama, Tai

Dai-29-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Yokoshu (Internet), 5 Pages, 2025/06

This paper describes an experimental study for establishing a passive creep-fatigue test technique that mainly utilizes the difference in thermal expansion coefficients of the materials as material surveillance test technique that can be applied to evaluate the structural integrity of the fast reactor components when the components are used beyond the period assumed in the design. Using the test article designed with the aid of a finite element analysis, a long-term creep-fatigue test data has been successfully obtained. In the designing of the test article, it was essential to generate a adequate strain at the gauge portion of the specimen due to the difference of thermal expansion coefficients of the materials, without buckling. After much trial and error, an optimal shape and dimensions of the test article and the cyclic thermal load conditions are established. In the future, miniaturization of the test article for applying the established test technique to the actual nuclear reactors will be required.

Clay minerals and metal ions; Unraveling the behavior of metal ions from a microscopic perspective

Yamaguchi, Akiko; Yoshimura, Takashi*; Okumura, Masahiko; Takahashi, Yoshio*

Kinzoku, 95(6), p.506 - 514, 2025/06

Clay minerals control behaviors of metal ions in the soil because they are widespread in the earth's surface layer and have a large cation exchange capacity. Due to the complex structure of clay minerals, it is necessary to clarify their microscopic structure and chemical reactions in order to understand how they work. In this article, we describe a study that reveals the mechanism by which clay minerals adsorb metal ions through systematic extended X-ray absorption fine structure (EXAFS) measurements and first principles calculations.

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2023

Kokubun, Yuji; Hosomi, Kenji; Nagaoka, Mika; Seya, Natsumi; Inoue, Kazumi; Koike, Yuko; Uchiyama, Rei; Sasaki, Kazuki; Maehara, Yushi; Matsuo, Kazuki; et al.

JAEA-Review 2024-054, 168 Pages, 2025/03

JAEA-Review-2024-054.pdf:2.73MB

The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2023 to March 2024 and the results of dose calculations for the surrounding public due to the release of radioactive materials from the plant into the atmosphere and ocean. In the results of the above environmental radiation monitoring, several items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Holdings, Inc. on April 1, 2016), which occurred in March 2011. In addition, environmental monitoring plan, analysis and measurement methods, monitoring data and their chronological change, meteorological data after statistical processing, status of radioactive waste release and evaluation results of the data over the normal range are included as appendices.

Adsorption structures and bonding states of cesium and barium adsorbed on various sites of vermiculite

Yamaguchi, Akiko; Okumura, Masahiko; Kawamura, Naomi*; Takahashi, Yoshio*

Science of the Total Environment, 964, p.178585_1 - 178585_13, 2025/02

https://doi.org/10.1016/j.scitotenv.2025.178585

There are many unresolved issues in the adsorption reactions of clay minerals. One of the reasons is the existence of multiple adsorption sites. It is known that the contribution of each adsorption site depends on the concentration of adsorbed ions, and there is a challenge in comprehensively correlate the results of atomic-level simulations that employ limited number of atoms and inevitably deal high-concentration samples with actual environmental samples where concentrations are orders of magnitude lower. In this study, we combined experiments using synchrotron radiation and first-principles calculations to comprehensively elucidate the systematic changes in the local structure of adsorption sites and adsorbed ions based on the adsorption concentration at the atomic level, and demonstrated that the interaction between adsorbed ions and clay minerals involves ionic bonding.

Development of an electron spin resonance spectroscopy code for measuring carbonate radicals in tooth enamel and verification of its practicality using irradiated Japanese macaque teeth

Yamashita, Takuma*; Hayashi, Teppei*; Mitsuyasu, Yusuke*; Ono, Kenta*; Iwami, Satone*; Kino, Yasushi*; Sekine, Tsutomu*; Oka, Toshitaka; Takahashi, Atsushi*; Shimizu, Yoshinaka*; et al.

International Journal of Radiation Biology, 8 Pages, 2025/00

https://doi.org/10.1080/09553002.2025.2510676

no abstracts in English

Improved multicomponent analysis method for electron spin resonance spectra of gamma-irradiated tooth enamel

Yamashita, Takuma*; Iwami, Satone*; Mitsuyasu, Yusuke*; Ono, Kenta*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

KEK Proceedings 2024-6, p.85 - 90, 2024/12

To clarify the radiation effects of the accident at the TEPCO's Fukushima Daiichi NPP on living organisms, it is important to accurately estimate the dose to each individual. We have developed a multi-component analysis program using random number optimization to extract only the components derived from carbonate radicals from the ESR spectra.

R&D status of digital technology on inverse estimation of radioactive source distributions and related source countermeasures; Fast Digital Twin Tech. in Decommissioning Field: 3D-ADRES-Indoor FrontEnd

Machida, Masahiko; Yamada, Susumu; Kim, M.; Tanaka, Satoshi*; Tobita, Yasuhiro*; Iwata, Ayako*; Aoki, Yuto; Aoki, Kazuhisa; Yanagisawa, Kenichi*; Yamaguchi, Takashi; et al.

RIST News, (70), p.3 - 22, 2024/09

Inside the Fukushima Daiichi Nuclear Power Plant (1F), there are many locations with high radiation levels due to contamination by radioactive materials that leaked from the reactor. These pose a significant obstacle to the smooth progress of decommissioning work. To help solve this issue, the Japan Atomic Energy Agency (JAEA), under a subsidy from the Ministry of Economy, Trade, and Industry's decommissioning and contaminated water management project, is conducting research and development on digital technologies to improve the radiation environment inside the decommissioning site. This project, titled "Development of Technology to Improve the Environment Inside Reactor Buildings (Enhancing Digital Technology for Environment and Source Distribution to Reduce Radiation Exposure)," began in April of FY 2023. In this project, the aim is to develop three interconnected systems: FrontEnd, Pro, and BackEnd. The FrontEnd system, based on the previously developed 3D-ADRES-Indoor (prototype) from FY 2021-2022, will be upgraded to a high-speed digital twin technology usable on-site. The Pro system will carry out detailed analysis in rooms such as the new office building at 1F, while the BackEnd system will serve as a database to centrally manage the collected and analyzed data. This report focuses on the FrontEnd system, which will be used on-site. After point cloud measurement, the system will quickly create a 3D mesh model, estimate the radiation source from dose rate measurements, and refine the position and intensity of the estimated source using recalculation techniques (re-observation instructions and re-estimation). The results of verification tests conducted on Unit 5 are also presented. Furthermore, the report briefly discusses the future research and development plans for this project.

Microbially formed Mn(IV) oxide as a novel adsorbent for removal of Radium

Tanaka, Kazuya; Yamaji, Keiko*; Masuya, Hayato*; Tomita, Jumpei; Ozawa, Mayumi*; Yamasaki, Shinya*; Tokunaga, Kohei; Fukuyama, Kenjin*; Ohara, Yoshiyuki*; Maamoun, I.*; et al.

Chemosphere, 355, p.141837_1 - 141837_11, 2024/05

https://doi.org/10.1016/j.chemosphere.2024.141837

In this study, biogenic Mn(IV) oxide was applied to remove Ra from mine water collected from a U mill tailings pond in the Ningyo-toge center. Just 7.6 mg of biogenic Mn(IV) oxide removed more than 98% of the Ra from 3 L of mine water, corresponding to a distribution coefficient of 10 mL/g for Ra at pH 7. The obtained value was convincingly high for practical application of biogenic Mn(IV) oxide in water treatment.

Molecular geochemistry of radium; A key to understanding cation adsorption reaction on clay minerals

Yamaguchi, Akiko; Kurihara, Yuichi*; Nagata, Kojiro*; Tanaka, Kazuya; Higaki, Shogo*; Kobayashi, Toru; Tanida, Hajime; Ohara, Yoshiyuki*; Yokoyama, Keiichi; Yaita, Tsuyoshi; et al.

Journal of Colloid and Interface Science, 661, p.317 - 332, 2024/05

https://doi.org/10.1016/j.jcis.2024.01.120

no abstracts in English