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Journal Articles

Proton-exchange mechanism of specific Cs$$^{+}$$ adsorption $$via$$ lattice defect sites of Prussian blue filled with coordination and crystallization water molecules

Ishizaki, Manabu*; Akiba, Sae*; Otani, Asako*; Hoshi, Yuji*; Ono, Kenta*; Matsuba, Mayu*; Togashi, Takanari*; Kanaizuka, Katsuhiko*; Sakamoto, Masatomi*; Takahashi, Akira*; et al.

Dalton Transactions, 42(45), p.16049 - 16055, 2013/12

https://doi.org/10.1039/c3dt51637g
 Times Cited Count：190 Percentile：99.56(Chemistry, Inorganic & Nuclear)

We have revealed the fundamental mechanism of specific Cs$$^{+}$$ adsorption into Prussian blue (PB) in order to develop high-performance PB-based Cs$$^{+}$$ adsorbents in the wake of the Fukushima nuclear accident. We compared two types of PB nanoparticles with formulae of Fe$$^{III}$$$$_{4}$$[Fe$$^{II}$$(CN)$$_{6}$$]3$$cdot$$xH$$_{2}$$O (x = 10-15) (PB-1) and (NH$$_{4}$$)0.70Fe$$^{III}$$1.10[Fe$$^{II}$$(CN)$$_{6}$$]$$cdot$$1.7H$$_{2}$$O (PB-2) with respect to the Cs$$^{+}$$ adsorption ability. The synthesised PB-1, by a common stoichiometric aqueous reaction between 4Fe$$^{3+}$$ and 3[Fe$$^{II}$$(CN)$$_{6}$$]$$^{4-}$$, showed much more efficient Cs$$^{+}$$ adsorption ability than did the commercially available PB-2.

Oral presentation

Development of and co-processing process; The Control of Pu/U ratio of product on the partitioning section

Namatame, Toshihiro; Masui, Kenji; Takahashi, Masatomi; Sato, Takehiko; Fujimoto, Ikuo; Tanaka, Yukiyoshi

no journal, , 

no abstracts in English

Oral presentation

The Supports for local governments used the walking survey

Terunuma, Hirotaka; Tanaka, Kiwamu; Kabumoto, Hiroshi; Haginoya, Masashi; Sano, Naruto; Takahashi, Masatomi; Hoshino, Masato; Aoki, Isao; Asazuma, Shinichiro

no journal, , 

no abstracts in English

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